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51. Manganese precipitation kinetics and cobalt adsorption on MnO2 from the ammoniacal ammonium sulfate leach liquor of Indian Ocean manganese nodule

Author

Nathsarma, K.C., Rout, P.C., and Sarangi, K.

Subjects
*MANGANESE oxides, *PRECIPITATION (Chemistry) kinetics, *COBALT, *METAL absorption & adsorption, *AMMONIUM sulfate, *LEACHING, *MANGANESE nodules
Abstract

Abstract: Precipitation of manganese from the SO2-roast leach ammoniacal ammonium sulfate solution bearing both high and low concentrations of manganese in the presence of copper, cobalt and nickel ions was carried out in a stainless steel reactor fitted with a turbo grid. Air/O2 was used to precipitate Mn as MnO2 from the solution. There was adsorption loss of cobalt from the solution. Precipitation of manganese from the solution was 57.2–99.9%. The maximum adsorption loss of Co was 22.1%. The precipitation of Mn and adsorption loss of cobalt from the solution followed the first order kinetics. The rate constants for the precipitation of manganese and loss of cobalt were evaluated and the experimental data were fitted to Freundlich and Langmuir adsorption isotherms. [Copyright &y& Elsevier]

Published
2013
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52. Process development for the recovery of high grade calcium tungstate from alkaline leach liquor of spent [sbnd]HDS catalyst.

Author

Ghadai, B., Rout, P.C., Mohapatra, D., Padh, B., and Reddy, B. Ramachandra

Subjects
*MOLYBDENUM, *SODIUM tungstate, *CALCIUM, *AMMONIUM paratungstate, *CATALYSTS, *TUNGSTEN, *LIQUORS
Abstract

Molybdenum is often associated with nickel-tungsten based spent HDS catalyst and must be removed from tungstate solution to obtain commercially acceptable tungsten products. In order to address this problem, a different approach has been proposed in the present work. A two step process based on selective thionization of Mo using Na 2 S at alkaline condition followed by W precipitation as calcium tungstate (CT) using lime (Ca(OH) 2) was studied. Various operating parameters were tested and optimum conditions for Mo thionization and W precipitation were developed. The CT produced by the conventional process was used as a reference to check the improvement in the proposed process with respect to Mo impurity. Under the optimum conditions, 92.7% Mo was rejected to the CT filtrate and 99.7% W converted to CT. The CT obtained from the proposed process contained 0.53% Mo, which was much less as compared to the CT obtained from the conventional process having 2.5% Mo using the same leach solution. High-grade ammonium paratungstate (APT) containing <100 ppm Mo was obtained by treating the CT, which can be used for the tools industry and other applications. • High grade CT preparation from sodium tungstate leach liquor was proposed. • Mo was separated from varying Mo bearing W leach liquors. • Selective thionisation of Mo is the key step to achieve high grade APT from the generated CT. • High grade APT containing <100 ppm Mo was obtained by treating the CT. • The process is simple, cost effective and can be applied industrially. [ABSTRACT FROM AUTHOR]

Published
2020
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53. Neutron Capture on the s -Process Branching Point Tm 171 via Time-of-Flight and Activation

Author

Guerrero, C., Lerendegui-Marco, J., Paul, M., Tessler, M., Heinitz, S., Domingo-Pardo, C., Cristallo, S., Dressler, R., Halfon, S., Kivel, N., Köster, U., Maugeri, E.a., Palchan-Hazan, T., Quesada, J.M., Rochman, D., Schumann, D., Weissman, L., Aberle, O., Amaducci, S., Andrzejewski, J., Audouin, L., Bécares, V., Bacak, M., Balibrea, J., Barak, A., Barbagallo, M., Barros, S., Bečvář, F., Beinrucker, C., Berkovits, D., Berthoumieux, E., Billowes, J., Bosnar, D., Brugger, M., Buzaglo, Y., Caamaño, M., Calviño, F., Calviani, M., Cano-Ott, D., Cardella, R., Casanovas, A., Castelluccio, D.M., Cerutti, F., Chen, Y.H., Chiaveri, E., Colonna, N., Cortés, G., Cortés-Giraldo, M.A., Cosentino, L., Dafna, H., Damone, A., Diakaki, M., Dietz, M., Dupont, E., Durán, I., Eisen, Y., Fernández-Domínguez, B., Ferrari, A., Ferreira, P., Finocchiaro, P., Furman, V., Göbel, K., García, A.R., Gawlik, A., Glodariu, T., Gonçalves, I.F., González-Romero, E., Goverdovski, A., Griesmayer, E., Gunsing, F., Harada, H., Heftrich, T., Heyse, J., Hirsh, T., Jenkins, D.G., Jericha, E., Käppeler, F., Kadi, Y., Kaizer, B., Katabuchi, T., Kavrigin, P., Ketlerov, V., Khryachkov, V., Kijel, D., Kimura, A., Kokkoris, M., Kriesel, A., Krtička, M., Leal-Cidoncha, E., Lederer-Woods, C., Leeb, H., Lo Meo, S., Lonsdale, S.J., Losito, R., Macina, D., Manna, A., Marganiec, J., Martínez, T., Massimi, C., Mastinu, P., Mastromarco, M., Matteucci, F., Mendoza, E., Mengoni, A., Milazzo, P.M., Millán-Callado, M.A., Mingrone, F., Mirea, M., Montesano, S., Musumarra, A., Nolte, R., Oprea, A., Patronis, N., Pavlik, A., Perkowski, J., Piersanti, L., Porras, I., Praena, J., Rajeev, K., Rauscher, T., Reifarth, R., Rodríguez-González, T., Rout, P.C., Rubbia, C., Ryan, J.A., Sabaté-Gilarte, M., Saxena, A., Schillebeeckx, P., Schmidt, S., Shor, A., Sedyshev, P., Smith, A.G., Stamatopoulos, A., Tagliente, G., Tain, J.L., Tarifeño-Saldivia, A., Tassan-Got, L., Tsinganis, A., Valenta, S., Vannini, G., Variale, V., Vaz, P., Ventura, A., Vlachoudis, V., Vlastou, R., Wallner, A., Warren, S., Weigand, M., Weiss, C., Wolf, C., Woods, P.J., Wright, T., Žugec, P., Institut Laue-Langevin (ILL), Institut de Physique Nucléaire d'Orsay (IPNO), Université Paris-Sud - Paris 11 (UP11)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Centre National de la Recherche Scientifique (CNRS), Institut de Recherches sur les lois Fondamentales de l'Univers (IRFU), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay, n_TOF, Guerrero C., Lerendegui-Marco J., Paul M., Tessler M., Heinitz S., Domingo-Pardo C., Cristallo S., Dressler R., Halfon S., Kivel N., Koster U., Maugeri E.A., Palchan-Hazan T., Quesada J.M., Rochman D., Schumann D., Weissman L., Aberle O., Amaducci S., Andrzejewski J., Audouin L., Becares V., Bacak M., Balibrea J., Barak A., Barbagallo M., Barros S., Becvar F., Beinrucker C., Berkovits D., Berthoumieux E., Billowes J., Bosnar D., Brugger M., Buzaglo Y., Caamano M., Calvino F., Calviani M., Cano-Ott D., Cardella R., Casanovas A., Castelluccio D.M., Cerutti F., Chen Y.H., Chiaveri E., Colonna N., Cortes G., Cortes-Giraldo M.A., Cosentino L., Dafna H., Damone A., Diakaki M., Dietz M., Dupont E., Duran I., Eisen Y., Fernandez-Dominguez B., Ferrari A., Ferreira P., Finocchiaro P., Furman V., Gobel K., Garcia A.R., Gawlik A., Glodariu T., Goncalves I.F., Gonzalez-Romero E., Goverdovski A., Griesmayer E., Gunsing F., Harada H., Heftrich T., Heyse J., Hirsh T., Jenkins D.G., Jericha E., Kappeler F., Kadi Y., Kaizer B., Katabuchi T., Kavrigin P., Ketlerov V., Khryachkov V., Kijel D., Kimura A., Kokkoris M., Kriesel A., Krticka M., Leal-Cidoncha E., Lederer-Woods C., Leeb H., Lo Meo S., Lonsdale S.J., Losito R., MacIna D., Manna A., Marganiec J., Martinez T., Massimi C., Mastinu P., Mastromarco M., Matteucci F., Mendoza E., Mengoni A., Milazzo P.M., Millan-Callado M.A., Mingrone F., Mirea M., Montesano S., Musumarra A., Nolte R., Oprea A., Patronis N., Pavlik A., Perkowski J., Piersanti L., Porras I., Praena J., Rajeev K., Rauscher T., Reifarth R., Rodriguez-Gonzalez T., Rout P.C., Rubbia C., Ryan J.A., Sabate-Gilarte M., Saxena A., Schillebeeckx P., Schmidt S., Shor A., Sedyshev P., Smith A.G., Stamatopoulos A., Tagliente G., Tain J.L., Tarifeno-Saldivia A., Tassan-Got L., Tsinganis A., Valenta S., Vannini G., Variale V., Vaz P., Ventura A., Vlachoudis V., Vlastou R., Wallner A., Warren S., Weigand M., Weiss C., Wolf C., Woods P.J., Wright T., Zugec P., Guerrero, C., Lerendegui-Marco, J., Paul, M., Tessler, M., Heinitz, S., Domingo-Pardo, C., Cristallo, S., Dressler, R., Halfon, S., Kivel, N., Koster, U., Maugeri, E. A., Palchan-Hazan, T., Quesada, J. M., Rochman, D., Schumann, D., Weissman, L., Aberle, O., Amaducci, S., Andrzejewski, J., Audouin, L., Becares, V., Bacak, M., Balibrea, J., Barak, A., Barbagallo, M., Barros, S., Becvar, F., Beinrucker, C., Berkovits, D., Berthoumieux, E., Billowes, J., Bosnar, D., Brugger, M., Buzaglo, Y., Caamano, M., Calvino, F., Calviani, M., Cano-Ott, D., Cardella, R., Casanovas, A., Castelluccio, D. M., Cerutti, F., Chen, Y. H., Chiaveri, E., Colonna, N., Cortes, G., Cortes-Giraldo, M. A., Cosentino, L., Dafna, H., Damone, A., Diakaki, M., Dietz, M., Dupont, E., Duran, I., Eisen, Y., Fernandez-Dominguez, B., Ferrari, A., Ferreira, P., Finocchiaro, P., Furman, V., Gobel, K., Garcia, A. R., Gawlik, A., Glodariu, T., Goncalves, I. F., Gonzalez-Romero, E., Goverdovski, A., Griesmayer, E., Gunsing, F., Harada, H., Heftrich, T., Heyse, J., Hirsh, T., Jenkins, D. G., Jericha, E., Kappeler, F., Kadi, Y., Kaizer, B., Katabuchi, T., Kavrigin, P., Ketlerov, V., Khryachkov, V., Kijel, D., Kimura, A., Kokkoris, M., Kriesel, A., Krticka, M., Leal-Cidoncha, E., Lederer-Woods, C., Leeb, H., Lo Meo, S., Lonsdale, S. J., Losito, R., Macina, D., Manna, A., Marganiec, J., Martinez, T., Massimi, C., Mastinu, P., Mastromarco, M., Matteucci, F., Mendoza, E., Mengoni, A., Milazzo, P. M., Millan-Callado, M. A., Mingrone, F., Mirea, M., Montesano, S., Musumarra, A., Nolte, R., Oprea, A., Patronis, N., Pavlik, A., Perkowski, J., Piersanti, L., Porras, I., Praena, J., Rajeev, K., Rauscher, T., Reifarth, R., Rodriguez-Gonzalez, T., Rout, P. C., Rubbia, C., Ryan, J. A., Sabate-Gilarte, M., Saxena, A., Schillebeeckx, P., Schmidt, S., Shor, A., Sedyshev, P., Smith, A. G., Stamatopoulos, A., Tagliente, G., Tain, J. L., Tarifeno-Saldivia, A., Tassan-Got, L., Tsinganis, A., Valenta, S., Vannini, G., Variale, V., Vaz, P., Ventura, A., Vlachoudis, V., Vlastou, R., Wallner, A., Warren, S., Weigand, M., Weiss, C., Wolf, C., Woods, P. J., Wright, T., Zugec, P., ILL, and Centre National de la Recherche Scientifique (CNRS)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Paris-Sud - Paris 11 (UP11)

