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A fundamental challenge in modern physics is bridging the gap between an exact description of few-body microscopic systems and the emergent description of many-body macroscopic systems. This gap may be bridged by tracing the properties of well-controlled intermediate-size mesoscopic systems. Here, we study mesoscopic signatures of a spatial self-organization phase transition in deterministically prepared arrays of between 10 and 22 atoms inside an optical cavity. Through precise engineering of the atom-cavity interactions, we reveal how critical behavior depends on atom number. We identify characteristic dynamical behaviors related to symmetry breaking and system size in the self-organized regime, and observe a finite optomechanical susceptibility at the critical point. This work opens the door to probing particle-number- and time-resolved properties of phase transitions in mesoscopic systems., Comment: 21 pages, 9 figures

We propose the use of collective states of matter as a resource for the deterministic generation of quantum states of light, which are fundamental for quantum information technologies. Our minimal model consists of three emitters coupled to a half-waveguide, i.e., a one-dimensional waveguide terminated by a mirror. Photon-mediated interactions between the emitters result in the emergence of bright and dark states. The dark states form a decoherence-free subspace, protected from dissipation. Local driving of the emitters and control of their resonance frequencies allows to perform arbitrary quantum gates within the decoherence-free subspace. Coupling to bright states facilitates photon emission, thereby enabling the realization of quantum gates between light and matter. We demonstrate that sequential application of these gates leads to the generation of photonic entangled states, such as Greenberger-Horne-Zeilinger and one- and two-dimensional cluster states.

We present a theoretical framework for 'collective transition quenching', a quantum many-body dissipative phenomenon that occurs in systems with multiple collective decay channels. Despite the competition, interactions suppress all but the dominant decay transition, leading to a 'winner takes all' dynamic where the system primarily settles into the dominant ground state. We prove that, in the presence of permutation symmetry, this problem is exactly solvable for any number of competing channels. Additionally, we develop an approximate model for the dynamics by mapping the evolution into a continuity equation for a fluid, and show analytically that the dominant transition ratio converges to unity with increasing system size as a power-law, for any branching ratio. This near-deterministic preparation of the dominant ground state has broad applicability. As an example we discuss a protocol for molecular photoassociation where collective dynamics effectively acts as a catalyst, amplifying the yield in a particular final state. Our results open new avenues for many-body strategies in the preparation and control of quantum systems., Comment: 5 pages, 3 figures

Quantum systems are open, continually exchanging energy and information with the surrounding environment. This interaction leads to decoherence and decay of quantum states. In complex systems, formed by many particles, decay can become correlated and enhanced. A fundamental question then arises: what is the maximal decay rate of a large quantum system, and how does it scale with its size? In this work, we address these issues by reformulating the problem into finding the ground state energy of a generic spin Hamiltonian. Inspired by recent work in Hamiltonian complexity theory, we establish rigorous and general upper and lower bounds on the maximal decay rate. These bounds are universal, as they hold for a broad class of Markovian many-body quantum systems. For many physically-relevant systems, the bounds are asymptotically tight, resulting in exact scaling laws with system size. Specifically, for large atomic arrays in free space, these scalings depend only on the arrays' dimensionality and are insensitive to details at short length-scales. The scaling laws establish fundamental limits on the decay rates of quantum states and offer valuable insights for research in many-body quantum dynamics, metrology, and fault tolerant quantum computation.

Subwavelength atomic arrays in free space are becoming a leading platform for exploring emergent many-body quantum phenomena. These arrays feature strong light-induced dipole-dipole interactions, resulting in subradiant collective resonances characterized by narrowed linewidths. In this work, we present a sideband cooling scheme for atoms trapped in subwavelength arrays that utilizes these narrow collective resonances. We derive an effective master equation for the atomic motion by adiabatically eliminating the internal degrees of freedom of the atoms, and validate its prediction with numerical simulations of the full system. Our results demonstrate that subradiant resonances enable the cooling of ensembles of atoms to temperatures lower than those achievable without dipole interactions, provided the atoms have different trap frequencies. Remarkably, narrow collective resonances can be sideband-resolved even when the individual atomic transition is not. In such scenarios, ground state cooling becomes feasible solely due to light-induced dipole-dipole interactions. This approach could be utilized for future quantum technologies based on dense ensembles of emitters, and paves the way towards harnessing many-body cooperative decay for enhanced motional control., Comment: 10 pages of main text and appendix, with 4 figures. 9 pages of Supplemental Material, with 4 figures

