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We report anisotropic magnetoresistance in Pt|Y3Fe5O12 bilayers. In spite of Y3Fe5O12 being a very good electrical insulator, the resistance of the Pt layer reflects its magnetization direction. The effect persists even when a Cu layer is inserted between Pt and Y3Fe5O12, excluding the contribution of induced equilibrium magnetization at the interface. Instead, we show that the effect originates from concerted actions of the direct and inverse spin Hall effects and therefore call it "spin Hall magnetoresistance.", Comment: 20 pages, 7 figures (including Supplemental Material)

Path entanglement constitutes an essential resource in quantum information and communication protocols. Here, we demonstrate frequency-degenerate entanglement between continuous-variable quantum microwaves propagating along two spatially separated paths. We combine a squeezed and a vacuum state using a microwave beam splitter. Via correlation measurements, we detect and quantify the path entanglement contained in the beam splitter output state. Our experiments open the avenue to quantum teleportation, quantum communication, or quantum radar with continuous variables at microwave frequencies., Comment: 16 pages, 14 figures

For gradiometric three-Josephson-junction flux qubits, we perform a systematic study on the tuning of the minimal transition frequency, the so-called qubit gap. By replacing one of the qubit's Josephson junctions by a dc SQUID, the critical current of this SQUID and, in turn, the qubit gap can be tuned in situ by a control flux threading the SQUID loop. We present spectroscopic measurements demonstrating a well-defined controllability of the qubit gap between zero and more than 10 GHz. In the future, this enables one to tune the qubit into and out of resonance with other superconducting quantum circuits, while operating the qubit at its symmetry point with optimal dephasing properties. The experimental data agree very well with model calculations based on the full qubit Hamiltonian. From a numerical fit, we determine the Josephson coupling and the charging energies of the qubit junctions. The derived values agree well with those measured for other junctions fabricated on the same chip. We also demonstrate the biasing of gradiometric flux qubits near the symmetry point by trapping an odd number of flux quanta in the gradiometer loop. In this way, we study the effect of the significant kinetic inductance, thereby obtaining valuable information for the qubit design., Comment: 23 pages, 9 figures

We present an extensive experimental and theoretical study of surface acoustic wave-driven ferromagnetic resonance. In a first modeling approach based on the Landau-Lifshitz-Gilbert equation, we derive expressions for the magnetization dynamics upon magnetoelastic driving that are used to calculate the absorbed microwave power upon magnetic resonance as well as the spin current density generated by the precessing magnetization in the vicinity of a ferromagnet/normal metal interface. In a second modeling approach, we deal with the backaction of the magnetization dynamics on the elastic wave by solving the elastic wave equation and the Landau-Lifshitz-Gilbert equation selfconsistently, obtaining analytical solutions for the acoustic wave phase shift and attenuation. We compare both modeling approaches with the complex forward transmission of a LiNbO$_3$/Ni surface acoustic wave hybrid device recorded experimentally as a function of the external magnetic field orientation and magnitude, rotating the field within three different planes and employing three different surface acoustic wave frequencies. We find quantitative agreement of the experimentally observed power absorption and surface acoustic wave phase shift with our modeling predictions using one set of parameters for all field configurations and frequencies., Comment: 13 pages, 9 figures

In this work we show that a tunable coupling between microwave resonators can be engineered by means of simple Josephson junctions circuits, such as dc- and rf-SQUIDs. We show that by controlling the time dependence of the coupling it is possible to switch on and off and modulate the cross-talk, boost the interaction towards the ultrastrong regime, as well as to engineer red and blue sideband couplings, nonlinear photon hopping and classical gauge fields. We discuss how these dynamically tunable superconducting circuits enable key applications in the fields of all optical quantum computing, continuous variable quantum information and quantum simulation - all within the reach of state of the art in circuit-QED experiments., Comment: 11 pages, 4 figures

We show that the resonant coupling of phonons and magnons can be exploited to generate spin currents at room temperature. Surface acoustic wave (SAW) pulses with a frequency of 1.55 GHz and duration of 300 ns provide coherent elastic waves in a ferromagnetic thin film/normal metal (Co/Pt) bilayer. We use the inverse spin Hall voltage in the Pt as a measure for the spin current and record its evolution as a function of time and external magnetic field magnitude and orientation. Our experiments show that a spin current is generated in the exclusive presence of a resonant elastic excitation. This establishes acoustic spin pumping as a resonant analogue to the spin Seebeck effect., Comment: New Appendix, minor revisions to main text

