Search

We present the first polarized neutron transmission image of a model Ne\'el ferrimagnetic material, polycrystalline terbium iron garnet (Tb$_{3}$Fe$_{5}$O$_{12}$, TbIG for short), as it is taken through its compensation temperature $T_{comp}$ where, according to the theory of ferrimagnetism, the internal magnetization should vanish. Our polarized neutron imaging data and the additional supporting measurements using neutron spin echo spectroscopy and SQUID magnetometry are all consistent with a vanishing internal magnetization at $T_{comp}$., Comment: 15 pages, 15 figures

The DArk Matter In CCDs at Modane (DAMIC-M) experiment is designed to search for light dark matter (m$_{\chi}$<10\,GeV/c$^2$) at the Laboratoire Souterrain de Modane (LSM) in France. DAMIC-M will use skipper charge-coupled devices (CCDs) as a kg-scale active detector target. Its single-electron resolution will enable eV-scale energy thresholds and thus world-leading sensitivity to a range of hidden sector dark matter candidates. A DAMIC-M prototype, the Low Background Chamber (LBC), has been taking data at LSM since 2022. The LBC provides a low-background environment, which has been used to characterize skipper CCDs, study dark current, and measure radiopurity of materials planned for DAMIC-M. It also allows testing of various subsystems like readout electronics, data acquisition software, and slow control. This paper describes the technical design and performance of the LBC.

The Goos-H\"anchen (GH) shift describes a phenomenon in which a specularly-reflected beam is laterally translated along the reflecting surface such that the incident and reflected rays no longer intersect at the surface. Using a neutron spin-echo technique and a specially-designed magnetic multilayer mirror, we have measured the relative phase between the reflected up and down neutron spin states in total reflection. The relative GH shift calculated from this phase shows a strong resonant enhancement at a particular incident neutron wavevector, which is due to a waveguiding effect in one of the magnetic layers. Calculations based on the observed phase difference between the neutron states indicate a propagation distance along the waveguide layer of 0.65 mm for the spin-down state, which we identify with the magnitude of the giant GH shift. The existence of a physical GH shift is confirmed by the observation of neutron absorption in the waveguide layer. We propose ways in which our experimental method may be exploited for neutron quantum-enhanced sensing of thin magnetic layers.

Cryogenic calorimetric experiments to search for neutrinoless double-beta decay ($0\nu\beta\beta$) are highly competitive, scalable and versatile in isotope. The largest planned detector array, CUPID, is comprised of about 1500 individual Li$_2^{100}$MoO$_{4}$ detector modules with a further scale up envisioned for a follow up experiment (CUPID-1T). In this article, we present a novel detector concept targeting this second stage with a low impedance TES based readout for the Li$_2$MoO$_{4}$ absorber that is easily mass-produced and lends itself to a multiplexed readout. We present the detector design and results from a first prototype detector operated at the NEXUS shallow underground facility at Fermilab. The detector is a 2-cm-side cube with 21$\,$g mass that is strongly thermally coupled to its readout chip to allow rise-times of $\sim$0.5$\,$ms. This design is more than one order of magnitude faster than present NTD based detectors and is hence expected to effectively mitigate backgrounds generated through the pile-up of two independent two neutrino decay events coinciding close in time. Together with a baseline resolution of 1.95$\,$keV (FWHM) these performance parameters extrapolate to a background index from pile-up as low as $5\cdot 10^{-6}\,$counts/keV/kg/yr in CUPID size crystals. The detector was calibrated up to the MeV region showing sufficient dynamic range for $0\nu\beta\beta$ searches. In combination with a SuperCDMS HVeV detector this setup also allowed us to perform a precision measurement of the scintillation time constants of Li$_2$MoO$_{4}$. The crystal showed a significant fast scintillation emission with O(10$\,\mu$s) time-scale, more than an order below the detector response of presently considered light detectors suggesting the possibility of further progress in pile-up rejection through better light detectors in the future.

