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Low-cost reduced graphene oxide sponges functionalized with manganese oxide were used as electrodes for the disinfection of Escherichia coli in water. Manganese oxide was doped with amino groups MnxOyNH2 to strengthen the bond with the graphene coating and improve the electrochemical stability of the sponge. The Mn II and Mn III incorporated into the graphene coating favored the formation of oxygen vacancies and enhanced the electric and catalytic properties of the anode. Electrooxidation of real tap water at 29 A m2 resulted in 2.2 log removal of E. coli. After storing the treated samples for 18 h at 25 and 37 {\deg}C, the removal of E. coli increased to 3.3 and 4.6 log, respectively, demonstrating the irreparable damage to the bacterial cells via low-voltage electroporation, and the key role of storage temperature in their further inactivation. The energy consumption of the system treating real low conductivity tap water was 1.2-1.6 kWh m-3. Finally, experiments with intermittent current suggest the contribution of the pseudo-capacitance of the graphene sponge to electrochemical disinfection during the OFF periods. This study demonstrates the feasibility of manganese oxide-functionalized graphene sponges for the chlorine-free disinfection of water., Comment: 33 pages, 7 figures, 1 table, and supplementary material with 14 figures and 7 tables

We present a low-resource and robust optical implementation of the four-dimensional Grover coin, a four-port linear-optical scatterer that augments the low dimensionality of a regular beam-splitter. While prior realizations of the Grover coin required a potentially unstable ring-cavity to be formed, this version of the scatterer does not exhibit any internal interference. When this Grover coin is placed in another system, it can be used for interferometry with a higher-dimensional set of optical field modes. In this case, we formed a Grover-Michelson interferometer, which results when the traditional beam-splitter of a Michelson interferometer is replaced with a four-port Grover coin. This replacement has been shown to remove a phase parameter redundancy in the original Michelson system, now allowing continuous tuning of the shape and slope of the interference pattern. We observed an intensity interferogram with $97\%$ visibility and a phase sensitivity more than an order of magnitude larger than a regular Michelson interferometer. Because this device is readily formed with nearly the same number of optomechanical resources as a Michelson interferometer, but can outperform it drastically in phase delay evaluation, it has a great potential to improve many interferometric sensing and control systems., Comment: 12 pages, 6 figures

Using symmetry considerations, we derive a unitary scattering matrix for a three-port optical Y-coupler or Y-branch. The result is shown to be unique up to external phase shifts. Unlike traditional passive linear-optical one-way splitters, coupling light into the conventional output ports of the Y-coupler results in strong coherent back-reflections, making the device a hybrid between feed-forward devices like the beam splitter, which do not reverse the direction of light, and a recently considered class of directionally unbiased multiport scatterers (with dimension greater than two) which do. While the device could immediately find use as a novel scattering vertex for the implementation of quantum walks, we also design a few simple but nonetheless useful optical systems that can be constructed by taking advantage of the symmetry of the scattering process. This includes an interference-free, resource-efficient implementation of the Grover four-port and a higher-dimensional Fabry-Perot interferometer with tunable finesse. Symmetry-breaking generalizations are also considered.

The Su-Schrieffer-Heeger (SSH) system is a popular model for exploring topological insulators and topological phases in one dimension. Recent interest in exceptional points has led to re-examination of non-Hermitian generalizations of many physical models, including the SSH model. In such non-Hermitian systems, singular points called exceptional points (EPs) appear that are of interest for applications in super-resolution sensing systems and topological lasers. Here, a non-Hermitian and non-PT-symmetric variation of the SSH model is introduced, in which the hopping amplitudes are non-reciprocal and vary monotonically along the chain. It is found that, while the existence of the EPs is due to the nonreciprocal couplings, the number, position, and order of the EPs can all be altered by the addition of the hopping amplitude gradient, adding a new tool for tailoring the spectrum of a non-Hermitian system.

Plasmonic nanoantennas with suitable far-field characteristics are of huge interest for utilization in optical wireless links, inter-/intra-chip communications, LiDARs, and photonic integrated circuits due to their exceptional modal confinement. Despite its success in shaping robust antenna design theories in radio frequency and millimeter-wave regimes, conventional transmission line theory finds its validity diminished in the optical frequencies, leading to a noticeable void in a generalized theory for antenna design in the optical domain. By utilizing neural networks and through a one-time training of the network, one can transform the plasmonic nanoantennas design into an automated, data-driven task. In this work, we have developed a multi-head deep convolutional neural network serving as an efficient inverse-design framework for plasmonic patch nanoantennas. Our framework is designed with the main goal of determining the optimal geometries of nanoantennas to achieve the desired (inquired by the designer) S 11 and radiation pattern simultaneously. The proposed approach preserves the one-to-many mappings, enabling us to generate diverse designs. In addition, apart from the primary fabrication limitations that were considered while generating the dataset, further design and fabrication constraints can also be applied after the training process. In addition to possessing an exceptionally rapid surrogate solver capable of predicting S 11 and radiation patterns throughout the entire design frequency spectrum, we are introducing what we believe to be the pioneering inverse design network.