Optical networks are the leading platform for the transfer of information due to their low loss and ability to scale to many information channels using optical frequency modes. To fully leverage the quantum properties of light in this platform, it is desired to manipulate higher-dimensional superpositions by orchestrating linear, beamsplitter-type interactions between several channels simultaneously. We propose a method of achieving simultaneous, all-to-all coupling between N optical frequency modes via N-way Bragg-scattering four-wave mixing. By exploiting the frequency degree of freedom, additional modes can be multiplexed in an interaction medium of fixed volume and loss, avoiding the introduction of excess noise. We generalize the theory of the frequency-encoded two-mode interaction to N modes under this four-wave mixing approach and experimentally verify the quantum nature of this scheme by demonstrating three-way multiphoton interference. The two input photons are shared among three frequency modes and display interference differing from that of two classical (coherent-state) inputs. These results show the potential of our approach for the scalability of photonic quantum information processing to general N-mode systems in the frequency domain.

Atoms are not two-level systems, and their rich internal structure often leads to complex phenomena in the presence of light. Here, we analyze off-resonant light scattering including the full hyperfine and magnetic structure. We find a set of frequency detunings where the induced atomic dipole is the same irrespective of the Zeeman state, and where two-photon transitions that alter the atomic state turn off. For alkali atoms and alkaline-earth ions, if the hyperfine splitting is dominated by the magnetic dipole moment contribution, these detunings approximately coincide. Therefore, at a given ``magical'' detuning, all Zeeman states in a hyperfine manifold behave almost identically, and can be traced out to good approximation. This feature prevents state decoherence due to light scattering, which impacts quantum optics experiments and quantum information applications., Comment: 12+9 pages, 4+1 figures, 2 tables. This version is in line with the published version

We realize collective enhancement and suppression of light scattered by an array of tweezer-trapped $^{87}$Rb atoms positioned within a strongly coupled Fabry-P\'{e}rot optical cavity. We illuminate the array with light directed transverse to the cavity axis, in the low saturation regime, and detect photons scattered into the cavity. For an array with integer-optical-wavelength spacing each atom scatters light into the cavity with nearly identical scattering amplitude, leading to an observed $N^2$ scaling of cavity photon number as the atom number increases stepwise from $N=1$ to $N=8$. By contrast, for an array with half-integer-wavelength spacing, destructive interference of scattering amplitudes yields a non-monotonic, sub-radiant cavity intensity versus $N$. By analyzing the polarization of light emitted from the cavity, we find that Rayleigh scattering can be collectively enhanced or suppressed with respect to Raman scattering. We observe also that atom-induced shifts and broadenings of the cavity resonance are precisely tuned by varying the atom number and positions. Altogether, tweezer arrays provide exquisite control of atomic cavity QED spanning from the single- to the many-body regime.

We study temporal oscillations, known as dynamical beats, developed by a propagating pulse due to its interaction with a near-resonant collective medium of $^{133}$Cs atoms randomly captured by a nanofiber-based optical lattice. A phenomenological theory provides an intuitive explanation and quantitative predictions, which are improved by an input-output theory considering multiple-scattering between the atoms. The results deepen our understanding of light propagation in waveguide QED, essential in time-frequency analysis and light engineering for probing, manipulating, and exploiting many-body quantum systems.

In inverted atomic ensembles, photon-mediated interactions give rise to Dicke superradiance, a form of many-body decay that results in a rapid release of energy as a photon burst. While originally studied in pointlike ensembles, this phenomenon persists in extended ordered systems if the inter-particle distance is below a certain bound. Here, we investigate Dicke superradiance in a realistic experimental setting using ordered arrays of alkaline-earth(-like) atoms, such as strontium and ytterbium. Such atoms offer exciting new opportunities for light-matter interactions as their internal structure allows for trapping at short interatomic distances compared to their long-wavelength transitions, providing the potential for collectively enhanced dissipative interactions. Despite their intricate electronic structure, we show that two-dimensional arrays of these atomic species should exhibit many-body superradiance for achievable lattice constants. Moreover, superradiance effectively ``closes'' transitions, such that multilevel atoms become more two-level like. This occurs because the avalanchelike decay funnels the emission of most photons into the dominant transition, overcoming the single-atom decay ratios dictated by their fine structure and Zeeman branching. Our work represents an important step in harnessing alkaline-earth atoms as quantum optical sources and as platforms to explore many-body dissipative dynamics., Comment: 10 + 9 pages, 7 + 3 figures, 2 tables. This version is in line with the published version

