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Our previous article [Phys. Rev. Lett. 104, 060401 (2010)] predicted that Casimir forces induced by the material-dispersion properties of certain dielectrics can give rise to stable configurations of objects. This phenomenon was illustrated via a dicluster configuration of non-touching objects consisting of two spheres immersed in a fluid and suspended against gravity above a plate. Here, we examine these predictions from the perspective of a practical experiment and consider the influence of non-additive, three-body, and nonzero-temperature effects on the stability of the two spheres. We conclude that the presence of Brownian motion reduces the set of experimentally realizable silicon/teflon spherical diclusters to those consisting of layered micro-spheres, such as the hollow- core (spherical shells) considered here., Comment: 11 pages, 9 figures

We demonstrate theoretical conditions for highly-efficient degenerate four-wave mixing in triply-resonant nonlinear (Kerr) cavities. We employ a general and accurate temporal coupled-mode analysis in which the interaction of light in arbitrary microcavities is expressed in terms a set of coupling coefficients that we rigorously derive from the full Maxwell equations. Using the coupled-mode theory, we show that light consisting of an input signal of frequency $\omega_0-\Delta \omega$ can, in the presence of pump light at $\omega_0$, be converted with quantum-limited efficiency into an output shifted signal of frequency $\omega_0 + \Delta \omega$, and we derive expressions for the critical input powers at which this occurs. We find that critical powers in the order of 10mW assuming very conservative cavity parameters (modal volumes $\sim10$ cubic wavelengths and quality factors $\sim1000$. The standard Manley-Rowe efficiency limits are obtained from the solution of the classical coupled-mode equations, although we also derive them from simple photon-counting "quantum" arguments. Finally, using a linear stability analysis, we demonstrate that maximal conversion efficiency can be retained even in the presence of self- and cross-phase modulation effects that generally act to disrupt the resonance condition., Comment: 13 pages, 8 figures. To appear in Physical Review A

We show how to compute Casimir forces at nonzero temperatures with time-domain electromagnetic simulations, for example using a finite-difference time-domain (FDTD) method. Compared to our previous zero-temperature time-domain method, only a small modification is required, but we explain that some care is required to properly capture the zero-frequency contribution. We validate the method against analytical and numerical frequency-domain calculations, and show a surprising high-temperature disappearance of a non-monotonic behavior previously demonstrated in a piston-like geometry., Comment: 5 pages, 2 figures, submitted to Physical Review A Rapid Communication

In this work we theoretically consider the Casimir force between two periodic arrays of nanowires (both in vacuum, and on a substrate separated by a fluid) at separations comparable to the period. Specifically, we compute the dependence of the exact Casimir force between the arrays under both lateral translations and rotations. Although typically the force between such structures is well-characterized by the Proximity Force Approximation (PFA), we find that in the present case the microstructure modulates the force in a way qualitatively inconsistent with PFA. We find instead that effective-medium theory, in which the slabs are treated as homogeneous, anisotropic dielectrics, gives a surprisingly accurate picture of the force, down to separations of half the period. This includes a situation for identical, fluid-separated slabs in which the exact force changes sign with the orientation of the wire arrays, whereas PFA predicts attraction. We discuss the possibility of detecting these effects in experiments, concluding that this effect is strong enough to make detection possible in the near future., Comment: 12 pages, 9, figure. Published version with expanded discussion

An experimental and theoretical study on the structure and energetics of stellated gold clusters at several sizes is presented. Systematic molecular dynamics simulations on Kepler-Poisont classified clusters are performed based on cubo-octahedral and icosahedral cores, following present and previous studies that suggest stellated clusters grew up from these seeds. For cluster sizes up to 10802 atoms full atomistic molecular dynamics simulations at room temperature have been carried out. Results show that stellated clusters in the bigger size regime maintain their star-like shape at room temperature, and by means of linear fitting of energy data to proper function models, it is predicted that the two type of stellated structures might coexist at room temperature for relatively large sizes, being these findings in good agreement with experimental results., Comment: 11 figures, plus 1 as graphical abstract