Subjects
PRIRODNE ZNANOSTI. Fizika, Physics, ddc:530, s process nucleosynthesis, n_TOF, neutron physics, 171Tm, Nuclear Physics - Experiment, [PHYS.NEXP]Physics [physics]/Nuclear Experiment [nucl-ex], NATURAL SCIENCES. Physics, Nuclear Physics
Abstract

International audience; The neutron capture cross sections of several unstable nuclides acting as branching points in the s process are crucial for stellar nucleosynthesis studies. The unstable Tm171 (t1/2=1.92 yr) is part of the branching around mass A∼170 but its neutron capture cross section as a function of the neutron energy is not known to date. In this work, following the production for the first time of more than 5 mg of Tm171 at the high-flux reactor Institut Laue-Langevin in France, a sample was produced at the Paul Scherrer Institute in Switzerland. Two complementary experiments were carried out at the neutron time-of-flight facility (n_TOF) at CERN in Switzerland and at the SARAF liquid lithium target facility at Soreq Nuclear Research Center in Israel by time of flight and activation, respectively. The result of the time-of-flight experiment consists of the first ever set of resonance parameters and the corresponding average resonance parameters, allowing us to make an estimation of the Maxwellian-averaged cross sections (MACS) by extrapolation. The activation measurement provides a direct and more precise measurement of the MACS at 30 keV: 384(40) mb, with which the estimation from the n_TOF data agree at the limit of 1 standard deviation. This value is 2.6 times lower than the JEFF-3.3 and ENDF/B-VIII evaluations, 25% lower than that of the Bao et al. compilation, and 1.6 times larger than the value recommended in the KADoNiS (v1) database, based on the only previous experiment. Our result affects the nucleosynthesis at the A∼170 branching, namely, the Yb171 abundance increases in the material lost by asymptotic giant branch stars, providing a better match to the available pre-solar SiC grain measurements compared to the calculations based on the current JEFF-3.3 model-based evaluation.

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54. Dissemination of data measured at the CERN n_TOF facility

Author

Dupont, E., Otuka, N., Cabellos, O., Aberle, O., Aerts, G., Altstadt, S., Alvarez, H., Alvarez-Velarde, F., Andriamonje, S., Andrzejewski, J., Audouin, L., Bacak, M., Badurek, G., Balibrea, J., Barbagallo, M., Barros, S., Baumann, P., Bécares, V., Bečvář, F., Beinrucker, C., Belloni, F., Berthier, B., Berthoumieux, E., Billowes, J., Boccone, V., Bosnar, D., Brown, A., Brugger, M., Caamaño, M., Calviani, M., Calviño, F., Cano-Ott, D., Capote, R., Cardella, R., Carrapiço, C., Casanovas, A., Castelluccio, D.M., Cennini, P., Cerutti, F., Chen, Y.H., Chiaveri, E., Chin, M., Colonna, N., Cortés, G., Cortés-Giraldo, M.A., Cosentino, L., Couture, A., Cox, J., Damone, L.A., David, S., Deo, K., Diakaki, M., Dillmann, I., Domingo-Pardo, C., Dressler, R., Dridi, W., Duran, I., Eleftheriadis, C., Embid-Segura, M., Fernández-Domínguez, B., Ferrant, L., Ferrari, A., Ferreira, P., Finocchiaro, P., Fraval, K., Frost, R.J.W., Fujii, K., Furman, W., Ganesan, S., Garcia, A.R., Gawlik, A., Gheorghe, I., Gilardoni, S., Giubrone, G., Glodariu, T., Göbel, K., Gomez-Hornillos, M.B., Goncalves, I.F., Gonzalez-Romero, E., Goverdovski, A., Gramegna, F., Griesmayer, E., Guerrero, C., Gunsing, F., Gurusamy, P., Haight, R., Harada, H., Heftrich, T., Heil, M., Heinitz, S., Hernández-Prieto, A., Heyse, J., Igashira, M., Isaev, S., Jenkins, D.G., Jericha, E., Kadi, Y., Kaeppeler, F., Kalamara, A., Karadimos, D., Karamanis, D., Katabuchi, T., Kavrigin, P., Kerveno, M., Ketlerov, V., Khryachkov, V., Kimura, A., Kivel, N., Kokkoris, M., Konovalov, V., Krtička, M., Kroll, J., Kurtulgil, D., Lampoudis, C., Langer, C., Leal-Cidoncha, E., Lederer, C., Leeb, H., Naour, C. Le, Lerendegui-Marco, J., Leong, L.S., Licata, M., Meo, S. Lo, Lonsdale, S.J., Losito, R., Lozano, M., Macina, D., Manousos, A., Marganiec, J., Martinez, T., Marrone, S., Masi, A., Massimi, C., Mastinu, P., Mastromarco, M., Matteucci, F., Maugeri, E.A., Mazzone, A., Mendoza, E., Mengoni, A., Milazzo, P.M., Mingrone, F., Mirea, M., Mondelaers, W., Montesano, S., Moreau, C., Mosconi, M., Musumarra, A., Negret, A., Nolte, R., O’Brien, S., Oprea, A., Palomo-Pinto, F.R., Pancin, J., Paradela, C., Patronis, N., Pavlik, A., Pavlopoulos, P., Perkowski, J., Perrot, L., Pigni, M.T., Plag, R., Plompen, A., Plukis, L., Poch, A., Porras, I., Praena, J., Pretel, C., Quesada, J.M., Radeck, D., Rajeev, K., Rauscher, T., Reifarth, R., Riego, A., Robles, M., Roman, F., Rout, P.C., Rudolf, G., Rubbia, C., Rullhusen, P., Ryan, J.A., Sabaté-Gilarte, M., Salgado, J., Santos, C., Sarchiapone, L., Sarmento, R., Saxena, A., Schillebeeckx, P., Schmidt, S., Schumann, D., Sedyshev, P., Smith, A.G., Sosnin, N.V., Stamatopoulos, A., Stephan, C., Suryanarayana, S.V., Tagliente, G., Tain, J.L., Tarifeño-Saldivia, A., Tarrío, D., Tassan-Got, L., Tavora, L., Terlizzi, R., Tsinganis, A., Valenta, S., Vannini, G., Variale, V., Vaz, P., Ventura, A., Versaci, R., Vermeulen, M.J., Villamarin, D., Vicente, M.C., Vlachoudis, V., Vlastou, R., Voss, F., Wallner, A., Walter, S., Ware, T., Warren, S., Weigand, M., Weiß, C., Wolf, C., Wiesher, M., Wisshak, K., Woods, P.J., Wright, T., Žugec, P., Plompen, A. [Hrsg.], Hambsch, F.-J. [Hrsg.], Schillebeeckx, P. [Hrsg.], Mondelaers, W. [Hrsg.], Heyse, J. [Hrsg.], Kopecky, S. [Hrsg.], Siegler, P. [Hrsg.], and Oberstedt, S. [Hrsg.]

Subjects
7. Clean energy

55. Selective leaching and recovery of V as iron vanadate from industrially generated Mo-V residue.

Author

Rout P.C., Mishra G.K., Mohapatra D., Padh B., Reddy B.R., Rout P.C., Mishra G.K., Mohapatra D., Padh B., and Reddy B.R.

Abstract

A commercial process was developed to treat a Ca-based Mo-V residue generated in a molybdenum processing plant. Vanadium was selectively leached using acetic acid and recovered as iron vanadate by the hydro process. Process conditions for selective V leaching and iron vanadate precipitation were investigated. V recovery efficiency of 90.3% was achieved with a V content of 26.5% and an Fe content of 29% in the iron vanadate cake suitable for the ferrovanadium industry. The overall Mo recovery in the whole process was 98.6%. The obtained leach residue containing 14.3% Mo with negligible impurities can be used as a feed material for the Mo production process or ferromolybdenum industry. This simple and economical process generates two product streams from a single operation and has the potential to solve a long standing problem of handling such a mixed Mo-V residue. (Authors.), A commercial process was developed to treat a Ca-based Mo-V residue generated in a molybdenum processing plant. Vanadium was selectively leached using acetic acid and recovered as iron vanadate by the hydro process. Process conditions for selective V leaching and iron vanadate precipitation were investigated. V recovery efficiency of 90.3% was achieved with a V content of 26.5% and an Fe content of 29% in the iron vanadate cake suitable for the ferrovanadium industry. The overall Mo recovery in the whole process was 98.6%. The obtained leach residue containing 14.3% Mo with negligible impurities can be used as a feed material for the Mo production process or ferromolybdenum industry. This simple and economical process generates two product streams from a single operation and has the potential to solve a long standing problem of handling such a mixed Mo-V residue. (Authors.)

56. A hydrometallurgical process for the recovery of metal values from spent Cu-Cr catalyst.

Author

Panigrahi J., Garnaik B., Rout P.C., Sarangi K., Panigrahi J., Garnaik B., Rout P.C., and Sarangi K.

Abstract

Copper-chromium catalyst has been used in many chemical processes and dumped in landfill after losing its catalytic property. Owing to the toxicity of Cr the dumping of catalyst is not environmentally acceptable, so metal values should be removed before disposal. One typical Cu-Cr catalyst was leached with sulphuric acid and from the leach liquor Cu and Cr were extracted using LIX 860N and NaD2EHPA, respectively. The McCabe-Thiele diagram at pH 3.5 with 20% LIX 860N indicated two stages at A:O=1:1 for quantitative extraction of Cu. The stripping of Cu was achieved by 10% sulphuric acid. After the extraction of Cu, the extraction of Cr was carried out with NaD2EHPA. The McCabe-Thiele diagram for Cr extraction with 0.5 M NaD2EHPA at pH 3.0 showed two stages at A:O ratio of 1:1. The loaded organic of Cr was stripped with a mixture of sodium carbonate, sodium hydroxide and hydrogen peroxide. (Authors)., Copper-chromium catalyst has been used in many chemical processes and dumped in landfill after losing its catalytic property. Owing to the toxicity of Cr the dumping of catalyst is not environmentally acceptable, so metal values should be removed before disposal. One typical Cu-Cr catalyst was leached with sulphuric acid and from the leach liquor Cu and Cr were extracted using LIX 860N and NaD2EHPA, respectively. The McCabe-Thiele diagram at pH 3.5 with 20% LIX 860N indicated two stages at A:O=1:1 for quantitative extraction of Cu. The stripping of Cu was achieved by 10% sulphuric acid. After the extraction of Cu, the extraction of Cr was carried out with NaD2EHPA. The McCabe-Thiele diagram for Cr extraction with 0.5 M NaD2EHPA at pH 3.0 showed two stages at A:O ratio of 1:1. The loaded organic of Cr was stripped with a mixture of sodium carbonate, sodium hydroxide and hydrogen peroxide. (Authors).

57. Solvent extraction of zinc, manganese, cobalt and nickel from nickel laterite bacterial leach liquor using sodium salts of TOPS-99 and Cyanex 272.

Author

Mishra R.K., Nathsarma K.C., Rout P.C., Sarangi K., Mishra R.K., Nathsarma K.C., Rout P.C., and Sarangi K.

