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1. Measurements of aerosol microphysical and chemical properties in the central Arctic atmosphere during MOSAiC

Author

Heutte, Benjamin, Bergner, Nora, Beck, Ivo, Angot, Hélène, Dada, Lubna, Quéléver, Lauriane L. J., Laurila, Tiia, Boyer, Matthew, Brasseur, Zoé, Daellenbach, Kaspar R., Henning, Silvia, Kuang, Chongai, Kulmala, Markku, Lampilahti, Janne, Lampimäki, Markus, Petäjä, Tuukka, Shupe, Matthew D., Sipilä, Mikko, Uin, Janek, Jokinen, Tuija, and Schmale, Julia

Published
2023
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2. Synergistic HNO3–H2SO4–NH3 upper tropospheric particle formation

Author

Wang, Mingyi, Xiao, Mao, Bertozzi, Barbara, Marie, Guillaume, Rörup, Birte, Schulze, Benjamin, Bardakov, Roman, He, Xu-Cheng, Shen, Jiali, Scholz, Wiebke, Marten, Ruby, Dada, Lubna, Baalbaki, Rima, Lopez, Brandon, Lamkaddam, Houssni, Manninen, Hanna E., Amorim, António, Ataei, Farnoush, Bogert, Pia, Brasseur, Zoé, Caudillo, Lucía, De Menezes, Louis-Philippe, Duplissy, Jonathan, Ekman, Annica M. L., Finkenzeller, Henning, Carracedo, Loïc Gonzalez, Granzin, Manuel, Guida, Roberto, Heinritzi, Martin, Hofbauer, Victoria, Höhler, Kristina, Korhonen, Kimmo, Krechmer, Jordan E., Kürten, Andreas, Lehtipalo, Katrianne, Mahfouz, Naser G. A., Makhmutov, Vladimir, Massabò, Dario, Mathot, Serge, Mauldin, Roy L., Mentler, Bernhard, Müller, Tatjana, Onnela, Antti, Petäjä, Tuukka, Philippov, Maxim, Piedehierro, Ana A., Pozzer, Andrea, Ranjithkumar, Ananth, Schervish, Meredith, Schobesberger, Siegfried, Simon, Mario, Stozhkov, Yuri, Tomé, António, Umo, Nsikanabasi Silas, Vogel, Franziska, Wagner, Robert, Wang, Dongyu S., Weber, Stefan K., Welti, André, Wu, Yusheng, Zauner-Wieczorek, Marcel, Sipilä, Mikko, Winkler, Paul M., Hansel, Armin, Baltensperger, Urs, Kulmala, Markku, Flagan, Richard C., Curtius, Joachim, Riipinen, Ilona, Gordon, Hamish, Lelieveld, Jos, El-Haddad, Imad, Volkamer, Rainer, Worsnop, Douglas R., Christoudias, Theodoros, Kirkby, Jasper, Möhler, Ottmar, and Donahue, Neil M.

Published
2022
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4. Ice-nucleating particles active below -24 °C in a Finnish boreal forest and their relationship to bioaerosols.

Author

Vogel, Franziska, Adams, Michael P., Lacher, Larissa, Foster, Polly B., Porter, Grace C. E., Bertozzi, Barbara, Höhler, Kristina, Schneider, Julia, Schorr, Tobias, Umo, Nsikanabasi S., Nadolny, Jens, Brasseur, Zoé, Heikkilä, Paavo, Thomson, Erik S., Büttner, Nicole, Daily, Martin I., Fösig, Romy, Harrison, Alexander D., Keskinen, Jorma, and Proske, Ulrike

Subjects
TAIGAS, CONIFEROUS forests, SPRING, HUMIDITY, AEROSOLS, MICROBIOLOGICAL aerosols, ICE clouds
Abstract

Cloud properties are strongly influenced by ice formation; hence, we need to understand the sources of ice-nucleating particles (INPs) around the globe. Boreal forests are known as sources of bioaerosol, and recent work indicates that these dominate the INP spectra above - 24 °C. To quantify the INP population at temperatures below - 24 °C , we deployed a portable cloud expansion chamber (PINE) in a Finnish boreal forest from 13 March 2018 to 11 May 2018. Using the 6 min time resolution PINE data, we present several lines of evidence that INPs below - 24 °C in this location are also from biological sources: (i) an INP parameterization developed for a pine forest site in Colorado, where many INPs were shown to be biological, produced a good fit to our measurements; a moderate correlation of INPs with aerosol concentration larger than 0.5 µm and the fluorescent bioaerosol concentration; (ii) a negative correlation with relative humidity that may relate to enhanced release of bioaerosol at low humidity from local sources such as the prolific lichen population in boreal forests; and (iii) the absence of correlation with ultra-fine particles (3.5 to 50 nm), indicating that new particle formation events are not sources of INPs. This study should motivate further work to establish whether the commonality in bioaerosol ice-nucleating properties between spring in Finland and summer in Colorado is more generally applicable to different coniferous forest locations and times and also to determine to what extent these bioaerosols are transported to locations where they may affect clouds. [ABSTRACT FROM AUTHOR]

Published
2024
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5. Vertical distribution of ice nucleating particles over the boreal forest of Hyytiälä, Finland.

Author

Brasseur, Zoé, Schneider, Julia, Lampilahti, Janne, Vakkari, Ville, Sinclair, Victoria A., Williamson, Christina J., Xavier, Carlton, Moisseev, Dmitri, Hartmann, Markus, Poutanen, Pyry, Lampimäki, Markus, Kulmala, Markku, Petäjä, Tuukka, Lehtipalo, Katrianne, Thomson, Erik S., Höhler, Kristina, Möhler, Ottmar, and Duplissy, Jonathan

Subjects
ICE clouds, BOUNDARY layer (Aerodynamics), TAIGAS, PARTICLE size distribution, FREE surfaces, TROPOSPHERIC aerosols
Abstract

Ice nucleating particles (INPs) play a crucial role in initiating ice crystal formation in clouds, influencing the dynamics and optical properties of clouds and their impacts on precipitation and the climate system. Despite their importance, there is limited knowledge about the vertical distribution of INPs. This study focuses on aircraft measurements conducted during spring 2018 above the boreal forest of Hyytiälä, Finland. Similarities between INP concentrations, activated fractions, particle concentrations, and size distributions observed at ground level and in the boundary layer aloft indicate that surface particles and INPs are efficiently transported and mixed within the boundary layer. INP concentrations observed in the boundary layer are best predicted by a parameterization describing near-surface INP concentrations driven by the abundance of biogenic aerosol in the Finnish boreal forest, suggesting that biogenic INPs are dominant in the boundary layer above the same environment. Most of the INP concentrations and activated fractions observed in the free troposphere are notably lower than in the boundary layer, and the distinct particle size distributions suggest that different aerosol populations, likely resulting from long-range transport, are present in the free troposphere. However, we show one case where higher INP concentrations are observed in the free troposphere and where a homogeneous particle population exists from the surface to the free troposphere. This indicates that surface particles and INPs from the boreal forest can occasionally reach the free troposphere, which is particularly important as the INPs in the free troposphere can further travel horizontally and/or vertically and impact cloud formation. [ABSTRACT FROM AUTHOR]

Published
2024
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6. A novel aerosol filter sampler for measuring the vertical distribution of ice-nucleating particles via fixed-wing uncrewed aerial vehicles.

