14 results on '"Nie, Wanyi"'
Search Results
2. Charged Hole‐Transporting Materials Based on Imidazolium for Defect Passivation in Inverted Perovskite Solar Cells.
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Tingare, Yogesh S., Li, Meng‐Che, Teng, Sheng‐Hung, Lin, Ja‐Hon, Su, Chaochin, Lin, Shan‐Jung, Lew, Xin‐Rui, Tsai, Hsinhan, Ghosh, Dibyajyoti, Nie, Wanyi, Yeh, Bao‐Lin, and Li, Wen‐Ren
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PASSIVATION ,SOLAR cells ,PEROVSKITE ,MASS production ,COUNTER-ions ,CRYSTAL structure - Abstract
The hole‐transporting material (HTM) in perovskite solar cells (PSCs) provides an ideal interface with the perovskite layer for hole collection while influencing the perovskite crystalline structure and morphology. This article presents SIM and DIM, two new dopant‐free imidazolium‐based HTMs with charged units accompanied by counter ions that show the potential to function as ionic HTMs and ionic liquid additives and help improve the efficiency and stability of inverted PSCs. DIM‐based PSCs demonstrates exceptional performance with a high‐power conversion efficiency of 19.15%, attributed to improved passivation of perovskite interface defects. Furthermore, these new imidazolium salt‐based HTMs can be manufactured economically, making them a viable option for mass production and PSC commercialization. [ABSTRACT FROM AUTHOR]
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- 2024
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3. Perovskite Solar Module: Promise and Challenges in Efficiency, Meta‐Stability, and Operational Lifetime.
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Le, Thanh‐Hai, Driscoll, Honora, Hou, Cheng‐Hung, Montgomery, Angelique, Li, Wayne, Stein, Joshua S., and Nie, Wanyi
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PEROVSKITE ,SOLAR cell efficiency ,SOLAR cells ,HYSTERESIS ,SOLAR energy ,DATABASES ,PHOTOVOLTAIC power generation - Abstract
Perovskite photovoltaics (PVs) are an emerging solar energy generation technology that is nearing commercialization. Despite the unprecedented progress in increasing power conversion efficiency (PCE) for perovskite solar cells (PSCs), up‐scaling lab‐made cells to solar modules remains a challenge. In this work, the recent progress of making perovskite mini‐modules is reviewed. In particular, a database summarizing the module size, performance, hysteresis, and operational lifetimes reported in the literature is built. After analyzing the performance losses from scaling PSCs to mini‐modules based on the data collected from the literature, the current key to high‐performance perovskite mini‐modules is found to be the coating method optimization. If the perovskite layer quality is well reserved, a >24% mini‐module efficiency is projected by only considering the losses from lateral resistivity and laser scribing area. Next, performance characteristics are explored including hysteresis and meta‐stable power outputs that must be overcome to correctly characterize perovskite modules. Finally, current challenges associated with the long‐term stability of perovskite modules are examined and the importance of such durability for commercialization is discussed. It is hoped that the findings in this review provide a bridge for the development of perovskite modules that will lead to commercialization in the near future. [ABSTRACT FROM AUTHOR]
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- 2023
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4. Benzimidazole Based Hole‐Transporting Materials for High‐performance Inverted Perovskite Solar Cells.