We examine a recent prediction for the chirality-dependence of the Casimir force in chiral metamaterials by numerical computation of the forces between the exact microstructures, rather than homogeneous approximations. We compute the exact force for a chiral bent-cross pattern, as well as forces for an idealized "omega"-particle medium in the dilute approximation and identify the effects of structural inhomogeneity (i.e. proximity forces and anisotropy). We find that these microstructure effects dominate the force for separations where chirality was predicted to have a strong influence. To get observations of chirality free from microstructure effects, one must go to large separations where the effect of chirality is at most $\sim10^{-4}$ of the total force., Comment: 5 pages, 4 figures

We propose a method of achieving large temperature sensitivity in the Casimir force that involves measuring the stable separation between dielectric objects immersed in fluid. We study the Casimir force between slabs and spheres using realistic material models, and find large > 2nm/K variations in their stable separations (hundreds of nanometers) near room temperature. In addition, we analyze the effects of Brownian motion on suspended objects, and show that the average separation is also sensitive to changes in temperature . Finally, this approach also leads to rich qualitative phenomena, such as irreversible transitions, from suspension to stiction, as the temperature is varied.

We give an example of a geometry in which two metallic objects in vacuum experience a repulsive Casimir force. The geometry consists of an elongated metal particle centered above a metal plate with a hole. We prove that this geometry has a repulsive regime using a symmetry argument and confirm it with numerical calculations for both perfect and realistic metals. The system does not support stable levitation, as the particle is unstable to displacements away from the symmetry axis., Comment: 4 pages, 4 figures; added references, replaced Fig. 3

We present a scheme for obtaining stable Casimir suspension of dielectric nontouching objects immersed in a fluid, validated here in various geometries consisting of ethanol-separated dielectric spheres and semi-infinite slabs. Stability is induced by the dispersion properties of real dielectric (monolithic) materials. A consequence of this effect is the possibility of stable configurations (clusters) of compact objects, which we illustrate via a "molecular" two-sphere dicluster geometry consiting of two bound spheres levitated above a gold slab. Our calculations also reveal a strong interplay between material and geometric dispersion, and this is exemplified by the qualitatively different stability behavior observed in planar versus spherical geometries.

Achieving efficient terahertz (THz) generation using compact turn-key sources operating at room temperature and modest power levels represents one of the critical challeges that must be overcome to realize truly practical applications based on THz. Up to now, the most efficient approaches to THz generation at room temperature -- relying mainly on optical rectification schemes -- require intricate phase-matching set-ups and powerful lasers. Here we show how the unique light-confining properties of triply-resonant photonic resonators can be tailored to enable dramatic enhancements of the conversion efficiency of THz generation via nonlinear frequency down-conversion processes. We predict that this approach can be used to reduce up to three orders of magnitude the pump powers required to reach quantum-limited conversion efficiency of THz generation in nonlinear optical material systems. Furthermore, we propose a realistic design readily accesible experimentally, both for fabrication and demonstration of optimal THz conversion efficiency at sub-W power levels.

We propose a scheme for efficient cavity-enhanced nonlinear THz generation via difference-frequency generation (DFG) processes using a triply resonant system based on photonic crystal cavities. We show that high nonlinear overlap can be achieved by coupling a THz cavity to a doubly-resonant, dual-polarization near-infrared (e.g. telecom band) photonic-crystal nanobeam cavity, allowing the mixing of three mutually orthogonal fundamental cavity modes through a chi(2) nonlinearity. We demonstrate through coupled-mode theory that complete depletion of the pump frequency - i.e., quantum-limited conversion - is possible in an experimentally feasible geometry, with the operating output power at the point of optimal total conversion efficiency adjustable by varying the mode quality (Q) factors., Comment: 8 pages, 3 figures