Author

Böhmländer, Alexander Julian, Lacher, Larissa, Brus, David, Doulgeris, Konstantinos-Matthaios, Brasseur, Zoé, Boyer, Matthew, Kuula, Joel, Leisner, Thomas, and Möhler, Ottmar

Subjects
SEA level, MICROPHYSICS, HUMIDITY, DETECTION limit, INFORMATION measurement
Abstract

A mobile sampler for the collection of aerosol particles on an uncrewed aerial vehicle (UAV) was developed and deployed during three consecutive Pallas Cloud Experiment campaigns in the vicinity of the Sammaltunturi Global Atmosphere Watch site (67°58' N, 24°7' E, 565 m above sea level). The sampler is designed to collect aerosol particles onto Nuclepore filters, which are subsequently analysed for the temperature-dependent number concentration of ice-nucleating particles of the sampled aerosol with the Ice Nucleation Spectrometer of the Karlsruhe Institute of Technology (INSEKT). This setup is an easy and flexible way to connect INP concentration measurements with cloud microphysics. The sampler was flown with a fixed-wing UAV in different altitudes up to 1000 m above ground level. The total flight time ranges from 1 hour to more than 1.5 hours, depending on environmental conditions. Pressure, temperature and relative humidity are also measured to provide information about the meteorological flight conditions. The flow over the filter was maintained by a micro-diaphragm pump, providing around 10 standard litres per minute over a small filter (diameter of 25 mm) and around 11 standard litres per minute over a larger filter (diameter of 47 mm) at a pressure corresponding to 500 m above sea level. For a typical flight time of 1.5 hours, this results in a sampled air volume of about 930 to 1000 standard litres per flight, giving an INP detection limit of approximately 1.1 × 10−3 and 1.0 × 10−3 INPs per standard litre, respectively. For comparison to the flight results, a similar setup was deployed at ground level. The comparison shows a clear distinction from the water and handling blank background for both setups, proving the technical feasibility of the setups. Furthermore, for some flights, a shift between the two INP populations can be seen, indicating that ground-based INP measurements deviate from the samples collected on-board the UAV. [ABSTRACT FROM AUTHOR]

Published
2024
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7. Ice-nucleating particles active below -24 °C in a Finnish boreal forest and their relationship to bioaerosols

Author

Vogel, Franziska, primary, Adams, Michael P., additional, Lacher, Larissa, additional, Foster, Polly, additional, Porter, Grace C. E., additional, Bertozzi, Barbara, additional, Höhler, Kristina, additional, Schneider, Julia, additional, Schorr, Tobias, additional, Umo, Nsikanabasi S., additional, Nadolny, Jens, additional, Brasseur, Zoé, additional, Heikkilä, Paavo, additional, Thomson, Erik S., additional, Büttner, Nicole, additional, Daily, Martin I., additional, Fösig, Romy, additional, Harrison, Alexander D., additional, Keskinen, Jorma, additional, Proske, Ulrike, additional, Duplissy, Jonathan, additional, Kulmala, Markku, additional, Petäjä, Tuukka, additional, Möhler, Ottmar, additional, and Murray, Benjamin J., additional

Published
2024
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8. Nitrate Radicals Suppress Biogenic New Particle Formation from Monoterpene Oxidation

Author

Li, Dandan, primary, Huang, Wei, additional, Wang, Dongyu, additional, Wang, Mingyi, additional, Thornton, Joel A., additional, Caudillo, Lucía, additional, Rörup, Birte, additional, Marten, Ruby, additional, Scholz, Wiebke, additional, Finkenzeller, Henning, additional, Marie, Guillaume, additional, Baltensperger, Urs, additional, Bell, David M., additional, Brasseur, Zoé, additional, Curtius, Joachim, additional, Dada, Lubna, additional, Duplissy, Jonathan, additional, Gong, Xianda, additional, Hansel, Armin, additional, He, Xu-Cheng, additional, Hofbauer, Victoria, additional, Junninen, Heikki, additional, Krechmer, Jordan E., additional, Kürten, Andreas, additional, Lamkaddam, Houssni, additional, Lehtipalo, Katrianne, additional, Lopez, Brandon, additional, Ma, Yingge, additional, Mahfouz, Naser G. A., additional, Manninen, Hanna E., additional, Mentler, Bernhard, additional, Perrier, Sebastien, additional, Petäjä, Tuukka, additional, Pfeifer, Joschka, additional, Philippov, Maxim, additional, Schervish, Meredith, additional, Schobesberger, Siegfried, additional, Shen, Jiali, additional, Surdu, Mihnea, additional, Tomaz, Sophie, additional, Volkamer, Rainer, additional, Wang, Xinke, additional, Weber, Stefan K., additional, Welti, André, additional, Worsnop, Douglas R., additional, Wu, Yusheng, additional, Yan, Chao, additional, Zauner-Wieczorek, Marcel, additional, Kulmala, Markku, additional, Kirkby, Jasper, additional, Donahue, Neil M., additional, George, Christian, additional, El-Haddad, Imad, additional, Bianchi, Federico, additional, and Riva, Matthieu, additional

Published
2024
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9. Development and characterization of the Portable Ice Nucleation Chamber 2 (PINCii)

Author

Castarède, Dimitri, primary, Brasseur, Zoé, additional, Wu, Yusheng, additional, Kanji, Zamin A., additional, Hartmann, Markus, additional, Ahonen, Lauri, additional, Bilde, Merete, additional, Kulmala, Markku, additional, Petäjä, Tuukka, additional, Pettersson, Jan B. C., additional, Sierau, Berko, additional, Stetzer, Olaf, additional, Stratmann, Frank, additional, Svenningsson, Birgitta, additional, Swietlicki, Erik, additional, Thu Nguyen, Quynh, additional, Duplissy, Jonathan, additional, and Thomson, Erik S., additional

Published
2023
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10. An intercomparison study of four different techniques for measuring the chemical composition of nanoparticles

Author

Caudillo, Lucía, primary, Surdu, Mihnea, additional, Lopez, Brandon, additional, Wang, Mingyi, additional, Thoma, Markus, additional, Bräkling, Steffen, additional, Buchholz, Angela, additional, Simon, Mario, additional, Wagner, Andrea C., additional, Müller, Tatjana, additional, Granzin, Manuel, additional, Heinritzi, Martin, additional, Amorim, Antonio, additional, Bell, David M., additional, Brasseur, Zoé, additional, Dada, Lubna, additional, Duplissy, Jonathan, additional, Finkenzeller, Henning, additional, He, Xu-Cheng, additional, Lamkaddam, Houssni, additional, Mahfouz, Naser G. A., additional, Makhmutov, Vladimir, additional, Manninen, Hanna E., additional, Marie, Guillaume, additional, Marten, Ruby, additional, Mauldin, Roy L., additional, Mentler, Bernhard, additional, Onnela, Antti, additional, Petäjä, Tuukka, additional, Pfeifer, Joschka, additional, Philippov, Maxim, additional, Piedehierro, Ana A., additional, Rörup, Birte, additional, Scholz, Wiebke, additional, Shen, Jiali, additional, Stolzenburg, Dominik, additional, Tauber, Christian, additional, Tian, Ping, additional, Tomé, António, additional, Umo, Nsikanabasi Silas, additional, Wang, Dongyu S., additional, Wang, Yonghong, additional, Weber, Stefan K., additional, Welti, André, additional, Zauner-Wieczorek, Marcel, additional, Baltensperger, Urs, additional, Flagan, Richard C., additional, Hansel, Armin, additional, Kirkby, Jasper, additional, Kulmala, Markku, additional, Lehtipalo, Katrianne, additional, Worsnop, Douglas R., additional, Haddad, Imad El, additional, Donahue, Neil M., additional, Vogel, Alexander L., additional, Kürten, Andreas, additional, and Curtius, Joachim, additional

Published
2023
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11. Measurement of the collision rate coefficients between atmospheric ions and multiply charged aerosol particles in the CERN CLOUD chamber

Author

Pfeifer, Joschka, Mahfouz, Naser G. A., Schulze, Benjamin C., Mathot, Serge, Stolzenburg, Dominik, Baalbaki, Rima, Brasseur, Zoé, Caudillo, Lucia, Dada, Lubna, Granzin, Manuel, He, Xu-Cheng, Lamkaddam, Houssni, Lopez, Brandon, Makhmutov, Vladimir, Marten, Ruby, Mentler, Bernhard, Müller, Tatjana, Onnela, Antti, Philippov, Maxim, Piedehierro, Ana A., Rörup, Birte, Schervish, Meredith, Tian, Ping, Umo, Nsikanabasi S., Wang, Dongyu S., Wang, Mingyi, Weber, Stefan K., Welti, André, Wu, Yusheng, Zauner-Wieczorek, Marcel, Amorim, Antonio, Haddad, Imad, Kulmala, Markku, Lehtipalo, Katrianne, Petäjä, Tuukka, Tomé, António, Mirme, Sander, Manninen, Hanna E., Donahue, Neil M., Flagan, Richard C., Kürten, Andreas, Curtius, Joachim, and Kirkby, Jasper

Abstract

Aerosol particles have an important role in Earth's radiation balance and climate, both directly and indirectly through aerosol–cloud interactions. Most aerosol particles in the atmosphere are weakly charged, affecting both their collision rates with ions and neutral molecules, as well as the rates by which they are scavenged by other aerosol particles and cloud droplets. The rate coefficients between ions and aerosol particles are important since they determine the growth rates and lifetimes of ions and charged aerosol particles, and so they may influence cloud microphysics, dynamics, and aerosol processing. However, despite their importance, very few experimental measurements exist of charged aerosol collision rates under atmospheric conditions, where galactic cosmic rays in the lower troposphere give rise to ion pair concentrations of around 1000 cm−3. Here we present measurements in the CERN CLOUD chamber of the rate coefficients between ions and small ( nm) aerosol particles containing up to 9 elementary charges, e. We find the rate coefficient of a singly charged ion with an oppositely charged particle increases from 2.0 (0.4–4.4) × 10−6 cm3 s−1 to 30.6 (24.9–45.1) × 10−6 cm3 s−1 for particles with charges of 1 to 9 e, respectively, where the parentheses indicate the ±1σ uncertainty interval. Our measurements are compatible with theoretical predictions and show excellent agreement with the model of Gatti and Kortshagen (2008).