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Tingare, Yogesh S., Su, Chaochin, Lin, Ja‐Hon, Hsieh, Yi‐Chun, Lin, Hong‐Jia, Hsu, Ya‐Chun, Li, Meng‐Che, Chen, Guan‐Lin, Tseng, Kai‐Wei, Yang, Yi‐Hsuan, Wang, Leeyih, Tsai, Hsinhan, Nie, Wanyi, and Li, Wen‐Ren
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SOLAR cells ,PEROVSKITE ,PHOTOVOLTAIC power systems ,HOLE mobility ,OPEN-circuit voltage ,CURRENT-voltage characteristics ,FREE material - Abstract
Interfaces play a decisive role in perovskite solar cells' power conversion efficiency and their long‐term durability. Small‐molecule hole‐transporting materials (HTMs) have grabbed enormous attention due to their structural flexibility, material properties, and stabilities, allowing for improved operational durability in perovskite photovoltaics. This study synthesizes and investigates a new class of benzimidazole‐based small molecules, named YJS001 and YJS003, serving as the HTMs to enable high‐efficiency mixed‐cation mixed‐halide perovskite solar cells. The benzimidazole‐based materials are dopant‐free HTMs composed of donor and acceptor building blocks that are designed to engineer the energy level alignment near the HTM/perovskite interface. Mixed‐cation mixed‐halide perovskites can be grown uniformly on both HTMs with large crystalline grains. It is discovered that the donor‐rich YJS003‐based solar cell exhibits a high open‐circuit voltage of 1.09 V with a champion power conversion efficiency of over 20%. Power‐dependent current–voltage characteristics of the solar cells are analyzed, from which the high performance of YJS003's excellent hole mobility and well‐aligned energy level is attributed. This work introduces a new class of benzimidazole‐based small molecules as HTMs, that paves the path for dopant free interface material development for commercialization of perovskite solar cells. [ABSTRACT FROM AUTHOR]
- Published
- 2022
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5. Two-Dimensional Halide Perovskites Incorporating Straight Chain Symmetric Diammonium Ions, (NH3CmH2mNH3)(CH3NH3)n−1PbnI3n+1 (m = 4–9; n = 1–4)
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Li, Xiaotong, Hoffman, Justin, Ke, Weijun, Chen, Michelle, Tsai, Hsinhan, Nie, Wanyi, Mohite, Aditya, Kepenekian, Mikael, Katan, Claudine, Even, Jacky, Wasielewski, Michael, Stoumpos, Constantinos, Kanatzidis, Mercouri, Northwestern University [Evanston], Rice University [Houston], Los Alamos National Laboratory (LANL), Institut des Sciences Chimiques de Rennes (ISCR), Centre National de la Recherche Scientifique (CNRS)-Institut de Chimie du CNRS (INC)-Université de Rennes 1 (UR1), Université de Rennes (UNIV-RENNES)-Université de Rennes (UNIV-RENNES)-Ecole Nationale Supérieure de Chimie de Rennes (ENSCR)-Institut National des Sciences Appliquées - Rennes (INSA Rennes), Institut National des Sciences Appliquées (INSA)-Université de Rennes (UNIV-RENNES)-Institut National des Sciences Appliquées (INSA), Institut des Fonctions Optiques pour les Technologies de l'informatiON (Institut FOTON), Université de Rennes 1 (UR1), Université de Rennes (UNIV-RENNES)-Université de Rennes (UNIV-RENNES)-Institut National des Sciences Appliquées - Rennes (INSA Rennes), Institut National des Sciences Appliquées (INSA)-Université de Rennes (UNIV-RENNES)-Institut National des Sciences Appliquées (INSA)-École Nationale Supérieure des Sciences Appliquées et de Technologie (ENSSAT)-Centre National de la Recherche Scientifique (CNRS)-IMT Atlantique Bretagne-Pays de la Loire (IMT Atlantique), Institut Mines-Télécom [Paris] (IMT)-Institut Mines-Télécom [Paris] (IMT), N00014-17-1-2231, Office of Naval Research, ANR-15-CE05-0018,TRANSHYPERO,Vers une compréhension des propriétés de transport électronique des cellules solaires basées sur les pérovskites hybrides(2015), Université de Rennes (UR)-Institut National des Sciences Appliquées - Rennes (INSA Rennes), Institut National des Sciences Appliquées (INSA)-Institut National des Sciences Appliquées (INSA)-Ecole Nationale Supérieure de Chimie de Rennes (ENSCR)-Institut de Chimie du CNRS (INC)-Centre National de la Recherche Scientifique (CNRS), and Institut National des Sciences Appliquées (INSA)-Institut National des Sciences Appliquées (INSA)-École Nationale Supérieure des Sciences Appliquées et de Technologie (ENSSAT)-Centre National de la Recherche Scientifique (CNRS)
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film stability ,excitons ,diammonium cation ,unconventional semiconductors ,solar cells ,2D perovskite ,[CHIM.MATE]Chemical Sciences/Material chemistry ,light emitting diodes - Abstract