Abstract

In India there is no primary nickel source but the chromite overburden of Sukinda in Odisha contains 0.3-0.9% Ni. Bacterial leaching produced a liquor containing 3.72 g/l Fe, 2.08 g/l Al, 0.22 g/l Cr, 0.14 g/l Zn, 0.13 g/l Mn, 0.02 g/l Co and 0.44 g/l Ni, for whose separation solvent extraction was considered the most suitable technique to investigate as there were a number of studies in the literature on extracting metals such as Mn, Zn and Ni from spent batteries. Initial precipitation with CaCO3 at pH 4.4 removed 100% of Fe, 96.98% of Al and 70.42% of Cr, the remaining Al and Cr being precipitated with 50% ammonia at pH 5.4. Extraction of Zn was then carried out with 0.1 mol/l TOPS-99, followed by Mn extraction with 0.04 mol/l NaTOPS-99; yields were 97.77% of Zn and 95.63% of Mn. Co was removed using 0.0125 mol/l NaCyanex 272 and finally Ni was extracted by 0.12 mol/l NaTOPS-99 with 99.84% yield.The loaded organic phases were stripped with dilute H2SO4. The sodium-salt extractants were prepared by saponifying commercial di(2-ethylhexyl)phosphoric acid (TOPS-99) and bis(2,4,4-trimethylpentyl)phosphinic acid (Cyanex 272) with sodium hydroxide solution., In India there is no primary nickel source but the chromite overburden of Sukinda in Odisha contains 0.3-0.9% Ni. Bacterial leaching produced a liquor containing 3.72 g/l Fe, 2.08 g/l Al, 0.22 g/l Cr, 0.14 g/l Zn, 0.13 g/l Mn, 0.02 g/l Co and 0.44 g/l Ni, for whose separation solvent extraction was considered the most suitable technique to investigate as there were a number of studies in the literature on extracting metals such as Mn, Zn and Ni from spent batteries. Initial precipitation with CaCO3 at pH 4.4 removed 100% of Fe, 96.98% of Al and 70.42% of Cr, the remaining Al and Cr being precipitated with 50% ammonia at pH 5.4. Extraction of Zn was then carried out with 0.1 mol/l TOPS-99, followed by Mn extraction with 0.04 mol/l NaTOPS-99; yields were 97.77% of Zn and 95.63% of Mn. Co was removed using 0.0125 mol/l NaCyanex 272 and finally Ni was extracted by 0.12 mol/l NaTOPS-99 with 99.84% yield.The loaded organic phases were stripped with dilute H2SO4. The sodium-salt extractants were prepared by saponifying commercial di(2-ethylhexyl)phosphoric acid (TOPS-99) and bis(2,4,4-trimethylpentyl)phosphinic acid (Cyanex 272) with sodium hydroxide solution.

58. A comparative study on extraction of Fe(III) from chloride leach liquor using TBP, Cyanex 921 and Cyanex 923.

Author

Mishra R.K., Nathsarma K.C., Rout P.C., Sarangi K., Mishra R.K., Nathsarma K.C., Rout P.C., and Sarangi K.

Abstract

A comparative study was carried out on the extraction of Fe(III) from the hydrochloric acid leach liquor of low-grade iron ore tailings using tri-n-butyl phosphate (TBP), Cyanex 921 (trioctylphosphine oxide) and Cyanex 923 (tertiary octyl and hexyl phosphine oxide mixture) in distilled kerosene. The percentage extraction of iron increased with increasing hydrochloric acid and extractant concentrations. The extraction efficiencies for Fe(III) were in the order TBP less than Cyanex 921 less than Cyanex 923, but the stripping of iron from the loaded Cyanex 923 was the least at 94.9%, compared with 99.8% from TBP and more than 99.9% from Cyanex 921. The extracted species in each case was found to be HFeCl4.S (where S is a molecule of extractant) and the Fourier transform infrared (FTIR) spectra indicated the interaction of the PO double bond with HFeCl4., A comparative study was carried out on the extraction of Fe(III) from the hydrochloric acid leach liquor of low-grade iron ore tailings using tri-n-butyl phosphate (TBP), Cyanex 921 (trioctylphosphine oxide) and Cyanex 923 (tertiary octyl and hexyl phosphine oxide mixture) in distilled kerosene. The percentage extraction of iron increased with increasing hydrochloric acid and extractant concentrations. The extraction efficiencies for Fe(III) were in the order TBP less than Cyanex 921 less than Cyanex 923, but the stripping of iron from the loaded Cyanex 923 was the least at 94.9%, compared with 99.8% from TBP and more than 99.9% from Cyanex 921. The extracted species in each case was found to be HFeCl4.S (where S is a molecule of extractant) and the Fourier transform infrared (FTIR) spectra indicated the interaction of the PO double bond with HFeCl4.

59. Measurement of the 76Ge(n, γ) cross section at the n_TOF facility at CERN

Author

Gawlik-Ramiega A., Lederer-Woods C., Krticka M., Valenta S., Battino U., Andrzejewski J., Perkowski J., Aberle O., Audouin L., Bacak M., Balibrea J., Barbagallo M., Barros S., Becares V., Becvar F., Beinrucker C., Berthoumieux E., Billowes J., Bosnar D., Brugger M., Caamano M., Calvino F., Calviani M., Cano-Ott D., Cardella R., Casanovas A., Castelluccio D. M., Cerutti F., Chen Y. H., Chiaveri E., Colonna N., Cortes G., Cortes-Giraldo M. A., Cosentino L., Damone L. A., Diakaki M., Dietz M., Domingo-Pardo C., Dressler R., Dupont E., Duran I., Fernandez-Dominguez B., Ferrari A., Ferreira P., Finocchiaro P., Furman V., Gobel K., Garcia A. R., Glodariu T., Goncalves I. F., Gonzalez-Romero E., Goverdovski A., Griesmayer E., Guerrero C., Gunsing F., Harada H., Heftrich T., Heinitz S., Heyse J., Jenkins D. G., Jericha E., Kappeler F., Kadi Y., Katabuchi T., Kavrigin P., Ketlerov V., Khryachkov V., Kimura A., Kivel N., Knapova I., Kokkoris M., Leal-Cidoncha E., Leeb H., Lerendegui-Marco J., Lo Meo S., Lonsdale S. J., Losito R., Macina D., Martinez T., Massimi C., Mastinu P., Mastromarco M., Matteucci F., Maugeri E. A., Mendoza E., Mengoni A., Milazzo P. M., Mingrone F., Mirea M., Montesano S., Musumarra A., Nolte R., Oprea A., Patronis N., Pavlik A., Porras J. I., Praena J., Quesada J. M., Rajeev K., Rauscher T., Reifarth R., Riego-Perez A., Rout P. C., Rubbia C., Ryan J. A., Sabate-Gilarte M., Saxena A., Schillebeeckx P., Schmidt S., Schumann D., Sedyshev P., Smith A. G., Stamatopoulos A., Tagliente G., Tain J. L., Tarifeno-Saldivia A., Tassan-Got L., Tattersall A., Tsinganis A., Vannini G., Variale V., Vaz P., Ventura A., Vlachoudis V., Vlastou R., Wallner A., Warren S., Weigand M., Weiss C., Wolf C., Woods P. J., Wright T., Zugec P., Gawlik-Ramiega A., Lederer-Woods C., Krticka M., Valenta S., Battino U., Andrzejewski J., Perkowski J., Aberle O., Audouin L., Bacak M., Balibrea J., Barbagallo M., Barros S., Becares V., Becvar F., Beinrucker C., Berthoumieux E., Billowes J., Bosnar D., Brugger M., Caamano M., Calvino F., Calviani M., Cano-Ott D., Cardella R., Casanovas A., Castelluccio D.M., Cerutti F., Chen Y.H., Chiaveri E., Colonna N., Cortes G., Cortes-Giraldo M.A., Cosentino L., Damone L.A., Diakaki M., Dietz M., Domingo-Pardo C., Dressler R., Dupont E., Duran I., Fernandez-Dominguez B., Ferrari A., Ferreira P., Finocchiaro P., Furman V., Gobel K., Garcia A.R., Glodariu T., Goncalves I.F., Gonzalez-Romero E., Goverdovski A., Griesmayer E., Guerrero C., Gunsing F., Harada H., Heftrich T., Heinitz S., Heyse J., Jenkins D.G., Jericha E., Kappeler F., Kadi Y., Katabuchi T., Kavrigin P., Ketlerov V., Khryachkov V., Kimura A., Kivel N., Knapova I., Kokkoris M., Leal-Cidoncha E., Leeb H., Lerendegui-Marco J., Lo Meo S., Lonsdale S.J., Losito R., Macina D., Martinez T., Massimi C., Mastinu P., Mastromarco M., Matteucci F., Maugeri E.A., Mendoza E., Mengoni A., Milazzo P.M., Mingrone F., Mirea M., Montesano S., Musumarra A., Nolte R., Oprea A., Patronis N., Pavlik A., Porras J.I., Praena J., Quesada J.M., Rajeev K., Rauscher T., Reifarth R., Riego-Perez A., Rout P.C., Rubbia C., Ryan J.A., Sabate-Gilarte M., Saxena A., Schillebeeckx P., Schmidt S., Schumann D., Sedyshev P., Smith A.G., Stamatopoulos A., Tagliente G., Tain J.L., Tarifeno-Saldivia A., Tassan-Got L., Tattersall A., Tsinganis A., Vannini G., Variale V., Vaz P., Ventura A., Vlachoudis V., Vlastou R., Wallner A., Warren S., Weigand M., Weiss C., Wolf C., Woods P.J., Wright T., and Zugec P.

Subjects
Physics::Instrumentation and Detectors, Astrophysics::High Energy Astrophysical Phenomena, s process, stellar nuceosinthesys, TOF, Nuclear Experiment
Abstract

The 76Ge(n, γ ) reaction has been measured at the n_TOF facility at CERN via the time-of-flight technique. Neutron capture cross sections on 76Ge are of interest to a variety of low-background experiments, such as neutrinoless double β decay searches, and to nuclear astrophysics. We have determined resonance capture kernels up to 52 keV neutron energy and used the new data to calculate Maxwellian-averaged neutron capture cross sections for kBT values of 5 to 100 keV.

Published
2021

60. Role of the cluster structure of 7Li in the dynamics of fragment capture

Author

Shrivastava, A., Navin, A., Diaz-Torres, A., Nanal, V., Ramachandran, K., Rejmund, M., Bhattacharyya, S., Chatterjee, A., Kailas, S., Lemasson, A., Palit, R., Parkar, V.V., Pillay, R.G., Rout, P.C., and Sawant, Y.