We study the validity and limitations of a macrospin model to describe the voltage-controlled manipulation of ferromagnetic magnetization in nickel thin film/piezoelectric actuator hybrid structures. To this end, we correlate simultaneously measured spatially resolved magneto-optical Kerr effect imaging and integral magnetotransport measurements at room temperature. Our results show that a macrospin approach is adequate to model the magnetoresistance as a function of the voltage applied to the hybrid, except for a narrow region around the coercive field - where the magnetization reorientation evolves via domain effects. Thus, on length scales much larger than the typical magnetic domain size, the voltage control of magnetization is well reproduced by a simple Stoner-Wohlfarth type macrospin model.

Superconducting qubits acting as artificial two-level atoms allow for controlled variation of the symmetry properties which govern the selection rules for single and multiphoton excitation. We spectroscopically analyze a superconducting qubit-resonator system in the strong coupling regime under one- and two-photon driving. Our results provide clear experimental evidence for the controlled transition from an operating point governed by dipolar selection rules to a regime where one- and two-photon excitations of the artificial atom coexist. We find that the vacuum coupling between qubit and resonator can be straightforwardly extracted from the two-photon spectra where the detuned two-photon drive does not populate the relevant resonator mode significantly., Comment: 8 pages, 5 figures

We report on the study of the Fermi surface of the electron-doped cuprate superconductor Nd$_{2-x}$Ce$_x$CuO$_{4}$ by measuring the interlayer magnetoresistance as a function of the strength and orientation of the applied magnetic field. We performed experiments in both steady and pulsed magnetic fields on high-quality single crystals with Ce concentrations of $x=0.13$ to 0.17. In the overdoped regime of $x > 0.15$ we found both semiclassical angle-dependent magnetoresistance oscillations (AMRO) and Shubnikov-de Haas (SdH) oscillations. The combined AMRO and SdH data clearly show that the appearance of fast SdH oscillations in strongly overdoped samples is caused by magnetic breakdown. This observation provides clear evidence for a reconstructed multiply-connected Fermi surface up to the very end of the overdoped regime at $x\simeq 0.17$. The strength of the superlattice potential responsible for the reconstructed Fermi surface is found to decrease with increasing doping level and likely vanishes at the same carrier concentration as superconductivity, suggesting a close relation between translational symmetry breaking and superconducting pairing. A detailed analysis of the high-resolution SdH data allowed us to determine the effective cyclotron mass and Dingle temperature, as well as to estimate the magnetic breakdown field in the overdoped regime., Comment: 23 pages, 8 figures

We systematically measured the DC voltage V_ISH induced by spin pumping together with the inverse spin Hall effect in ferromagnet/platinum bilayer films. In all our samples, comprising ferromagnetic 3d transition metals, Heusler compounds, ferrite spinel oxides, and magnetic semiconductors, V_ISH invariably has the same polarity. V_ISH furthermore scales with the magnetization precession cone angle with a universal prefactor, irrespective of the magnetic properties, the charge carrier transport mechanism or type. These findings quantitatively corroborate the present theoretical understanding of spin pumping in combination with the inverse spin Hall effect.

Superconducting circuit quantum electrodynamics experiments with propagating microwaves require devices acting as beam splitters. Using niobium thin films on silicon and sapphire substrates, we fabricated superconducting 180{\deg} microstrip hybrid ring couplers, acting as beam splitters with center frequencies of about 6GHz. For the magnitude of the coupling and isolation we find -3.5+/-0.5dB and at least -15dB, respectively, in a bandwidth of 2GHz. We also investigate the effect of reflections at the superconductor-normal conductor contact by means of low temperature laser scanning microscopy. Our measurements show that our hybrid rings are well suited for on-chip applications in circuit quantum electrodynamics experiments.