Photon-mediated interactions within an excited ensemble of emitters can result in Dicke superradiance, where the emission rate is greatly enhanced, manifesting as a high-intensity burst at short times. The superradiant burst is most commonly observed in systems with long-range interactions between the emitters, although the minimal interaction range remains unknown. Here, we put forward a new theoretical method to bound the maximum emission rate by upper bounding the spectral radius of an auxiliary Hamiltonian. We harness this tool to prove that for an arbitrary ordered array with only nearest-neighbor interactions in all dimensions, a superradiant burst is not physically observable. We show that Dicke superradiance requires minimally the inclusion of next-nearest-neighbor interactions. For exponentially decaying interactions, the critical coupling is found to be asymptotically independent of the number of emitters in all dimensions, thereby defining the threshold interaction range where the collective enhancement balances out the decoherence effects. Our findings provide key physical insights to the understanding of collective decay in many-body quantum systems, and the designing of superradiant emission in physical systems for applications such as energy harvesting and quantum sensing., Comment: 5 pages, 4 figures

We propose metasurface holograms as a novel platform to generate optical trap arrays for cold atoms with high fidelity, efficiency, and thermal stability. We developed design and fabrication methodologies to create dielectric, phase-only metasurface holograms based on titanium dioxide. We experimentally demonstrated optical trap arrays of various geometries, including periodic and aperiodic configurations with dimensions ranging from 1D to 3D and the number of trap sites up to a few hundred. We characterized the performance of the holographic metasurfaces in terms of the positioning accuracy, size and intensity uniformity of the generated traps, and power handling capability of the dielectric metasurfaces. Our proposed platform has great potential for enabling fundamental studies of quantum many-body physics, and quantum simulation and computation tasks. The compact form factor, passive nature, good power handling capability, and scalability of generating high-quality, large-scale arrays also make the metasurface platform uniquely suitable for realizing field-deployable devices and systems based on cold atoms.

The many-body decay of extended collections of two-level systems remains an open problem. Here, we investigate whether an array of emitters coupled to a one-dimensional bath undergoes Dicke superradiance. This is a process whereby a completely inverted system becomes correlated via dissipation, leading to the release of all the energy in the form of a rapid photon burst. We derive the minimal conditions for the burst to happen as a function of the number of emitters, the chirality of the waveguide, and the single-emitter optical depth, both for ordered and disordered ensembles. Many-body superradiance occurs because the initial fluctuation that triggers the emission is amplified throughout the decay process. In one-dimensional baths, this avalanchelike behavior leads to a spontaneous mirror symmetry breaking, with large shot-to-shot fluctuations in the number of photons emitted to the left and right. Superradiant bursts may thus be a smoking gun for the generation of correlated photon states of exotic quantum statistics., Comment: 16 pages, 9 figures

Subradiant excited states in finite chains of two-level quantum emitters coupled to a one-dimensional reservoir are a resource for superior photon storage and controlled photon manipulation. Typically, states storing multiple excitations exhibit fermionic correlations and are thus characterized by an anti-symmetric wavefunction, which makes them hard to prepare experimentally. Here we identify a class of quasi-localized dark states with up to half of the qubits excited, which appear for lattice constants that are an integer multiple of the guided-mode wavelength. They allow for a high-fidelity preparation and minimally invasive read out in state-of-the-art setups. In particular, we suggest an experimental implementation using a coplanar wave-guide coupled to superconducting transmon qubits on a chip. As free space and intrinsic losses are minimal, virtually perfect dark states can be achieved even for a low number of qubits, enabling fast preparation and manipulation with high fidelity., Comment: 11 pages, 6 figures

When a broadband signal propagates through a dispersive medium, some frequency components move faster than the center of the pulse. This leads to the appearance of precursors, transient signals that emerge from the medium earlier than the main part of the pulse and seem to propagate superluminally. Here, we investigate the microscopic origin of precursors in a minimal setup: an array of qubits coupled to a waveguide. The linear transmission function only converges to that of a continuous medium for large qubit numbers. Nevertheless, the dispersion produced by only two qubits is enough to produce oscillatory transients. Precursors are best observed under conditions of electromagnetically-induced transparency, as the center of the pulse is significantly delayed. Under these conditions, just a single qutrit is enough to generate a precursor. Our results pave the way towards dispersion engineering of light with just a few qubits, and can be realized with superconducting qubits coupled to transmission lines or atoms coupled to optical waveguides., Comment: 10 pages, 6 figures