Subjects
*MICROCLUSTERS, *TRAJECTORY optimization, *MOLECULAR dynamics, *LITHIUM, *NUCLEAR cross sections, *COULOMB functions
Abstract

Abstract: Exclusive measurements of prompt γ-rays from the heavy-residues with various light charged particles in the 7Li+ 198Pt system, at an energy near the Coulomb barrier () are reported. Recent dynamic classical trajectory calculations, constrained by the measured fusion, α- and t-capture cross-sections have been used to explain the excitation energy dependence of the residue cross-sections. These calculations distinctly illustrate a two-step process, breakup followed by fusion, in case of the capture of t and α clusters; whereas for and configurations, massive transfer is inferred to be the dominant mechanism. The present work clearly demonstrates the role played by the cluster structures of 7Li in understanding the reaction dynamics at energies around the Coulomb barrier. [Copyright &y& Elsevier]

Published
2013
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61. Measurement of the Ge 70 (n,γ) cross section up to 300 keV at the CERN n-TOF facility

Author

Gawlik A., Lederer-Woods C., Andrzejewski J., Battino U., Ferreira P., Gunsing F., Heinitz S., Krticka M., Massimi C., Mingrone F., Perkowski J., Reifarth R., Tattersall A., Valenta S., Weiss C., Aberle O., Audouin L., Bacak M., Balibrea J., Barbagallo M., Barros S., Becares V., Becvar F., Beinrucker C., Berthoumieux E., Billowes J., Bosnar D., Brugger M., Caamano M., Calvino F., Calviani M., Cano-Ott D., Cardella R., Casanovas A., Castelluccio D. M., Cerutti F., Chen Y. H., Chiaveri E., Colonna N., Cortes G., Cortes-Giraldo M. A., Cosentino L., Damone L. A., Diakaki M., Dietz M., Domingo-Pardo C., Dressler R., Dupont E., Duran I., Fernandez-Dominguez B., Ferrari A., Finocchiaro P., Furman V., Gobel K., Garcia A. R., Glodariu T., Goncalves I. F., Gonzalez-Romero E., Goverdovski A., Griesmayer E., Guerrero C., Harada H., Heftrich T., Heyse J., Jenkins D. G., Jericha E., Kappeler F., Kadi Y., Katabuchi T., Kavrigin P., Ketlerov V., Khryachkov V., Kimura A., Kivel N., Knapova I., Kokkoris M., Leal-Cidoncha E., Leeb H., Lerendegui-Marco J., Lo Meo S., Lonsdale S. J., Losito R., MacIna D., Marganiec J., Martinez T., Mastinu P., Mastromarco M., Matteucci F., Maugeri E. A., Mendoza E., Mengoni A., Milazzo P. M., Mirea M., Montesano S., Musumarra A., Nolte R., Oprea A., Patronis N., Pavlik A., Porras J. I., Praena J., Quesada J. M., Rajeev K., Rauscher T., Riego-Perez A., Rout P. C., Rubbia C., Ryan J. A., Sabate-Gilarte M., Saxena A., Schillebeeckx P., Schmidt S., Schumann D., Sedyshev P., Smith A. G., Stamatopoulos A., Tagliente G., Tain J. L., Tarifeno-Saldivia A., Tassan-Got L., Tsinganis A., Vannini G., Variale V., Vaz P., Ventura A., Vlachoudis V., Vlastou R., Wallner A., Warren S., Weigand M., Wolf C., Woods P. J., Wright T., Zugec P., Gawlik A., Lederer-Woods C., Andrzejewski J., Battino U., Ferreira P., Gunsing F., Heinitz S., Krticka M., Massimi C., Mingrone F., Perkowski J., Reifarth R., Tattersall A., Valenta S., Weiss C., Aberle O., Audouin L., Bacak M., Balibrea J., Barbagallo M., Barros S., Becares V., Becvar F., Beinrucker C., Berthoumieux E., Billowes J., Bosnar D., Brugger M., Caamano M., Calvino F., Calviani M., Cano-Ott D., Cardella R., Casanovas A., Castelluccio D.M., Cerutti F., Chen Y.H., Chiaveri E., Colonna N., Cortes G., Cortes-Giraldo M.A., Cosentino L., Damone L.A., Diakaki M., Dietz M., Domingo-Pardo C., Dressler R., Dupont E., Duran I., Fernandez-Dominguez B., Ferrari A., Finocchiaro P., Furman V., Gobel K., Garcia A.R., Glodariu T., Goncalves I.F., Gonzalez-Romero E., Goverdovski A., Griesmayer E., Guerrero C., Harada H., Heftrich T., Heyse J., Jenkins D.G., Jericha E., Kappeler F., Kadi Y., Katabuchi T., Kavrigin P., Ketlerov V., Khryachkov V., Kimura A., Kivel N., Knapova I., Kokkoris M., Leal-Cidoncha E., Leeb H., Lerendegui-Marco J., Lo Meo S., Lonsdale S.J., Losito R., MacIna D., Marganiec J., Martinez T., Mastinu P., Mastromarco M., Matteucci F., Maugeri E.A., Mendoza E., Mengoni A., Milazzo P.M., Mirea M., Montesano S., Musumarra A., Nolte R., Oprea A., Patronis N., Pavlik A., Porras J.I., Praena J., Quesada J.M., Rajeev K., Rauscher T., Riego-Perez A., Rout P.C., Rubbia C., Ryan J.A., Sabate-Gilarte M., Saxena A., Schillebeeckx P., Schmidt S., Schumann D., Sedyshev P., Smith A.G., Stamatopoulos A., Tagliente G., Tain J.L., Tarifeno-Saldivia A., Tassan-Got L., Tsinganis A., Vannini G., Variale V., Vaz P., Ventura A., Vlachoudis V., Vlastou R., Wallner A., Warren S., Weigand M., Wolf C., Woods P.J., Wright T., Zugec P., Gawlik, A., Lederer-Woods, C., Andrzejewski, J., Battino, U., Ferreira, P., Gunsing, F., Heinitz, S., Krticka, M., Massimi, C., Mingrone, F., Perkowski, J., Reifarth, R., Tattersall, A., Valenta, S., Weiss, C., Aberle, O., Audouin, L., Bacak, M., Balibrea, J., Barbagallo, M., Barros, S., Becares, V., Becvar, F., Beinrucker, C., Berthoumieux, E., Billowes, J., Bosnar, D., Brugger, M., Caamano, M., Calvino, F., Calviani, M., Cano-Ott, D., Cardella, R., Casanovas, A., Castelluccio, D. M., Cerutti, F., Chen, Y. H., Chiaveri, E., Colonna, N., Cortes, G., Cortes-Giraldo, M. A., Cosentino, L., Damone, L. A., Diakaki, M., Dietz, M., Domingo-Pardo, C., Dressler, R., Dupont, E., Duran, I., Fernandez-Dominguez, B., Ferrari, A., Finocchiaro, P., Furman, V., Gobel, K., Garcia, A. R., Glodariu, T., Goncalves, I. F., Gonzalez-Romero, E., Goverdovski, A., Griesmayer, E., Guerrero, C., Harada, H., Heftrich, T., Heyse, J., Jenkins, D. G., Jericha, E., Kappeler, F., Kadi, Y., Katabuchi, T., Kavrigin, P., Ketlerov, V., Khryachkov, V., Kimura, A., Kivel, N., Knapova, I., Kokkoris, M., Leal-Cidoncha, E., Leeb, H., Lerendegui-Marco, J., Lo Meo, S., Lonsdale, S. J., Losito, R., Macina, D., Marganiec, J., Martinez, T., Mastinu, P., Mastromarco, M., Matteucci, F., Maugeri, E. A., Mendoza, E., Mengoni, A., Milazzo, P. M., Mirea, M., Montesano, S., Musumarra, A., Nolte, R., Oprea, A., Patronis, N., Pavlik, A., Porras, J. I., Praena, J., Quesada, J. M., Rajeev, K., Rauscher, T., Riego-Perez, A., Rout, P. C., Rubbia, C., Ryan, J. A., Sabate-Gilarte, M., Saxena, A., Schillebeeckx, P., Schmidt, S., Schumann, D., Sedyshev, P., Smith, A. G., Stamatopoulos, A., Tagliente, G., Tain, J. L., Tarifeno-Saldivia, A., Tassan-Got, L., Tsinganis, A., Vannini, G., Variale, V., Vaz, P., Ventura, A., Vlachoudis, V., Vlastou, R., Wallner, A., Warren, S., Weigand, M., Wolf, C., Woods, P. J., Wright, T., and Zugec, P.

Subjects
Astrophysics::High Energy Astrophysical Phenomena, s process TOF neutron cross section, Astrophysics::Solar and Stellar Astrophysics, Nuclear Experiment
Abstract

Neutron capture data on intermediate mass nuclei are of key importance to nucleosynthesis in the weak component of the slow neutron capture processes, which occurs in massive stars. The (n,γ) cross section on Ge70, which is mainly produced in the s process, was measured at the neutron time-of-flight facility n-TOF at CERN. Resonance capture kernels were determined up to 40 keV neutron energy and average cross sections up to 300 keV. Stellar cross sections were calculated from kT=5 keV to kT=100 keV and are in very good agreement with a previous measurement by Walter and Beer (1985) and recent evaluations. Average cross sections are in agreement with Walter and Beer (1985) over most of the neutron energy range covered, while they are systematically smaller for neutron energies above 150 keV. We have calculated isotopic abundances produced in s-process environments in a 25 solar mass star for two initial metallicities (below solar and close to solar). While the low metallicity model reproduces best the solar system germanium isotopic abundances, the close to solar model shows a good global match to solar system abundances in the range of mass numbers A=60-80.

Published
2019

62. New measurement of the 242Pu(n,γ) cross section at n-TOF-EAR1 for MOX fuels: Preliminary results in the RRR

Author

Simone Gilardoni, P. C. Rout, Ignacio Porras, Rene Reifarth, J. Billowes, C. Lederer, E. Leal-Cidoncha, J. M. Quesada, L. Tassan-Got, A. Gawlik, Thomas Rauscher, R. Cardella, P. Vaz, P. Schillebeeckx, M. Diakaki, A. Casanovas, Alberto Ventura, A. Mengoni, M. Kokkoris, Hideo Harada, J. Marganiec, G. Vannini, M. Caamaño, A. Oprea, J. Heyse, N. Patronis, L. Cosentino, M. Sabaté-Gilarte, S. Warren, E. A. Maugeri, A. Pavlik, M. A. Cortés-Giraldo, C. Domingo-Pardo, F. Cerutti, Ariel Tarifeño-Saldivia, S. J. Lonsdale, E. Mendoza, E. Jericha, R. Nolte, S. Valenta, P. F. Mastinu, T. Glodariu, J. Lerendegui-Marco, V. Variale, Arnd R. Junghans, A. R. García, Paolo Finocchiaro, Marco Calviani, A. Kimura, J. A. Ryan, A. Saxena, A. G. Smith, P. M. Milazzo, I. F. Gonçalves, M. Mastromarco, Philip Woods, F. Calviño, H. Leeb, A. S. Brown, Anton Wallner, R. Vlastou, J. Perkowski, M. B. Gómez-Hornillos, I. Duran, Javier Praena, S. Lo Meo, F. Gunsing, P. Ferreira, Y. H. Chen, Mario Barbagallo, D. Schumann, F. Mingrone, J. Andrzejewski, J. Balibrea, E. Chiaveri, A. Masi, G. Tagliente, S. Heinitz, Damir Bosnar, D. Cano-Ott, Carlo Rubbia, G. Cortes, Cristian Massimi, A. Stamatopoulos, Y. Kadi, D. G. Jenkins, K. Göbel, R. Dressler, V. Vlachoudis, D. Macina, P. Kavrigin, Alfredo Ferrari, E. González, T. Wright, E. Griesmayer, L. A. Damone, M. Krtička, O. Aberle, T. Martinez, N. V. Sosnin, Annamaria Mazzone, Petar Žugec, B. Fernández-Domínguez, J. L. Tain, Alexandru Negret, F. Käppeler, N. Kivel, Klaus Eberhardt, D. Radeck, E. Berthoumieux, L. Audouin, A. Kalamara, A. Musumarra, Deniz Kurtulgil, Nicola Colonna, Carlos Guerrero, E. Dupont, F. Bečvář, M. Bacak, Institut de Physique Nucléaire d'Orsay (IPNO), Université Paris-Sud - Paris 11 (UP11)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Centre National de la Recherche Scientifique (CNRS), Institut de Recherches sur les lois Fondamentales de l'Univers (IRFU), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay, n_TOF, Mengoni, A., Centre National de la Recherche Scientifique (CNRS)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Paris-Sud - Paris 11 (UP11), Universidad de Sevilla. Departamento de Física Atómica, Molecular y Nuclear, Ministerio de Economía y Competitividad (MINECO). España, Lerendegui-Marco, J., Guerrero, C., Cortés-Giraldo, M.A., Quesada, J.M., Mendoza, E., Cano-Ott, D., Eberhardt, K., Junghans, A., Aberle, O., Andrzejewski, J., Audouin, L., Bacak, M., Balibrea, J., Barbagallo, M., Bečvář, F., Berthoumieux, E., Billowes, J., Bosnar, D., Brown, A., Caamaño, M., Calviño, F., Calviani, M., Cardella, R., Casanovas, A., Cerutti, F., Chen, Y.H., Chiaveri, E., Colonna, N., Cortés, G., Cosentino, L., Damone, L.A., Diakaki, M., Domingo-Pardo, C., Dressler, R., Dupont, E., Durán, I., Fernández-Domínguez, B., Ferrari, A., Ferreira, P., Finocchiaro, P., Göbel, K., Gómez-Hornillos, M.B., García, A.R., Gawlik, A., Gilardoni, S., Glodariu, T., Gonçalves, I.F., González, E., Griesmayer, E., Gunsing, F., Harada, H., Heinitz, S., Heyse, J., Jenkins, D.G., Jericha, E., Käppeler, F., Kadi, Y., Kalamara, A., Kavrigin, P., Kimura, A., Kivel, N., Kokkoris, M., Krtička, M., Kurtulgil, D., Leal-Cidoncha, E., Lederer, C., Leeb, H., Meo, S. Lo, Lonsdale, S.J., Macina, D., Marganiec, J., Martínez, T., Masi, A., Massimi, C., Mastinu, P., Mastromarco, M., Maugeri, E.A., Mazzone, A., Milazzo, P.M., Mingrone, F., Musumarra, A., Negret, A., Nolte, R., Oprea, A., Patronis, N., Pavlik, A., Perkowski, J., Porras, I., Praena, J., Radeck, D., Rauscher, T., Reifarth, R., Rout, P.C., Rubbia, C., Ryan, J.A., Sabaté-Gilarte, M., Saxena, A., Schillebeeckx, P., Schumann, D., Smith, A.G., Sosnin, N.V., Stamatopoulos, A., Tagliente, G., Tain, J.L., Tarifeño-Saldivia, A., Tassan-Got, L., Valenta, S., Vannini, G., Variale, V., Vaz, P., Ventura, A., Vlachoudis, V., Vlastou, R., Wallner, A., Warren, S., Woods, P.J., Wright, T., Ž Ugec, P., Universitat Politècnica de Catalunya. Departament de Física, Universitat Politècnica de Catalunya. Institut de Tècniques Energètiques, Universitat Politècnica de Catalunya. Departament de Física i Enginyeria Nuclear, and Universitat Politècnica de Catalunya. ANT - Advanced Nuclear Technologies Research Group