We report on semiclassical angle-dependent magnetoresistance oscillations (AMRO) and the Shubnikov-de Haas effect in the electron-overdoped cuprate superconductor Nd$_{2-x}$Ce$_x$CuO$_4$. Our data provide convincing evidence for magnetic breakdown in the system. This shows that a reconstructed multiply-connected Fermi surface persists, at least at strong magnetic fields, up to the highest doping level of the superconducting regime. Our results suggest an intimate relation between translational symmetry breaking and the superconducting pairing in the electron-doped cuprate superconductors., Comment: 5 pages, 4 figures, submitted to PRL

We report on the fabrication of Nb/AlO_x/Pd_{0.82}Ni_{0.18}/Nb superconductor/insulator/ferromagnetic metal/superconductor (SIFS) Josephson junctions with high critical current densities, large normal resistance times area products, high quality factors, and very good spatial uniformity. For these junctions a transition from 0- to \pi-coupling is observed for a thickness d_F ~ 6 nm of the ferromagnetic Pd_{0.82}Ni_{0.18} interlayer. The magnetic field dependence of the \pi-coupled junctions demonstrates good spatial homogeneity of the tunneling barrier and ferromagnetic interlayer. Magnetic characterization shows that the Pd_{0.82}Ni_{0.18} has an out-of-plane anisotropy and large saturation magnetization, indicating negligible dead layers at the interfaces. A careful analysis of Fiske modes provides information on the junction quality factor and the relevant damping mechanisms up to about 400 GHz. Whereas losses due to quasiparticle tunneling dominate at low frequencies, the damping is dominated by the finite surface resistance of the junction electrodes at high frequencies. High quality factors of up to 30 around 200 GHz have been achieved. Our analysis shows that the fabricated junctions are promising for applications in superconducting quantum circuits or quantum tunneling experiments., Comment: 15 pages, 9 figures

We use a correlation function analysis of the field quadratures to characterize both the black body radiation emitted by a 50 Ohm load resistor and the quantum properties of two types of beam splitters in the microwave regime. To this end, we first study vacuum fluctuations as a function of frequency in a Planck spectroscopy experiment and then measure the covariance matrix of weak thermal states. Our results provide direct experimental evidence that vacuum fluctuations represent the fundamental minimum quantum noise added by a beam splitter to any given input signal., Comment: 5 pages, 4 figures

In cavity quantum electrodynamics (QED), light-matter interaction is probed at its most fundamental level, where individual atoms are coupled to single photons stored in three-dimensional cavities. This unique possibility to experimentally explore the foundations of quantum physics has greatly evolved with the advent of circuit QED, where on-chip superconducting qubits and oscillators play the roles of two-level atoms and cavities, respectively. In the strong coupling limit, atom and cavity can exchange a photon frequently before coherence is lost. This important regime has been reached both in cavity and circuit QED, but the design flexibility and engineering potential of the latter allowed for increasing the ratio between the atom-cavity coupling rate and the cavity transition frequency above the percent level. While these experiments are well described by the renowned Jaynes-Cummings model, novel physics is expected in the ultrastrong coupling limit. Here, we report on the first experimental realization of a superconducting circuit QED system in the ultrastrong coupling limit and present direct evidence for the breakdown of the Jaynes-Cummings model., Comment: 5 pages, 3 figures

Quantum state reconstruction involves measurement devices that are usually described by idealized models, but not known in full detail in experiments. For weak propagating microwaves, the detection process requires linear amplifiers which obscure the signal with random noise. Here, we introduce a theory which nevertheless allows one to use these devices for measuring all quadrature moments of propagating quantum microwaves based on cross-correlations from a dual-path amplification setup. Simultaneously, the detector noise properties are determined, allowing for tomography. We demonstrate the feasibility of our novel concept by proof-of-principle experiments with classical mixtures of weak coherent microwaves., Comment: 11 pages, 3 figures

The integration of ferromagnetic and ferroelectric materials into hybrid heterostructures yields multifunctional systems with improved or novel functionality. We here report on the structural, electronic and magnetic properties of the ferromagnetic double perovskite Sr2CrReO6, grown as epitaxial thin film onto ferroelectric BaTiO3. As a function of temperature, the crystal-structure of BaTiO3 undergoes phase transitions, which induce qualitative changes in the magnetic anisotropy of the ferromagnet. We observe abrupt changes in the coercive field of up to 1.2T along with resistance changes of up to 6.5%. These results are attributed to the high sensitivity of the double perovskites to mechanical deformation., Comment: 3 figures