International audience; Low-dimensional halide perovskites have recently attracted intense interest as alternatives to the three-dimensional (3D) perovskites because of their greater tunability and higher environmental stability. Herein, we present the new homologous 2D series (NHC HNH)(CHNH) Pb I ( m = 4-9; n = 1-4), where m represents the carbon-chain number and n equals layer-thickness number. Multilayer ( n > 1) 2D perovskites incorporating diammonium cations were successfully synthesized by the solid-state grinding method for m = 4 and 6 and by the solution method for m = 7-9. Structural characterization by single-crystal X-ray diffraction for the m = 8 and m = 9 series ( n = 1-4) reveals that these compounds adopt the Cc space group for even n members and Pc for odd n members. The optical bandgaps are 2.15 eV for two-layer ( n = 2), 2.01 eV for three-layer ( n = 3), and 1.90 eV for four-layer ( n = 4). The materials exhibit excellent solution processability, and casting thin-films of the n = 3 members was successfully accomplished. The films show a clear tendency for the higher- m members to have preferred orientation on the glass substrate, with m = 8 exhibiting almost perfect vertical layer orientation and m = 9 displaying both vertical and parallel layer orientation, as confirmed by grazing-incidence wide-angle X-ray scattering (GIWAXS) measurements. The vertical layer orientation for the (NHCHNH)(CHNH)PbI member results in the best thermal, light, and air stability within this series, thus showing excellent potential for solar cell applications.
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- 2018
6. Critical role of Interface and perovskite lattice in high-efficiency and photostable solar cells
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Durand, Olivier, Nie, Wanyi, Tsai, Hsinhan, Asadpour, Reza, Blancon, Jean-Christophe, Liu, Fangze, Stoumpos, Constantinos, Strzalka, Joseph, Crochet, Jared, Ajayan, Pulickel, Traoré, Boubacar, Kepenekian, Mikael, Katan, Claudine, Tretiak, Sergei, Kanatzidis, Mercouri, Alam, Muhammad, Even, Jacky, Mohite, Aditya, Institut des Fonctions Optiques pour les Technologies de l'informatiON (Institut FOTON), Université de Rennes 1 (UR1), Université de Rennes (UNIV-RENNES)-Université de Rennes (UNIV-RENNES)-Institut National des Sciences Appliquées - Rennes (INSA Rennes), Institut National des Sciences Appliquées (INSA)-Université de Rennes (UNIV-RENNES)-Institut National des Sciences Appliquées (INSA)-École Nationale Supérieure des Sciences Appliquées et de Technologie (ENSSAT)-Centre National de la Recherche Scientifique (CNRS)-IMT Atlantique Bretagne-Pays de la Loire (IMT Atlantique), Institut Mines-Télécom [Paris] (IMT)-Institut Mines-Télécom [Paris] (IMT), Los Alamos National Laboratory (LANL), Rice University [Houston], Purdue University [West Lafayette], Northwestern University [Evanston], Argonne National Laboratory [Lemont] (ANL), Institut des Sciences Chimiques de Rennes (ISCR), Centre National de la Recherche Scientifique (CNRS)-Institut de Chimie du CNRS (INC)-Université de Rennes 1 (UR1), Université de Rennes (UNIV-RENNES)-Université de Rennes (UNIV-RENNES)-Ecole Nationale Supérieure de Chimie de Rennes (ENSCR)-Institut National des Sciences Appliquées - Rennes (INSA Rennes), Institut National des Sciences Appliquées (INSA)-Université de Rennes (UNIV-RENNES)-Institut National des Sciences Appliquées (INSA), Telluride Science Research Center, Université de Rennes (UR)-Institut National des Sciences Appliquées - Rennes (INSA Rennes), Institut National des Sciences Appliquées (INSA)-Institut National des Sciences Appliquées (INSA)-École Nationale Supérieure des Sciences Appliquées et de Technologie (ENSSAT)-Centre National de la Recherche Scientifique (CNRS), and Institut National des Sciences Appliquées (INSA)-Institut National des Sciences Appliquées (INSA)-Ecole Nationale Supérieure de Chimie de Rennes (ENSCR)-Institut de Chimie du CNRS (INC)-Centre National de la Recherche Scientifique (CNRS)
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[PHYS]Physics [physics] ,solar cells ,halide perovskites ,[SPI.OPTI]Engineering Sciences [physics]/Optics / Photonic ,[CHIM]Chemical Sciences ,Synchrotron X-ray diffraction ,ComputingMilieux_MISCELLANEOUS ,[SPI.MAT]Engineering Sciences [physics]/Materials - Abstract
International audience; Los Alamos National laboratory (LANL) developed an efficient growth procedure for 3D halide perovskites in inverted perovskite cell architecture using PEDOT-PSS as a p-type hole transporting material (HTM). The initial collaboration between FOTON/ISCR and LANL led to the observation of a reversible self-healing mechanism under light soaking and showed that the aging of the precursor solution plays a role in the nucleation of the perovskite crystallites. In this study, we show that growth of methylammonium lead perovskites (MAPbI3) on nickel oxide (NiO) HTM, results in the formation of ordered and crystalline thin-films with enhanced crystallinity, leading to characteristic XRD Bragg peak width reminiscent of exclusively observed in the tetragonal phase in single-crystals.