Dicke superradiance in ordered atomic arrays is a phenomenon where atomic synchronization gives rise to a burst in photon emission. This superradiant burst only occurs if there is one -- or just a few -- dominant decay channels. For a fixed atom number, this happens only below a critical interatomic distance. Here we show that array dimensionality is the determinant factor that drives superradiance. In 2D and 3D arrays, superradiance occurs due to constructive interference, which grows stronger with atom number. This leads to a critical distance that scales sublogarithmically with atom number in 2D, and as a power law in 3D. In 1D arrays, superradiance occurs due to destructive interference that effectively switches off certain decay channels, yielding a critical distance that saturates with atom number. Our results provide a guide to explore many-body decay in state-of-the art experimental setups., Comment: 13 pages, 6 figures. This version is in line with the published version

Dicke superradiance is an example of emergence of macroscopic quantum coherence via correlated dissipation. Starting from an initially incoherent state, a collection of excited atoms synchronizes as they decay, generating a macroscopic dipole moment and emitting a short and intense pulse of light. While well understood in cavities, superradiance remains an open problem in extended systems due to the exponential growth of complexity with atom number. Here we show that Dicke superradiance is a universal phenomenon in ordered arrays. We present a theoretical framework -- which circumvents the exponential complexity of the problem -- that allows us to predict the critical distance beyond which Dicke superradiance disappears. This critical distance is highly dependent on the dimensionality and atom number. Our predictions can be tested in state of the art experiments with arrays of neutral atoms, molecules, and solid-state emitters and pave the way towards understanding the role of many-body decay in quantum simulation, metrology, and lasing., Comment: 7+9 pages, 4+4 figures. This version is in line with the published version

At the quantum many-body level, atom-light interfaces generally remain challenging to solve for or understand in a non-perturbative fashion. Here, we consider a waveguide quantum electrodynamics model, where two-level atoms interact with and via propagating photons in a one-dimensional waveguide, and specifically investigate the interplay of atomic position disorder, multiple scattering of light, quantum nonlinear interactions and dissipation. We develop qualitative arguments and present numerical evidence that such a system exhibits a many-body localized~(MBL) phase, provided that atoms are less than half excited. Interestingly, while MBL is usually formulated with respect to closed systems, this system is intrinsically open. However, as dissipation originates from transport of energy to the system boundaries and the subsequent radiative loss, the lack of transport in the MBL phase makes the waveguide QED system look essentially closed and makes applicable the notions of MBL. Conversely, we show that if the system is initially in a delocalized phase due to a large excitation density, rapid initial dissipation can leave the system unable to efficiently transport energy at later times, resulting in a dynamical transition to an MBL phase. These phenomena can be feasibly realized in state-of-the-art experimental setups., Comment: 19 pages, 10 figures, pre-print

Fully inverted atoms placed at exactly the same location synchronize as they deexcite, and light is emitted in a burst (known as "Dicke's superradiance"). We investigate the role of finite interatomic separation on correlated decay in mesoscopic chains, and provide an understanding in terms of collective jump operators. We show that the superradiant burst survives at small distances, despite Hamiltonian dipole-dipole interactions. However, for larger separations, competition between different jump operators leads to dephasing, suppressing superradiance. Collective effects are still significant for arrays with lattice constants of the order of a wavelength, and lead to a photon emission rate that decays nonexponentially in time. We calculate the two-photon correlation function and demonstrate that emission is correlated and directional, as well as sensitive to small changes in the interatomic distance. These features can be measured in current experimental setups, and are robust to realistic imperfections., Comment: 17 pages, 13 figures

Broken symmetries induce strong nonlinear optical responses in materials and at interfaces. Twist angle can give complete control over the presence or lack of inversion symmetry at a crystal interface, and is thus an appealing knob for tuning nonlinear optical systems. In contrast to conventional nonlinear crystals with rigid lattices, the weak interlayer coupling in van der Waals (vdW) heterostructures allows for arbitrary selection of twist angle, making nanomechanical manipulation of fundamental interfacial symmetry possible within a single device. Here we report highly tunable second harmonic generation (SHG) from nanomechanically rotatable stacks of bulk hexagonal boron nitride (BN) crystals, and introduce the term twistoptics to describe studies of optical properties in dynamically twistable vdW systems. We observe SHG intensity modulated by a factor of more than 50, polarization patterns determined by moir\'e interface symmetry, and enhanced conversion efficiency for bulk crystals by stacking multiple pieces of BN joined by symmetry-broken interfaces. Our study provides a foundation for compact twistoptics architectures aimed at efficient, scalable, and tunable frequency-conversion, and demonstrates SHG as a robust probe of buried vdW interfaces., Comment: 23 Pages, 17 Figures