Published
2023

12. A full year of aerosol size distribution data from the central Arctic under an extreme positive Arctic Oscillation : insights from the Multidisciplinarydrifting Observatory for the Study of Arctic Climate (MOSAiC) expedition

Author

Boyer, Matthew, Aliaga, Diego, Pernov, Jakob Boyd, Angot, Hélène, Quéléver, Lauriane L. J., Dada, Lubna, Heutte, Benjamin, Dall'Osto, Manuel, Beddows, David C. S., Brasseur, Zoé, Beck, Ivo, Bucci, Silvia, Duetsch, Marina, Stohl, Andreas, Laurila, Tiia, Asmi, Eija, Massling, Andreas, Thomas, Daniel Charles, Klenø Nøjgaard, Jakob, Chan, Tak, Sharma, Sangeeta, Tunved, Peter, Krejci, Radovan, Hansson, Hans-Christen, Bianchi, Federico, Lehtipalo, Katrianne, Wiedensohler, Alfred, Weinhold, Kay, Kulmala, Markku, Petäjä, Tuukka, Sipilä, Mikko, Schmale, Julia, Jokinen, Tuija, Boyer, Matthew, Aliaga, Diego, Pernov, Jakob Boyd, Angot, Hélène, Quéléver, Lauriane L. J., Dada, Lubna, Heutte, Benjamin, Dall'Osto, Manuel, Beddows, David C. S., Brasseur, Zoé, Beck, Ivo, Bucci, Silvia, Duetsch, Marina, Stohl, Andreas, Laurila, Tiia, Asmi, Eija, Massling, Andreas, Thomas, Daniel Charles, Klenø Nøjgaard, Jakob, Chan, Tak, Sharma, Sangeeta, Tunved, Peter, Krejci, Radovan, Hansson, Hans-Christen, Bianchi, Federico, Lehtipalo, Katrianne, Wiedensohler, Alfred, Weinhold, Kay, Kulmala, Markku, Petäjä, Tuukka, Sipilä, Mikko, Schmale, Julia, and Jokinen, Tuija

Abstract

The Arctic environment is rapidly changing due to accelerated warming in the region. The warming trend is driving a decline in sea ice extent, which thereby enhances feedback loops in the surface energy budget in the Arctic. Arctic aerosols play an important role in the radiative balance and hence the climate response in the region, yet direct observations of aerosols over the Arctic Ocean are limited. In this study, we investigate the annual cycle in the aerosol particle number size distribution (PNSD), particle number concentration (PNC), and black carbon (BC) mass concentration in the central Arctic during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition. This is the first continuous, year-long data set of aerosol PNSD ever collected over the sea ice in the central Arctic Ocean. We use a k-means cluster analysis, FLEXPART simulations, and inverse modeling to evaluate seasonal patterns and the influence of different source regions on the Arctic aerosol population. Furthermore, we compare the aerosol observations to land-based sites across the Arctic, using both long-term measurements and observations during the year of the MOSAiC expedition (2019–2020), to investigate interannual variability and to give context to the aerosol characteristics from within the central Arctic. Our analysis identifies that, overall, the central Arctic exhibits typical seasonal patterns of aerosols, including anthropogenic influence from Arctic haze in winter and secondary aerosol processes in summer. The seasonal pattern corresponds to the global radiation, surface air temperature, and timing of sea ice melting/freezing, which drive changes in transport patterns and secondary aerosol processes. In winter, the Norilsk region in Russia/Siberia was the dominant source of Arctic haze signals in the PNSD and BC observations, which contributed to higher accumulation-mode PNC and BC mass concentrations in the central Arctic than at land-based obse

Published
2023
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13. Iodine oxoacids enhance nucleation of sulfuric acid particles in the atmosphere

Author

He, Xu-Cheng, Simon, Mario, Iyer, Siddharth, Xie, Hong-Bin, Rörup, Birte, Shen, Jiali, Finkenzeller, Henning, Stolzenburg, Dominik, Zhang, Rongjie, Baccarini, Andrea, Tham, Yee Jun, Wang, Mingyi, Amanatidis, Stavros, Piedehierro, Ana A., Amorim, Antonio, Baalbaki, Rima, Brasseur, Zoé, Caudillo, Lucía, Chu, Biwu, Dada, Lubna, Duplissy, Jonathan, El Haddad, Imad, Flagan, Richard C., Granzin, Manuel, Hansel, Armin, Heinritzi, Martin, Hofbauer, Victoria, Jokinen, Tuija, Kemppainen, Deniz, Kong, Weimeng, Krechmer, Jordan, Kürten, Andreas, Lamkaddam, Houssni, Lopez, Brandon, Ma, Fangfang, Mahfouz, Naser G. A., Makhmutov, Vladimir, Manninen, Hanna E., Marie, Guillaume, Marten, Ruby, Massabò, Dario, Mauldin, Roy L., Mentler, Bernhard, Onnela, Antti, Petäjä, Tuukka, Pfeifer, Joschka, Philippov, Maxim, Ranjithkumar, Ananth, Rissanen, Matti P., Schobesberger, Siegfried, Scholz, Wiebke, Schulze, Benjamin, Surdu, Mihnea, Thakur, Roseline C., Tomé, António, Wagner, Andrea C., Wang, Dongyu, Wang, Yonghong, Weber, Stefan K., Welti, André, Winkler, Paul M., Zauner-Wieczorek, Marcel, Baltensperger, Urs, Curtius, Joachim, Kurtén, Theo, Worsnop, Douglas R., Volkamer, Rainer, Lehtipalo, Katrianne, Kirkby, Jasper, Donahue, Neil M., Sipilä, Mikko, Kulmala, Markku, He, Xu-Cheng, Simon, Mario, Iyer, Siddharth, Xie, Hong-Bin, Rörup, Birte, Shen, Jiali, Finkenzeller, Henning, Stolzenburg, Dominik, Zhang, Rongjie, Baccarini, Andrea, Tham, Yee Jun, Wang, Mingyi, Amanatidis, Stavros, Piedehierro, Ana A., Amorim, Antonio, Baalbaki, Rima, Brasseur, Zoé, Caudillo, Lucía, Chu, Biwu, Dada, Lubna, Duplissy, Jonathan, El Haddad, Imad, Flagan, Richard C., Granzin, Manuel, Hansel, Armin, Heinritzi, Martin, Hofbauer, Victoria, Jokinen, Tuija, Kemppainen, Deniz, Kong, Weimeng, Krechmer, Jordan, Kürten, Andreas, Lamkaddam, Houssni, Lopez, Brandon, Ma, Fangfang, Mahfouz, Naser G. A., Makhmutov, Vladimir, Manninen, Hanna E., Marie, Guillaume, Marten, Ruby, Massabò, Dario, Mauldin, Roy L., Mentler, Bernhard, Onnela, Antti, Petäjä, Tuukka, Pfeifer, Joschka, Philippov, Maxim, Ranjithkumar, Ananth, Rissanen, Matti P., Schobesberger, Siegfried, Scholz, Wiebke, Schulze, Benjamin, Surdu, Mihnea, Thakur, Roseline C., Tomé, António, Wagner, Andrea C., Wang, Dongyu, Wang, Yonghong, Weber, Stefan K., Welti, André, Winkler, Paul M., Zauner-Wieczorek, Marcel, Baltensperger, Urs, Curtius, Joachim, Kurtén, Theo, Worsnop, Douglas R., Volkamer, Rainer, Lehtipalo, Katrianne, Kirkby, Jasper, Donahue, Neil M., Sipilä, Mikko, and Kulmala, Markku

Abstract

The main nucleating vapor in the atmosphere is thought to be sulfuric acid (H2SO4), stabilized by ammonia (NH3). However, in marine and polar regions, NH3 is generally low, and H2SO4 is frequently found together with iodine oxoacids [HIOx, i.e., iodic acid (HIO3) and iodous acid (HIO2)]. In experiments performed with the CERN CLOUD (Cosmics Leaving OUtdoor Droplets) chamber, we investigated the interplay of H2SO4 and HIOx during atmospheric particle nucleation. We found that HIOx greatly enhances H2SO4(-NH3) nucleation through two different interactions. First, HIO3 strongly binds with H2SO4 in charged clusters so they drive particle nucleation synergistically. Second, HIO2 substitutes for NH3, forming strongly bound H2SO4-HIO2 acid-base pairs in molecular clusters. Global observations imply that HIOx is enhancing H2SO4(-NH3) nucleation rates 10- to 10,000-fold in marine and polar regions.