Subjects
Nuclear reaction, nTOF, QC1-999, Nuclear engineering, Context (language use), CERN nTOF, Neutron, [PHYS.NEXP]Physics [physics]/Nuclear Experiment [nucl-ex], 01 natural sciences, 7. Clean energy, Physics and Astronomy (all), Nuclear reactors, Reactors nuclears, 0103 physical sciences, CERN, Neutron cross section, Nuclear Physics - Experiment, ddc:530, 242Pu neutron capture, 010306 general physics, MOX fuel, Neutrons, Energies::Energia nuclear [Àrees temàtiques de la UPC], Fissile material, Cross section, Física [Àrees temàtiques de la UPC], 010308 nuclear & particles physics, Physics, Spent nuclear fuel, Neutron temperature, 13. Climate action, neutron time-of-flight measurement
Abstract

The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with 238U to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. The use of MOX fuels in thermal and fast reactors requires accurate capture and fission cross sections. For the particular case of 242Pu, the previous neutron capture cross section measurements were made in the 70’s, providing an uncertainty of about 35% in the keV region. In this context, the Nuclear Energy Agency recommends in its “High Priority Request List” and its report WPEC-26 that the capture cross section of 242Pu should be measured with an accuracy of at least 7–12% in the neutron energy range between 500 eV and 500 keV. This work presents a brief description of the measurement performed at n TOF-EAR1, the data reduction process and the first ToF capture measurement on this isotope in the last 40 years, providing preliminary individual resonance parameters beyond the current energy limits in the evaluations, as well as a preliminary set of average resonance parameters., This measurement has received funding from the EC FP7 Programme under the projects NEUTANDALUS (Grant No. 334315) and CHANDA (Grant No. 605203), and the Spanish Ministry of Economy and Competitiveness projects FPA2013- 45083-P and FPA2014-53290-C2-2-P.

Published
2017

63. Characterization of the n-TOF EAR-2 neutron beam

Author

M. Sabaté-Gilarte, Enrique Casarejos, F. Gunsing, A. Musumarra, Cristian Massimi, A. Pavlik, P. Ferreira, C. Domingo-Pardo, P. M. Milazzo, N. Kivel, M. Krtička, R. Nolte, G. Tagliente, M. A. Cortés-Giraldo, Ariel Tarifeño-Saldivia, S. J. Lonsdale, P. C. Rout, M. Caamaño, F. Cerutti, Alfredo Ferrari, R. Cardella, T. Martinez, Javier Praena, S. Lo Meo, K. Göbel, C. Lederer, G. Vannini, S. Warren, A. Kimura, Tatsuya Katabuchi, E. Leal-Cidoncha, Tanja Heftrich, F. Mingrone, J. Andrzejewski, Mario Weigand, V. Variale, J. Marganiec, O. Aberle, T. Wright, E. Chiaveri, D. Cano-Ott, D. Macina, J. L. Tain, Carlo Rubbia, E. González, V. Vlachoudis, S. Barros, A. Gawlik, M. Kokkoris, J. I. Porras, Thomas Rauscher, Rene Reifarth, D. M. Castelluccio, A. Riego-Perez, J. Lerendegui-Marco, Stefan Schmidt, Mario Barbagallo, P. F. Mastinu, V. Khryachkov, M. Mirea, D. Schumann, P. Vaz, L. Cosentino, J. M. Quesada, C. Le Naour, L. Tassan-Got, Alberto Ventura, I. F. Gonçalves, M. Bacak, D. G. Jenkins, F. Käppeler, E. Mendoza, V. Bécares, F. Calviño, H. Leeb, A. Oprea, G. Cortes, A. Casanovas, J. Perkowski, S. Montesano, Y. H. Chen, J. Heyse, A. R. García, M. B. Gómez-Hornillos, B. Fernández-Domínguez, S. Heinitz, N. Patronis, Carlos Guerrero, M. Brugger, I. Duran, S. Valenta, Marco Calviani, A. Stamatopoulos, C. Beinrucker, A. Saxena, E. Jericha, C. Wolf, A. G. Smith, Roberto Losito, T. Glodariu, Paolo Finocchiaro, K. Rajeev, Philip Woods, Alberto Mengoni, J. A. Ryan, P. Schillebeeckx, Francesca Matteucci, V. Ketlerov, C. Weiss, R. Vlastou, A. Goverdovski, R. Dressler, A. Tsinganis, Damir Bosnar, Y. Kadi, P. Kavrigin, P. V. Sedyshev, F. Bečvář, Nicola Colonna, Hideo Harada, E. Dupont, J. Billowes, E. Griesmayer, M. Mastromarco, L. A. Damone, M. S. Robles, Anton Wallner, E. A. Maugeri, J. Balibrea, L. Audouin, M. Diakaki, E. Berthoumieux, V. Furman, Petar Žugec, Institut de Physique Nucléaire d'Orsay (IPNO), Université Paris-Sud - Paris 11 (UP11)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Centre National de la Recherche Scientifique (CNRS), Institut de Recherches sur les lois Fondamentales de l'Univers (IRFU), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay, n_TOF, Universitat Politècnica de Catalunya. Departament de Física, Universitat Politècnica de Catalunya. Institut de Tècniques Energètiques, Universitat Politècnica de Catalunya. ANT - Advanced Nuclear Technologies Research Group, Universitat Politècnica de Catalunya. NEMEN - Nanoenginyeria de materials aplicats a l'energia, Universidad de Sevilla. Departamento de Física Atómica, Molecular y Nuclear, Gobierno de España, Centre National de la Recherche Scientifique (CNRS)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Paris-Sud - Paris 11 (UP11), Chen, Y.H., Tassan-Got, L., Audouin, L., Le Naour, C., Durán, I., Casarejos, E., Aberle, O., Andrzejewski, J., Bécares, V., Bacak, M., Balibrea, J., Barbagallo, M., Barros, S., Bečvář, F., Beinrucker, C., Berthoumieux, E., Billowes, J., Bosnar, D., Brugger, M., Caamaño, M., Calviño, F., Calviani, M., Cano-Ott, D., Cardella, R., Casanovas, A., Castelluccio, D.M., Cerutti, F., Chiaveri, E., Colonna, N., Cortés, G., Cortés-Giraldo, M.A., Cosentino, L., Damone, L.A., Diakaki, M., Domingo-Pardo, C., Dressler, R., Dupont, E., Fernández-Domínguez, B., Ferrari, A., Ferreira, P., Finocchiaro, P., Furman, V., Göbel, K., Gómez-Hornillos, M.B., García, A.R., Gawlik, A., Glodariu, T., Gonçalves, I.F., González, E., Goverdovski, A., Griesmayer, E., Guerrero, C., Gunsing, F., Harada, H., Heftrich, T., Heinitz, S., Heyse, J., Jenkins, D.G., Jericha, E., Käppeler, F., Kadi, Y., Katabuchi, T., Kavrigin, P., Ketlerov, V., Khryachkov, V., Kimura, A., Kivel, N., Kokkoris, M., Krtička, M., Leal-Cidoncha, E., Lederer, C., Leeb, H., Lerendegui-Marco, J., Meo, S. Lo, Lonsdale, S.J., Losito, R., Macina, D., Marganiec, J., Martínez, T., Massimi, C., Mastinu, P., Mastromarco, M., Matteucci, F., Maugeri, E.A., Mendoza, E., Mengoni, A., Milazzo, P.M., Mingrone, F., Mirea, M., Montesano, S., Musumarra, A., Nolte, R., Oprea, A., Patronis, N., Pavlik, A., Perkowski, J., Porras, J.I., Praena, J., Quesada, J.M., Rajeev, K., Rauscher, T., Reifarth, R., Riego-Perez, A., Robles, M., Rout, P.C., Rubbia, C., Ryan, J.A., Sabaté-Gilarte, M., Saxena, A., Schillebeeckx, P., Schmidt, S., Schumann, D., Sedyshev, P., Smith, A.G., Stamatopoulos, A., Tagliente, G., Tain, J.L., Tarifeño-Saldivia, A., Tsinganis, A., Valenta, S., Vannini, G., Variale, V., Vaz, P., Ventura, A., Vlachoudis, V., Vlastou, R., Wallner, A., Warren, S., Weigand, M., Weiss, C., Wolf, C., Woods, P.J., Wright, T., Ugec, P., and Lo Meo, S.

Subjects
nTOF, QC1-999, [PHYS.PHYS.PHYS-ACC-PH]Physics [physics]/Physics [physics]/Accelerator Physics [physics.acc-ph], Neutron, 01 natural sciences, Nuclear physics, Physics and Astronomy (all), CERN, 0103 physical sciences, ddc:530, 010306 general physics, Neutrons, Physics, Flux, Large Hadron Collider, Física [Àrees temàtiques de la UPC], 010308 nuclear & particles physics, Beam, Neutron radiation, Accelerators and Storage Rings, Parallel plate, Characterization (materials science), Beam (structure)
Abstract

The experimental area 2 (EAR-2) at CERNs neutron time-of-flight facility (n TOF), which is operational since 2014, is designed and built as a short-distance complement to the experimental area 1 (EAR-1). The Parallel Plate Avalanche Counter (PPAC) monitor experiment was performed to characterize the beam profile and the shape of the neutron flux at EAR-2. The prompt γ-flash which is used for calibrating the time-of-flight at EAR-1 is not seen by PPAC at EAR-2, shedding light on the physical origin of this γ-flash., The USC group contribution has been partly supported by Spanish grant FPA2013-46236-P.