We measure space- and time-correlated charge jumps on a four-qubit device, operating 107 meters below the Earth's surface in a low-radiation, cryogenic facility designed for the characterization of low-threshold particle detectors. The rock overburden of this facility reduces the cosmic ray muon flux by over 99% compared to laboratories at sea level. Combined with 4$\pi$ coverage of a movable lead shield, this facility enables quantifiable control over the flux of ionizing radiation on the qubit device. Long-time-series charge tomography measurements on these weakly charge-sensitive qubits capture discontinuous jumps in the induced charge on the qubit islands, corresponding to the interaction of ionizing radiation with the qubit substrate. The rate of these charge jumps scales with the flux of ionizing radiation on the qubit package, as characterized by a series of independent measurements on another energy-resolving detector operating simultaneously in the same cryostat with the qubits. Using lead shielding, we achieve a minimum charge jump rate of 0.19$^{+0.04}_{-0.03}$ mHz, almost an order of magnitude lower than that measured in surface tests, but a factor of roughly eight higher than expected based on reduction of ambient gammas alone. We operate four qubits for over 22 consecutive hours with zero correlated charge jumps at length scales above three millimeters., Comment: 12 pages, 6 figures, 4 tables. Minor update to the measured gamma flux ratio (Page 4 and Supplemental Section F) in the LMO detector, from 23 to 20. Typos corrected, references added. Extraneous .tex files have been removed that were causing errors with the "HTML (experimental)" arxiv feature

We have developed a calibration system based on a micro-electromechanical systems (MEMS) mirror that is capable of delivering an optical beam over a wavelength range of 180 -- 2000 nm (0.62 -- 6.89 eV) in a sub-Kelvin environment. This portable, integrated system can steer the beam over a $\sim$3 cm $\times$ 3 cm area on the surface of any sensor with a precision of $\sim$100 $\mu$m, enabling characterization of device response as a function of position. This fills a critical need in the landscape of calibration tools for sub-Kelvin devices, including those used for dark matter detection and quantum computing. These communities have a shared goal of understanding the impact of ionizing radiation on device performance, which can be pursued with our system. This paper describes the design of the first-generation calibration system and the results from successfully testing its performance at room temperature and 20 mK., Comment: 17 pages, 7 figures, submitted to SPIE

In recent years, the lack of a conclusive detection of WIMP dark matter at the 10 GeV/c$^{2}$ mass scale and above has encouraged development of low-threshold detector technology aimed at probing lighter dark matter candidates. Detectors based on Cooper-pair-breaking sensors have emerged as a promising avenue for this detection due to the low (meV-scale) energy required for breaking a Cooper pair in most superconductors. Among them, devices based on superconducting qubits are interesting candidates for sensing due to their observed sensitivity to broken Cooper pairs. We have developed an end-to-end G4CMP-based simulation framework and have used it to evaluate performance metrics of qubit-based devices operating in a gate-based "energy relaxation" readout scheme, akin to those used in recent studies of qubit sensitivity to ionizing radiation. We find that for this readout scheme, the qubit acts as a phonon sensor with an energy threshold ranging down to $\simeq$0.4 eV for near-term performance parameters., Comment: 17 pages, 10 figures

Dark Matter (DM) particles with sufficiently large cross sections may scatter as they travel through Earth's bulk. The corresponding changes in the DM flux give rise to a characteristic daily modulation signal in detectors sensitive to DM-electron interactions. Here, we report results obtained from the first underground operation of the DAMIC-M prototype detector searching for such a signal from DM with MeV-scale mass. A model-independent analysis finds no modulation in the rate of 1$e^-$ events with sidereal period, where a DM signal would appear. We then use these data to place exclusion limits on DM in the mass range [0.53, 2.7] MeV/c$^2$ interacting with electrons via a dark photon mediator. Taking advantage of the time-dependent signal we improve by $\sim$2 orders of magnitude on our previous limit obtained from the total rate of 1$e^-$ events, using the same data set. This daily modulation search represents the current strongest limit on DM-electron scattering via ultralight mediators for DM masses around 1 MeV/c$^2$.

We present results from a 3.25 kg-day target exposure of two silicon charge-coupled devices (CCDs), each with 24 megapixels and skipper readout, deployed in the DAMIC setup at SNOLAB. With a reduction in pixel readout noise of a factor of 10 relative to the previous detector, we investigate the excess population of low-energy events in the CCD bulk previously observed above expected backgrounds. We address the dominant systematic uncertainty of the previous analysis through a depth fiducialization designed to reject surface backgrounds on the CCDs. The measured bulk ionization spectrum confirms the presence of an excess population of low-energy events in the CCD target with characteristic rate of ${\sim}7$ events per kg-day and electron-equivalent energies of ${\sim}80~$eV, whose origin remains unknown., Comment: 8 pages, 4 figures

We report constraints on sub-GeV dark matter particles interacting with electrons from the first underground operation of DAMIC-M detectors. The search is performed with an integrated exposure of 85.23 g days, and exploits the subelectron charge resolution and low level of dark current of DAMIC-M charge-coupled devices (CCDs). Dark-matter-induced ionization signals above the detector dark current are searched for in CCD pixels with charge up to 7e$^-$. With this dataset we place limits on dark matter particles of mass between 0.53 and 1000 MeV/$c^2$, excluding unexplored regions of parameter space in the mass ranges [1.6,1000] MeV/$c^2$ and [1.5,15.1] MeV/$c^2$ for ultralight and heavy mediator interactions, respectively.