Published
2023

14. A full year of aerosol size distribution data from the central Arctic under an extreme positive Arctic Oscillation: insights from the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition

Author

European Commission, Academy of Finland, Department of Energy (US), Swiss Polar Institute, Agencia Estatal de Investigación (España), Boyer, Matthew, Aliaga, Diego, Pernov, Jakob Boyd, Angot, Hélène, Quéléver, Lauriane L.J., Dada, Lubna, Heutte, Benjamin, Dall'Osto, Manuel, Beddows, David C. S., Brasseur, Zoé, Beck, Ivo, Bucci, Silvia, Duetsch, Marina, Stohl, Andreas, Laurila, Tiia, Asmi, Eija, Massling, Andreas, Thomas, Daniel Charles, Nøjgaard, Jacob Klenø, Chan, Tak, Sharma, Sangeeta, Tunved, Peter, Krejci, Radovan, Hansson, Hans-Christien, Bianchi, Federico, Lehtipalo, Katrianne, Wiedensohler, Alfred, Weinhold, Kay, Kulmala, Markku, Petäjä, Tuukka, Sipilä, Mikko, Schmale, Julia, Jokinen, Tuija, European Commission, Academy of Finland, Department of Energy (US), Swiss Polar Institute, Agencia Estatal de Investigación (España), Boyer, Matthew, Aliaga, Diego, Pernov, Jakob Boyd, Angot, Hélène, Quéléver, Lauriane L.J., Dada, Lubna, Heutte, Benjamin, Dall'Osto, Manuel, Beddows, David C. S., Brasseur, Zoé, Beck, Ivo, Bucci, Silvia, Duetsch, Marina, Stohl, Andreas, Laurila, Tiia, Asmi, Eija, Massling, Andreas, Thomas, Daniel Charles, Nøjgaard, Jacob Klenø, Chan, Tak, Sharma, Sangeeta, Tunved, Peter, Krejci, Radovan, Hansson, Hans-Christien, Bianchi, Federico, Lehtipalo, Katrianne, Wiedensohler, Alfred, Weinhold, Kay, Kulmala, Markku, Petäjä, Tuukka, Sipilä, Mikko, Schmale, Julia, and Jokinen, Tuija

Abstract

The Arctic environment is rapidly changing due to accelerated warming in the region. The warming trend is driving a decline in sea ice extent, which thereby enhances feedback loops in the surface energy budget in the Arctic. Arctic aerosols play an important role in the radiative balance and hence the climate response in the region, yet direct observations of aerosols over the Arctic Ocean are limited. In this study, we investigate the annual cycle in the aerosol particle number size distribution (PNSD), particle number concentration (PNC), and black carbon (BC) mass concentration in the central Arctic during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition. This is the first continuous, year-long data set of aerosol PNSD ever collected over the sea ice in the central Arctic Ocean. We use a k-means cluster analysis, FLEXPART simulations, and inverse modeling to evaluate seasonal patterns and the influence of different source regions on the Arctic aerosol population. Furthermore, we compare the aerosol observations to land-based sites across the Arctic, using both long-term measurements and observations during the year of the MOSAiC expedition (2019–2020), to investigate interannual variability and to give context to the aerosol characteristics from within the central Arctic. Our analysis identifies that, overall, the central Arctic exhibits typical seasonal patterns of aerosols, including anthropogenic influence from Arctic haze in winter and secondary aerosol processes in summer. The seasonal pattern corresponds to the global radiation, surface air temperature, and timing of sea ice melting/freezing, which drive changes in transport patterns and secondary aerosol processes. In winter, the Norilsk region in Russia/Siberia was the dominant source of Arctic haze signals in the PNSD and BC observations, which contributed to higher accumulation-mode PNC and BC mass concentrations in the central Arctic than at land-based obse

Published
2023

17. Nitrate radicals suppress biogenic new particle formation from monoterpene oxidation

Author

Li, Dandan, primary, Huang, Wei, additional, Wang, Dongyu, additional, Wang, Mingyi, additional, Thornton, Joel, additional, Caudillo, Lucía, additional, Rörup, Birte, additional, Marten, Ruby, additional, Scholz, Wiebke, additional, Finkenzeller, Henning, additional, Marie, Guillaume, additional, Bell, David, additional, Brasseur, Zoé, additional, Curtius, Joachim, additional, Dada, Lubna, additional, Duplissy, Jonathan, additional, Gong, Xianda, additional, Hansel, Armin, additional, He, Xu-cheng, additional, Hofbauer, Victoria, additional, Junninen, Heikki, additional, Krechmer, Jordan E., additional, Kurten, Andreas, additional, Lamkaddam, Houssni, additional, LEHTIPALO, Katrianne, additional, Lopez, Brandon, additional, Ma, Yingge, additional, Mahfouz, Naser, additional, Manninen, Hanna E., additional, Mentler, Bernhard, additional, Perrier, Sebastien, additional, Petäjä, Tuukka, additional, Pfeifer, Joschka, additional, Philippov, Maxim, additional, Schervish, Meredith, additional, Schobesberger, Siegfried, additional, Shen, Jiali, additional, Surdu, Mihnea, additional, Tomaz, Sophie, additional, Volkamer, Rainer, additional, Wang, Xinke, additional, Weber, Stefan, additional, Welti, André, additional, Worsnop, Douglas, additional, wu, yusheng, additional, Yan, Chao, additional, Zauner-Wieczorek, Marcel, additional, Kulmala, Markku, additional, Kirkby, Jasper, additional, Donahue, Neil, additional, George, Christian, additional, El-Haddad, Imad, additional, Bianchi, Federico, additional, and Riva, Matthieu, additional

Published
2023
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18. Molecular Understanding of the Enhancement in Organic Aerosol Mass at High Relative Humidity

Author

Surdu, Mihnea, primary, Lamkaddam, Houssni, additional, Wang, Dongyu S., additional, Bell, David M., additional, Xiao, Mao, additional, Lee, Chuan Ping, additional, Li, Dandan, additional, Caudillo, Lucía, additional, Marie, Guillaume, additional, Scholz, Wiebke, additional, Wang, Mingyi, additional, Lopez, Brandon, additional, Piedehierro, Ana A., additional, Ataei, Farnoush, additional, Baalbaki, Rima, additional, Bertozzi, Barbara, additional, Bogert, Pia, additional, Brasseur, Zoé, additional, Dada, Lubna, additional, Duplissy, Jonathan, additional, Finkenzeller, Henning, additional, He, Xu-Cheng, additional, Höhler, Kristina, additional, Korhonen, Kimmo, additional, Krechmer, Jordan E., additional, Lehtipalo, Katrianne, additional, Mahfouz, Naser G. A., additional, Manninen, Hanna E., additional, Marten, Ruby, additional, Massabò, Dario, additional, Mauldin, Roy, additional, Petäjä, Tuukka, additional, Pfeifer, Joschka, additional, Philippov, Maxim, additional, Rörup, Birte, additional, Simon, Mario, additional, Shen, Jiali, additional, Umo, Nsikanabasi Silas, additional, Vogel, Franziska, additional, Weber, Stefan K., additional, Zauner-Wieczorek, Marcel, additional, Volkamer, Rainer, additional, Saathoff, Harald, additional, Möhler, Ottmar, additional, Kirkby, Jasper, additional, Worsnop, Douglas R., additional, Kulmala, Markku, additional, Stratmann, Frank, additional, Hansel, Armin, additional, Curtius, Joachim, additional, Welti, André, additional, Riva, Matthieu, additional, Donahue, Neil M., additional, Baltensperger, Urs, additional, and El Haddad, Imad, additional

