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Despite the crucial role of the Southern Hemisphere (SH) westerlies in modulating modern and past climate evolution, little is known about their behavior and possible forcing mechanisms during the early Cenozoic. We probe changes in the hydroclimate of southwest Australia during 62–51 Ma, based on sedimentary proxy records from the International Ocean Discovery Program Site U1514 in the Mentelle Basin. Our results reveal a transition from a less humid climate to wetter conditions at mid–high latitudes starting from the early Eocene, which suggests poleward migration of the SH westerlies. This long‐term trend is punctuated by short‐lived events of aridification during the Mid‐Paleocene Biotic Event and wetter intervals during the Paleocene‐Eocene Thermal Maximum, indicating additional short‐term meridional shifting of the westerlies. We propose that the evolution of SH westerlies was driven by the equator‐to‐pole temperature gradient regulated by global warming and ephemeral growth of the Antarctic ice sheet. Plain Language Summary: The Southern Hemisphere (SH) westerlies, which are the dominant atmospheric circulation patterns in the middle latitudes, play a key role in regulating global and regional climate. Currently, the knowledge of past changes in SH westerlies relies mainly on the late Quaternary. Its dynamics over longer timescales, especially under early Cenozoic greenhouse climate states, remain poorly understood. The Mentelle Basin off southwest Australia was located at a more southerly location than at the present day, and was potentially under the influence of SH westerlies. To examine the long‐term hydroclimate changes in southwest Australia during the mid‐late Paleocene to the early Eocene (62–51 Ma), we measured neodymium and hafnium isotopic compositions of fine‐grained detrital sediments from a borehole (IODP Site U1514) drilled in the Mentelle Basin, in addition to clay mineralogy, and elemental abundances. Our results suggest a gradual wetting of southwest Australia since the early Eocene, which we relate to the poleward migration of SH westerlies in response to a reduced latitudinal temperature gradient. An abrupt northward shift of SH westerlies was observed during the short‐lived Middle Paleocene Biotic Event (∼59 Ma), possibly driven by ephemeral growth of the Antarctica ice sheet. Key Points: We reconstruct the hydroclimate evolution of southwest Australia during 62–51 MaThe Southern Hemisphere (SH) westerlies remained relatively stable during the mid‐late Paleocene and shifted poleward since the early EoceneProcesses related to variations of pole‐equator temperature gradients drove meridional migration of the SH westerlies [ABSTRACT FROM AUTHOR]

The Eocene was a critical period of global plate reorganization and it also saw the Earth's climate transition from the warmhouse state to the coolhouse state. Reconstructing the Eocene sedimentary history in the climate-sensitive Southern Ocean is important for understanding paleoenvironmental changes in response to the accelerated Australia/Antarctica separation and global cooling throughout the middle and late Eocene. Here, we present the first detailed multiproxy record of a continuous sequence from International Ocean Discovery Program (IODP) Site U1514 in the Mentelle Basin off southwestern Australia. Our aim is to reconstruct the sediment provenances and paleoenvironmental evolution in response to the abovementioned climatic and tectonic changes in the mid-high southern latitudes during the Eocene. Provenance analyses based on Sr-Nd isotopes, trace elements, and clay mineral assemblages suggest that Eocene sediments at Site U1514 predominantly originated from the southwestern Australian continent and the Naturaliste Plateau. Sediment provenance variations during the middle Eocene indicate that the onset of fast separation between Australia and Antarctica at 43 Ma caused an increased supply of volcanic materials from the Naturaliste Plateau between 43 and 38 Ma. Terrigenous inputs to the Mentelle Basin during the middle Eocene were primarily controlled by paleoclimate changes rather than tectonic processes because coeval clay mineralogical changes (higher kaolinite/smectite ratio and MAR kaolinite) indicate a period of stronger physical erosion and chemical weathering on the western Australian continent that resulted in increased terrigenous materials delivered to the Mentelle Basin. Our results reveal a 5 Myr-long (43–38 Ma) warming reversal in the southern mid-high latitudes, providing an exception to the generally short-lived (10–100 kyr-long) hyperthermals that interrupted the long-term global cooling throughout the middle to late Eocene. As for the late Eocene (38–37 Ma), tectonic processes related to the sudden acceleration in seafloor spreading in the Tasman Sea led to the exposure of shallower areas, resulting in rapid detritus accumulation at the study site. During the late Eocene (37–34 Ma), major sediment provenance shifted from distal source areas (e.g., the Yilgarn Craton) to relatively proximal sources (e.g., the Leeuwin Block and Perth Basin). We interpret that the regional uplift in southwestern Australia and coeval climate cooling resulted in the diversion and inactivation of large drainage systems, thus blocking the transportation of sediment from distant regions. • First detailed record of the Eocene source-to-sink process in the Mentelle Basin. • The onset of fast Australia/Antarctica separation caused increased volcanic input. • Regional warming led to enhanced chemical weathering in Australia during 43–38 Ma. • Regional uplift and global cooling induced sediment source change during 37–34 Ma. [ABSTRACT FROM AUTHOR]