Published
2017
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64. 7Be(n,α) and 7Be(n,p) cross-section measurement for the cosmological lithium problem at the n-TOF facility at CERN

Author

M. Mirea, J. Marganiec, F. Calviño, H. Leeb, V. Bécares, J. Perkowski, Petar Žugec, P. F. Mastinu, A. Musumarra, D. G. Jenkins, Tanja Heftrich, F. Gunsing, P. Vaz, V. Furman, Y. H. Chen, Tatsuya Katabuchi, A. Riego-Perez, L. Cosentino, Cristian Massimi, S. Heinitz, A. Casanovas, E. A. Maugeri, Alberto Ventura, A. Saxena, Ariel Tarifeño-Saldivia, S. J. Lonsdale, S. Barros, G. Vannini, C. Wolf, J. Lerendegui-Marco, O. Aberle, F. Käppeler, A. Tsinganis, E. Berthoumieux, M. Krtička, I. F. Gonçalves, A. Kimura, Alfredo Ferrari, Mario Weigand, J. Billowes, N. Kivel, T. Martinez, Nicola Colonna, E. Dupont, M. A. Cortés-Giraldo, A. Stamatopoulos, E. Chiaveri, G. Cortes, D. Cano-Ott, Rene Reifarth, V. Khryachkov, E. González, Alberto Mengoni, P. Ferreira, Stefan Schmidt, Mario Barbagallo, D. Schumann, J. I. Porras, J. M. Quesada, L. Tassan-Got, F. Bečvář, R. Cardella, A. Pavlik, G. Tagliente, C. Domingo-Pardo, K. Rajeev, B. Fernández-Domínguez, Francesca Matteucci, E. Jericha, T. Glodariu, Paolo Finocchiaro, J. L. Tain, P. Schillebeeckx, M. Bacak, J. A. Ryan, M. Caamaño, M. Diakaki, F. Cerutti, Roberto Losito, P. V. Sedyshev, L. Audouin, A. Oprea, J. Heyse, Hideo Harada, D. M. Castelluccio, M. Mastromarco, Javier Praena, S. Lo Meo, Carlos Guerrero, Anton Wallner, S. Montesano, J. Balibrea, S. Warren, M. Sabaté-Gilarte, V. Variale, R. Nolte, A. Goverdovski, E. Leal-Cidoncha, A. Gawlik, Thomas Rauscher, P. C. Rout, C. Lederer, S. Valenta, F. Mingrone, J. Andrzejewski, Marco Calviani, Carlo Rubbia, V. Vlachoudis, A. G. Smith, V. Ketlerov, Philip Woods, P. M. Milazzo, C. Weiss, R. Vlastou, A. R. García, Damir Bosnar, Y. Kadi, M. Brugger, K. Göbel, C. Beinrucker, T. Wright, M. Kokkoris, N. Patronis, I. Duran, R. Dressler, P. Kavrigin, E. Griesmayer, L. A. Damone, E. Mendoza, D. Macina, Universidad de Sevilla. Departamento de Física Atómica, Molecular y Nuclear, Mengoni, A., Lo Meo, S., Castelluccio, D. M., Universitat Politècnica de Catalunya. Departament de Física, Universitat Politècnica de Catalunya. Institut de Tècniques Energètiques, Universitat Politècnica de Catalunya. ANT - Advanced Nuclear Technologies Research Group, Universitat Politècnica de Catalunya. NEMEN - Nanoenginyeria de materials aplicats a l'energia, Barbagallo, M., Colonna, N., Aberle, O., Andrzejewski, J., Audouin, L., Bécares, V., Bacak, M., Balibrea, J., Barros, S., Bečvář, F., Beinrucker, C., Berthoumieux, E., Billowes, J., Bosnar, D., Brugger, M., Caamaño, M., Calviño, F., Calviani, M., Cano-Ott, D., Cardella, R., Casanovas, A., Castelluccio, D.M., Cerutti, F., Chen, Y.H., Chiaveri, E., Cortés, G., Cortés-Giraldo, M.A., Cosentino, L., Damone, L.A., Diakaki, M., Domingo-Pardo, C., Dressler, R., Dupont, E., Durán, I., Fernández-Domínguez, B., Ferrari, A., Ferreira, P., Finocchiaro, P., Furman, V., Göbel, K., García, A.R., Gawlik, A., Glodariu, T., Gonçalves, I.F., González, E., Goverdovski, A., Griesmayer, E., Guerrero, C., Gunsing, F., Harada, H., Heftrich, T., Heinitz, S., Heyse, J., Jenkins, D.G., Jericha, E., Käppeler, F., Kadi, Y., Katabuchi, T., Kavrigin, P., Ketlerov, V., Khryachkov, V., Kimura, A., Kivel, N., Kokkoris, M., Krtička, M., Leal-Cidoncha, E., Lederer, C., Leeb, H., Lerendegui-Marco, J., Meo, S. Lo, Lonsdale, S.J., Losito, R., Macina, D., Marganiec, J., Martínez, T., Massimi, C., Mastinu, P., Mastromarco, M., Matteucci, F., Maugeri, E.A., Mendoza, E., Milazzo, P.M., Mingrone, F., Mirea, M., Montesano, S., Musumarra, A., Nolte, R., Oprea, A., Patronis, N., Pavlik, A., Perkowski, J., Porras, J.I., Praena, J., Quesada, J.M., Rajeev, K., Rauscher, T., Reifarth, R., Riego-Perez, A., Rout, P.C., Rubbia, C., Ryan, J.A., Sabaté-Gilarte, M., Saxena, A., Schillebeeckx, P., Schmidt, S., Schumann, D., Sedyshev, P., Smith, A.G., Stamatopoulos, A., Tagliente, G., Tain, J.L., Tarifeño-Saldivia, A., Tassan-Got, L., Tsinganis, A., Valenta, S., Vannini, G., Variale, V., Vaz, P., Ventura, A., Vlachoudis, V., Vlastou, R., Wallner, A., Warren, S., Weigand, M., Weiss, C., Wolf, C., Woods, P.J., Wright, T., and Ugec, P.

Subjects
Astrofísica, nTOF, QC1-999, chemistry.chemical_element, Neutron, Astrophysics, 01 natural sciences, 7. Clean energy, Nuclear physics, Physics and Astronomy (all), Big Bang nucleosynthesis, Nucleosynthesis, CERN, 0103 physical sciences, Nuclear astrophysics, Astrophysics::Solar and Stellar Astrophysics, 010306 general physics, Nuclear Experiment, Astrophysics::Galaxy Astrophysics, Energies::Energia nuclear [Àrees temàtiques de la UPC], Neutrons, Physics, Alpha, Large Hadron Collider, Física [Àrees temàtiques de la UPC], 010308 nuclear & particles physics, Stars, chemistry, Lithium, Halo, Nucleosíntesi
Abstract

One of the most puzzling problems in Nuclear Astrophysics is the “Cosmological Lithium Problem”, i.e the discrepancy between the primordial abundance of \(^{7}\)Li observed in metal poor halo stars (Asplund et al. in Astrophys J 644:229–259, 2006, [1]), and the one predicted by Big Bang Nucleosynthesis (BBN). One of the reactions that could have an impact on the problem is \(^{7}\)Be(n,p)\(^{7}\)Li. Despite of the importance of this reaction in BBN, the cross-section has never been directly measured at the energies of interest for BBN. Taking advantage of the innovative features of the second experimental area at the n\(\_\)TOF facility at CERN (Sabate-Gilarte et al. in Eur Phys J A 53:210, 2017, [2]; Weiss et al. in NIMA 799:90, 2015, [3]), an accurate measurement of \(^{7}\)Be(n,p) cross section has been recently performed at n\(\_\)TOF, with a pure \(^{7}\)Be target produced by implantation of a \(^{7}\)Be beam at ISOLDE. The mesurement started in April 2016 and lasted for two months. The experimental procedure, the setup used in the measurement and the results obtained so far will be here presented.

Published
2017

65. Time-of-flight and activation experiments on 147Pm and 171Tm for astrophysics

Author

E. Leal-Cidoncha, P. M. Milazzo, M. Mastromarco, Rene Reifarth, O. Aberle, Simone Gilardoni, A. Gawlik, J. M. Quesada-Molina, Thomas Rauscher, D. Radeck, Michael Paul, J. Marganiec, R. Cardella, E. Berthoumieux, Javier Praena, S. Lo Meo, Leonid Weissman, M. Diakaki, M. Kokkoris, A. S. Brown, L. Tassan-Got, Anton Wallner, M. Caamaño, F. Cerutti, M. Tessler, L. Cosentino, J. Balibrea, S. Valenta, G. Cortes, A. Stamatopoulos, Deniz Kurtulgil, A. Oprea, N. V. Sosnin, J. Heyse, Marco Calviani, F. Mingrone, J. Andrzejewski, A. G. Smith, A. Kimura, D. Macina, Ariel Tarifeño-Saldivia, S. J. Lonsdale, J. L. Tain, A. Saxena, A. R. García, F. Gunsing, N. Patronis, Annamaria Mazzone, Petar Žugec, M. Bacak, I. Duran, P. Schillebeeckx, Philip Woods, S. Halfon, A. Casanovas, P. F. Mastinu, Ulli Köster, J. Lerendegui-Marco, P. Ferreira, Hideo Harada, Alfredo Ferrari, Mario Barbagallo, S. Warren, R. Dressler, Cristian Massimi, V. Variale, A. Kalamara, C. Weiss, D. Schumann, R. Vlastou, G. Tagliente, P. Kavrigin, I. F. Gonçalves, M. Sabaté-Gilarte, P. C. Rout, E. Mendoza, Y. H. Chen, Alexandru Negret, E. Griesmayer, R. Nolte, L. A. Damone, S. Heinitz, F. Becvar, A. Tsinganis, C. Lederer, A. Masi, E. Jericha, T. Glodariu, Paolo Finocchiaro, Damir Bosnar, Y. Kadi, F. Käppeler, J. A. Ryan, D. G. Jenkins, E. A. Maugeri, K. Göbel, N. Kivel, Ignacio Porras, Nicola Colonna, E. Dupont, G. Vannini, T. Wright, M. Krtička, E. González, M. A. Cortés-Giraldo, B. Fernández-Domínguez, T. Martinez, F. Calviño, L. Audouin, H. Leeb, Alberto Mengoni, J. Perkowski, Carlo Rubbia, V. Vlachoudis, Carlos Guerrero, P. Vaz, Alberto Ventura, A. Musumarra, E. Chiaveri, D. Cano-Ott, A. Pavlik, C. Domingo-Pardo, J. Billowes, Universitat Politècnica de Catalunya. Departament de Física, Universitat Politècnica de Catalunya. Institut de Tècniques Energètiques, Universitat Politècnica de Catalunya. ANT - Advanced Nuclear Technologies Research Group, Universitat Politècnica de Catalunya. NEMEN - Nanoenginyeria de materials aplicats a l'energia, Vannini, G., Mengoni, A., Lo Meo, S., Guerrero, C., Lerendegui-Marco, J., Domingo-Pardo, C., Casanovas, A., Dressler, R., Halfon, S., Heinitz, S., Kivel, N., Köster, U., Paul, M., Quesada-Molina, J.M., Schumann, D., Tarifeño-Saldivia, A., Tessler, M., Weissman, L., Aberle, O., Andrzejewski, J., Audouin, L., Bacak, M., Balibrea, J., Barbagallo, M., Becvar, F., Berthoumieux, E., Billowes, J., Bosnar, D., Brown, A., Caamaño, M., Calviño, F., Calviani, M., Cano-Ott, D., Cardella, R., Cerutti, F., Chen, Y.H., Chiaveri, E., Colonna, N., Cortés, G., Cortés-Giraldo, M.A., Cosentino, L., Damone, L.A., Diakaki, M., Dupont, E., Durán, I., Fernández-Domínguez, B., Ferrari, A., Ferreira, P., Finocchiaro, P., Göbel, K., García, A.R., Gawlik, A., Gilardoni, S., Glodariu, T., Gonçalves, I.F., González, E., Griesmayer, E., Gunsing, F., Harada, H., Heyse, J., Jenkins, D.G., Jericha, E., Käppeler, F., Kadi, Y., Kalamara, A., Kavrigin, P., Kimura, A., Kokkoris, M., Krticka, M., Kurtulgil, D., Leal-Cidoncha, E., Lederer, C., Leeb, H., Meo, S. Lo, Lonsdale, S.J., Macina, D., Marganiec, J., Martínez, T., Masi, A., Massimi, C., Mastinu, P., Mastromarco, M., Maugeri, E.A., Mazzone, A., Mendoza, E., Milazzo, P.M., Mingrone, F., Musumarra, A., Negret, A., Nolte, R., Oprea, A., Patronis, N., Pavlik, A., Perkowski, J., Porras, I., Praena, J., Radeck, D., Rauscher, T., Reifarth, R., Rout, P.C., Rubbia, C., Ryan, J.A., Sabaté-Gilarte, M., Saxena, A., Schillebeeckx, P., Smith, A.G., Sosnin, N.V., Stamatopoulos, A., Tagliente, G., Tain, J.L., Tassan-Got, L., Tsinganis, A., Valenta, S., Variale, V., Vaz, P., Ventura, A., Vlachoudis, V., Vlastou, R., Wallner, A., Warren, S., Weiss, C., Woods, P.J., Wright, T., Ugec, P., and Universidad de Sevilla. Departamento de Física Atómica, Molecular y Nuclear