Published
2023
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19. A full year of aerosol size distribution data from the central Arctic under an extreme positive Arctic Oscillation: insights from the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition

Author

Boyer, Matthew, primary, Aliaga, Diego, additional, Pernov, Jakob Boyd, additional, Angot, Hélène, additional, Quéléver, Lauriane L. J., additional, Dada, Lubna, additional, Heutte, Benjamin, additional, Dall'Osto, Manuel, additional, Beddows, David C. S., additional, Brasseur, Zoé, additional, Beck, Ivo, additional, Bucci, Silvia, additional, Duetsch, Marina, additional, Stohl, Andreas, additional, Laurila, Tiia, additional, Asmi, Eija, additional, Massling, Andreas, additional, Thomas, Daniel Charles, additional, Nøjgaard, Jakob Klenø, additional, Chan, Tak, additional, Sharma, Sangeeta, additional, Tunved, Peter, additional, Krejci, Radovan, additional, Hansson, Hans Christen, additional, Bianchi, Federico, additional, Lehtipalo, Katrianne, additional, Wiedensohler, Alfred, additional, Weinhold, Kay, additional, Kulmala, Markku, additional, Petäjä, Tuukka, additional, Sipilä, Mikko, additional, Schmale, Julia, additional, and Jokinen, Tuija, additional

Published
2023
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20. Supplementary material to "Measurement of the rate coefficients between atmospheric ions and multiply charged aerosol particles in the CERN CLOUD chamber"

Author

Pfeifer, Joschka, primary, Mahfouz, Naser G., additional, Schulze, Ben, additional, Mathot, Serge, additional, Stolzenburg, Dominik, additional, Baalbaki, Rima, additional, Brasseur, Zoé, additional, Caudillo, Lucia, additional, Dada, Lubna, additional, Granzin, Manuel, additional, He, Xu-Cheng, additional, Lamkaddam, Houssni, additional, Lopez, Brandon, additional, Makhmutov, Vladimir, additional, Marten, Ruby, additional, Mentler, Bernhard, additional, Müller, Tatjana, additional, Onnela, Antti, additional, Philippov, Maxim, additional, Piedehierro, Ana A., additional, Rörup, Birte, additional, Schervish, Meredith, additional, Tian, Ping, additional, Umo, Nsikanabasi S., additional, Wang, Dongyu S., additional, Wang, Mingyi, additional, Weber, Stefan K., additional, Welti, André, additional, Wu, Yusheng, additional, Zauner-Wieczorek, Marcel, additional, Amorim, Antonio, additional, El Haddad, Imad, additional, Kulmala, Markku, additional, Lehtipalo, Katrianne, additional, Petäjä, Tuukka, additional, Tomé, António, additional, Mirme, Sander, additional, Manninen, Hanna E., additional, Donahue, Neil M., additional, Flagan, Richard C., additional, Kürten, Andreas, additional, Curtius, Joachim, additional, and Kirkby, Jasper, additional

Published
2022
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21. Measurement of the rate coefficients between atmospheric ions and multiply charged aerosol particles in the CERN CLOUD chamber

Author

Pfeifer, Joschka, primary, Mahfouz, Naser G., additional, Schulze, Ben, additional, Mathot, Serge, additional, Stolzenburg, Dominik, additional, Baalbaki, Rima, additional, Brasseur, Zoé, additional, Caudillo, Lucia, additional, Dada, Lubna, additional, Granzin, Manuel, additional, He, Xu-Cheng, additional, Lamkaddam, Houssni, additional, Lopez, Brandon, additional, Makhmutov, Vladimir, additional, Marten, Ruby, additional, Mentler, Bernhard, additional, Müller, Tatjana, additional, Onnela, Antti, additional, Philippov, Maxim, additional, Piedehierro, Ana A., additional, Rörup, Birte, additional, Schervish, Meredith, additional, Tian, Ping, additional, Umo, Nsikanabasi S., additional, Wang, Dongyu S., additional, Wang, Mingyi, additional, Weber, Stefan K., additional, Welti, André, additional, Wu, Yusheng, additional, Zauner-Wieczorek, Marcel, additional, Amorim, Antonio, additional, El Haddad, Imad, additional, Kulmala, Markku, additional, Lehtipalo, Katrianne, additional, Petäjä, Tuukka, additional, Tomé, António, additional, Mirme, Sander, additional, Manninen, Hanna E., additional, Donahue, Neil M., additional, Flagan, Richard C., additional, Kürten, Andreas, additional, Curtius, Joachim, additional, and Kirkby, Jasper, additional

Published
2022
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22. High Gas-Phase Methanesulfonic Acid Production in the OH-Initiated Oxidation of Dimethyl Sulfide at Low Temperatures

Author

Shen, Jiali, primary, Scholz, Wiebke, additional, He, Xu-Cheng, additional, Zhou, Putian, additional, Marie, Guillaume, additional, Wang, Mingyi, additional, Marten, Ruby, additional, Surdu, Mihnea, additional, Rörup, Birte, additional, Baalbaki, Rima, additional, Amorim, Antonio, additional, Ataei, Farnoush, additional, Bell, David M., additional, Bertozzi, Barbara, additional, Brasseur, Zoé, additional, Caudillo, Lucía, additional, Chen, Dexian, additional, Chu, Biwu, additional, Dada, Lubna, additional, Duplissy, Jonathan, additional, Finkenzeller, Henning, additional, Granzin, Manuel, additional, Guida, Roberto, additional, Heinritzi, Martin, additional, Hofbauer, Victoria, additional, Iyer, Siddharth, additional, Kemppainen, Deniz, additional, Kong, Weimeng, additional, Krechmer, Jordan E., additional, Kürten, Andreas, additional, Lamkaddam, Houssni, additional, Lee, Chuan Ping, additional, Lopez, Brandon, additional, Mahfouz, Naser G. A., additional, Manninen, Hanna E., additional, Massabò, Dario, additional, Mauldin, Roy L., additional, Mentler, Bernhard, additional, Müller, Tatjana, additional, Pfeifer, Joschka, additional, Philippov, Maxim, additional, Piedehierro, Ana A., additional, Roldin, Pontus, additional, Schobesberger, Siegfried, additional, Simon, Mario, additional, Stolzenburg, Dominik, additional, Tham, Yee Jun, additional, Tomé, António, additional, Umo, Nsikanabasi Silas, additional, Wang, Dongyu, additional, Wang, Yonghong, additional, Weber, Stefan K., additional, Welti, André, additional, Wollesen de Jonge, Robin, additional, Wu, Yusheng, additional, Zauner-Wieczorek, Marcel, additional, Zust, Felix, additional, Baltensperger, Urs, additional, Curtius, Joachim, additional, Flagan, Richard C., additional, Hansel, Armin, additional, Möhler, Ottmar, additional, Petäjä, Tuukka, additional, Volkamer, Rainer, additional, Kulmala, Markku, additional, Lehtipalo, Katrianne, additional, Rissanen, Matti, additional, Kirkby, Jasper, additional, El-Haddad, Imad, additional, Bianchi, Federico, additional, Sipilä, Mikko, additional, Donahue, Neil M., additional, and Worsnop, Douglas R., additional

Published
2022
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23. Supplementary material to "A full year of aerosol size distribution data from the central Arctic under an extreme positive Arctic Oscillation: Insights from the MOSAiC expedition"

Author

Boyer, Matthew, primary, Aliaga, Diego, additional, Pernov, Jakob Boyd, additional, Angot, Hélène, additional, Quéléver, Lauriane L. J., additional, Dada, Lubna, additional, Heutte, Benjamin, additional, Dall’Osto, Manuel, additional, Beddows, David C. S., additional, Brasseur, Zoé, additional, Beck, Ivo, additional, Bucci, Silvia, additional, Duetsch, Marina, additional, Stohl, Andreas, additional, Laurila, Tiia, additional, Asmi, Eija, additional, Massling, Andreas, additional, Thomas, Daniel Charles, additional, Nøjgaard, Jakob Klenø, additional, Chan, Tak, additional, Sharma, Sangeeta, additional, Tunved, Peter, additional, Krejci, Radovan, additional, Hansson, Hans Christen, additional, Kulmala, Markku, additional, Petäjä, Tuukka, additional, Sipilä, Mikko, additional, Schmale, Julia, additional, and Jokinen, Tuija, additional

