51. Radioactivity study of EAST structural materials based on neutron activation system.
- Author
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Zhang, Ruixue, Hu, Liqun, Huang, Liangsheng, Li, Kai, Zhang, Yongqiang, Xu, Mingyuan, Yang, Li, Zhang, Yubo, and Zhong, Guoqiang
- Subjects
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CONSTRUCTION materials , *NEUTRONS , *RADIOISOTOPES , *NEUTRON irradiation , *RADIOACTIVITY , *GAMMA rays - Abstract
• Selected structural materials including SS316L, SS304L, Al, Cu and W, the self- absorption factor and detection efficiency of gamma rays were calculated to optimize the sample size. • The samples were transported to the activation terminal for irradiation, and single shot activation experiment was repeated to calculate the specific activities under a wide range of neutron fluences. • Neutron spectrum and neutron transport coefficients at the activation terminal were calculated. Subsequently, activation prediction using FIAPACT-II and comparison with experimental results were discussed. The plasma operation in the Experimental Advanced Superconducting Tokamak (EAST) would generate 2.45 MeV neutrons and a small fraction of 14 MeV neutrons. Neutrons react with structural materials, leading to the production of radioactive isotopes. The identification of nuclides and the determination of radioactive activity are of great significance for radiation protection and fusion material applications. In this study, structural materials including stainless steel 316L(SS316L), stainless steel 304L(SS304L), aluminum(Al), tungsten(W) and copper(Cu) were transported to the activation terminal for fusion neutron irradiation. The gamma ray spectra were measured using high-purity germanium (HPGe) detector, and the main radioactive nuclides of SS316L and SS304L are 56Mn, while the main radioactive nuclide of Al is 28Al. For Cu and W, the main radionuclides resulting from neutron reactions are 66Cu and 187W, respectively. The uncertainty of the radioactivity is 2.27∼7.94 % for W, 1.95∼5.84 % for SS316L, 2.10∼6.07 % for SS304L, 0.68∼1.69 % for Al and 2.59∼6.75 % for Cu. The specific activity of radionuclides is proportional to neutron yield, so the material activation is the main source of radiation dose during irradiation with high-yield neutron. The neutron activation coefficients of SS316L, SS304L, Al, Cu and W are 2.74538 × 10−14, 3.6411 × 10−14, 2.50711 × 10−12, 1.76506 × 10−12 and 3.51725 × 10−14, respectively. The coefficient represents the radioactive activity generated by each fusion neutron. In addition, the predicted activity was calculated using FISPACT program and compared with experiments. [ABSTRACT FROM AUTHOR]
- Published
- 2023
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