101. Anisotropic electronic state via spontaneous phase separation in strained vanadium dioxide films
- Author
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Jiwei Lu, Alexander McLeod, Dimitri Basov, Zhe Fei, Salinporn Kittiwatanakul, Michael Goldflam, Mengkun Liu, Stuart A. Wolf, Elsa Abreu, Richard D. Averitt, Siyuan Dai, Martin Wagner, and Michael M. Fogler
- Subjects
Phase transition ,Mesoscopic physics ,General Physics ,Materials science ,Condensed matter physics ,Isotropy ,Oxide ,General Physics and Astronomy ,Infrared spectroscopy ,Mathematical Sciences ,chemistry.chemical_compound ,Condensed Matter::Materials Science ,Engineering ,chemistry ,Rutile ,Phase (matter) ,Physical Sciences ,Condensed Matter::Strongly Correlated Electrons ,Anisotropy - Abstract
We resolved the enigma of anisotropic electronic transport in strained vanadium dioxide (VO2) films by inquiring into the role that strain plays in the nanoscale phase separation in the vicinity of the insulator-to-metal transition. The root source of the anisotropy was visualized as the formation of a peculiar unidirectional stripe state which accompanies the phase transition. Furthermore, nanoscale infrared spectroscopy unveils distinct facets of electron-lattice interplay at three different stages of the phase transition. These stages include the initial formation of sparse nonpercolating metallic domains without noticeable involvement of the lattice followed by an electron-lattice coupled anisotropic stripe state close to percolation which ultimately evolves into a nearly isotropic rutile metallic phase. Our results provide a unique mesoscopic perspective for the tunable macroscopic phenomena in strained metal oxide films. © 2013 American Physical Society.
- Published
- 2013