- Published
- 2018
7. Facile Fabrication of Self‐Assembly Functionalized Polythiophene Hole Transporting Layer for High Performance Perovskite Solar Cells.
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Chang, Chi‐Yuan, Huang, Hsin‐Hsiang, Tsai, Hsinhan, Lin, Shu‐Ling, Liu, Pang‐Hsiao, Chen, Wei, Hsu, Fang‐Chi, Nie, Wanyi, Chen, Yang‐Fang, and Wang, Leeyih
- Subjects
DYE-sensitized solar cells ,SOLAR cells ,SILICON solar cells ,PEROVSKITE ,SEMICONDUCTORS ,INDIUM tin oxide ,POLYTHIOPHENES - Abstract
Crystallinity and crystal orientation have a predominant impact on a materials' semiconducting properties, thus it is essential to manipulate the microstructure arrangements for desired semiconducting device performance. Here, ultra‐uniform hole‐transporting material (HTM) by self‐assembling COOH‐functionalized P3HT (P3HT‐COOH) is fabricated, on which near single crystal quality perovskite thin film can be grown. In particular, the self‐assembly approach facilitates the P3HT‐COOH molecules to form an ordered and homogeneous monolayer on top of the indium tin oxide (ITO) electrode facilitate the perovskite crystalline film growth with high quality and preferred orientations. After detailed spectroscopy and device characterizations, it is found that the carboxylic acid anchoring groups can down‐shift the work function and passivate the ITO surface, retarding the interface carrier recombination. As a result, the device made with the self‐assembled HTM show high open‐circuit voltage over 1.10 V and extend the lifetime over 4,300 h when storing at 30% relative humidity. Moreover, the cell works efficiently under much reduced light power, making it useful as power source under dim‐light conditions. The demonstration suggests a new facile way of fabricating monolayer HTM for high efficiency perovskite devices, as well as the interconnecting layer needed for tandem cell. [ABSTRACT FROM AUTHOR]
- Published
- 2021
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8. Effect of Cation Composition on the Mechanical Stability of Perovskite Solar Cells.
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Rolston, Nicholas, Printz, Adam D., Tracy, Jared M., Weerasinghe, Hasitha C., Vak, Doojin, Haur, Lew Jia, Priyadarshi, Anish, Mathews, Nripan, Slotcavage, Daniel J., McGehee, Michael D., Kalan, Roghi E., Zielinski, Kenneth, Grimm, Ronald L., Tsai, Hsinhan, Nie, Wanyi, Mohite, Aditya D., Gholipour, Somayeh, Saliba, Michael, Grätzel, Michael, and Dauskardt, Reinhold H.
