1. Greatly amplified spontaneous emission of colloidal quantum dots mediated by a dielectric-plasmonic hybrid nanoantenna.
- Author
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Yang, Guoce, Niu, Yijie, Wei, Hong, Bai, Benfeng, and Sun, Hong-Bo
- Subjects
SEMICONDUCTOR nanocrystals ,SURFACE plasmons ,ELECTROMAGNETIC waves ,SUBSTRATE integrated waveguides ,METAL quenching ,ENERGY harvesting ,OPTICAL losses ,QUANTUM dots - Abstract
Optical nanoantennas can efficiently harvest electromagnetic energy from nanoscale space and boost the local radiation to the far field. The dielectric-metal nanogap is a novel design that can help to overcome the core issue of optical loss in all-metal nanostructures while enabling photon density of states larger than that in all-dielectric counterparts. This article reports that a crystalline spherical silicon nanoparticle on metal film (SiNPoM) nanoantenna can largely enhance the spontaneous emission intensity of quantum dots by an area-normalized factor of 69 and the decay rate by 42-fold compared with quantum dots on glass. A high total quantum efficiency of over 80%, including ~20% for far-field radiation and ~60% for surface plasmon polaritons, is obtained in simulation. Thanks to not only the low optical loss in dielectric nanoparticles but also the appropriate gap thickness which weakens the non-radiative decay due to the quenching from metal. Mie resonant modes additionally provide the flexible control of far-field emission patterns. Such a simple optical nanoantenna can be combined with various nanoscale optical emitters and easily extended to form large area metasurfaces functioning as active regions in light-emitting devices in applications such as advanced display, wireless optical communication, and quantum technology. [ABSTRACT FROM AUTHOR]
- Published
- 2019
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