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Urban forests have important functions to alleviate air pollution, adjust the regional climate, and promote visitors' mental health and well-being. Humans' perceptions towards both atmospheric particulate matter (PM) and meteorological factors can be a gauge for assessing the functional services of urban forests. The geographical locations of host cities experiencing urbanization could take part in effects on emotional states of forest visitors. In this study, a total of 6309 facial photos of urban forest visitors were obtained from social networks in 42 cities of mainland China. Happy, sad, and neutral emotions were rated as percent scores in 2020, when the same-day air pollutants, meteorological factors, and socioeconomic indicators were recorded. The positive emotional index (PEI) was calculated as the difference between happy scores and sad scores. The results reveal that severe air pollutants (jointly PM2.5 > 75 μg/m3, PM10 > 150 μg/m3, and AQI > 150) were more frequently found in cities in the northeastern and northern areas of China. The forest visitors in the northeastern cities showed higher happiness scores compared to the visitors in other regions. The Quasi-Poisson regression suggested that high scores of happiness were frequently disclosed in weathers with low PM10. High scores of sadness were regressed on exposure to cities with a low GDP per capita and low total retail sales but with a high GDP at low-longitudinal and high-latitudinal locations with low levels of PM2.5 pollution, relative humidity, and wind velocity and a high temperature. The happiness score and PEI showed high-value aggregations in mega-sized cities (population over 10 million), such as Beijing and Zhengzhou, and in a metro-sized city (population of 5–10 million in Langfang) from climate regions of China. [ABSTRACT FROM AUTHOR]