We report on the direct probing of the Fermi surface in the bulk of the electron-doped superconductor Nd$_{2-x}$Ce$_x$CuO$_4$ at different doping levels by means of magnetoresistance quantum oscillations. Our data reveal a sharp qualitative change in the Fermi surface topology, due to translational symmetry breaking in the electronic system which occurs at a critical doping level significantly exceeding the optimal doping. This result implies that the $(\pi/a,\pi/a)$ ordering, known to exist at low doping levels, survives up to the overdoped superconducting regime., Comment: 12 pages, 4 figures; submitted to PRL

We present a method for measuring the internal state of a superconducting qubit inside an on-chip microwave resonator. We show that one qubit state can be associated with the generation of an increasingly large cavity coherent field, while the other remains associated with the vacuum. By measuring the outgoing resonator field with conventional devices, an efficient single-shot QND-like qubit readout can be achieved, enabling a high-fidelity measurement in the spirit of the electron-shelving technique for trapped ions. We expect that the proposed ideas can be adapted to different superconducting qubit designs and contribute to the further improvement of qubit readout fidelity., Comment: 4 pages, 3 figures

The double perovskite Sr2CrReO6 is an interesting material for spintronics, showing ferrimagnetism up to 635 K with a predicted high spin polarization of about 86%. We fabricated Sr2CrReO6 epitaxial films by pulsed laser deposition on (001)-oriented SrTiO3 substrates. Phase-pure films with optimum crystallographic and magnetic properties were obtained by growing at a substrate temperature of 700 degree C in pure O2 of 6.6x10-4 mbar. The films are c-axis oriented, coherently strained, and show less than 20% anti-site defects. The magnetization curves reveal high saturation magnetization of 0.8 muB per formula unit and high coercivity of 1.1 T, as well as a strong magnetic anisotropy., Comment: accepted for publication

Superconducting quantum circuits are promising systems for experiments testing fundamental quantum mechanics on a macroscopic scale and for applications in quantum information processing. We report on the fabrication and characterization of superconducting flux qubits, readout dc SQUIDs, on-chip shunting capacitors, and high-quality coplanar waveguide resonators. Furthermore, we discuss the tunability and fundamental symmetry aspects inherent to all superconducting qubits, which can be regarded as artificial solid-state atoms. Comparing them to their natural counterparts, we discuss first and second-order energy shifts due to static control fields. Additionally, we present an intuitive derivation of the first- and second-order matrix elements for level transitions in the presence of a coherent microwave driving., Comment: 20 pages, 7 figures, accepted for publication in Supercond. Sci. Technol

The control of magnetic properties by means of an electric field is an important aspect in magnetism and magnetoelectronics. We here utilize magnetoelastic coupling in ferromagnetic/piezoelectric hybrids to realize a voltage control of magnetization orientation at room temperature. The samples consist of polycrystalline nickel thin films evaporated onto piezoelectric actuators. The magnetic properties of these multifunctional hybrids are investigated at room temperature as a function of the voltage controlled stress exerted by the actuator on the Ni film. Ferromagnetic resonance spectroscopy shows that the magnetic easy axis in the Ni film plane is rotated by 90 degree upon changing the polarity of the voltage Vp applied to the actuator. In other words, the in-plane uniaxial magnetic anisotropy of the Ni film can be inverted via the application of an appropriate voltage Vp. Using SQUID magnetometry, the evolution of the magnetization vector is recorded as a function of Vp and of the external magnetic field. Changing Vp allows to reversibly adjust the magnetization orientation in the Ni film plane within a range of approximately 70 degree. All magnetometry data can be quantitatively understood in terms of the magnetic free energy determined from the ferromagnetic resonance experiments. These results demonstrate that magnetoelastic coupling in hybrid structures indeed is a viable option to control magnetization orientation in technologically relevant ferromagnetic thin films at room temperature.