Published
2022
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24. A full year of aerosol size distribution data from the central Arctic under an extreme positive Arctic Oscillation: Insights from the MOSAiC expedition

Author

Boyer, Matthew, primary, Aliaga, Diego, additional, Pernov, Jakob Boyd, additional, Angot, Hélène, additional, Quéléver, Lauriane L. J., additional, Dada, Lubna, additional, Heutte, Benjamin, additional, Dall’Osto, Manuel, additional, Beddows, David C. S., additional, Brasseur, Zoé, additional, Beck, Ivo, additional, Bucci, Silvia, additional, Duetsch, Marina, additional, Stohl, Andreas, additional, Laurila, Tiia, additional, Asmi, Eija, additional, Massling, Andreas, additional, Thomas, Daniel Charles, additional, Nøjgaard, Jakob Klenø, additional, Chan, Tak, additional, Sharma, Sangeeta, additional, Tunved, Peter, additional, Krejci, Radovan, additional, Hansson, Hans Christen, additional, Kulmala, Markku, additional, Petäjä, Tuukka, additional, Sipilä, Mikko, additional, Schmale, Julia, additional, and Jokinen, Tuija, additional

Published
2022
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25. An intercomparison study of four different techniques for measuring the chemical composition of nanoparticles

Author

Caudillo, Lucía, primary, Surdu, Mihnea, additional, Lopez, Brandon, additional, Wang, Mingyi, additional, Thoma, Markus, additional, Bräkling, Steffen, additional, Buchholz, Angela, additional, Simon, Mario, additional, Wagner, Andrea C., additional, Müller, Tatjana, additional, Granzin, Manuel, additional, Heinritzi, Martin, additional, Amorim, Antonio, additional, Bell, David M., additional, Brasseur, Zoé, additional, Dada, Lubna, additional, Duplissy, Jonathan, additional, Finkenzeller, Henning, additional, He, Xu-Cheng, additional, Lamkaddam, Houssni, additional, Mahfouz, Naser G. A., additional, Makhmutov, Vladimir, additional, Manninen, Hanna E., additional, Marie, Guillaume, additional, Marten, Ruby, additional, Mauldin, Roy L., additional, Mentler, Bernhard, additional, Onnela, Antti, additional, Petäjä, Tuukka, additional, Pfeifer, Joschka, additional, Philippov, Maxim, additional, Piedehierro, Ana A., additional, Rörup, Birte, additional, Scholz, Wiebke, additional, Shen, Jiali, additional, Stolzenburg, Dominik, additional, Tauber, Christian, additional, Tian, Ping, additional, Tomé, António, additional, Umo, Nsikanabasi Silas, additional, Wang, Dongyu S., additional, Wang, Yonghong, additional, Weber, Stefan K., additional, Welti, André, additional, Zauner-Wieczorek, Marcel, additional, Baltensperger, Urs, additional, Flagan, Richard C., additional, Hansel, Armin, additional, Kirkby, Jasper, additional, Kulmala, Markku, additional, Lehtipalo, Katrianne, additional, Worsnop, Douglas R., additional, Haddad, Imad El, additional, Donahue, Neil M., additional, Vogel, Alexander L., additional, Kürten, Andreas, additional, and Curtius, Joachim, additional

Published
2022
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26. Supplementary material to "An intercomparison study of four different techniques for measuring the chemical composition of nanoparticles"

Author

Caudillo, Lucía, primary, Surdu, Mihnea, additional, Lopez, Brandon, additional, Wang, Mingyi, additional, Thoma, Markus, additional, Bräkling, Steffen, additional, Buchholz, Angela, additional, Simon, Mario, additional, Wagner, Andrea C., additional, Müller, Tatjana, additional, Granzin, Manuel, additional, Heinritzi, Martin, additional, Amorim, Antonio, additional, Bell, David M., additional, Brasseur, Zoé, additional, Dada, Lubna, additional, Duplissy, Jonathan, additional, Finkenzeller, Henning, additional, He, Xu-Cheng, additional, Lamkaddam, Houssni, additional, Mahfouz, Naser G. A., additional, Makhmutov, Vladimir, additional, Manninen, Hanna E., additional, Marie, Guillaume, additional, Marten, Ruby, additional, Mauldin, Roy L., additional, Mentler, Bernhard, additional, Onnela, Antti, additional, Petäjä, Tuukka, additional, Pfeifer, Joschka, additional, Philippov, Maxim, additional, Piedehierro, Ana A., additional, Rörup, Birte, additional, Scholz, Wiebke, additional, Shen, Jiali, additional, Stolzenburg, Dominik, additional, Tauber, Christian, additional, Tian, Ping, additional, Tomé, António, additional, Umo, Nsikanabasi Silas, additional, Wang, Dongyu S., additional, Wang, Yonghong, additional, Weber, Stefan K., additional, Welti, André, additional, Zauner-Wieczorek, Marcel, additional, Baltensperger, Urs, additional, Flagan, Richard C., additional, Hansel, Armin, additional, Kirkby, Jasper, additional, Kulmala, Markku, additional, Lehtipalo, Katrianne, additional, Worsnop, Douglas R., additional, Haddad, Imad El, additional, Donahue, Neil M., additional, Vogel, Alexander L., additional, Kürten, Andreas, additional, and Curtius, Joachim, additional

Published
2022
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27. Overview of the MOSAiC expedition - Atmosphere

Author

Shupe, Matthew D., Rex, Markus, Blomquist, Byron, Persson, P. Ola G., Schmale, Julia, Uttal, Taneil, Althausen, Dietrich, Angot, Hélène, Archer, Stephen, Bariteau, Ludovic, Beck, Ivo, Bilberry, John, Bucci, Silvia, Buck, Clifton, Boyer, Matt, Brasseur, Zoé, Brooks, Ian M., Calmer, Radiance, Cassano, John, Castro, Vagner, Chu, David, Costa, David, Cox, Christopher J., Creamean, Jessie, Crewell, Susanne, Dahlke, Sandro, Damm, Ellen, de Boer, Gijs, Deckelmann, Holger, Dethloff, Klaus, Dütsch, Marina, Ebell, Kerstin, Ehrlich, André, Ellis, Jody, Engelmann, Ronny, Fong, Allison A., Frey, Markus M., Gallagher, Michael R., Ganzeveld, Laurens, Gradinger, Rolf, Graeser, Jürgen, Greenamyer, Vernon, Griesche, Hannes, Griffiths, Steele, Hamilton, Jonathan, Heinemann, Günther, Helmig, Detlev, Herber, Andreas, Heuzé, Céline, Hofer, Julian, Houchens, Todd, Howard, Dean, Inoue, Jun, Jacobi, Hans-Werner, Jaiser, Ralf, Jokinen, Tuija, Jourdan, Olivier, Jozef, Gina, King, Wessley, Kirchgaessner, Amelie, Klingebiel, Marcus, Krassovski, Misha, Krumpen, Thomas, Lampert, Astrid, Landing, William, Laurila, Tiia, Lawrence, Dale, Lonardi, Michael, Loose, Brice, Lüpkes, Christof, Maahn, Maximilian, Macke, Andreas, Maslowski, Wieslaw, Marsay, Christopher, Maturilli, Marion, Mech, Mario, Morris, Sara, Moser, Manuel, Nicolaus, Marcel, Ortega, Paul, Osborn, Jackson, Pätzold, Falk, Perovich, Donald K., Petäjä, Tuukka, Pilz, Christian, Pirazzini, Roberta, Posman, Kevin, Powers, Heath, Pratt, Kerri A., Preußer, Andreas, Quéléver, Lauriane, Radenz, Martin, Rabe, Benjamin, Rinke, Annette, Sachs, Torsten, Schulz, Alexander, Siebert, Holger, Silva, Tercio, Solomon, Amy, Sommerfeld, Anja, Spreen, Gunnar, Stephens, Mark, Stohl, Andreas, Svensson, Gunilla, Uin, Janek, Viegas, Juarez, Voigt, Christiane, von der Gathen, Peter, Wehner, Birgit, Welker, Jeffrey M., Wendisch, Manfred, Werner, Martin, Xie, ZhouQing, Yue, Fange, Shupe, Matthew D., Rex, Markus, Blomquist, Byron, Persson, P. Ola G., Schmale, Julia, Uttal, Taneil, Althausen, Dietrich, Angot, Hélène, Archer, Stephen, Bariteau, Ludovic, Beck, Ivo, Bilberry, John, Bucci, Silvia, Buck, Clifton, Boyer, Matt, Brasseur, Zoé, Brooks, Ian M., Calmer, Radiance, Cassano, John, Castro, Vagner, Chu, David, Costa, David, Cox, Christopher J., Creamean, Jessie, Crewell, Susanne, Dahlke, Sandro, Damm, Ellen, de Boer, Gijs, Deckelmann, Holger, Dethloff, Klaus, Dütsch, Marina, Ebell, Kerstin, Ehrlich, André, Ellis, Jody, Engelmann, Ronny, Fong, Allison A., Frey, Markus M., Gallagher, Michael R., Ganzeveld, Laurens, Gradinger, Rolf, Graeser, Jürgen, Greenamyer, Vernon, Griesche, Hannes, Griffiths, Steele, Hamilton, Jonathan, Heinemann, Günther, Helmig, Detlev, Herber, Andreas, Heuzé, Céline, Hofer, Julian, Houchens, Todd, Howard, Dean, Inoue, Jun, Jacobi, Hans-Werner, Jaiser, Ralf, Jokinen, Tuija, Jourdan, Olivier, Jozef, Gina, King, Wessley, Kirchgaessner, Amelie, Klingebiel, Marcus, Krassovski, Misha, Krumpen, Thomas, Lampert, Astrid, Landing, William, Laurila, Tiia, Lawrence, Dale, Lonardi, Michael, Loose, Brice, Lüpkes, Christof, Maahn, Maximilian, Macke, Andreas, Maslowski, Wieslaw, Marsay, Christopher, Maturilli, Marion, Mech, Mario, Morris, Sara, Moser, Manuel, Nicolaus, Marcel, Ortega, Paul, Osborn, Jackson, Pätzold, Falk, Perovich, Donald K., Petäjä, Tuukka, Pilz, Christian, Pirazzini, Roberta, Posman, Kevin, Powers, Heath, Pratt, Kerri A., Preußer, Andreas, Quéléver, Lauriane, Radenz, Martin, Rabe, Benjamin, Rinke, Annette, Sachs, Torsten, Schulz, Alexander, Siebert, Holger, Silva, Tercio, Solomon, Amy, Sommerfeld, Anja, Spreen, Gunnar, Stephens, Mark, Stohl, Andreas, Svensson, Gunilla, Uin, Janek, Viegas, Juarez, Voigt, Christiane, von der Gathen, Peter, Wehner, Birgit, Welker, Jeffrey M., Wendisch, Manfred, Werner, Martin, Xie, ZhouQing, and Yue, Fange

