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Ozone (O3) pollution has negative impacts on human health and property. The Guangdong–Hong Kong–Macao Greater Bay Area (GBA) is facing severe O3 pollution problems due to rapid economic development. In this paper, we used sensitivity experiments and GeoDetector to analyze the effects of meteorological factors, anthropogenic emissions, and landscape patterns on O3 concentrations as well as the contributions of NOx and NMVOC (non-methane volatile organic compounds) to the variation of O3 concentrations and the causes of sectoral emissions in the GBA in 2017. The results revealed that, in GBA, the contribution of meteorology to the variation of O3 concentration was dominant both in terms of region and extent, and the contribution of emissions was relatively weak. The contribution of meteorology and emissions to O3 production was mainly contributory. Meteorology contributed significantly to O3, and its non-linear interaction with anthropogenic emissions and surface landscape affected O3 concentration changes. The degree of contribution of NOx and NMVOC varied widely among seasons, and the variation of their relative contribution areas was related to residential sector emissions and agricultural sector emissions. This article enriches the exploration of the O3 formation mechanism in the GBA and provides theoretical support for the implementation of differentiated regional and seasonal mitigation strategies for O3 concentration. [ABSTRACT FROM AUTHOR]