Search

Filming atomic motion within molecules is an active pursuit of molecular physics and quantum chemistry. A promising method is laser-induced Coulomb Explosion Imaging (CEI) where a laser pulse rapidly ionizes many electrons from a molecule, causing the remaining ions to undergo Coulomb repulsion. The ion momenta are used to reconstruct the molecular geometry which is tracked over time (i.e. filmed) by ionizing at an adjustable delay with respect to the start of interatomic motion. Results are distorted, however, by ultrafast motion during the ionizing pulse. We studied this effect in water and filmed the rapid "slingshot" motion that enhances ionization and distorts CEI results. Our investigation uncovered both the geometry and mechanism of the enhancement which may inform CEI experiments in many other polyatomic molecules.

Investigations of cosmic ray anisotropies and their relationship to concurrent magnetic field data are reported. These investigations range in scope from the examination of data very late in the decay phase of a solar particle event where long term (approximately 6 hour) averages are used and definite interplanetary effects sought after to an examination of the change in low energy particle anisotropy as the satellite approaches the bow shock and the magnetopause.

During the period 1967-1973 data were obtained from five satellites in order to investigate bidirectional anisotropies in low-energy solar protons and to study electron events. Detailed consideration is given to the characteristics of two observed solar electron events. It is particularly noted that (1) the mean duration of bidirectional anisotropy is about 9 hours, (2) for most events the bidirectional anisotropy occurs at the minimum of the associated Forbush decrease, (3) the existence of bidirectional anisotropy in subrelativistic electrons associated with an interplanetary shock is not expected as anisotropies in impulsive solar electron events usually decay quickly within a time of not more than an hour at 1 AU, and (4) simultaneous observations show a significant difference in the nature of the angular distributions first between electrons and protons and second between different proton energies. The formation of bidirectional anisotropy by propagation and by energy change is also discussed.

Solar low energy cosmic ray population anisotropy from satellite observations during flare event, describing rise time, decay, field alignment and time constant

Anisotropy of solar cosmic ray electrons, considering parallel diffusion coefficients for ions and electrons

Satellite-borne anisotropy and energy spectra measurement instruments for cosmic ray electrons and protons and solar and galactic X-rays

Solar cosmic ray anisotropy measurement by Explorer 34 satellite during solar flare events

Low energy, positive ion flux from inner radiation zone, noting losses due to charge exchange, night sky emissions and lifetimes

Rocket measurements of midlatitude nightglow and particle fluxes indicate different sources for aurorae and 5577 angstrom line

The anisotropy of the particle distribution and its variation with time at 1 AU early in a solar cosmic-ray event can provide information on the pitch-angle scattering of the particles in the interplanetary medium. One proton event (7.6-55 MeV) is described in which the anisotropy remained large well into the decay of the omnidirectional intensity. A Monte Carlo technique which gives the pitch-angle distribution is employed to investigate two models put forward to explain the sustained anisotropy. It is shown that the observed event is consistent with a model in which the injection of particles at the sun reaches a peak 1.5 hours after flare maximum before decaying with an e-folding time of 7 hours. The uniform diffusion coefficient in this model corresponds to a classical mean free path of 1.6 AU.