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SOLAR cells ,STABILITY (Mechanics) ,CATIONS ,OPTOELECTRONICS ,COHESION ,FRACTURE toughness ,HARDNESS testing - Abstract
Abstract: Photoactive perovskite semiconductors are highly tunable, with numerous inorganic and organic cations readily incorporated to modify optoelectronic properties. However, despite the importance of device reliability and long service lifetimes, the effects of various cations on the mechanical properties of perovskites are largely overlooked. In this study, the cohesion energy of perovskites containing various cation combinations of methylammonium, formamidinium, cesium, butylammonium, and 5‐aminovaleric acid is reported. A trade‐off is observed between the mechanical integrity and the efficiency of perovskite devices. High efficiency devices exhibit decreased cohesion, which is attributed to reduced grain sizes with the inclusion of additional cations and PbI
2 additives. Microindentation hardness testing is performed to estimate the fracture toughness of single‐crystal perovskite, and the results indicated perovskites are inherently fragile, even in the absence of grain boundaries and defects. The devices found to have the highest fracture energies are perovskites infiltrated into a porous TiO2 /ZrO2 /C triple layer, which provide extrinsic reinforcement and shielding for enhanced mechanical and chemical stability. [ABSTRACT FROM AUTHOR]- Published
- 2018
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9. Understanding Film Formation Morphology and Orientation in High Member 2D Ruddlesden-Popper Perovskites for High-Efficiency Solar Cells.
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Soe, Chan Myae Myae, Nie, Wanyi, Stoumpos, Constantinos C., Tsai, Hsinhan, Blancon, Jean‐Christophe, Liu, Fangze, Even, Jacky, Marks, Tobin J., Mohite, Aditya D., and Kanatzidis, Mercouri G.
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THIN films , *CRYSTAL morphology , *PEROVSKITE , *SOLAR cells , *TWO-dimensional models , *BAND gaps - Abstract
2D Ruddlesden-Popper (RP) perovskites have recently emerged as promising candidates for hybrid perovskite photovoltaic cells, realizing power-conversion efficiencies (PCEs) of over 10% with technologically relevant stability. To achieve solar cell performance comparable to the state-of-the-art 3D perovskite cells, it is highly desirable to increase the conductivity and lower the optical bandgap for enhanced near-IR region absorption by increasing the perovskite slab thickness. Here, the use of the 2D higher member ( n = 5) RP perovskite ( n-butyl-NH3)2(MeNH3)4Pb5I16 in depositing highly oriented thin films from dimethylformamide/dimethylsulfoxide mixtures using the hot-casting method is reported. In addition, they exhibit superior environmental stability over thin films of their 3D counterpart. These films are assembled into high-efficiency solar cells with an open-circuit voltage of ≈1 V and PCE of up to 10%. This is achieved by fine-tuning the solvent ratio, crystal growth orientation, and grain size in the thin films. The enhanced performance of the optimized devices is ascribed to the growth of micrometer-sized grains as opposed to more typically obtained nanometer grain size and highly crystalline, densely packed microstructures with the majority of the inorganic slabs preferentially aligned out of plane to the substrate, as confirmed by X-ray diffraction and grazing-incidence wide-angle X-ray scattering mapping. [ABSTRACT FROM AUTHOR]
- Published
- 2018
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10. Effect of Precursor Solution Aging on the Crystallinity and Photovoltaic Performance of Perovskite Solar Cells.
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Tsai, Hsinhan, Nie, Wanyi, Lin, Yen‐Hao, Blancon, Jean Christophe, Tretiak, Sergei, Even, Jacky, Gupta, Gautam, Ajayan, Pulickel M., and Mohite, Aditya D.
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CRYSTALLINITY , *PHOTOVOLTAIC power systems , *PEROVSKITE , *SOLAR cells , *X-ray diffraction - Abstract
Perovskite materials due to their exceptional photophysical properties are beginning to dominate the field of thin-film optoelectronic devices. However, one of the primary challenges is the processing-dependent variability in the properties, thus making it imperative to understand the origin of such variations. Here, it is discovered that the precursor solution aging time before it is cast into a thin film, is a subtle but a very important factor that dramatically affects the overall thin-film formation and crystallinity and therein factors such as grain growth, phase purity, surface uniformity, trap state density, and overall solar cell performance. It is shown that progressive aging of the precursor promotes efficient formation of larger seeds after the fast nucleation of a large density of small seeds. The hot-casting method then leads to the growth of large grains in uniform thin-films with excellent crystallinity validated using scanning microscopy images and X-ray diffraction patterns. The high-quality films cast from aged solution is ideal for thin-film photovoltaic device fabrication with reduced shunt current and good charge transport. This observation is a significant step toward achieving highly crystalline thin-films with reliability in device performance and establishes the subtle but dramatic effect of solution aging before fabricating perovskite thin-films. [ABSTRACT FROM AUTHOR]
- Published
- 2017
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11. Silver Nanoparticle-Doped Titanium Oxide Thin Films for Intermediate Layers in Organic Tandem Solar Cell.