PICO bubble chambers have exceptional sensitivity to inelastic dark matter-nucleus interactions due to a combination of their extended nuclear recoil energy detection window from a few keV to $O$(100 keV) or more and the use of iodine as a heavy target. Inelastic dark matter-nucleus scattering is interesting for studying the properties of dark matter, where many theoretical scenarios have been developed. This study reports the results of a search for dark matter inelastic scattering with the PICO-60 bubble chambers. The analysis reported here comprises physics runs from PICO-60 bubble chambers using CF$_{3}$I and C$_{3}$F$_{8}$. The CF$_{3}$I run consisted of 36.8 kg of CF$_{3}$I reaching an exposure of 3415 kg-day operating at thermodynamic thresholds between 7 and 20 keV. The C$_{3}$F$_{8}$ runs consisted of 52 kg of C$_{3}$F$_{8}$ reaching exposures of 1404 kg-day and 1167 kg-day running at thermodynamic thresholds of 2.45 keV and 3.29 keV, respectively. The analysis disfavors various scenarios, in a wide region of parameter space, that provide a feasible explanation of the signal observed by DAMA, assuming an inelastic interaction, considering that the PICO CF$_{3}$I bubble chamber used iodine as the target material., Comment: 7 pages, 3 figures

The DAMIC-M (DArk Matter In CCDs at Modane) experiment employs thick, fully depleted silicon charged-coupled devices (CCDs) to search for dark matter particles with a target exposure of 1 kg-year. A novel skipper readout implemented in the CCDs provides single electron resolution through multiple non-destructive measurements of the individual pixel charge, pushing the detection threshold to the eV-scale. DAMIC-M will advance by several orders of magnitude the exploration of the dark matter particle hypothesis, in particular of candidates pertaining to the so-called "hidden sector." A prototype, the Low Background Chamber (LBC), with 20g of low background Skipper CCDs, has been recently installed at Laboratoire Souterrain de Modane and is currently taking data. We will report the status of the DAMIC-M experiment and first results obtained with LBC commissioning data., Comment: 10 pages, 6 figures, Submission to SciPost Physics Proceedings: 14th International Conference on Identification of Dark Matter (IDM) 2022

Experiments aiming to directly detect dark matter through particle recoils can achieve energy thresholds of $\mathcal{O}(1\,\mathrm{eV})$. In this regime, ionization signals from small-angle Compton scatters of environmental $\gamma$-rays constitute a significant background. Monte Carlo simulations used to build background models have not been experimentally validated at these low energies. We report a precision measurement of Compton scattering on silicon atomic shell electrons down to 23$\,$eV. A skipper charge-coupled device (CCD) with single-electron resolution, developed for the DAMIC-M experiment, was exposed to a $^{241}$Am $\gamma$-ray source over several months. Features associated with the silicon K, L$_{1}$, and L$_{2,3}$-shells are clearly identified, and scattering on valence electrons is detected for the first time below 100$\,$eV. We find that the relativistic impulse approximation for Compton scattering, which is implemented in Monte Carlo simulations commonly used by direct detection experiments, does not reproduce the measured spectrum below 0.5$\,$keV. The data are in better agreement with $ab$ $initio$ calculations originally developed for X-ray absorption spectroscopy., Comment: 12 pages, 10 figures

The bubble nucleation efficiency of low-energy nuclear recoils in superheated liquids plays a crucial role in interpreting results from direct searches for weakly interacting massive particle (WIMP) dark matter. The PICO Collaboration presents the results of the efficiencies for bubble nucleation from carbon and fluorine recoils in superheated C$_3$F$_8$ from calibration data taken with 5 distinct neutron spectra at various thermodynamic thresholds ranging from 2.1 keV to 3.9 keV. Instead of assuming any particular functional forms for the nuclear recoil efficiency, a generalized piecewise linear model is proposed with systematic errors included as nuisance parameters to minimize model-introduced uncertainties. A Markov-Chain Monte-Carlo (MCMC) routine is applied to sample the nuclear recoil efficiency for fluorine and carbon at 2.45 keV and 3.29 keV thermodynamic thresholds simultaneously. The nucleation efficiency for fluorine was found to be $\geq 50\, \%$ for nuclear recoils of 3.3 keV (3.7 keV) at a thermodynamic Seitz threshold of 2.45 keV (3.29 keV), and for carbon the efficiency was found to be $\geq 50\, \%$ for recoils of 10.6 keV (11.1 keV) at a threshold of 2.45 keV (3.29 keV). Simulated data sets are used to calculate a p-value for the fit, confirming that the model used is compatible with the data. The fit paradigm is also assessed for potential systematic biases, which although small, are corrected for. Additional steps are performed to calculate the expected interaction rates of WIMPs in the PICO-60 detector, a requirement for calculating WIMP exclusion limits., Comment: 17 pages, 22 figures, 5 tables

