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Measurements of water vapor and clouds in the polar regions are difficult, because conventional instruments show little sensitivity (∼1.3 K/mm) to low amounts. On the other hand, millimeter- and submillimeter-wavelength radiometry offers greatly enhanced sensitivity (up to 51.4 K/mm, depending upon frequency). For this reason, the National Oceanic and Atmospheric Administration's Physical Science Division designed a new instrument, the Ground-Based Scanning Radiometer (GSR), for continuous and unattended observations at millimeter and submillimeter wavelengths (50-380 GHz). The GSR was deployed for the first time during the Arctic winter radiometric experiment in March-April 2004. In this paper, we discuss the GSR calibration procedure, which allows for accurate measurements during clear and cloudy skies. Error-budget analysis and comparison with independent measurements show an absolute accuracy on the order of 1-2 K. Examples of multifrequency and multiangle GSR observations are illustrated, representing a valuable new data set for the study of water vapor, clouds, and atmospheric absorption models in the Arctic. [ABSTRACT FROM AUTHOR]