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We report a unified framework describing all existing protocols for spin manipulation and signal creation in frequency-modulation magnetic resonance force microscopy using classical perturbation theory. The framework is well suited for studying the dependence of the frequency shift on the cantilever amplitude via numerical simulation. We demonstrate the formalism by recovering an exact result for a single spin signal and by simulating, for the first time as a function of cantilever amplitude, the frequency shift due to a volume of noninteracting spins inverted by an adiabatic rapid passage. We show that an optimal cantilever amplitude exists that maximizes the signal. Our findings suggest that understanding the amplitude dependence of the spin signal will be important for designing future high-sensitivity experiments. [ABSTRACT FROM AUTHOR]

We report an approach that extends the applicability of ultrasensitive force-gradient detection of magnetic resonance to samples with spin-lattice relaxation times (T1) as short as a single cantilever period. To demonstrate the generality of the approach, which relies on detecting either cantilever frequency or phase, we used it to detect electron spin resonance from a T1 = 1 ms nitroxide spin probe in a thin film at 4.2 K and 0.6 T. By using a custom-fabricated cantilever with a 4 μm-diameter nickel tip, we achieve a magnetic resonance sensitivity of 400 Bohr magnetons in a 1 Hz bandwidth. A theory is presented that quantitatively predicts both the line-shape and the magnitude of the observed cantilever frequency shift as a function of field and cantilever-sample separation. Good agreement was found between nitroxide T1's measured mechanically and inductively, indicating that the cantilever magnet is not an appreciable source of spin-lattice relaxation here. We suggest that the new approach has a number of advantages that make it well suited to push magnetic resonance detection and imaging of nitroxide spin labels in an individual macromolecule to single-spin sensitivity. [ABSTRACT FROM AUTHOR]

We introduce and demonstrate a method of measuring small force gradients acting on a harmonic oscillator in which the force-gradient signal of interest is used to parametrically up-convert a forced oscillation below resonance into an amplitude signal at the oscillator’s resonance frequency. The approach, which we demonstrate in a mechanically detected electron spin resonance experiment, allows the force-gradient signal to evade detector frequency noise by converting a slowly modulated frequency signal into an amplitude signal. [ABSTRACT FROM AUTHOR]

Present research on no-insulation (NI) rare earth barium copper oxide (REBCO) magnets have demonstrated their ability to produce high fields due to their compact nature. NI magnets have often been demonstrated to be self-protecting. However, evidence of mechanical damage in recent high field magnets, suggests that there are some issues about quench that must be resolved for this otherwise promising technology. This article attempts to explain multi-physics phenomena occurring during the quench of an NI magnet that can be used to elucidate quench behavior through experiments and simulations. A lumped circuit model is used for the circuit analysis where each coil is modeled as a single inductor with variable quench resistance in series and characteristic contact resistance in parallel. Three case studies have been analyzed: (1) a 3 double pancake (DP) standalone magnet, (2) a 2 DP coil in 31 T background, and (3) a high temperature superconductor/low temperature superconductor (HTS/LTS) hybrid user magnet that consists of a 13 T HTS insert and a 6 T LTS background magnet. Lessons learned from these analyses include: (1) characteristic resistance of NI coil rises during quench with the temperature rise; (2) influence of Hall effect exists on the voltage rise during quench; (3) over-current during quench can over-stress the coil; and (4) quench propagation from one end of the magnet generates significant unbalanced forces. This approach is expected to be used in the preliminary design of an ultra high field (>40 T) user magnet currently under design at the National High Magnetic Field Laboratory. [ABSTRACT FROM AUTHOR]

A conduction-cooled 3 T 100 mm winding bore multi-width and no-insulation (NI) all-REBCO magnet was designed, constructed and tested at 13 K. The magnet consists of a stack of double pancake (DP) coils wound with, for the first time, REBCO tapes having a 1 μm thick layer of stainless steel, named ‘metallic cladding’, that surrounds the tapes in a hermetic way to substantially reduce the NI charging delay. After construction, the magnet was cooled down to the target operating temperature of 13 K using a two-stage pulse-tube cryo-cooler. During charging–discharging tests up to 200 A, magnetic center field, voltage of each DP coil, power supply current, and magnet temperature were monitored. The charging time constant of the magnet was measured to be about 10.1 s, 13 times smaller than that of its NI counterpart. The magnet experienced, due to an unexpected power supply trip, a sudden discharge at a peak coil current density of 353 A mm2, yet it survived without any degradation. The results demonstrated strong potential of the metallic cladding NI-REBCO magnet for significant charging-delay reduction and self-protecting operation. [ABSTRACT FROM AUTHOR]