Many compelling models predict dark matter coupling to the electromagnetic current through higher multipole interactions, while remaining electrically neutral. Different multipole couplings have been studied, among them anapole moment, electric and magnetic dipole moments, and millicharge. This study sets limits on the couplings for these photon-mediated interactions using non-relativistic contact operators in an effective field theory framework. Using data from the PICO-60 bubble chamber leading limits for dark matter masses between 2.7 GeV/c$^2$ and 24 GeV/c$^2$ are reported for the coupling of these photon-mediated dark matter-nucleus interactions. The detector was filled with 52 kg of C$_3$F$_8$ operating at thermodynamic thresholds of 2.45 keV and 3.29 keV, reaching exposures of 1404 kg-day and 1167 kg-day, respectively.

The search for particle-like dark matter with meV-to-GeV masses has developed rapidly in the past few years. We summarize the science case for these searches, the recent progress, and the exciting upcoming opportunities. Funding for Research and Development and a portfolio of small dark matter projects will allow the community to capitalize on the substantial recent advances in theory and experiment and probe vast regions of unexplored dark-matter parameter space in the coming decade., Comment: Contribution to Snowmass 2021. v2: includes endorsers and minor changes

Many low-threshold experiments observe sharply rising event rates of yet unknown origins below a few hundred eV, and larger than expected from known backgrounds. Due to the significant impact of this excess on the dark matter or neutrino sensitivity of these experiments, a collective effort has been started to share the knowledge about the individual observations. For this, the EXCESS Workshop was initiated. In its first iteration in June 2021, ten rare event search collaborations contributed to this initiative via talks and discussions. The contributing collaborations were CONNIE, CRESST, DAMIC, EDELWEISS, MINER, NEWS-G, NUCLEUS, RICOCHET, SENSEI and SuperCDMS. They presented data about their observed energy spectra and known backgrounds together with details about the respective measurements. In this paper, we summarize the presented information and give a comprehensive overview of the similarities and differences between the distinct measurements. The provided data is furthermore publicly available on the workshop's data repository together with a plotting tool for visualization., Comment: 44 pages, 20 figures; Editors: A. Fuss, M. Kaznacheeva, F. Reindl, F. Wagner; updated copyright statements and funding information

We construct the first comprehensive radioactive background model for a dark matter search with charge-coupled devices (CCDs). We leverage the well-characterized depth and energy resolution of the DAMIC at SNOLAB detector and a detailed GEANT4-based particle-transport simulation to model both bulk and surface backgrounds from natural radioactivity down to 50 eV$_{\text{ee}}$. We fit to the energy and depth distributions of the observed ionization events to differentiate and constrain possible background sources, for example, bulk $^{3}$H from silicon cosmogenic activation and surface $^{210}$Pb from radon plate-out. We observe the bulk background rate of the DAMIC at SNOLAB CCDs to be as low as $3.1 \pm 0.6$ counts kg$^{-1}$ day$^{-1}$ keV$_{\text{ee}}^{-1}$, making it the most sensitive silicon dark matter detector. Finally, we discuss the properties of a statistically significant excess of events over the background model with energies below 200 eV$_{\text{ee}}$., Comment: 27 pages, 19 figures

As the Milky Way and its satellite system become more entrenched in near field cosmology efforts, the need for an accurate mass estimate of the Milky Way's dark matter halo is increasingly critical. With the second and early third data releases of stellar proper motions from {\it Gaia}, several groups calculated full $6$D phase-space information for the population of Milky Way satellite galaxies. Utilizing these data in comparison to subhalo properties drawn from the Phat ELVIS simulations, we constrain the Milky Way dark matter halo mass to be $\sim 1-1.2\times10^{12}~\msun$. We find that the kinematics of subhalos drawn from more- or less-massive hosts (i.e. $>1.2\times10^{12}~\msun$ or $<10^{12}~\msun$) are inconsistent, at the $3\sigma$ confidence level, with the observed velocities of the Milky Way satellites. The preferred host halo mass for the Milky Way is largely insensitive to the exclusion of systems associated with the Large Magellanic Cloud, changes in galaxy formation thresholds, and variations in observational completeness. As more Milky Way satellites are discovered, their velocities (radial, tangential, and total) plus Galactocentric distances will provide further insight into the mass of the Milky Way dark matter halo., Comment: Key Figures: 4 and 5; 15 pages; 8 figures; accepted for publication in MNRAS 3 May 2022

