51. Slater to Mott crossover in the metal to insulator transition of Nd2Ir2O7
- Author
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Nakayama, M., Kondo, Takeshi, Tian, Z., Ishikawa, J. J., Halim, M., Bareille, C., Malaeb, W., Kuroda, K., Tomita, T., Ideta, S., Tanaka, K., Matsunami, M., Kimura, S., Inami, N., Ono, K., Kumigashira, H., Balents, L., Nakatsuji, S., and Shin, S.
- Subjects
Condensed Matter - Strongly Correlated Electrons ,Condensed Matter - Materials Science - Abstract
We present an angle-resolved photoemission study of the electronic structure of the three-dimensional pyrochlore iridate Nd2Ir2O7 through its magnetic metal-insulator transition. Our data reveal that metallic Nd2Ir2O7 has a quadratic band, touching the Fermi level at the Gamma point, similarly to that of Pr2Ir2O7. The Fermi node state is, therefore, a common feature of the metallic phase of the pyrochlore iridates. Upon cooling below the transition temperature, this compound exhibits a gap opening with an energy shift of quasiparticle peaks like a band gap insulator. The quasiparticle peaks are strongly suppressed, however, with further decrease of temperature, and eventually vanish at the lowest temperature, leaving a non-dispersive flat band lacking long-lived electrons. We thereby identify a remarkable crossover from Slater to Mott insulators with decreasing temperature. These observations explain the puzzling absence of Weyl points in this material, despite its proximity to the zero temperature metal-insulator transition.
- Published
- 2016
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