Oxide based ferromagnet/semiconductor heterostructures offer substantial advantages for spin electronics. We have grown (111) oriented Fe3O4 thin films and Fe3O4/ZnO heterostructures on ZnO(0001) and Al2O3(0001) substrates by pulsed laser deposition. High quality crystalline films with mosaic spread as small as 0.03 degree, sharp interfaces, and rms surface roughness of 0.3 nm were achieved. Magnetization measurements show clear ferromagnetic behavior of the magnetite layers with a saturation magnetization of 3.2 muB/f.u. at 300 K. Our results demonstrate that the Fe3O4/ZnO system is an intriguing and promising candidate for the realization of multi-functional heterostructures., Comment: 4 pages, 3 figures

Superconducting qubits behave as artificial two-level atoms and are used to investigate fundamental quantum phenomena. In this context, the study of multi-photon excitations occupies a central role. Moreover, coupling superconducting qubits to on-chip microwave resonators has given rise to the field of circuit QED. In contrast to quantum-optical cavity QED, circuit QED offers the tunability inherent to solid-state circuits. In this work, we report on the observation of key signatures of a two-photon driven Jaynes-Cummings model, which unveils the upconversion dynamics of a superconducting flux qubit coupled to an on-chip resonator. Our experiment and theoretical analysis show clear evidence for the coexistence of one- and two-photon driven level anticrossings of the qubit-resonator system. This results from the symmetry breaking of the system Hamiltonian, when parity becomes a not well-defined property. Our study provides deep insight into the interplay of multiphoton processes and symmetries in a qubit-resonator system., Comment: Accepted for publication in Nature Physics, 8 pages, 4 figures

We have investigated the magnetic properties of a piezoelectric actuator/ferromagnetic semiconductor hybrid structure. Using a GaMnAs epilayer as the ferromagnetic semiconductor and applying the piezo-stress along its [110] direction, we quantify the magnetic anisotropy as a function of the voltage V_p applied to the piezoelectric actuator using anisotropic magnetoresistance techniques. We find that the easy axis of the strain-induced uniaxial magnetic anisotropy contribution can be inverted from the [110] to the [1-10] direction via the application of appropriate voltages V_p. At T=5K the magnetoelastic term is a minor contribution to the magnetic anisotropy. Nevertheless, we show that the switching fields of rho(H) loops are shifted as a function of V_p at this temperature. At 50K - where the magnetoelastic term dominates the magnetic anisotropy - we are able to tune the magnetization orientation by about 70 degree solely by means of the electrical voltage V_p applied. Furthermore, we derive the magnetostrictive constant lambda_111 as a function of temperature and find values consistent with earlier results. We argue that the piezo-voltage control of magnetization orientation is directly transferable to other ferromagnetic/piezoelectric hybrid structures, paving the way to innovative multifunctional device concepts. As an example, we demonstrate piezo-voltage induced irreversible magnetization switching at T=40K, which constitutes the basic principle of a nonvolatile memory element.

We introduce a systematic formalism for two-resonator circuit QED, where two on-chip microwave resonators are simultaneously coupled to one superconducting qubit. Within this framework, we demonstrate that the qubit can function as a quantum switch between the two resonators, which are assumed to be originally independent. In this three-circuit network, the qubit mediates a geometric second-order circuit interaction between the otherwise decoupled resonators. In the dispersive regime, it also gives rise to a dynamic second-order perturbative interaction. The geometric and dynamic coupling strengths can be tuned to be equal, thus permitting to switch on and off the interaction between the two resonators via a qubit population inversion or a shifting of the qubit operation point. We also show that our quantum switch represents a flexible architecture for the manipulation and generation of nonclassical microwave field states as well as the creation of controlled multipartite entanglement in circuit QED. In addition, we clarify the role played by the geometric interaction, which constitutes a fundamental property characteristic of superconducting quantum circuits without counterpart in quantum-optical systems. We develop a detailed theory of the geometric second-order coupling by means of circuit transformations for superconducting charge and flux qubits. Furthermore, we show the robustness of the quantum switch operation with respect to decoherence mechanisms. Finally, we propose a realistic design for a two-resonator circuit QED setup based on a flux qubit and estimate all the related parameters. In this manner, we show that this setup can be used to implement a superconducting quantum switch with available technology., Comment: Published in Phys. Rev. B, major changes, 24 pages, 8 figures, REVTeX 4

