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The rapid advancement of deep learning has facilitated the automated processing of electron microscopy (EM) big data stacks. However, designing a framework that eliminates manual labeling and adapts to domain gaps remains challenging. Current research remains entangled in the dilemma of pursuing complete automation while still requiring simulations or slight manual annotations. Here we demonstrate tandem generative adversarial network (tGAN), a fully label-free and simulation-free pipeline capable of generating EM images for computer vision training. The tGAN can assimilate key features from new data stacks, thus producing a tailored virtual dataset for the training of automated EM analysis tools. Using segmenting nanoparticles for analyzing size distribution of supported catalysts as the demonstration, our findings showcased that the recognition accuracy of tGAN even exceeds the manually-labeling method by 5%. It can also be adaptively deployed to various data domains without further manual manipulation, which is verified by transfer learning from HAADF-STEM to BF-TEM. This generalizability may enable it to extend its application to a broader range of imaging characterizations, liberating microscopists and materials scientists from tedious dataset annotations.

Federated Learning (FL) has increasingly been recognized as an innovative and secure distributed model training paradigm, aiming to coordinate multiple edge clients to collaboratively train a shared model without uploading their private datasets. The challenge of encouraging mobile edge devices to participate zealously in FL model training procedures, while mitigating the privacy leakage risks during wireless transmission, remains comparatively unexplored so far. In this paper, we propose a novel approach, named QI-DPFL (Quality-Aware and Incentive-Boosted Federated Learning with Differential Privacy), to address the aforementioned intractable issue. To select clients with high-quality datasets, we first propose a quality-aware client selection mechanism based on the Earth Mover's Distance (EMD) metric. Furthermore, to attract high-quality data contributors, we design an incentive-boosted mechanism that constructs the interactions between the central server and the selected clients as a two-stage Stackelberg game, where the central server designs the time-dependent reward to minimize its cost by considering the trade-off between accuracy loss and total reward allocated, and each selected client decides the privacy budget to maximize its utility. The Nash Equilibrium of the Stackelberg game is derived to find the optimal solution in each global iteration. The extensive experimental results on different real-world datasets demonstrate the effectiveness of our proposed FL framework, by realizing the goal of privacy protection and incentive compatibility., Comment: To be published in IJCNN 2024

We report on the development and performance evaluation of an ultra-stable clock laser for an $\rm ^{27}Al^+$ optical clock. The thermal noise limited ultra-stable laser is developed based on a 30 cm long ultra-stable cavity. Three independent evaluation methods, including the frequency noise summation method, the three-cornered hat (TCH) method, and the optical clock transition detection method, are used to evaluate the clock laser performance. The summation result of various frequency noise terms is compared with the result of the TCH method. In addition, the $\rm ^{27}Al^+$ ion optical clock transition with ultra-narrow linewidth is also used to detect the frequency noise of the laser at lower Fourier frequencies. The results of the three methods show good agreements, showing a frequency instability level of $1.3\times10^{-16}$, and giving us confidence that these evaluation methods may provides guidance for accurate evaluations of high stability laser sources.

Federated Learning (FL) has emerged as a crucial distributed training paradigm, enabling discrete devices to collaboratively train a shared model under the coordination of a central server, while leveraging their locally stored private data. Nonetheless, the non-independent-and-identically-distributed (Non-IID) data generated on heterogeneous clients and the incessant information exchange among participants may significantly impede training efficacy, retard the model convergence rate and increase the risk of privacy leakage. To alleviate the divergence between the local and average model parameters and obtain a fast model convergence rate, we propose an adaptive FEDerated learning algorithm called FedAgg by refining the conventional stochastic gradient descent (SGD) methodology with an AGgregated Gradient term at each local training epoch and adaptively adjusting the learning rate based on a penalty term that quantifies the local model deviation. To tackle the challenge of information exchange among clients during local training and design a decentralized adaptive learning rate for each client, we introduce two mean-field terms to approximate the average local parameters and gradients over time. Through rigorous theoretical analysis, we demonstrate the existence and convergence of the mean-field terms and provide a robust upper bound on the convergence of our proposed algorithm. The extensive experimental results on real-world datasets substantiate the superiority of our framework in comparison with existing state-of-the-art FL strategies for enhancing model performance and accelerating convergence rate under IID and Non-IID datasets.

Federated Learning (FL) has emerged as a prominent distributed machine learning framework that enables geographically discrete clients to train a global model collaboratively while preserving their privacy-sensitive data. However, due to the non-independent-and-identically-distributed (Non-IID) data generated by heterogeneous clients, the performances of the conventional federated optimization schemes such as FedAvg and its variants deteriorate, requiring the design to adaptively adjust specific model parameters to alleviate the negative influence of heterogeneity. In this paper, by leveraging entropy as a new metric for assessing the degree of system disorder, we propose an adaptive FEDerated learning algorithm based on ENTropy theory (FedEnt) to alleviate the parameter deviation among heterogeneous clients and achieve fast convergence. Nevertheless, given the data disparity and parameter deviation of heterogeneous clients, determining the optimal dynamic learning rate for each client becomes a challenging task as there is no communication among participating clients during the local training epochs. To enable a decentralized learning rate for each participating client, we first introduce the mean-field terms to estimate the components associated with other clients' local parameters. Furthermore, we provide rigorous theoretical analysis on the existence and determination of the mean-field estimators. Based on the mean-field estimators, the closed-form adaptive learning rate for each client is derived by constructing the Hamilton equation. Moreover, the convergence rate of our proposed FedEnt is proved. The extensive experimental results on the real-world datasets (i.e., MNIST, EMNIST-L, CIFAR10, and CIFAR100) show that our FedEnt algorithm surpasses FedAvg and its variants (i.e., FedAdam, FedProx, and FedDyn) under Non-IID settings and achieves a faster convergence rate., Comment: 16 pages, 13 figures

We report precision measurement of aluminum atoms ${^{2}P_{1/2}}-{^{2}S_{1/2}}$ transition at 394 nm and ${^{2}P_{3/2}}-{^{2}S_{1/2}}$ transition at 396 nm in a hollow-cathode lamp (HCL). Both absorption spectroscopy and saturated absorption spectroscopy (SAS) are performed. From the absorption spectroscopy the Doppler linewidth is estimated to be 2.6 GHz. The SAS spectroscopy is analyzed based on the velocity-changing-effect model. With a frequency comb calibrated wavemeter, the frequencies of ${^{2}P_{1/2}},{F=3}-{^{2}S_{1/2}},{F=2}$ transition and ${^{2}P_{3/2}},{F=4}-{^{2}S_{1/2}},{F=3}$ transition are measured to be 759.905401(10) THz and 756.547403(10) THz, respectively. The hyperfine structure constants of aluminum atoms are determined and compared with previously reported measurement results and theoretical calculation. Reasonable agreement is found for the magnetic dipole constant (A constant), while the electric quadrupole constant (B constant) has a large deviation., Comment: 11 pages, 5 figures