1. Tracing the geographic origin of CTC black tea based on colorimetric sensor array response to taste substances combined with chemometrics.
- Author
-
Shen, Jingfei, Li, Tiehan, Chen, Yurong, Zhou, Huan, Dong, Shuai, Wei, Yuming, Li, Feilan, Ning, Jingming, and Li, Luqing
- Subjects
- *
SENSOR arrays , *TASTE , *CHEMOMETRICS , *SUPPORT vector machines , *GALLIC acid - Abstract
The quality of crush–tear–curl black tea (CTC-BT) varies greatly by geographic origin. Origin traceability is crucial for consumer interest protection, market order regulation, and food safety monitoring. This paper proposes a fast and accurate method for qualitative discrimination of CTC-BT origins and quantitative detection of its key taste-presenting substances. The method involves a simple colorimetric sensor array and ultraviolet–visible spectroscopy. The effects of various variable screening methods on modeling results were compared. A particle swarm optimization–based support vector machine achieved the highest performance in qualitative discrimination, with a correct classification rate of 99.48%. Based on their origin-distinguishing contributions and dose-over-thresholds, seven key taste-presenting substances were screened, namely, theaflavin, caffine, vitexin-2- O -rhamnoside, rutin, epigallocatechin gallate, epicatechin gallate, gallic acid. A least squares-support vector regression model achieved accurate quantification of the seven aforementioned compounds (square root of determination coefficient of prediction >0.9698, residual prediction deviation >2). [Display omitted] • A simple method for CTC black tea origin tracing and taste evaluation was developed. • Stable and simplified solution phase-colorimetric sensing array was built. • SG-PSO-SVM model achieved best CCR of 99.48% in origin discrimination. • Taste compounds were screened by origin-distinguishing contributions and thresholds. • Accurate quantification (Rp > 0.9698, RPD>2) of 7 taste compounds were achieved. [ABSTRACT FROM AUTHOR]
- Published
- 2024
- Full Text
- View/download PDF