The field of dark matter detection is a highly visible and highly competitive one. In this paper, we propose recommendations for presenting dark matter direct detection results particularly suited for weak-scale dark matter searches, although we believe the spirit of the recommendations can apply more broadly to searches for other dark matter candidates, such as very light dark matter or axions. To translate experimental data into a final published result, direct detection collaborations must make a series of choices in their analysis, ranging from how to model astrophysical parameters to how to make statistical inferences based on observed data. While many collaborations follow a standard set of recommendations in some areas, for example the expected flux of dark matter particles (to a large degree based on a paper from Lewin and Smith in 1995), in other areas, particularly in statistical inference, they have taken different approaches, often from result to result by the same collaboration. We set out a number of recommendations on how to apply the now commonly used Profile Likelihood Ratio method to direct detection data. In addition, updated recommendations for the Standard Halo Model astrophysical parameters and relevant neutrino fluxes are provided. The authors of this note include members of the DAMIC, DarkSide, DARWIN, DEAP, LZ, NEWS-G, PandaX, PICO, SBC, SENSEI, SuperCDMS, and XENON collaborations, and these collaborations provided input to the recommendations laid out here. Wide-spread adoption of these recommendations will make it easier to compare and combine future dark matter results., Comment: 20 pages, 8 figures, 4 tables, version 2 to match publication

The development of direct probes of entanglement is integral to the rapidly expanding field of complex quantum materials. Here we test the robustness of entangled neutrons as a quantum probe by measuring the Clauser-Horne-Shimony-Holt contextuality witness while varying the beam properties. Specifically, we prove that the entanglement of the spin and path subsystems of individual neutrons prepared in two different experiments using two different apparatuses persists even after varying the entanglement length, coherence length, and neutron energy difference of the paths. The two independent apparatuses acting as entangler-disentangler pairs are static-field magnetic Wollaston prisms and resonance-field radio frequency flippers. Our results show that the spatial and energy properties of the neutron beam may be significantly altered without reducing the contextuality witness value below the Tsirelson bound, meaning that maximum entanglement is preserved. We also show that two paths may be considered distinguishable even when separated by less than the neutron coherence length. This work is the key step in the realization of the new modular, robust technique of entangled neutron scattering.

We present measurements of bulk radiocontaminants in the high-resistivity silicon CCDs from the DAMIC at SNOLAB experiment. We utilize the exquisite spatial resolution of CCDs to discriminate between $\alpha$ and $\beta$ decays, and to search with high efficiency for the spatially-correlated decays of various radioisotope sequences. Using spatially-correlated $\beta$ decays, we measure a bulk radioactive contamination of $^{32}$Si in the CCDs of $140 \pm 30$ $\mu$Bq/kg, and place an upper limit on bulk $^{210}$Pb of $< 160~\mu$Bq/kg. Using similar analyses of spatially-correlated bulk $\alpha$ decays, we set limits of $< 11$ $\mu$Bq/kg (0.9 ppt) on $^{238}$U and of $< 7.3$ $\mu$Bq/kg (1.8 ppt) on $^{232}$Th. The ability of DAMIC CCDs to identify and reject spatially-coincident backgrounds, particularly from $^{32}$Si, has significant implications for the next generation of silicon-based dark matter experiments, where $\beta$'s from $^{32}$Si decay will likely be a dominant background. This capability demonstrates the readiness of the CCD technology to achieve kg-scale dark matter sensitivity., Comment: 7 pages, 2 figures

We present constraints on the existence of weakly interacting massive particles (WIMPs) from an 11 kg-day target exposure of the DAMIC experiment at the SNOLAB underground laboratory. The observed energy spectrum and spatial distribution of ionization events with electron-equivalent energies $>$200 eV$_{\rm ee}$ in the DAMIC CCDs are consistent with backgrounds from natural radioactivity. An excess of ionization events is observed above the analysis threshold of 50 eV$_{\rm ee}$. While the origin of this low-energy excess requires further investigation, our data exclude spin-independent WIMP-nucleon scattering cross sections $\sigma_{\chi-n}$ as low as $3\times 10^{-41}$ cm$^2$ for WIMPs with masses $m_{\chi}$ from 7 to 10 GeV$c^{-2}$ . These results are the strongest constraints from a silicon target on the existence of WIMPs with $m_{\chi}$$<$9 GeV$c^{-2}$ and are directly relevant to any dark matter interpretation of the excess of nuclear-recoil events observed by the CDMS silicon experiment in 2013., Comment: 6 pages, 4 figures