Atom arrays are a new type of quantum light-matter interface. Here, we propose to employ one-dimensional ordered arrays as atomic waveguides. These arrays support optical guided modes that do not decay into free space. We show that these modes can be harnessed to mediate tunable, long-range interactions between additional "impurity qubits" coupled to the chain, without need for photonic structures. The efficient coupling between qubits and atomic waveguides enables the realization of tunable qubit-qubit interactions, which can be short- or long-range, dissipative or coherent, as well as chiral. Moreover, owing to the two-level nature of atoms, these waveguides are intrinsically quantum. In contrast to classical waveguides, where photons do not interact with each other, atomic waveguides display strong non-linearities, which create a tunable dissipative channel for qubit-qubit interactions, and opens the door to the exploration of many-body physics between guided photons. This physics is universal as it only relies on photon interference and can also be observed with other types of quantum emitters, such as those in molecular or solid-state systems., Comment: 17 pages, 11 figures. In this version, we have fixed a numerical integration error that overestimated the scattering into free space in Fig. 3(b), the inset to Fig. 6(b), and in Fig. 11. We have also corrected an error in Fig. 5

Waveguide quantum electrodynamics studies photon-mediated interactions of quantum emitters in a one-dimensional radiation channel. Although signatures of such interactions have been observed previously in a variety of physical systems, observation of coherent cooperative dynamics has been obscured by radiative decay of atoms into the waveguide. Employing transmon qubits as artificial atoms coupled to a microwave coplanar waveguide, here we observe dynamical oscillations in an open system where a designated probe qubit interacts with an entangled dark state of an array of qubits which effectively traps radiation as an atomic cavity. The qubit-cavity system is shown to achieve a large cooperativity of $\mathcal{C}=172$ due to collective enhancement of photon-mediated interactions, entering the strong coupling regime. The quantum coherence of the dark state cavity is also explored through its nonlinear response at the single-excitation level. With realistic refinements, this system is suitable for studying the many-body dynamics of large ($N>10$) quantum spin chains, synthesizing highly non-classical radiation fields on demand, and implementing universal quantum logic operations with high fidelity on information encoded within decoherence-free subspaces., Comment: 19 pages, 8 figures, 5 appendices

The properties of coupled emitters can differ dramatically from those of their individual constituents. Canonical examples include sub- and super-radiance, wherein the decay rate of a collective excitation is reduced or enhanced due to correlated interactions with the environment. Here, we systematically study the properties of collective excitations for regularly spaced arrays of quantum emitters coupled to a one-dimensional (1D) waveguide. We find that, for low excitation numbers, the modal properties are well-characterized by spin waves with a definite wavevector. Moreover, the decay rate of the most subradiant modes obeys a universal scaling with a cubic suppression in the number of emitters. Multi-excitation subradiant eigenstates can be built from fermionic combinations of single excitation eigenstates; such "fermionization" results in multiple excitations that spatially repel one another. We put forward a method to efficiently create and measure such subradiant states, which can be realized with superconducting qubits. These measurement protocols probe both real-space correlations (using on-site dispersive readout) and temporal correlations in the emitted field (using photon correlation techniques)., Comment: 21 pages, 9 figures

We examine theoretically how dipole-dipole interactions arising from multiple photon scattering lead to a modified distribution of ground state populations in a driven, ordered 1D array of multilevel atoms. Specifically, we devise a level configuration in which a ground-state population accumulated due solely to dipole-dipole interactions can be up to 20\% in regimes accessible to current experiments with neutral atom arrays. For much larger systems, the steady state can consist of an equal distribution of population across the ground state manifold. Our results illustrate how dipole-dipole interactions can be accentuated through interference, and regulated by the geometry of ordered atom arrays. More generally, control techniques for multilevel atoms that can be degraded by multiple scattering, such as optical pumping, will benefit from an improved understanding and control of dipole-dipole interactions available in ordered arrays., Comment: paper is now identical to published version

The rotational dynamics of particles subject to external illumination is found to produce light amplification and inelastic scattering at high rotation velocities. Light emission at frequencies shifted with respect to the incident light by twice the rotation frequency dominates over elastic scattering within a wide range of light and rotation frequencies. Remarkably, net amplification of the incident light is produced in this classical linear system via stimulated emission. Large optically-induced acceleration rates are predicted in vacuum accompanied by moderate heating of the particle, thus supporting the possibility of observing these effects under extreme rotation conditions., Comment: 6 figures, 8 pages