Our preceding paper introduced a method to compute Casimir forces in arbitrary geometries and for arbitrary materials that was based on a finite-difference time-domain (FDTD) scheme. In this manuscript, we focus on the efficient implementation of our method for geometries of practical interest and extend our previous proof-of-concept algorithm in one dimension to problems in two and three dimensions, introducing a number of new optimizations. We consider Casimir piston-like problems with nonmonotonic and monotonic force dependence on sidewall separation, both for previously solved geometries to validate our method and also for new geometries involving magnetic sidewalls and/or cylindrical pistons. We include realistic dielectric materials to calculate the force between suspended silicon waveguides or on a suspended membrane with periodic grooves, also demonstrating the application of PML absorbing boundaries and/or periodic boundaries. In addition we apply this method to a realizable three-dimensional system in which a silica sphere is stably suspended in a fluid above an indented metallic substrate. More generally, the method allows off-the-shelf FDTD software, already supporting a wide variety of materials (including dielectric, magnetic, and even anisotropic materials) and boundary conditions, to be exploited for the Casimir problem., Comment: 11 pages, 12 figures. Includes additional examples (dispersive materials and fully three-dimensional systems)

We introduce an efficient technique for computing Casimir energies and forces between objects of arbitrarily complex 3D geometries. In contrast to other recently developed methods, our technique easily handles non-spheroidal, non-axisymmetric objects and objects with sharp corners. Using our new technique, we obtain the first predictions of Casimir interactions in a number of experimentally relevant geometries, including crossed cylinders and tetrahedral nanoparticles., Comment: 4 pages, 4 figures

We introduce a method to compute Casimir forces in arbitrary geometries and for arbitrary materials based on the finite-difference time-domain (FDTD) scheme. The method involves the time-evolution of electric and magnetic fields in response to a set of current sources, in a modified medium with frequency-independent conductivity. The advantage of this approach is that it allows one to exploit existing FDTD software, without modification, to compute Casimir forces. In this manuscript, part I, we focus on the derivation, implementation choices, and essential properties of the time-domain algorithm, considered both analytically and illustrated in the simplest parallel-plate geometry. Part II presents results for more complex two- and three-dimensional geometries.

We present a comprehensive study of second-order nonlinear difference frequency generation in triply resonant cavities using a theoretical framework based on coupled-mode theory. We show that optimal quantum-limited conversion efficiency can be achieved at any pump power when the powers at the pump and idler frequencies satisfy a critical relationship. We demonstrate the existence of a broad parameter range in which all triply-resonant DFG processes exhibit monostable conversion. We also demonstrate the existence of a geometry-dependent bistable region., Comment: 10 pages, 3 figures

We present the basic ingredients of a technique to compute quantum Casimir forces at micrometer scales using antenna measurements at tabletop, e.g. centimeter, scales, forming a type of analog computer for the Casimir force. This technique relies on a correspondence that we derive between the contour integration of the Casimir force in the complex frequency plane and the electromagnetic response of a physical dissipative medium in a finite, real frequency bandwidth.

We describea theoretical analysis of the nonlinear dynamics of third-harmonic generation ($\omega\to3\omega$) via Kerr ($\chithree$) nonlinearities in a resonant cavity with resonances at both $\omega$ and $3\omega$. Such a doubly resonant cavity greatly reduces the required power for efficient harmonic generation, by a factor of $\sim V/Q^2$ where $V$ is the modal volume and $Q$ is the lifetime, and can even exhibit 100% harmonic conversion efficiency at a critical input power. However, we show that it also exhibits a rich variety of nonlinear dynamics, such as multistable solutions and long-period limit cycles.We describe how to compensate for self/cross-phase modulation (which otherwise shifts the cavity frequencies out of resonance), and how to excite the different stable solutions (and especially the high-efficiency solutions) by specially modulated input pulses., Comment: 12 pages, 12 figures

Using an exact numerical method for finite nonplanar objects, we demonstrate a stable mechanical suspension of a silica cylinder within a metallic cylinder separated by ethanol, via a repulsive Casimir force between the silica and the metal. We investigate cylinders with both circular and square cross sections, and show that the latter exhibit a stable orientation as well as a stable position, via a method to compute Casimir torques for finite objects. Furthermore, the stable orientation of the square cylinder is shown to undergo an unusual 45 degrees transition as a function of the separation lengthscale, which is explained as a consequence of material dispersion., Comment: Published in Physical Review Letters. Vol. 101, page, 190404 (2008)