Abstract

With the Arctic rapidly changing, the needs to observe, understand, and model the changes are essential. To support these needs, an annual cycle of observations of atmospheric properties, processes, and interactions were made while drifting with the sea ice across the central Arctic during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition from October 2019 to September 2020. An international team designed and implemented the comprehensive program to document and characterize all aspects of the Arctic atmospheric system in unprecedented detail, using a variety of approaches, and across multiple scales. These measurements were coordinated with other observational teams to explore cross-cutting and coupled interactions with the Arctic Ocean, sea ice, and ecosystem through a variety of physical and biogeochemical processes. This overview outlines the breadth and complexity of the atmospheric research program, which was organized into 4 subgroups: atmospheric state, clouds and precipitation, gases and aerosols, and energy budgets. Atmospheric variability over the annual cycle revealed important influences from a persistent large-scale winter circulation pattern, leading to some storms with pressure and winds that were outside the interquartile range of past conditions suggested by long-term reanalysis. Similarly, the MOSAiC location was warmer and wetter in summer than the reanalysis climatology, in part due to its close proximity to the sea ice edge. The comprehensiveness of the observational program for characterizing and analyzing atmospheric phenomena is demonstrated via a winter case study examining air mass transitions and a summer case study examining vertical atmospheric evolution. Overall, the MOSAiC atmospheric program successfully met its objectives and was the most comprehensive atmospheric measurement program to date conducted over the Arctic sea ice. The obtained data will support a broad range of coupled-system

Published
2022

28. Measurement report: Introduction to the HyICE-2018 campaign for measurements of ice-nucleating particles and instrument inter-comparison in the Hyytiälä boreal forest

Author

Brasseur, Zoé, primary, Castarède, Dimitri, additional, Thomson, Erik S., additional, Adams, Michael P., additional, Drossaart van Dusseldorp, Saskia, additional, Heikkilä, Paavo, additional, Korhonen, Kimmo, additional, Lampilahti, Janne, additional, Paramonov, Mikhail, additional, Schneider, Julia, additional, Vogel, Franziska, additional, Wu, Yusheng, additional, Abbatt, Jonathan P. D., additional, Atanasova, Nina S., additional, Bamford, Dennis H., additional, Bertozzi, Barbara, additional, Boyer, Matthew, additional, Brus, David, additional, Daily, Martin I., additional, Fösig, Romy, additional, Gute, Ellen, additional, Harrison, Alexander D., additional, Hietala, Paula, additional, Höhler, Kristina, additional, Kanji, Zamin A., additional, Keskinen, Jorma, additional, Lacher, Larissa, additional, Lampimäki, Markus, additional, Levula, Janne, additional, Manninen, Antti, additional, Nadolny, Jens, additional, Peltola, Maija, additional, Porter, Grace C. E., additional, Poutanen, Pyry, additional, Proske, Ulrike, additional, Schorr, Tobias, additional, Silas Umo, Nsikanabasi, additional, Stenszky, János, additional, Virtanen, Annele, additional, Moisseev, Dmitri, additional, Kulmala, Markku, additional, Murray, Benjamin J., additional, Petäjä, Tuukka, additional, Möhler, Ottmar, additional, and Duplissy, Jonathan, additional

Published
2022
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29. Overview of the MOSAiC expedition: Atmosphere

Author

Shupe, Matthew, Rex, Markus, Blomquist, Byron, Ola, P, Persson, G, Schmale, Julia, Uttal, Taneil, Althausen, Dietrich, Lè Ne Angot, Hé, Archer, Stephen, Bariteau, Ludovic, Beck, Ivo, Bilberry, John, Bucci, Silvia, Buck, Clifton, Boyer, Matt, Brasseur, Zoé, Brooks, Ian, Cassano, John, Castro, Vagner, Chu, David, Costa, David, Cox, Christopher, Creamean, Jessie, Crewell, Susanne, Dahlke, Sandro, Damm, Ellen, de Boer, Gijs, Deckelmann, Holger, Dethloff, Klaus, Dütsch, Marina, Ebell, Kerstin, Ehrlich, André, Ellis, Jody, Engelmann, Ronny, Fong, Allison, Frey, Markus, Gallagher, Michael, Ganzeveld, Laurens, Gradinger, Rolf, Graeser, Jürgen, Greenamyer, Vernon, Griesche, Hannes, Griffiths, Steele, Hamilton, Jonathan, Heinemann, Günther, Helmig, Detlev, Herber, Andreas, Line Heuzé, Cé, Hofer, Julian, Houchens, Todd, Inoue, Jun, Jacobi, Hans-Werner, Jaiser, Ralf, Jokinen, Tuija, Jourdan, Olivier, King, Wessley, Kirchgaessner, Amelie, Klingebiel, Marcus, Krassovski, Misha, Krumpen, Thomas, Lampert, Astrid, Landing, William, Laurila, Tiia, Lawrence, Dale, Lonardi, Michael, Loose, Brice, Lüpkes, Christof, Maahn, Maximilian, Macke, Andreas, Maslowski, Wieslaw, Marsay, Christopher, Maturilli, Marion, Mech, Mario, Morris, Sara, Moser, Manuel, Nicolaus, Marcel, Ortega, Paul, Osborn, Jackson, Pätzold, Falk, Perovich, Donald, Petäjä, Tuukka, Pilz, Christian, Pirazzini, Roberta, Posman, Kevin, Powers, Heath, Pratt, Kerri, Preusser, Andreas, Qué Lé Ver, Lauriane, Radenz, Martin, Rabe, Benjamin, Rinke, Annette, Sachs, Torsten, Schulz, Alexander, Siebert, Holger, Silva, Tercio, Solomon, Amy, Sommerfeld, Anja, Spreen, Gunnar, Stephens, Mark, Stohl, Andreas, Svensson, Gunilla, Uin, Janek, Viegas, Juarez, Voigt, Christiane, von Der Gathen, Peter, Wehner, Birgit, Welker, Jeffrey, Wendisch, Manfred, Werner, Martin, Xie, Zhouqing, Yue, Fange, Jourdan, Olivier, Laboratoire de Météorologie Physique (LaMP), and Institut national des sciences de l'Univers (INSU - CNRS)-Université Clermont Auvergne [2017-2020] (UCA [2017-2020])-Centre National de la Recherche Scientifique (CNRS)

