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After launching from the martian surface via the Mars Ascent Vehicle (MAV), the MAV and the Orbiting Sample (OS) capsule containing the samples collected on Mars by the Perseverance rover are to be identified by the Narrow Angle Camera (NAC) on the Earth Return Orbiter (ERO) spacecraft in order to determine the exact orbit of the capsule before rendezvous. To ensure detection of the OS, noise and straylight contributions to the NAC must be well characterized. Here, we assess the radiometric environment at Mars likely to be encountered by the NAC—from the surface through the middle atmosphere—using the High Resolution Stereo Camera (HRSC) onboard Mars Express (MEx) and the Mars Climate Sounder (MCS) onboard the Mars Reconnaissance Orbiter (MRO). The results show that the radiance values in general tend to increase as phase angle increases, as the season progresses from L s = 60° to L s = 230°, and as altitude decreases. We compare HRSC and MCS profiles where observing conditions were similar and find good agreement. At specific latitudes, high-altitude aerosols are present in 1–5% of observations and significantly increase the worst-case radiance contribution above 50 km. We construct envelope profiles from the maximum radiances at 5 km intervals from 0 to 90 km that provide important input for straylight calculations of the NAC and for the validation of models that may be used as input for straylight calculations. [ABSTRACT FROM AUTHOR]