We describe a three-dimensional geometry that exhibits a repulsive Casimir force using ordinary metallic materials, as computed via an exact numerical method (no uncontrolled approximations). The geometry consists of a zippelike, glide-symmetric structure formed of interleaved metal brackets attached to parallel plates. Depending on the separation, the perpendicular force between the plates/brackets varies from attractive (large separations) to repulsive (intermediate distances) and back to attractive (close separations), with one point of stable equilibrium in the perpendicular direction. This geometry was motivated by a simple intuition of attractive interactions between surfaces, and so we also consider how a rough proximity force approximation of pairwise attractions compares to the exact calculations.

Previous methods for determining photonic quasicrystal (PQC) spectra have relied on the use of large supercells to compute the eigenfrequencies and/or local density of states (LDOS). In this manuscript, we present a method by which the energy spectrum and the eigenstates of a PQC can be obtained by solving Maxwells equations in higher dimensions for any PQC defined by the standard cut-and-project construction, to which a generalization of Blochs theorem applies. In addition, we demonstrate how one can compute band structures with defect states in the higher-dimensional superspace with no additional computational cost. As a proof of concept, these general ideas are demonstrated for the simple case of one-dimensional quasicrystals, which can also be solved by simple transfer-matrix techniques., Comment: Published in Physical Review B, 77 104201, 2008

We analyze the Casimir force between two parallel infinite metal cylinders, with nearby metal plates (sidewalls), using complementary methods for mutual confirmation. The attractive force between cylinders is shown to have a nonmonotonic dependence on the separation to the plates. This intrinsically multi-body phenomenon, which occurs with either one or two sidewalls (generalizing an earlier result for squares between two sidewalls), does not follow from any simple two-body force description. We can, however, explain the nonmonotonicity by considering the screening (enhancement) of the interactions by the fluctuating charges (currents) on the two cylinders, and their images on the nearby plate(s). Furthermore, we show that this effect also implies a nonmonotonic dependence of the cylinder-plate force on the cylinder-cylinder separation., Comment: 5 pages, 4 figures

Using the ray-optics approximation, we analyze the Casimir force in a two dimensional domain formed by two metallic blocks adjacent to parallel metallic sidewalls, which are separated from the blocks by a finite distance h. For h > 0, the ray-optics approach is not exact because diffraction effects are neglected. Nevertheless, we show that ray optics is able to qualitatively reproduce a surprising effect recently identified in an exact numerical calculation: the force between the blocks varies non-monotonically with h. In this sense, the ray-optics approach captures an essential part of the physics of multi-body interactions in this system, unlike simpler pairwise-interaction approximations such as PFA. Furthermore, by comparison to the exact numerical results, we are able to quantify the impact of diffraction on Casimir forces in this geometry.

Infrared, visible and near-UV reflectivity measurements are used to obtain conductivity as a function of temperature and frequency in YbInCu_4, which exhibits an isostructural phase-transition into a mixed-valent phase below T_v=42 K. In addition to a gradual loss of spectral weight with decreasing temperature extending up to 1.5 eV, a sharp resonance appears at 0.25 eV in the mixed-valent phase. This feature can be described in terms of excitations into the Kondo (Abrikosov-Suhl) resonance, and, like the sudden reduction of resistivity, provides a direct reflection of the onset of coherence in this strongly correlated electron system., Comment: 4 pages, 3 figures (to appear in Phys. Rev. B)

Infrared measurements are used to obtain conductivity as a function of temperature and frequency in YbInCu_4, which exhibits an isostructural transition to a mixed-valent state at T_v \simeq 42 K. In addition to a gradual loss of spectral weight with decreasing temperature extending up to 1.5 eV, sharp resonances appear in the mixed-valent state at 0 and 0.25 eV . These features may be key to understanding both YbInCu_4 and the nature of the mixed-valent Kondo state., Comment: 4 pages, 3 postscript figures