We present a finite-element approach for computing the aggregate scattering matrix of a network of linear coherent scatterers. These might be optical scatterers or more general scattering coins studied in quantum walk theory. While techniques exist for two-dimensional lattices of feed-forward scatterers, the present approach is applicable to any network configuration of any collection of scatterers. Unlike traditional finite-element methods in optics, this method does not directly solve Maxwell's equations; instead it is used to assemble and solve a linear, coupled scattering problem that emerges after Maxwell's equations are abstracted within the scattering matrix method. With this approach, a global unitary is assembled corresponding to one time step of the quantum walk on the network. After applying the relevant boundary conditions to this global matrix, the problem becomes non-unitary, and possesses a steady-state solution which is the output scattering state. We provide an algorithm to obtain this steady-state solution exactly using a matrix inversion, yielding the scattering state without requiring a direct calculation of the eigenspectrum. The approach is then numerically validated on a coupled-cavity interferometer example that possesses a known, closed-form solution. Finally, the method is shown to be a generalization of the Redheffer star product, which describes scatterers on one-dimensional lattices (2-regular graphs) and is often applied to the design of thin-film optics, making the current approach an invaluable tool for the design and validation of high-dimensional phase-reprogrammable optical devices and study of quantum walks on arbitrary graphs.

We combine lossless, phase-only transformations with fully-transmitting linear-optical scatterers to define the principle of linear-optical phase amplification. This enables a physical phase shift $\phi$ to be nonlinearly mapped to a new space $\gamma(\phi)$ using linear optics, resulting in a completely general and enhanced phase shifter that can replace any standard one. A particular phase amplifier is experimentally realized, allowing the phase enhancement parameter $d\gamma/d\phi$ to be continuously tuned. Placing this enhanced phase shifter in one arm of a Mach-Zehnder interferometer led to an intensity-phase slope more than twenty times steeper than what can be obtained with its unamplified counterpart.

The efficient frontier (EF) is a fundamental resource allocation problem where one has to find an optimal portfolio maximizing a reward at a given level of risk. This optimal solution is traditionally found by solving a convex optimization problem. In this paper, we introduce NeuralEF: a fast neural approximation framework that robustly forecasts the result of the EF convex optimization problem with respect to heterogeneous linear constraints and variable number of optimization inputs. By reformulating an optimization problem as a sequence to sequence problem, we show that NeuralEF is a viable solution to accelerate large-scale simulation while handling discontinuous behavior., Comment: Accepted at the Thirty-seventh Conference on Neural Information Processing Systems (NeurIPS 2023)

Here we introduce interferometric devices by combining optical feedback (cavities) with unbiased multiports, which unlike traditional beam dividers, allow light to reflect back out of the port from which it originated. By replacing the traditional, directionally-biased beam-splitter in a Michelson interferometer with an unbiased multiport, the functional dependence of the scattering amplitudes changes. As a result, the derivative of transmittance with respect to an external phase perturbation can be made substantially large. This significantly enhances the resolution of phase measurement, and allows the phase response curves to be altered in real time by tuning an externally-controllable phase shift.

This article presents the early results of synchronous multiwavelength observations of one of the brightest gamma-ray bursts (GRBs) GRB 160625B with the detailed continuous fast optical photometry of its optical counterpart obtained by MASTER and with hard X-ray and gamma-ray emission, obtained by the Lomonosov and Konus-Wind spacecraft. The detailed photometry led us to detect the quasi-periodical emission components in the intrinsic optical emission. As a result of our analysis of synchronous multiwavelength observations, we propose a three-stage collapse scenario for this long and bright GRB. We suggest that quasiperiodic fluctuations may be associated with forced precession of a self-gravitating rapidly rotating superdense body (spinar), whose evolution is determined by a powerful magnetic field. The spinar's mass allows it to collapse into a black hole at the end of evolution., Comment: 22 pages, 12 figures, 4 tables, accepted for publication in ApJ

