1. Size spectra and source apportionment of fine particulates in tropical urban environment during southwest monsoon season.
- Author
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Zong Y, Botero ML, Yu LE, and Kraft M
- Subjects
- Atmosphere analysis, Dust analysis, Humans, Particle Size, Seasons, Singapore, Tropical Climate, Air Pollutants analysis, Air Pollution analysis, Environmental Monitoring methods, Particulate Matter analysis, Vehicle Emissions analysis
- Abstract
In this study, we carried out high time-resolution measurements of particle number concentration and size distribution (5-1000 nm) in Singapore, which represents a tropical urban environment. The measurements were taken during the southwest monsoon season in 2017 using a fast-response differential mobility spectrometer at a sampling rate of 1 Hz. In the measurement, short-lived nucleation events were found prominent at early afternoon because of the abundant incoming radiation that enhances the photochemical reactions in atmosphere. For the first time in the region, a five-factor positive matrix factorization approach was applied to the size spectra data. Based on particle number concentration, two sources within nucleation mode (<30 nm) were resolved and account for 43% of total number concentration, which is higher than the available monitoring data in other big cities. Among the sources, O
3 -related atmospheric photochemical reactions with peak size at 10-12 nm is a unique factor and prominent in early afternoon nucleation events. The findings of this work can serve as a baseline for assessing influence of local and cross-border airborne emissions during various seasons in the future., (Copyright © 2018 Elsevier Ltd. All rights reserved.)- Published
- 2019
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