We present a systematic study of the phase-coherent dynamics of a superconducting three-Josephson-junction flux qubit. The qubit state is detected with the integrated-pulse method, which is a variant of the pulsed switching DC SQUID method. In this scheme the DC SQUID bias current pulse is applied via a capacitor instead of a resistor, giving rise to a narrow band-pass instead of a pure low-pass filter configuration of the electromagnetic environment. Measuring one and the same qubit with both setups allows a direct comparison. With the capacitive method about four times faster switching pulses and an increased visibility are achieved. Furthermore, the deliberate engineering of the electromagnetic environment, which minimizes the noise due to the bias circuit, is facilitated. Right at the degeneracy point the qubit coherence is limited by energy relaxation. We find two main noise contributions. White noise is limiting the energy relaxation and contributing to the dephasing far from the degeneracy point. 1/f-noise is the dominant source of dephasing in the direct vicinity of the optimal point. The influence of 1/f-noise is also supported by non-random beatings in the Ramsey and spin echo decay traces. Numeric simulations of a coupled qubit-oscillator system indicate that these beatings are due to the resonant interaction of the qubit with at least one point-like fluctuator, coupled especially strongly to the qubit., Comment: Minor changes. 21 pages, 15 figures

We investigate in-plane quasiparticle tunneling across thin film grain boundary junctions (GBJs) of the electron-doped cuprate La$_{2-x}$Ce$_{x}$CuO$_4$ in magnetic fields up to $B=16 $T, perpendicular to the CuO$_2$ layers. The differential conductance in the superconducting state shows a zero bias conductance peak (ZBCP) due to zero energy surface Andreev bound states. With increasing temperature $T$, the ZBCP vanishes at the critical temperature $T_c\approx29 $K if B=0, and at $T=12 $K for B=16 T. As the ZBCP is related to the macroscopic phase coherence of the superconducting state, we argue that the disappearance of the ZBCP at a field $B_{ZBCP}(T)$ must occur below the upper critical field $B_{c2}(T)$ of the superconductor. We find $B_{ZBCP}(0) \approx 25 $T which is at least a factor of 2.5 higher than previous estimates of $B_{c2}(0)$., Comment: 4 pages, 4 figures

We consider a superconducting charge qubit coupled to distinct orthogonal electromagnetic field modes belonging to a coplanar wave guide and a microstrip transmission line resonators. This architecture allows the simultaneous implementation of a Jaynes-Cummings and anti-Jaynes-Cummings dynamics, a resonant method for generating mesoscopic qubit-field superpositions and for field-state reconstruction. Furthermore, we utilize this setup to propose a field measurement technique that is, in principle, robust to qubit dephasing and field relaxation due to a fast pre-measurement., Comment: 4 pages and 1 figure, minor changes, added references and improved figured, submitted for publication

We present a comprehensive study relating the nanostructure of Ge_0.95Mn_0.05 films to their magnetic properties. The formation of ferromagnetic nanometer sized inclusions in a defect free Ge matrix fabricated by low temperature molecular beam epitaxy is observed down to substrate temperatures T_S as low as 70 deg. Celsius. A combined transmission electron microscopy (TEM) and electron energy-loss spectroscopy (EELS) analysis of the films identifies the inclusions as precipitates of the ferromagnetic compound Mn_5Ge_3. The volume and amount of these precipitates decreases with decreasing T_S. Magnetometry of the films containing precipitates reveals distinct temperature ranges: Between the characteristic ferromagnetic transition temperature of Mn_5Ge_3 at approximately room temperature and a lower, T_S dependent blocking temperature T_B the magnetic properties are dominated by superparamagnetism of the Mn_5Ge_3 precipitates. Below T_B, the magnetic signature of ferromagnetic precipitates with blocked magnetic moments is observed. At the lowest temperatures, the films show features characteristic for a metastable state., Comment: accepted for publication in Phys. Rev. B 74 (01.12.2006). High resolution images ibidem

We present a detailed study of the magnetic properties of low-temperature-molecular-beam-epitaxy grown Ge:Mn dilute magnetic semiconductor films. We find strong indications for a frozen state of Ge_{1-x}Mn_{x}, with freezing temperatures of T_f=12K and T_f=15K for samples with x=0.04 and x=0.2, respectively, determined from the difference between field-cooled and zero-field-cooled magnetization. For Ge_{0.96}Mn_{0.04}, ac susceptibility measurements show a peak around T_f, with the peak position T'_f shifting as a function of the driving frequency f by Delta T_f' / [T_f' Delta log f] ~ 0.06, whereas for sample Ge_{0.8}Mn_{0.2} a more complicated behavior is observed. Furthermore, both samples exhibit relaxation effects of the magnetization after switching the magnitude of the external magnetic field below T_f which are in qualitative agreement with the field- and zero-field-cooled magnetization measurements. These findings consistently show that Ge:Mn exhibits a frozen magnetic state at low temperatures and that it is not a conventional ferromagnet., Comment: Revised version contains extended interpretation of experimental data