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Nie, Wanyi, Coffin, Robert C., and Carroll, David L.
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SILVER nanoparticles , *TITANIUM dioxide films , *INTERMEDIATES (Chemistry) , *SOLAR cells , *PHOTOVOLTAIC cells , *CURRENT-voltage curves - Abstract
In this work we investigate the Ag nanoparticle doping of TiOx used as an intermediate layer between subcells of a tandem organic photovoltaic. We use a model polymer cell structure of P3HT:TiOx:PEDOT:P3HT to observe charge-trapping effects as a function of nanoparticle content in the TiOx, as determined by the shape of the dark and illuminated current voltage curves of the devices. There is a direct correlation between the amount ofAg nanoparticles in theTiOx, and interfacial charge buildup, and charge trapping being completely mitigated at around 0.2%mol. This suggests that such doping schemes might provide a simple approach to the creation and use of TiOx layers for tandem cells. [ABSTRACT FROM AUTHOR]
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- 2013
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12. High efficiency organic solar cells with spray coated active layers comprised of a low band gap conjugated polymer.
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Nie, Wanyi, Coffin, Robert C., Liu, Jiwen, Li, Yuan, Peterson, Eric D., MacNeill, Christopher M., Noftle, Ronald E., and Carroll, David L.
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SOLAR cells , *CONJUGATED polymers , *PHOTOVOLTAIC cells , *QUANTUM efficiency , *AIRBRUSHES - Abstract
Airbrush is a promising tool for large scale organic thin film deposition in photovoltaic devices fabrication. This paper reports a detailed study on solar cell performance using airbrush spray deposition for active layer composed with recently developed low band gap donor material poly[4,8-bis(1-pentylhexyloxy)benzo[1,2-b:4,5-b′]dithiophene-2,6-diyl-alt-2,1,3-benzoxadiazole-4,7-diyl and [6,6]-phenyl-C61-butyric acid methyl ester. The effect of carrier solvent and substrate temperature on film morphology are studied; a formula in 1,2-dichlorobenzene sprayed at a substrate temperature of 80 °C is found to be the optimum condition that produces a peak power conversion efficiency of 5.8%. [ABSTRACT FROM AUTHOR]
- Published
- 2012
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13. Thickness dependence of the MoO3 blocking layers on ZnO nanorod-inverted organic photovoltaic devices.
- Author
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Wang, Mingjun, Li, Yuan, Huang, Huihui, Peterson, Eric D., Nie, Wanyi, Zhou, Wei, Zeng, Wei, Huang, Wenxiao, Fang, Guojia, Sun, Nanhai, Zhao, Xingzhong, and Carroll, David L.
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THICK films ,MOLYBDENUM oxides ,PHOTOVOLTAIC cells ,ZINC oxide ,SOLAR cells ,BUTYRIC acid ,ENERGY conversion - Abstract
Organic solar cells based on vertically aligned zinc oxide nanorod arrays (ZNR) in an inverted structure of indium tin oxide (ITO)/ZNR/poly(3-hexylthiophene): (6,6)-phenyl C61 butyric acid methyl ester(P3HT:PCBM)/MoO
3 /aluminum(Al) were studied. We found that the optimum MoO3 layer thickness condition of 20 nm, the MoO3 can effectively decrease the probability of bimolecular recombination either at the Al interface or within the active layer itself. For this optimum condition we get a power conversion efficiency of 2.15%, a short-circuit current density of 9.02 mA/cm2 , an open-circuit voltage of 0.55V, and a fill factor of 0.44 under 100 mW/cm2 irradiation. Our investigations also show that the highly crystallized ZNR can create short and continuous pathways for electron transport and increase the contact area between the ZNR and the organic materials. [ABSTRACT FROM AUTHOR]- Published
- 2011
- Full Text
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14. Single-Crystal Halide Perovskites for Transistor Applications
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Li, Feng, Nie, Wanyi, editor, and Iniewski, Krzysztof (Kris), editor
- Published
- 2023
- Full Text
- View/download PDF
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