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Multimode optical fibers represent the ideal platform for transferring multidimensional light states. However, dispersion degrades the correlations between the light's degrees of freedom, thus limiting the effective transport of ultrashort pulses between distant nodes of optical networks. Here, we demonstrate that tailoring the spatiotemporal structure of ultrashort light pulses can overcome the physical limitations imposed by both chromatic and modal dispersion in multimode optical fibers. We synthesize these light states with predefined spatial and chromatic dynamics through applying a sequence of transformations to shape the optical field in all its dimensions. Similar methods can also be used to overcome dispersion processes in other physical settings like acoustics and electron optics. Our results will enable advancements in laser-based technologies, including multimode optical communications, imaging, ultrafast light-matter interactions, and high brightness fiber sources., Comment: 15 pages, 4 figures

Supercontinuum (SC) generation based on ultrashort pulse compression constitutes one of the most promising technologies towards an ultra-wide bandwidth, high-brightness and spatially coherent light sources for applications such as spectroscopy and microscopy. Here, multi-octave SC generation in a gas-filled hollow-core antiresonant fiber (HC-ARF) is reported spanning from 200 nm in the deep ultraviolet (DUV) to 4000 nm in the mid-infrared (mid-IR). A measured average output power of 5 mW was obtained by pumping at the center wavelength of the first anti-resonance transmission window (2460 nm) with ~100 fs pulses and an injected pulse energy of ~7-8 {\mu}J. The mechanism behind the extreme spectral broadening relies upon intense soliton-plasma nonlinear dynamics which leads to efficient soliton self-compression and phase-matched dispersive wave (DW) emission in the DUV region. The strongest DW is observed at 275 nm having an estimated pulse energy of 1.42 {\mu}J, corresponding to 28.4 % of the total output energy. Furthermore, the effect of changing the pump pulse energy and gas pressure on the nonlinear dynamics and their direct impact on SC generation was investigated. The current work paves a new way towards novel investigations of gas-based ultrafast nonlinear optics in the emerging mid-IR spectral regime.

In this work, we numerically investigate an experimentally feasible design of a tapered Ne-filled hollow-core anti-resonant fiber and we report the generation of multiple dispersive waves (DWs) in the range 90-120 nm, well into the extreme ultraviolet (UV) region. The simulations assume an 800 nm pump pulse with 30 fs 10 $\mu$J pulse energy, launched into a 9 bar Ne-filled fiber with $34~\mu$m initial core diameter that is then tapered to a $10~\mu$m core diameter. The simulations were performed using a new model that provides a realistic description of both loss and dispersion of the resonant and anti-resonant spectral bands of the fiber, and also importantly includes the material loss of silica in the UV. We show that by first generating solitons that emit DWs in the far-UV region in the pre-taper section, optimization of the following taper structure can allow re-collision with the solitons and further up-conversion of the far-UV DWs to the extreme-UV with energies up to 190 nJ in the 90-120 nm range. This process provides a new way to generate light in the extreme-UV spectral range using relatively low gas pressure.