Nanoscale strain has emerged as a powerful tool for controlling single-photon emitters (SPEs) in atomically thin transition metal dichalcogenides (TMDCs)(1, 2). However, quantum emitters in monolayer TMDCs are typically unstable in ambient conditions. Multilayer two-dimensional (2D) TMDCs could be a solution, but they suffer from low quantum efficiency, resulting in low brightness of the SPEs. Here, we report the deterministic spatial localization of strain-induced single-photon emitters in multilayer GaSe by nanopillar arrays. The strain-controlled quantum confinement effect introduces well-isolated sub-bandgap photoluminescence and corresponding suppression of the broad band edge photoluminescence. Clear photon-antibunching behavior is observed from the quantum dot-like GaSe sub-bandgap exciton emission at 3.5 Kelvin. The strain-dependent confinement potential and the brightness are found to be strongly correlated, suggesting a promising route for tuning and controlling SPEs. The comprehensive investigations of strain-engineered GaSe SPEs provide a solid foundation for the development of 2D devices for quantum photonic technologies., Comment: 18 pages, 4 figures in the maintext; 21 figures in the supporting information

Grover multiports are higher-dimensional generalizations of beam splitters, in which input to any one of the four ports has equal probability of exiting at any of the same four ports, including the input port. In this paper, we demonstrate that interferometers built from such multiports have novel features. For example, when combined with two-photon input and coincidence measurements, it is shown that such interferometers have capabilities beyond those of standard beam-splitter-based interferometers, such as easily controlled interpolation between Hong-Ou-Mandel (HOM) and anti-HOM behavior. Further, it is shown that the Grover-based analog of the Mach-Zehnder interferometer can make three separate phase measurements simultaneously. By arranging the transmission lines between the two multiports to lie in different planes, the same interferometer acts as a higher-dimensional Sagnac interferometer, allowing rotation rates about three different axes to be measured with a single device.

Reconfigurable distribution of entangled states is essential for operation of quantum networks connecting multiple devices such as quantum memories and quantum computers. We introduce new quantum distribution network architecture enabling control of the entangled state propagation direction using linear-optical devices and phase shifters and offering reconfigurable connections between multiple quantum nodes. The basic two-photon entanglement distribution scheme is first introduced to illustrate the principle of operation. The scheme is then extended to a network structure with increased number of spatial modes connecting potential end-users. We present several examples of controllable network configuration modifications using time-dependent phase shifters.

The intriguing analogy between quantum physics and optics has inspired the design of unconventional integrated photonics devices. In this paper, we numerically demonstrate a broadband integrated polarization beam splitter (PBS) by implementing the stimulated Raman adiabatic passage (STIRAP) technique in a three-waveguide plasmonic system. Our proposed PBS exhibits >250 nm TM bandwidth with <-40 dB extinction and >150 nm TE bandwidth with <-20 dB extinction, covering the entire S-, C- and L-band and partly E-band. Moreover, near-lossless light transfer is achieved in our system despite the incorporation of a plasmonic hybrid waveguide because of the unique loss mitigating feature of the STIRAP scheme. Through this approach, various broadband integrated devices that were previously impossible can be realized, which will allow innovation in integrated optics.

Lithium niobate on insulator (LNOI) waveguides, as an emerging technology, have proven to offer a promising platform for integrated optics, due to their strong optical confinement comparable to silicon on insulator (SOI) waveguides, while possessing the versatile properties of lithium niobate, such as high electro-optic coefficients. In this paper, we show that mode hybridization, a phenomenon widely found in vertically asymmetric waveguides, can be efficiently modulated in an LNOI ridge waveguide by electro-optic effect, leading to a polarization mode converter with 97% efficiency. Moreover, the proposed device does not require tapering or periodic poling, thereby greatly simplifying the fabrication process. It can also be actively switched by external fields. Such a platform facilitates technological progress of photonic circuits and sensors.

We expand the two-photon Hong-Ou-Mandel (HOM) effect onto a higher-dimensional set of spatial modes and introduce an effect that allows controllable redistribution of quantum states over these modes using directionally unbiased linear-optical four-ports without post-selection. The original HOM effect only allows photon pairs to exit in two directions in space. But when accompanied by beam splitters and phase shifters, the result is a directionally controllable two-photon HOM effect in four spatial modes, with direction controlled by changing the phases in the system. This controllable quantum amplitude manipulation also allows demonstration of a "delayed" HOM effect by exploiting phase shifters in a system of two connected multiport devices. By this means, both spatial and temporal control of the propagation of the two-photon superposition state through a network can be achieved.

We present the earliest astronomical observation of a high energy neutrino error box in which its variability was discovered after high-energy neutrinos detection. The one robotic telescope of the MASTER global international network (Lipunov et al. 2010) automatically imaged the error box of the very high-energy neutrino event IceCube-170922A. Observations were carried out in minute after the IceCube-170922A neutrino event was detected by the IceCube observatory at the South Pole. MASTER found the blazar TXS 0506+056 to be in the off-state after one minute and then switched to the on-state no later than two hours after the event. The effect is observed at a 50-sigma significance level. Also we present own unique 16-years light curve of blazar TXS 0506+056 (518 data set)., Comment: 17 pages, 3 figures, 1 Table accepted to The Astrophysical Journal Letters