Tao, Yuqiang, Zhang, Ya, Cao, Jicheng, Wu, Zifan, Yao, Shuchun, and Xue, Bin
Burial in sediments is a crucial way to reduce mobilization and risks of hydrophobic organic contaminants (HOCs), but ability of sediments to bury HOCs may be altered if the environment is changed. Whether the ability of sediments to bury HOCs has been affected by climate change remains largely unclear. We excluded the impacts of anthropogenic emissions and eutrophication from that of climate change, and for the first time found that not only the rising surface air temperature but also the declining wind speed and the reducing days with precipitation had weakened the ability of Chinese lakes to bury 16 polycyclic aromatic hydrocarbon (PAHs) by 69.2% ± 9.4%–85.7% ± 3.6% from 1951 to 2017. The relative contributions of the climatic variables to the reduced burial ability depended on the properties of the PAHs, and lakes. Burial ability of the PAHs responded differently to climate change, and was correlated to their volatilization and aqueous solubility, and lake area, catchment area/lake area ratio, and water depth. Our study suggests that not only the rising surface air temperature but also the declining wind speed and the reducing days with precipitation can undermine global efforts to reduce environmental and human exposure to PAHs. Image 1 • Methodological approach was used to study climate change and burial ability of PAHs. • Temperature, wind speed, and days with precipitation weakened the burial ability. • Contribution of the climatic variables to the reduced burial ability was estimated. • The reduced burial ability was correlated to the properties of PAHs, and the lakes. For the first time we find not only rising surface air temperature but also declining wind speed and reducing days with precipitation weakens the ability of lakes to bury PAHs. [ABSTRACT FROM AUTHOR]