The violation of Baryon Number, $\mathcal{B}$, is an essential ingredient for the preferential creation of matter over antimatter needed to account for the observed baryon asymmetry in the universe. However, such a process has yet to be experimentally observed. The HIBEAM/NNBAR %experiment program is a proposed two-stage experiment at the European Spallation Source (ESS) to search for baryon number violation. The program will include high-sensitivity searches for processes that violate baryon number by one or two units: free neutron-antineutron oscillation ($n\rightarrow \bar{n}$) via mixing, neutron-antineutron oscillation via regeneration from a sterile neutron state ($n\rightarrow [n',\bar{n}'] \rightarrow \bar{n}$), and neutron disappearance ($n\rightarrow n'$); the effective $\Delta \mathcal{B}=0$ process of neutron regeneration ($n\rightarrow [n',\bar{n}'] \rightarrow n$) is also possible. The program can be used to discover and characterise mixing in the neutron, antineutron, and sterile neutron sectors. The experiment addresses topical open questions such as the origins of baryogenesis, the nature of dark matter, and is sensitive to scales of new physics substantially in excess of those available at colliders. A goal of the program is to open a discovery window to neutron conversion probabilities (sensitivities) by up to three orders of magnitude compared with previous searches. The opportunity to make such a leap in sensitivity tests should not be squandered. The experiment pulls together a diverse international team of physicists from the particle (collider and low energy) and nuclear physics communities, while also including specialists in neutronics and magnetics.

The European Spallation Source (ESS), presently well on its way to completion, will soon provide the most intense neutron beams for multi-disciplinary science. Fortuitously, it will also generate the largest pulsed neutrino flux suitable for the detection of Coherent Elastic Neutrino-Nucleus Scattering (CE$\nu$NS), a process recently measured for the first time at ORNL's Spallation Neutron Source. We describe innovative detector technologies maximally able to profit from the order-of-magnitude increase in neutrino flux provided by the ESS, along with their sensitivity to a rich particle physics phenomenology accessible through high-statistics, precision CE$\nu$NS measurements., Comment: 21 pages, 15 figures. v2: Minor changes, typo corrected in Fig 6. Version accepted for publication in JHEP

The development of qualitatively new measurement capabilities is often a prerequisite for critical scientific and technological advances. The dramatic progress made by modern probe techniques to uncover the microscopic structure of matter is fundamentally rooted in our control of two defining traits of quantum mechanics: discreteness of physical properties and interference phenomena. Magnetic Resonance Imaging, for instance, exploits the fact that protons have spin and can absorb photons at frequencies that depend on the medium to image the anatomy and physiology of living systems. Scattering techniques, in which photons, electrons, protons or neutrons are used as probes, make use of quantum interference to directly image the spatial position of individual atoms, their magnetic structure, or even unveil their concomitant dynamical correlations. None of these probes have so far exploited a unique characteristic of the quantum world: entanglement. Here we introduce a fundamentally new quantum probe, an entangled neutron beam, where individual neutrons can be entangled in spin, trajectory and energy. Its tunable entanglement length from nanometers to microns and energy differences from peV to neV will enable new investigations of microscopic magnetic correlations in systems with strongly entangled phases, such as those believed to emerge in unconventional superconductors. We develop an interferometer to prove entanglement of these distinguishable properties of the neutron beam by observing clear violations of both Clauser-Horne-Shimony-Holt and Mermin contextuality inequalities in the same experimental setup. Our work opens a pathway to a future era of entangled neutron scattering in matter., Comment: 11 pages, 4 figures

Adopting the Standard Halo Model (SHM) of an isotropic Maxwellian velocity distribution for dark matter (DM) particles in the Galaxy, the most stringent current constraints on their spin-dependent scattering cross-section with nucleons come from the IceCube neutrino observatory and the PICO-60 C$_3$F$_8$ superheated bubble chamber experiments. The former is sensitive to high energy neutrinos from the self-annihilation of DM particles captured in the Sun, while the latter looks for nuclear recoil events from DM scattering off nucleons. Although slower DM particles are more likely to be captured by the Sun, the faster ones are more likely to be detected by PICO. Recent N-body simulations suggest significant deviations from the SHM for the smooth halo component of the DM, while observations hint at a dominant fraction of the local DM being in substructures. We use the method of Ferrer et al. (2015) to exploit the complementarity between the two approaches and derive conservative constraints on DM-nucleon scattering. Our results constrain $\sigma_{\mathrm{SD}} \lesssim 3 \times 10^{-39} \mathrm{cm}^2$ (6 $ \times 10^{-38} \mathrm{cm}^2$) at $\gtrsim 90\%$ C.L. for a DM particle of mass 1~TeV annihilating into $\tau^+ \tau^-$ ($b\bar{b}$) with a local density of $\rho_{\mathrm{DM}} = 0.3~\mathrm{ GeV/cm}^3$. The constraints scale inversely with $\rho_{\mathrm{DM}}$ and are independent of the DM velocity distribution., Comment: 9 pages, 3 figures, 1 table. To appear in Eur.Phys.J. C

