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Urban trees store and sequester large amounts of carbon and are a vital component of natural climate solutions. Despite the well-recognized carbon benefits of urban trees, there is limited effort to examine how spatial distribution of carbon density varies across distinctive social, demographic, and built dimensions of urban landscapes. Moreover, it is unclear whether specific aspects of landscape structure and design could help increase carbon densities in urban trees. Here, we produced a fine-resolution carbon density map of urban trees in New York City (NYC) by integrating high-resolution land cover map, LiDAR-derived tree metrics, i-Tree Eco, and field survey data. We then explored spatial variations of carbon density across the gradients of urban development intensity, social deprivation index, and neighborhood age, and we examined the relationships between carbon density, and fragmentation, aggregation, size, and shape of tree canopy cover. We find that carbon stored in urban trees in NYC is estimated as 1078 Gg, with an average density of 13.8 Mg/ha. This large amount of carbon is unevenly distributed, with carbon densities being highest in Bronx and in open parks and street trees. Furthermore, carbon densities are negatively associated with urban development intensity and the social gradient of deprivation. Regarding the impacts of tree morphology on carbon density, our results show that while the amount of tree cover is the most influential factor in determining carbon density, small-sized forest patches and moderate levels of forest edges are also conductive to increasing carbon densities of urban trees. To incorporate urban forestry into developing innovative, effective, and equitable climate mitigation strategies, planners and decision makers need to identify the optimal spatial configuration of urban forests and invest in tree planting programs in marginalized communities. • Carbon density in urban trees in New York City is estimated as 13.8 Mg/ha. • Socially deprived areas are associated with lower carbon densities. • Small-sized forest patches and moderate levels of forest edges are beneficial to increase carbon densities of urban trees. • The findings provide implications to incorporate urban forestry to develop effective and equitable climate mitigation strategies. [ABSTRACT FROM AUTHOR]