We have measured Re 5d spin and orbital magnetic moments in the ferrimagnetic double perovskite Sr2CrReO6 by X-ray magnetic circular dichroism at the L_{2,3} edges. In fair agreement with recent band-structure calculations [Vaitheeswaran et. al., Ref 1], at the Re site a large 5d spin magnetic moment of -0.68 mu_B and a considerable orbital moment of +0.25 mu_B have been detected. We found that the Curie temperature of the double perovskites A2BB'O6 scales with the spin magnetic moment of the 'non-magnetic' B' ion., Comment: 3 pages, 3 figures

Using low-temperature scanning laser microscopy we directly image electric transport in a magnetoresistive element, a manganite thin film intersected by a grain boundary (GB). Imaging at variable temperature allows reconstruction and comparison of the local resistance vs temperature for both, the manganite film and the GB. Imaging at low temperature also shows that the GB switches between different resistive states due to the formation and growth of magnetic domains along the GB. We observe different types of domain wall growth; in most cases a domain wall nucleates at one edge of the bridge and then proceeds towards the other edge., Comment: 5 pages, 4 figures; submitted to Phys. Rev. Lett

We propose a method to couple metastable flux-based qubits to superconductive resonators based on a quantum-optical Raman excitation scheme that allows for the deterministic generation of stationary and propagating microwave Fock states and other weak quantum fields. Moreover, we introduce a suitable microwave quantum homodyne technique, with no optical counterpart, that enables the measurement of relevant field observables, even in the presence of noisy amplification devices., Comment: Four pages and two figures. Submitted for publication. Significant changes in the microwave measurement procedure

We have investigated the magnetic moment of the W ion in the ferrimagnetic double perovskites Sr2CrWO6 and Ca2CrWO6 by X-ray magnetic circular dichroism (XMCD) at the W L(2,3) edges. In both compounds a finite negative spin and positive orbital magnetic moment was detected. The experimental results are in good agreement with band-structure calculations for (Sr/Ca)2CrWO6 using the full-potential linear muffin-tin orbital method. It is remarkable, that the magnetic ordering temperature, TC, is correlated with the magnetic moment at the 'non-magnetic' W atom., Comment: accepted for publication

Magnetite (Fe3O4) based tunnel junctions with turret/mesa structure have been investigated for different barrier materials (SrTiO3, NdGaO3, MgO, SiO2, and Al2O(3-x)). Junctions with a Ni counter electrode and an aluminium oxide barrier showed reproducibly a tunneling magnetoresistance (TMR) effect at room temperature of up to 5% with almost ideal switching behavior. This number only partially reflects the intrinsic high spin polarization of Fe3O4. It is considerably decreased due to an additional series resistance within the junction. Only SiO2 and Al2O(3-x) barriers provide magnetically decoupled electrodes as necessary for sharp switching. The observed decrease of the TMR effect as a function of increasing temperature is due to a decrease in spin polarization and an increase in spin-scattering in the barrier. Among the oxide half-metals magnetite has the potential to enhance the performance of TMR based devices.

We have studied the magnetic properties of Ba_2FeNbO_6 and Ba_2MnNbO_6. it is seen that Ba_2FeNbO_6 is an antiferromagnet with a weak ferromagnetic behaviour at 5K while Ba_2MnNbO_6 shows two magnetic transitions one at 45 K and the other at 12K. Electron spin resonance (ESR) measurements at room temperature show that the Mn compound does not show any Jahn-Teller distortion. It is also seen that the Neel temperature of the A_2FeNbO_6 (A=Ba,Sr, BaSr) compounds do not vary significantly. However variations in the average A-site ionic radius influence the formation of short range correlations that persist above T_N., Comment: 10 oages, 5 figures, MMM, to appear in J.Appl.Phys