Subjects
QC1-999, Neutron, Scintillator, 01 natural sciences, Nuclear physics, Physics and Astronomy (all), Stellar nucleosynthesis, Nucleosynthesis, 0103 physical sciences, Neutron cross section, 010306 general physics, Nuclear Experiment, Physics, Energies::Energia nuclear [Àrees temàtiques de la UPC], Neutrons, Isotope, Física [Àrees temàtiques de la UPC], 010308 nuclear & particles physics, Tof, Time of flight, Neutron capture, 13. Climate action, Nucleosíntesi
Abstract

The neutron capture cross section of several key unstable isotopes acting as branching points in the s-process are crucial for stellar nucleosynthesis studies, but they are very challenging to measure due to the difficult production of sufficient sample material, the high activity of the resulting samples, and the actual (n,γ ) measurement, for which high neutron fluxes and effective background rejection capabilities are required. As part of a new program to measure some of these important branching points, radioactive targets of 147Pm and 171Tm have been produced by irradiation of stable isotopes at the ILL high flux reactor. Neutron capture on 146Nd and 170Er at the reactor was followed by beta decay and the resulting matrix was purified via radiochemical separation at PSI. The radioactive targets have been used for time-of-flight measurements at the CERN n TOF facility using the 19 and 185m beam lines during 2014 and 2015. The capture cascades were detected using a set of four C6D6 scintillators, allowing to observe the associated neutron capture resonances. The results presented in this work are the first ever determination of the resonance capture cross section of 147Pm and 171Tm. Activation experiments on the same 147Pm and 171Tm targets with a high-intensity 30 keV quasi-Maxwellian flux of neutrons will be performed using the SARAF accelerator and the Liquid-Lithium Target (LiLiT) in order to extract the corresponding Maxwellian Average Cross Section (MACS). The status of these experiments and preliminary results will be presented and discussed as well., The authors acknowledge financial support by Spanish FPA2013-45083-P and FPA2014-53290-C2-2-P projects and the EC FP7 projects NeutAndalus (Grant No. 334315) and CHANDA (Grant No. 605203).

Published
2017

66. Monte carlo simulations of the n_TOF lead spallation target with the Geant4 toolkit: A benchmark study

Author

S. Warren, J. Andrzejewski, V. Variale, M. Mastromarco, Pedro G. Ferreira, G. Vannini, M. A. Cortés-Giraldo, Rugard Dressler, N. Patronis, A. K. Saxena, Arnaud Ferrari, J. Billowes, J. Marganiec, E. Jericha, Paolo Finocchiaro, Anton Wallner, M. Caamaño, Nicola Colonna, A. Musumarra, Dorothea Schumann, E. Chiaveri, P. F. Mastinu, J. Balibrea, J. A. Ryan, Vasilis Vlachoudis, C. Rubbia, A. Tarifeño-Saldivia, G. Cortes, E. González, A. Pavlik, L. Audouin, A. Ventura, M. Sabaté-Gilarte, F. Calviño, H. Leeb, J. Perkowski, A. Casanovas, Y. H. Chen, P. C. Rout, C. Domingo-Pardo, M. Bacak, A. Kimura, J. L. Tain, F. Gunsing, T. Glodariu, F. Mingrone, A. Masi, D. G. Jenkins, E. Dupont, Cristian Massimi, C. Lederer, M. Diakaki, Niko Kivel, F. Cerutti, M. Krtička, Kathrin Göbel, A. S. Brown, Alexandru Negret, S. J. Lonsdale, J. Lerendegui-Marco, E. Mendoza, T. Martinez, B. Fernández-Domínguez, F. Käppeler, Jan Heyse, Mario Barbagallo, M.B. Gómez-Hornillos, A. Oprea, A. Kalamara, I. F. Gonçalves, Javier Praena, S. Lo Meo, P. M. Milazzo, A. Stamatopoulos, S. Heinitz, Ignacio Porras, F. Bečvář, T. J. Wright, D. Mancussi, Simone Gilardoni, Hideo Harada, Rene Reifarth, R. Cardella, A. Mengoni, O. Aberle, Peter Schillebeeckx, J. M. Quesada, L. Tassan-Got, Deniz Kurtulgil, R. Vlastou, P. Vaz, D. Radeck, E. Berthoumieux, L. Cosentino, N. V. Sosnin, Annamaria Mazzone, Petar Žugec, D. Bosnar, D. Macina, Carlos Guerrero, G. Tagliente, D. Cano-Ott, Y. Kadi, S. Valenta, Marco Calviani, A. G. Smith, Philip Woods, A. R. García, Emilio Andrea Maugeri, M. Kokkoris, E. Leal-Cidoncha, A. Gawlik, Thomas Rauscher, I. Duran, P. Kavrigin, Ralf Nolte, E. Griesmayer, L. A. Damone, Institut de Recherches sur les lois Fondamentales de l'Univers (IRFU), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay, Institut de Physique Nucléaire d'Orsay (IPNO), Université Paris-Sud - Paris 11 (UP11)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Centre National de la Recherche Scientifique (CNRS), n_TOF, Lerendegui-Marco, J., Cortés-Giraldo, M.A., Guerrero, C., Quesada, J.M., Meo, S. Lo, Massimi, C., Barbagallo, M., Colonna, N., Mancussi, D., Mingrone, F., Sabaté-Gilarte, M., Vannini, G., Vlachoudis, V., Aberle, O., Andrzejewski, J., Audouin, L., Bacak, M., Balibrea, J., Bečvář, F., Berthoumieux, E., Billowes, J., Bosnar, D., Brown, A., Caamaño, M., Calviño, F., Calviani, M., Cano-Ott, D., Cardella, R., Casanovas, A., Cerutti, F., Chen, Y.H., Chiaveri, E., Cortés, G., Cosentino, L., Damone, L.A., Diakaki, M., Domingo-Pardo, C., Dressler, R., Dupont, E., Durán, I., Fernández-Domínguez, B., Ferrari, A., Ferreira, P., Finocchiaro, P., Göbel, K., Gómez-Hornillos, M.B., García, A.R., Gawlik, A., Gilardoni, S., Glodariu, T., Gonçalves, I.F., González, E., Griesmayer, E., Gunsing, F., Harada, H., Heinitz, S., Heyse, J., Jenkins, D.G., Jericha, E., Käppeler, F., Kadi, Y., Kalamara, A., Kavrigin, P., Kimura, A., Kivel, N., Kokkoris, M., Krtička, M., Kurtulgil, D., Leal-Cidoncha, E., Lederer, C., Leeb, H., Lonsdale, S.J., Macina, D., Marganiec, J., Martínez, T., Masi, A., Mastinu, P., Mastromarco, M., Maugeri, E.A., Mazzone, A., Mendoza, E., Mengoni, A., Milazzo, P.M., Musumarra, A., Negret, A., Nolte, R., Oprea, A., Patronis, N., Pavlik, A., Perkowski, J., Porras, I., Praena, J., Radeck, D., Rauscher, T., Reifarth, R., Rout, P.C., Rubbia, C., Ryan, J.A., Saxena, A., Schillebeeckx, P., Schumann, D., Smith, A.G., Sosnin, N.V., Stamatopoulos, A., Tagliente, G., Tain, J.L., Tarifeño-Saldivia, A., Tassan-Got, L., Valenta, S., Variale, V., Vaz, P., Ventura, A., Vlastou, R., Wallner, A., Warren, S., Woods, P.J., Wright, T., Ugec, P., Universitat Politècnica de Catalunya. Departament de Física, Universitat Politècnica de Catalunya. Institut de Tècniques Energètiques, Universitat Politècnica de Catalunya. ANT - Advanced Nuclear Technologies Research Group, Universitat Politècnica de Catalunya. NEMEN - Nanoenginyeria de materials aplicats a l'energia, Centre National de la Recherche Scientifique (CNRS)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Paris-Sud - Paris 11 (UP11), and Universidad de Sevilla. Departamento de Física Atómica, Molecular y Nuclear

Subjects
nTOF, [PHYS.NUCL]Physics [physics]/Nuclear Theory [nucl-th], QC1-999, Astrophysics::High Energy Astrophysical Phenomena, Montecarlo, Mètode de, Monte Carlo method, Context (language use), Neutron, 01 natural sciences, Nuclear physics, Physics and Astronomy (all), Informàtica [Àrees temàtiques de la UPC], Neutron flux, CERN, 0103 physical sciences, Spallation, 010306 general physics, Nuclear Experiment, Monte Carlo, Neutrons, Physics, Large Hadron Collider, Física [Àrees temàtiques de la UPC], 010308 nuclear & particles physics, Neutron radiation, Cascade, Nuclear Physics - Theory
Abstract

Monte Carlo (MC) simulations are an essential tool to determine fundamental features of a neutron beam, such as the neutron flux or the γ -ray background, that sometimes can not be measured or at least not in every position or energy range. Until recently, the most widely used MC codes in this field had been MCNPX and FLUKA. However, the Geant4 toolkit has also become a competitive code for the transport of neutrons after the development of the native Geant4 format for neutron data libraries, G4NDL. In this context, we present the Geant4 simulations of the neutron spallation target of the n TOF facility at CERN, done with version 10.1.1 of the toolkit. The first goal was the validation of the intra-nuclear cascade models implemented in the code using, as benchmark, the characteristics of the neutron beam measured at the first experimental area (EAR1), especially the neutron flux and energy distribution, and the time distribution of neutrons of equal kinetic energy, the so-called Resolution Function. The second goal was the development of aMonte Carlo tool aimed to provide useful calculations for both the analysis and planning of the upcoming measurements at the new experimental area (EAR2) of the facility., The research that led to these results has received funding from the EC FP7 Programme under the projects NEUTANDALUS (Grant No. 334315) and CHANDA (Grant No. 605203), and the Spanish Ministry of Economy and Competitiveness projects FPA2011-28770- C3-02, FPA2013-45083-P and FPA2014- 53290-C2-2-P. The simulations have been performed at the computing cluster FISATOM, hosted at CICA (Seville, Spain), and of INFN-CNAF, University of Bologna; we thank the staff of both institutions for the operational maintenance of the machines.

