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We analysed the variability of equivalent black carbon (BC) and ozone (O3) at the global WMO/GAW station Nepal Climate Observatory-Pyramid (NCO-P, 5079 m a.s.l.) in the southern Himalayas, for evaluating the possible contribution of open vegetation fires to the variability of these short-lived climate forcers/pollutants (SLCF/SLCP) in the Himalayan region. We found that 162 days (9% of the data-set) were characterised by acute pollution events with enhanced BC and O3 in respect to the climatological values. By using satellite observations (MODIS fire products and the USGS Land Use Cover Characterization) and air mass back-trajectories, we deduced that 56% of these events were likely to be affected by emissions from open fires along the Himalayas foothills, the Indian Subcontinent and the Northern Indo-Gangetic Plain. These results suggest that open fire emissions are likely to play an important role in modulating seasonal and inter-annual BC and O3 variability over south Himalayas. [Copyright &y& Elsevier]

To study the influence of polluted air-mass transport carrying ozone (O 3 ) and black carbon (BC) in the high Himalayas, since March 2006 the Nepal Climate Observatory at Pyramid (NCO-P) GAW-WMO global station (Nepal, 5079 m a.s.l.) is operative. During the first 5-year measurements, the O 3 and BC concentrations have shown a mean value of 48 ± 12 ppb (± standard deviation) and 208 ± 374 ng/m 3 , respectively. Both O 3 and BC showed well defined seasonal cycles with maxima during pre-monsoon (O 3 : 61.3 ± 7.7 ppbV; BC: 444 ± 433 ng/m 3 ) and minima during the summer monsoon (O 3 : 40.1 ± 12.4 ppbV; BC: 64 ± 101 ng/m 3 ). The analysis of the days characterised by the presence of a significant BC increase with respect to the typical seasonal cycle identified 156 days affected by “acute” pollution events, corresponding to 9.1% of the entire data-set. Such events mostly occur in the pre-monsoon period, when the O 3 diurnal variability is strongly related to the transport of polluted air-mass rich on BC. On average, these “acute” pollution events were characterised by dramatic increases of BC (352%) and O 3 (29%) levels compared with the remaining days. [ABSTRACT FROM AUTHOR]