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To investigate the impact of combining aluminum sulfate with straw and irrigation water to enhance soil quality in soda saline–alkali soil, in this study a field experiment was conducted in Tongliao City, Inner Mongolia Autonomous Region, China. With beet IM1162 as the indicator crop, four levels of aluminum sulfate dosage (30, 60, 90, 120 g m−2) and four levels of drip irrigation water quota (225, 270, 315, 360 m3 ha−1) were set. The study examined the impact of varying levels of aluminum sulfate and irrigation water on soil water salt and crop yield. Next, using a comprehensive evaluation method, the optimal quantities of aluminum sulfate and irrigation water needed for effective soil improvement were determined. The research findings indicate that the most effective treatment (W2S3) involved an aluminum sulfate dosage of 90 g m−2 and an irrigation quota of 270 m3 ha−1. This treatment resulted in significant improvements compared to the control (CK) group. Specifically, in the 0–50 cm soil layer, the following improvements were observed: the water storage capacity (SWS) increased by 51.7%; evapotranspiration (ET) increased by 16.2%; water use efficiency (WUE) increased by 55.0%; and irrigation water use efficiency (IWUE) increased by 98.1% (p < 0.05). These results emphasize the importance of optimizing the combination of aluminum sulfate dosage and irrigation water quota to improve soil conditions and crop performance. It is worth nothing that this study highlights the potential for enhancing water use efficiency and crop yield in agricultural practices, which can contribute to sustainable and efficient farming practices. The study results revealed significant improvements in soil quality and crop yield when compared to the control group (CK). Specifically, in the 0–50 cm soil layer: the soil salt content decreased by 19.8%, soil pH increased by 8.7%, and exchangeable sodium percentage (ESP) decreased by 34.0%. Moreover, the crop yield in the treatment group increased significantly, by 32.1%. These findings indicate the positive impact of the intervention on soil health and agricultural productivity. The study employed the game theory combination weighting method to comprehensively evaluate soil water, salt, and various yield indicators. The results showed that the sustainability weight for crop yield reached 0.116, emphasizing the aim of soil improvement: the sustainable enhancement of crop yield. This approach underscores the importance of balanced soil management practices to ensure long-term agricultural productivity and environmental sustainability. The comprehensive evaluation results of grey relation analysis and the TOPSIS coupling model showed that the soil improvement effect score was the highest when the dosage of aluminum sulfate was 61.7–120.0 g m−2, and the irrigation quota was 250.4–319.4 m3 ha−1, which was the recommended range for the local area. The research findings discussed in the provided sources contribute to the theoretical basis for soil improvement in soda–saline–alkali land. [ABSTRACT FROM AUTHOR]