Published
2016

67. Dissemination of data measured at the CERN n TOF facility

Author

Dupont, E., Otuka, N., Cabellos, O., Aberle, O., Aerts, G., Altstadt, S., Alvarez, H., Alvarez-Velarde, F., Andriamonje, S., Andrzejewski, J., Audouin, L., Bacak, M., Badurek, G., Balibrea, J., Barbagallo, M., Barros, S., Baumann, P., Bécares, V., Bečvář, F., Beinrucker, C., Belloni, F., Berthier, B., Berthoumieux, E., Billowes, J., Boccone, V., Bosnar, D., Brown, A., Brugger, M., Caamaño, M., Calviani, M., Calviño, F., Cano-Ott, D., Capote, R., Cardella, R., Carrapiço, C., Casanovas, A., Castelluccio, D. M., Cennini, P., Cerutti, F., Chen, Y. H., Chiaveri, E., Chin, M., Colonna, N., Cortés, G., Cortés-Giraldo, M. A., Cosentino, L., Couture, A., Cox, J., Damone, L. A., David, S., Deo, K., Diakaki, M., Dillmann, I., Domingo-Pardo, C., Dressler, R., Dridi, W., Duran, I., Eleftheriadis, C., Embid-Segura, M., Fernández-Domínguez, B., Ferrant, L., Ferrari, A., Ferreira, P., Finocchiaro, P., Fraval, K., Frost, R. J. W., Fujii, K., Furman, W., Ganesan, S., Garcia, A. R., Gawlik, A., Gheorghe, I., Gilardoni, S., Giubrone, G., Glodariu, T., Göbel, K., Gomez-Hornillos, M. B., Goncalves, I. F., Gonzalez-Romero, E., Goverdovski, A., Gramegna, F., Griesmayer, E., Guerrero, C., Gunsing, F., Gurusamy, P., Haight, R., Harada, H., Heftrich, T., Heil, M., Heinitz, S., Hernández-Prieto, A., Heyse, J., Igashira, M., Isaev, S., Jenkins, D. G., Jericha, E., Kadi, Y., Kaeppeler, F., Kalamara, A., Karadimos, D., Karamanis, D., Katabuchi, T., Kavrigin, P., Kerveno, M., Ketlerov, V., Khryachkov, V., Kimura, A., Kivel, N., Kokkoris, M., Konovalov, V., Krtička, M., Kroll, J., Kurtulgil, D., Lampoudis, C., Langer, C., Leal-Cidoncha, E., Lederer, C., Leeb, H., Naour, C. Le, Lerendegui-Marco, J., Leong, L. S., Licata, M., Meo, S. Lo, Lonsdale, S. J., Losito, R., Lozano, M., Macina, D., Manousos, A., Marganiec, J., Martinez, T., Marrone, S., Masi, A., Massimi, C., Mastinu, P., Mastromarco, M., Matteucci, F., Maugeri, E. A., Mazzone, A., Mendoza, E., Mengoni, A., Milazzo, P. M., Mingrone, F., Mirea, M., Mondelaers, W., Montesano, S., Moreau, C., Mosconi, M., Musumarra, A., Negret, A., Nolte, R., O’Brien, S., Oprea, A., Palomo-Pinto, F. R., Pancin, J., Paradela, C., Patronis, N., Pavlik, A., Pavlopoulos, P., Perkowski, J., Perrot, L., Pigni, M. T., Plag, R., Plompen, A., Plukis, L., Poch, A., Porras, I., Praena, J., Pretel, C., Quesada, J. M., Radeck, D., Rajeev, K., Rauscher, T., Reifarth, R., Riego, A., Robles, M., Roman, F., Rout, P. C., Rudolf, G., Rubbia, C., Rullhusen, P., Ryan, J. A., Sabaté-Gilarte, M., Salgado, J., Santos, C., Sarchiapone, L., Sarmento, R., Saxena, A., Schillebeeckx, P., Schmidt, S., Schumann, D., Sedyshev, P., Smith, A. G., Sosnin, N. V., Stamatopoulos, A., Stephan, C., Suryanarayana, S. V., Tagliente, G., Tain, J. L., Tarifeño-Saldivia, A., Tarrío, D., Tassan-Got, L., Tavora, L., Terlizzi, R., Tsinganis, A., Valenta, S., Vannini, G., Variale, V., Vaz, P., Ventura, A., Versaci, R., Vermeulen, M. J., Villamarin, D., Vicente, M. C., Vlachoudis, V., Vlastou, R., Voss, F., Wallner, A., Walter, S., Ware, T., Warren, S., Weigand, M., Weiß, C., Wolf, C., Wiesher, M., Wisshak, K., Woods, P. J., Wright, T., Žugec, P., Hambsch, F.-J., Kopecky, S., Siegler, P., Oberstedt, S., Universitat Politècnica de Catalunya. Departament de Física, Universitat Politècnica de Catalunya. Institut de Tècniques Energètiques, Universitat Politècnica de Catalunya. ANT - Advanced Nuclear Technologies Research Group, Mengoni, A., Lo Meo, S., Castelluccio, D. M., Universidad de Sevilla. Departamento de Física Atómica, Molecular y Nuclear, Institut de Recherches sur les lois Fondamentales de l'Univers (IRFU), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay, Institut de Physique Nucléaire d'Orsay (IPNO), Université Paris-Sud - Paris 11 (UP11)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Centre National de la Recherche Scientifique (CNRS), Institut Pluridisciplinaire Hubert Curien (IPHC), Université de Strasbourg (UNISTRA)-Centre National de la Recherche Scientifique (CNRS), n_TOF, Université de Strasbourg (UNISTRA)-Université de Haute-Alsace (UHA) Mulhouse - Colmar (Université de Haute-Alsace (UHA))-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Centre National de la Recherche Scientifique (CNRS), Centre National de la Recherche Scientifique (CNRS)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Paris-Sud - Paris 11 (UP11), Université de Strasbourg (UNISTRA)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Centre National de la Recherche Scientifique (CNRS), Dupont, E., Otuka, N., Cabellos, O., Aberle, O., Aerts, G., Altstadt, S., Alvarez, H., Alvarez-Velarde, F., Andriamonje, S., Andrzejewski, J., Audouin, L., Bacak, M., Badurek, G., Balibrea, J., Barbagallo, M., Barros, S., Baumann, P., Bécares, V., Bečvář, F., Beinrucker, C., Belloni, F., Berthier, B., Berthoumieux, E., Billowes, J., Boccone, V., Bosnar, D., Brown, A., Brugger, M., Caamaño, M., Calviani, M., Calviño, F., Cano-Ott, D., Capote, R., Cardella, R., Carrapiço, C., Casanovas, A., Castelluccio, D.M., Cennini, P., Cerutti, F., Chen, Y.H., Chiaveri, E., Chin, M., Colonna, N., Cortés, G., Cortés-Giraldo, M.A., Cosentino, L., Couture, A., Cox, J., Damone, L.A., David, S., Deo, K., Diakaki, M., Dillmann, I., Domingo-Pardo, C., Dressler, R., Dridi, W., Duran, I., Eleftheriadis, C., Embid-Segura, M., Fernández-Domínguez, B., Ferrant, L., Ferrari, A., Ferreira, P., Finocchiaro, P., Fraval, K., Frost, R.J.W., Fujii, K., Furman, W., Ganesan, S., Garcia, A.R., Gawlik, A., Gheorghe, I., Gilardoni, S., Giubrone, G., Glodariu, T., Göbel, K., Gomez-Hornillos, M.B., Goncalves, I.F., Gonzalez-Romero, E., Goverdovski, A., Gramegna, F., Griesmayer, E., Guerrero, C., Gunsing, F., Gurusamy, P., Haight, R., Harada, H., Heftrich, T., Heil, M., Heinitz, S., Hernández-Prieto, A., Heyse, J., Igashira, M., Isaev, S., Jenkins, D.G., Jericha, E., Kadi, Y., Kaeppeler, F., Kalamara, A., Karadimos, D., Karamanis, D., Katabuchi, T., Kavrigin, P., Kerveno, M., Ketlerov, V., Khryachkov, V., Kimura, A., Kivel, N., Kokkoris, M., Konovalov, V., Krtička, M., Kroll, J., Kurtulgil, D., Lampoudis, C., Langer, C., Leal-Cidoncha, E., Lederer, C., Leeb, H., Naour, C. Le, Lerendegui-Marco, J., Leong, L.S., Licata, M., Meo, S. Lo, Lonsdale, S.J., Losito, R., Lozano, M., Macina, D., Manousos, A., Marganiec, J., Martinez, T., Marrone, S., Masi, A., Massimi, C., Mastinu, P., Mastromarco, M., Matteucci, F., Maugeri, E.A., Mazzone, A., Mendoza, E., Milazzo, P.M., Mingrone, F., Mirea, M., Mondelaers, W., Montesano, S., Moreau, C., Mosconi, M., Musumarra, A., Negret, A., Nolte, R., O'Brien, S., Oprea, A., Palomo-Pinto, F.R., Pancin, J., Paradela, C., Patronis, N., Pavlik, A., Pavlopoulos, P., Perkowski, J., Perrot, L., Pigni, M.T., Plag, R., Plompen, A., Plukis, L., Poch, A., Porras, I., Praena, J., Pretel, C., Quesada, J.M., Radeck, D., Rajeev, K., Rauscher, T., Reifarth, R., Riego, A., Robles, M., Roman, F., Rout, P.C., Rudolf, G., Rubbia, C., Rullhusen, P., Ryan, J.A., Sabaté-Gilarte, M., Salgado, J., Santos, C., Sarchiapone, L., Sarmento, R., Saxena, A., Schillebeeckx, P., Schmidt, S., Schumann, D., Sedyshev, P., Smith, A.G., Sosnin, N.V., Stamatopoulos, A., Stephan, C., Suryanarayana, S.V., Tagliente, G., Tain, J.L., Tarifeño-Saldivia, A., Tarrío, D., Tassan-Got, L., Tavora, L., Terlizzi, R., Tsinganis, A., Valenta, S., Vannini, G., Variale, V., Vaz, P., Ventura, A., Versaci, R., Vermeulen, M.J., Villamarin, D., Vicente, M.C., Vlachoudis, V., Vlastou, R., Voss, F., Wallner, A., Walter, S., Ware, T., Warren, S., Weigand, M., Weiß, C., Wolf, C., Wiesher, M., Wisshak, K., Woods, P.J., Wright, T., Ž Ugec, P., and Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université de Strasbourg (UNISTRA)-Centre National de la Recherche Scientifique (CNRS)

Subjects
Nuclear reaction, nTOF, Physics::Instrumentation and Detectors, Chemistry & allied sciences, QC1-999, Nuclear Theory, Neutron, [PHYS.NEXP]Physics [physics]/Nuclear Experiment [nucl-ex], 01 natural sciences, Nuclear physics, Physics and Astronomy (all), 0103 physical sciences, CERN, Nuclear astrophysics, Nuclear Physics - Experiment, 010306 general physics, Nuclear Experiment, Physics, Energies::Energia nuclear [Àrees temàtiques de la UPC], Neutrons, Large Hadron Collider, Física [Àrees temàtiques de la UPC], Cross section, Reaccions nuclears, 010308 nuclear & particles physics, Nuclear data, Nuclear technology, ddc:540, Nuclear reactions
Abstract

The n-TOF neutron time-of-flight facility at CERN is used for high quality nuclear data measurements from thermal energy up to hundreds of MeV. In line with the CERN open data policy, the n-TOF Collaboration takes actions to preserve its unique data, facilitate access to them in standardised format, and allow their re-use by a wide community in the fields of nuclear physics, nuclear astrophysics and various nuclear technologies. The present contribution briefly describes the n-TOF outcomes, as well as the status of dissemination and preservation of n-TOF final data in the international EXFOR library. © The Authors, published by EDP Sciences, 2017.

Published
2016

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