We report direct-detection constraints on light dark matter particles interacting with electrons. The results are based on a method that exploits the extremely low levels of leakage current of the DAMIC detector at SNOLAB of 2-6$\times$10$^{-22}$ A cm$^{-2}$. We evaluate the charge distribution of pixels that collect $<10~\rm{e^-}$ for contributions beyond the leakage current that may be attributed to dark matter interactions. Constraints are placed on so-far unexplored parameter space for dark matter masses between 0.6 and 100 MeV$c^{-2}$. We also present new constraints on hidden-photon dark matter with masses in the range $1.2$-$30$ eV$c^{-2}$., Comment: 6 pages, 4 figures

The primary advantage of moderately superheated bubble chamber detectors is their simultaneous sensitivity to nuclear recoils from WIMP dark matter and insensitivity to electron recoil backgrounds. A comprehensive analysis of PICO gamma calibration data demonstrates for the first time that electron recoils in C$_3$F$_8$ scale in accordance with a new nucleation mechanism, rather than one driven by a hot-spike as previously supposed. Using this semi-empirical model, bubble chamber nucleation thresholds may be tuned to be sensitive to lower energy nuclear recoils while maintaining excellent electron recoil rejection. The PICO-40L detector will exploit this model to achieve thermodynamic thresholds as low as 2.8 keV while being dominated by single-scatter events from coherent elastic neutrino-nucleus scattering of solar neutrinos. In one year of operation, PICO-40L can improve existing leading limits from PICO on spin-dependent WIMP-proton coupling by nearly an order of magnitude for WIMP masses greater than 3 GeV c$^{-2}$ and will have the ability to surpass all existing non-xenon bounds on spin-independent WIMP-nucleon coupling for WIMP masses from 3 to 40 GeV c$^{-2}$., Comment: 18 pages, 12 figures

Final results are reported from operation of the PICO-60 C$_3$F$_8$ dark matter detector, a bubble chamber filled with 52 kg of C$_3$F$_8$ located in the SNOLAB underground laboratory. The chamber was operated at thermodynamic thresholds as low as 1.2 keV without loss of stability. A new blind 1404-kg-day exposure at 2.45 keV threshold was acquired with approximately the same expected total background rate as the previous 1167-kg-day exposure at 3.3 keV. This increased exposure is enabled in part by a new optical tracking analysis to better identify events near detector walls, permitting a larger fiducial volume. These results set the most stringent direct-detection constraint to date on the WIMP-proton spin-dependent cross section at 2.5 $\times$ 10$^{-41}$ cm$^2$ for a 25 GeV WIMP, and improve on previous PICO results for 3-5 GeV WIMPs by an order of magnitude., Comment: 9 pages, 8 figures

The identification of non-signal events is a major hurdle to overcome for bubble chamber dark matter experiments such as PICO-60. The current practice of manually developing a discriminator function to eliminate background events is difficult when available calibration data is frequently impure and present only in small quantities. In this study, several different discriminator input/preprocessing formats and neural network architectures are applied to the task. First, they are optimized in a supervised learning context. Next, two novel semi-supervised learning algorithms are trained, and found to replicate the Acoustic Parameter (AP) discriminator previously used in PICO-60 with a mean of 97% accuracy., Comment: 27 pages, 10 figures