Magnetite epitaxial thin films have been prepared by pulsed laser deposition at 340 C on MgO and Si substrates. One key result is that the thin film properties are almost identical to the properties of bulk material. For 40 - 50 nm thick films, the saturation magnetization and conductivity are respectively 453 emu/cm^3 and 225 1/(Ohm cm) at room temperature. The Verwey transition is at 117 K. The Hall effect indicates an electron concentration corresponding to 0.22 electrons per formula unit at room temperature. Normal and anomalous Hall effect both have a negative sign.

he structural, transport, magnetic and optical properties of the double perovskite $A_2$CrWO$_6$ with $A=\text{Sr, Ba, Ca}$ have been studied. By varying the alkaline earth ion on the $A$ site, the influence of steric effects on the Curie temperature $T_C$ and the saturation magnetization has been determined. A maximum $T_C=458$ K was found for Sr$_2$CrWO$_6$ having an almost undistorted perovskite structure with a tolerance factor $f\simeq 1$. For Ca$_2$CrWO$_6$ and Ba$_2$CrWO$_6$ structural changes result in a strong reduction of $T_C$. Our study strongly suggests that for the double perovskites in general an optimum $T_C$ is achieved only for $f \simeq 1$, that is, for an undistorted perovskite structure. Electron doping in Sr$_2$CrWO$_6$ by a partial substitution of Sr$^{2+}$ by La$^{3+}$ was found to reduce both $T_C$ and the saturation magnetization $M_s$. The reduction of $M_s$ could be attributed both to band structure effects and the Cr/W antisites induced by doping. Band structure calculations for Sr$_2$CrWO$_6$ predict an energy gap in the spin-up band, but a finite density of states for the spin-down band. The predictions of the band structure calculation are consistent with our optical measurements. Our experimental results support the presence of a kinetic energy driven mechanism in $A_2$CrWO$_6$, where ferromagnetism is stabilized by a hybridization of states of the nonmagnetic W-site positioned in between the high spin Cr-sites., Comment: 14 pages, 10 figures

Epitaxy of oxide materials on silicon (Si) substrates is of great interest for future functional devices using the large variety of physical properties of the oxides as ferroelectricity, ferromagnetism, or superconductivity. Recently, materials with high spin polarization of the charge carriers have become interesting for semiconductor-oxide hybrid devices in spin electronics. Here, we report on pulsed laser deposition of magnetite (Fe3O4) on Si(001) substrates cleaned by an in situ laser beam high temperature treatment. After depositing a double buffer layer of titanium nitride (TiN) and magnesium oxide (MgO), a high quality epitaxial magnetite layer can be grown as verified by RHEED intensity oscillations and high resolution x-ray diffraction., Comment: submitted

We report on the preparation and characterization of epitaxial thin films of the double-perovskite Sr$_2$CrWO$_6$ by Pulsed Laser Deposition (PLD). On substrates with low lattice mismatch like SrTiO$_3$, epitaxial Sr$_2$CrWO$_6$ films with high crystalline quality can be grown in a molecular layer-by-layer growth mode. Due to the similar ionic radii of Cr and W, these elements show no sublattice order. Nevertheless, the measured Curie temperature is well above 400 K. Due to the reducing growth atmosphere required for double perovskites, the SrTiO$_3$ substrate surface undergoes an insulator-metal transition impeding the separation of thin film and substrate electric transport properties., Comment: 3 pages, 5 figures

We have performed a systematic analysis of the low frequency 1/f-noise in single grain boundary junctions in the colossal magnetoresistance material La_{2/3}Ca_{1/3}MnO_{3-delta}. The grain boundary junctions were formed in epitaxial La_{2/3}Ca_{1/3}MnO_{3-delta} films deposited on SrTiO_3 bicrystal substrates and show a large tunneling magnetoresistance of up to 300% at 4.2 K as well as ideal, rectangular shaped resistance versus applied magnetic field curves. Below the Curie temperature T_C the measured 1/f noise is dominated by the grain boundary. The dependence of the noise on bias current, temperature and applied magnetic field gives clear evidence that the large amount of low frequency noise is caused by localized sites with fluctuating magnetic moments in a heavily disordered grain boundary region. At 4.2 K additional temporally unstable Lorentzian components show up in the noise spectra that are most likely caused by fluctuating clusters of interacting magnetic moments. Noise due to fluctuating domains in the junction electrodes is found to play no significant role., Comment: 9 pages, 7 figures