A single pancake no-insulation (NI) coil was wound in a hermetic way with REBCO tape having a thin (1–2 μm) cladding layer of stainless steel. With an electric heater embedded at the innermost turn of the coil, heater-induced quench tests were performed under a background field of 15 T in a bath of liquid helium at 4.2 K. Despite the large average contact surface resistance of 1.63 cm2 times larger than those of pure NI coils, ‘thermal recovery’ was observed at a coil current density (Je) below 700 A mm−2 mainly due to the local current sharing. The coil experienced nine consecutive ‘thermal runaway’ quenches at Je of 700–820 A mm−2 (power supply limit), yet no discernible coil degradation or damage was observed. The results demonstrated that the stainless steel cladding REBCO tape may be effective at reducing the charging delay of high field NI REBCO magnets without sacrificing the self-protecting feature. [ABSTRACT FROM AUTHOR]

This paper presents a design of a 35 T 40 mm winding diameter no-insulation standalone magnet that consists of a stack of 52 double pancake (DP) coils wound with multi-width REBCO tapes. The inner and outer diameters and height of the magnet are 40 mm, 221.6 mm, and 628 mm, respectively. It is designed to generate 35 T at an operating current (Iop) of 179.8 A in a bath of liquid helium at 4.2 K. All the DP coils will be ‘dry’ wound without epoxy, making turns within the DP coils to be essentially ‘self-supporting,’ which is effective to reduce the magnetic stress. To reduce the magnet charging time constant, the so-called ‘metallic cladding’ REBCO tapes will be adopted, where a 1–2 μm thick stainless steel layer surrounds the tapes hermetically. With an average surface contact resistance (Rct) of 170 cm−2, experimentally obtained from a charging test of our recent 3 T 100 mm stainless steel cladding REBCO magnet, the charging time constant of the 35 T magnet was estimated to be 3.01 minutes, though the magnet will be energized substantially slower over a few hours to reduce ac loss and Joule heating from radial turn-to-turn leak currents. A preliminary post-quench analysis, based on our lumped equivalent circuit model, was performed; the total stored energy of 1.79 MJ (magnet inductance: 110.5 H) was expected to be discharged in approximately 1.28 seconds after a quench due to the fast electromagnetic quench propagation among the DP coils, while the peak hot spot temperature was estimated to rise to 94 K, acceptable for a safe quench of a REBCO magnet. [ABSTRACT FROM AUTHOR]

We describe a magnetic resonance force microscopy experiment carried out using both a fast-relaxing spin system and a frequency-modulation mode detection method, presenting a validation of the measured signal and sensitivity. The detection method applied along with a self-excited cantilever oscillation worked stably without any serious interference due to spurious cantilever excitation despite application of first-harmonic microwave modulation, and thereby successfully created almost the maximum available signal. The signal could be measured without distortion while the magnetic field was swept at a rate of 1.9 G s[?]1. The measured sensitivity approached the thermal noise limit of the cantilever with a high quality factor. The experimental results for both signal and noise were in good agreement with theoretical predictions. [ABSTRACT FROM AUTHOR]

Hydrogen gas is introduced to multi-walled carbon nanotubes and 1H nuclear magnetic resonances are measured as the functions of hydrogen gas pressure and temperature. The resonance frequency is shifted in inverse proportion to temperature due to the super-paramagnetic Fe catalysts that remained in the nanotubes. By the differences in relaxation times, the signal from hydrogen adsorbed on carbon nanotubes is differentiated from that of gas phase hydrogen. [Copyright &y& Elsevier]

We demonstrate an efficient control of 29Si nuclear spins for specific lattice sites near 31P donors in silicon at temperatures below 1 K and in a high magnetic field of 4.6 T. Excitation of the forbidden electron-nuclear transitions leads to a pattern of well-resolved holes and peaks in the electron spin resonance (ESR) lines of 31P. The pattern originates from dynamic polarization (DNP) of the 29Si nuclear spins near the donors via the solid effect. DNP of 29Si is demonstrated also with the Overhauser effect where the allowed ESR transitions are excited. In this case mostly the remote 29Si nuclei having weak interaction with the donors are polarized, which results in a single hole and a sharp peak pair in the ESR spectrum. Our work shows that the solid effect can be used for initialization of 29Si nuclear spin qubits near the donors. [ABSTRACT FROM AUTHOR]