A 30-g xenon bubble chamber, operated at Northwestern University in June and November 2016, has for the first time observed simultaneous bubble nucleation and scintillation by nuclear recoils in a superheated liquid. This chamber is instrumented with a CCD camera for near-IR bubble imaging, a solar-blind photomultiplier tube to detect 175-nm xenon scintillation light, and a piezoelectric acoustic transducer to detect the ultrasonic emission from a growing bubble. The time of nucleation determined from the acoustic signal is used to correlate specific scintillation pulses with bubble-nucleating events. We report on data from this chamber for thermodynamic "Seitz" thresholds from 4.2 to 15.0 keV. The observed single- and multiple-bubble rates when exposed to a $^{252}$Cf neutron source indicate that, for an 8.3-keV thermodynamic threshold, the minimum nuclear recoil energy required to nucleate a bubble is $19\pm6$ keV (1$\sigma$ uncertainty). This is consistent with the observed scintillation spectrum for bubble-nucleating events. We see no evidence for bubble nucleation by gamma rays at any of the thresholds studied, setting a 90% C.L. upper limit of $6.3\times10^{-7}$ bubbles per gamma interaction at a 4.2-keV thermodynamic threshold. This indicates stronger gamma discrimination than in CF$_3$I bubble chambers, supporting the hypothesis that scintillation production suppresses bubble nucleation by electron recoils while nuclear recoils nucleate bubbles as usual. These measurements establish the noble-liquid bubble chamber as a promising new technology for the detection of weakly interacting massive particle dark matter and coherent elastic neutrino-nucleus scattering., Comment: 6 pages, 4 figures. Published version

New results are reported from the operation of the PICO-60 dark matter detector, a bubble chamber filled with 52 kg of C$_3$F$_8$ located in the SNOLAB underground laboratory. As in previous PICO bubble chambers, PICO-60 C$_3$F$_8$ exhibits excellent electron recoil and alpha decay rejection, and the observed multiple-scattering neutron rate indicates a single-scatter neutron background of less than 1 event per month. A blind analysis of an efficiency-corrected 1167-kg-day exposure at a 3.3-keV thermodynamic threshold reveals no single-scattering nuclear recoil candidates, consistent with the predicted background. These results set the most stringent direct-detection constraint to date on the WIMP-proton spin-dependent cross section at 3.4 $\times$ 10$^{-41}$ cm$^2$ for a 30-GeV$\thinspace$c$^{-2}$ WIMP, more than one order of magnitude improvement from previous PICO results., Comment: 6 pages, 6 figures

New data are reported from a second run of the 2-liter PICO-2L C$_3$F$_8$ bubble chamber with a total exposure of 129$\,$kg-days at a thermodynamic threshold energy of 3.3$\,$keV. These data show that measures taken to control particulate contamination in the superheated fluid resulted in the absence of the anomalous background events observed in the first run of this bubble chamber. One single nuclear-recoil event was observed in the data, consistent both with the predicted background rate from neutrons and with the observed rate of unambiguous multiple-bubble neutron scattering events. The chamber exhibits the same excellent electron-recoil and alpha decay rejection as was previously reported. These data provide the most stringent direct detection constraints on weakly interacting massive particle (WIMP)-proton spin-dependent scattering to date for WIMP masses $<$ 50$\,$GeV/c$^2$.

New data are reported from the operation of the PICO-60 dark matter detector, a bubble chamber filled with 36.8 kg of CF$_3$I and located in the SNOLAB underground laboratory. PICO-60 is the largest bubble chamber to search for dark matter to date. With an analyzed exposure of 92.8 livedays, PICO-60 exhibits the same excellent background rejection observed in smaller bubble chambers. Alpha decays in PICO-60 exhibit frequency-dependent acoustic calorimetry, similar but not identical to that reported recently in a C$_3$F$_8$ bubble chamber. PICO-60 also observes a large population of unknown background events, exhibiting acoustic, spatial, and timing behaviors inconsistent with those expected from a dark matter signal. These behaviors allow for analysis cuts to remove all background events while retaining $48.2\%$ of the exposure. Stringent limits on weakly interacting massive particles interacting via spin-dependent proton and spin-independent processes are set, and most interpretations of the DAMA/LIBRA modulation signal as dark matter interacting with iodine nuclei are ruled out., Comment: v3 to reflect published version

New data are reported from the operation of a 2-liter C$_3$F$_8$ bubble chamber in the 2100 meter deep SNOLAB underground laboratory, with a total exposure of 211.5 kg-days at four different recoil energy thresholds ranging from 3.2 keV to 8.1 keV. These data show that C3F8 provides excellent electron recoil and alpha rejection capabilities at very low thresholds, including the first observation of a dependence of acoustic signal on alpha energy. Twelve single nuclear recoil event candidates were observed during the run. The candidate events exhibit timing characteristics that are not consistent with the hypothesis of a uniform time distribution, and no evidence for a dark matter signal is claimed. These data provide the most sensitive direct detection constraints on WIMP-proton spin-dependent scattering to date, with significant sensitivity at low WIMP masses for spin-independent WIMP-nucleon scattering., Comment: 6 pages, 6 figures, v2 to match published version

This paper summarizes the relevant theoretical developments, outlines some ideas to improve experimental searches for free neutron-antineutron oscillations, and suggests avenues for future improvement in the experimental sensitivity., Comment: Submitted to Physics Reports