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Snowfall is critical in the mountainous cryosphere cycle and is vulnerable to climate change. Due to data-scarcity and strong surface heterogeneity, its information is not sufficiently revealed across the Third Pole (TP) under warming. Accordingly, this study investigated the spatiotemporal variability of snowfall and its entropy information across the TP from 1980 to 2020 based on a new high-accuracy snowfall dataset (TPHiS), which was estimated from a long-term high-resolution precipitation dataset for the TP (TPHiPr) and High Asia Refined analysis version 2 reanalysis data (HARv2) using a threshold temperature method. The results indicated that the correlation coefficient, mean bias, and root-mean-square error of the daily TPHiS were 0.77, 0.03 mm/daily, and 0.18 mm/daily, respectively, compared against in-situ observation, illustrating that this dataset performs better than other snowfall datasets. The annual mean snowfall measured 259.38 mm across the TP and experienced a slight negative trend (−0.77 mm/decade, p > 0.05). A significantly positive trend in annual snowfall was observed in the intersection of the West Kunlun, Karakoram, and Western Inner Tibet, with elevations over 5500 m. In contrast, a significantly negative trend prevailed in the Pamir, Hengduan Shan, and West and Central Himalaya intersections, especially at elevations varied from 3000 to 4500 m. Compared with other seasons, a significantly negative trend in snowfall was observed in summer (−1.94 mm/decade, p < 0.05). Change in snowfall frequency entropy was more significant than that in snowfall amount entropy. A significantly positive trend in light snowfall frequency dominated the augmentation in snowfall frequency, causing a negative trend in snowfall frequency entropy, while a substantial reduction in snowfall frequency associated with the decline in light snowfall frequency induced a positive trend in snowfall frequency entropy. The outcomes provide a finer snowfall dataset for regional cryospheric research and might inform sustainable water resource management in alpines. • A new daily snowfall dataset (TPHiS) covering the TP was estimated from the TPHiPr precipitation and HARv2 reanalysis dataset using a threshold temperature method. • The daily TPHiS (CC = 0.77, MB = 0.03 mm/daily, and RMSE = 0.18 mm/daily) performed better than other snowfall datasets. • The annual mean snowfall measured 259.38 mm across the TP, and summer snowfall exhibited a significantly negative trend (-1.94 mm/decade, p < 0.05). [ABSTRACT FROM AUTHOR]