51. The dominant role of critical valence fluctuations on high Tc superconductivity in heavy fermions
- Author
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DQMP, University of Geneva, Geneva 1211, Switzerland, Institute of Natural Sciences, Westlake Institute For Advanced Study, Westlake University, 18 Shilongshan Road, Hangzhou 310024, P. R. China, Department of Basic Sciences, Kyushu Institute of Technology, Kitakyushu, Fukuoka 804-8550, Japan, PHELIQS, UMR-E 9001, CEA-INAC/UJF-Grenoble 1, 38054 Grenoble, France, PHELIQS, UMR-E 9001, CEA-INAC/UJF-Grenoble 1, 38054 Grenoble, France, Institute for Materials Research, Tohoku University, Oarai, Ibaraki 311-1313, Japan, Center for Advanced High Magnetic Field Science, Osaka University, Toyonaka, Osaka 560-0043, Japan, Scheerer, Gernot W., Ren, Zhi, Watanabe, Shinji, Lapertot, Gérard, Aoki, Dai, Jaccard, Didier, Miyake, Kazumasa, DQMP, University of Geneva, Geneva 1211, Switzerland, Institute of Natural Sciences, Westlake Institute For Advanced Study, Westlake University, 18 Shilongshan Road, Hangzhou 310024, P. R. China, Department of Basic Sciences, Kyushu Institute of Technology, Kitakyushu, Fukuoka 804-8550, Japan, PHELIQS, UMR-E 9001, CEA-INAC/UJF-Grenoble 1, 38054 Grenoble, France, PHELIQS, UMR-E 9001, CEA-INAC/UJF-Grenoble 1, 38054 Grenoble, France, Institute for Materials Research, Tohoku University, Oarai, Ibaraki 311-1313, Japan, Center for Advanced High Magnetic Field Science, Osaka University, Toyonaka, Osaka 560-0043, Japan, Scheerer, Gernot W., Ren, Zhi, Watanabe, Shinji, Lapertot, Gérard, Aoki, Dai, Jaccard, Didier, and Miyake, Kazumasa
- Abstract
type:Journal Article, Despite almost 40 years of research, the origin of heavy-fermion superconductivity is still strongly debated. Especially, the pressure-induced enhancement of superconductivity in CeCu2Si2 away from the magnetic breakdown is not sufficiently taken into consideration. As recently reported in CeCu2Si2 and several related compounds, optimal superconductivity occurs at the pressure of a valence crossover, which arises from a virtual critical end point at negative temperature Tcr. In this context, we did a meticulous analysis of a vast set of top-quality high-pressure electrical resistivity data of several Ce-based heavy fermion compounds. The key novelty is the salient correlation between the superconducting transition temperature Tc and the valence instability parameter Tcr, which is in line with theory of enhanced valence fluctuations. Moreover, it is found that, in the pressure region of superconductivity, electrical resistivity is governed by the valence crossover, which most often manifests in scaling behavior. We develop the new idea that the optimum superconducting Tc of a given sample is mainly controlled by the compound’s Tcr and limited by non-magnetic disorder. In this regard, the present study provides compelling evidence for the crucial role of critical valence fluctuations in the formation of Cooper pairs in Ce-based heavy fermion superconductors besides the contribution of spin fluctuations near magnetic quantum critical points, and corroborates a plausible superconducting mechanism in strongly correlated electron systems in general.
- Published
- 2019