Subjects
[SDU.OCEAN]Sciences of the Universe [physics]/Ocean, Atmosphere, Arctic, Field campaign, Atmosphere, [SDU.OCEAN] Sciences of the Universe [physics]/Ocean, Atmosphere
Abstract

International audience; With the Arctic rapidly changing, the needs to observe, understand, and model the changes are essential. To support these needs, an annual cycle of observations of atmospheric properties, processes, and interactions were made while drifting with the sea ice across the central Arctic during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition from October 2019 to September 2020. An international team designed and implemented the comprehensive program to document and characterize all aspects of the Arctic atmospheric system in unprecedented detail, using a variety of approaches, and across multiple scales. These measurements were coordinated with other observational teams to explore crosscutting and coupled interactions with the Arctic Ocean, sea ice, and ecosystem through a variety of physical and biogeochemical processes. This overview outlines the breadth and complexity of the atmospheric research program, which was organized into 4 subgroups: atmospheric state, clouds and precipitation, gases and aerosols, and energy budgets. Atmospheric variability over the annual cycle revealed important influences from a persistent large-scale winter circulation pattern, leading to some storms with pressure and winds that were outside the interquartile range of past conditions suggested by long-term reanalysis. Similarly, the MOSAiC location was warmer and wetter in summer than the reanalysis climatology, in part due to its close proximity to the sea ice edge.The comprehensiveness of the observational program for characterizing and analyzing atmospheric phenomena is demonstrated via a winter case study examining air mass transitions and a summer case study examining vertical atmospheric evolution. Overall, the MOSAiC atmospheric program successfully met its objectives and was the most comprehensive atmospheric measurement program to date conducted over the Arctic sea ice. The obtained data will support a broad range of coupled-system scientific research and provide an important foundation for advancing multiscale modeling capabilities in the Arctic.

Published
2022

30. Measurement of the rate coefficients between atmospheric ions and multiply charged aerosol particles in the CERN CLOUD chamber.

Author

Pfeifer, Joschka, Mahfouz, Naser G. A., Schulze, Benjamin C., Mathot, Serge, Stolzenburg, Dominik, Baalbaki, Rima, Brasseur, Zoé, Caudillo, Lucia, Dada, Lubna, Granzin, Manuel, Xu-Cheng He, Lamkaddam, Houssni, Lopez, Brandon, Makhmutov, Vladimir, Marten, Ruby, Mentler, Bernhard, Müller, Tatjana, Onnela, Antti, Philippov, Maxim, and Piedehierro, Ana A.

Abstract

Aerosol particles have an important role in Earth's radiation balance and climate, both directly and indirectly through aerosol-cloud interactions. Most aerosol particles in the atmosphere are weakly charged, affecting both their collision rates with ions and neutral molecules, as well as the rates by which they are scavenged by other aerosol particles and cloud droplets. The rate coefficients between ions and aerosol particles are important since they determine the growth rates and lifetimes of ions and charged aerosol particles, and so may influence cloud dynamics and aerosol processing. However, despite their importance, very few experimental measurements exist of charged aerosol collision rates under atmospheric conditions, where galactic cosmic rays in the lower troposphere give rise to ion pair concentrations of around 1000 cm-3. Here we present measurements in the CERN CLOUD chamber of the rate coefficients between ions and small (<10 nm) aerosol particles containing up to 9 elementary charges, e. We find the rate coefficient of a singly charged ion with an oppositely charged particle increases from 2.0 (0.4-4.4) x 10-6 cm³ s-1 to 30.6 (24.9-45.1) x 10-6 cm³s-1 for particles with charges of 1 e to 9 e, respectively, where the parentheses indicate the ±1σ uncertainty interval. Our measurements are compatible with theoretical predictions and show excellent agreement with the model of Gatti and Kortshagen (2008). [ABSTRACT FROM AUTHOR]

Published
2022
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31. Chemical composition of nanoparticles from &lt;i&gt;α&lt;/i&gt;-pinene nucleation and the influence of isoprene and relative humidity at low temperature

Author

Caudillo, Lucía, primary, Rörup, Birte, additional, Heinritzi, Martin, additional, Marie, Guillaume, additional, Simon, Mario, additional, Wagner, Andrea C., additional, Müller, Tatjana, additional, Granzin, Manuel, additional, Amorim, Antonio, additional, Ataei, Farnoush, additional, Baalbaki, Rima, additional, Bertozzi, Barbara, additional, Brasseur, Zoé, additional, Chiu, Randall, additional, Chu, Biwu, additional, Dada, Lubna, additional, Duplissy, Jonathan, additional, Finkenzeller, Henning, additional, Gonzalez Carracedo, Loïc, additional, He, Xu-Cheng, additional, Hofbauer, Victoria, additional, Kong, Weimeng, additional, Lamkaddam, Houssni, additional, Lee, Chuan P., additional, Lopez, Brandon, additional, Mahfouz, Naser G. A., additional, Makhmutov, Vladimir, additional, Manninen, Hanna E., additional, Marten, Ruby, additional, Massabò, Dario, additional, Mauldin, Roy L., additional, Mentler, Bernhard, additional, Molteni, Ugo, additional, Onnela, Antti, additional, Pfeifer, Joschka, additional, Philippov, Maxim, additional, Piedehierro, Ana A., additional, Schervish, Meredith, additional, Scholz, Wiebke, additional, Schulze, Benjamin, additional, Shen, Jiali, additional, Stolzenburg, Dominik, additional, Stozhkov, Yuri, additional, Surdu, Mihnea, additional, Tauber, Christian, additional, Tham, Yee Jun, additional, Tian, Ping, additional, Tomé, António, additional, Vogt, Steffen, additional, Wang, Mingyi, additional, Wang, Dongyu S., additional, Weber, Stefan K., additional, Welti, André, additional, Yonghong, Wang, additional, Yusheng, Wu, additional, Zauner-Wieczorek, Marcel, additional, Baltensperger, Urs, additional, El Haddad, Imad, additional, Flagan, Richard C., additional, Hansel, Armin, additional, Höhler, Kristina, additional, Kirkby, Jasper, additional, Kulmala, Markku, additional, Lehtipalo, Katrianne, additional, Möhler, Ottmar, additional, Saathoff, Harald, additional, Volkamer, Rainer, additional, Winkler, Paul M., additional, Donahue, Neil M., additional, Kürten, Andreas, additional, and Curtius, Joachim, additional

Published
2021
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32. Measurement report: Introduction to the HyICE-2018 campaign for measurements of ice nucleating particles in the Hyytiälä boreal forest

Author

Brasseur, Zoé, primary, Castarède, Dimitri, additional, Thomson, Erik S., additional, Adams, Michael P., additional, Drossaart van Dusseldorp, Saskia, additional, Heikkilä, Paavo, additional, Korhonen, Kimmo, additional, Lampilahti, Janne, additional, Paramonov, Mikhail, additional, Schneider, Julia, additional, Vogel, Franziska, additional, Wu, Yusheng, additional, Abbat, Jonathan P. D., additional, Atanasova, Nina S., additional, Bamford, Dennis H., additional, Bertozzi, Barbara, additional, Boyer, Matthew, additional, Brus, David, additional, Daily, Martin I., additional, Fösig, Romy, additional, Gute, Ellen, additional, Harrison, Alexander D., additional, Hietala, Paula, additional, Höhler, Kristina, additional, Kanji, Zamin A., additional, Keskinen, Jorma, additional, Lacher, Larissa, additional, Lampimäki, Markus, additional, Levula, Janne, additional, Manninen, Antti, additional, Nadolny, Jens, additional, Peltola, Maija, additional, Porter, Grace C. E., additional, Poutanen, Pyry, additional, Proske, Ulrike, additional, Schorr, Tobias, additional, Silas Umo, Nsikanabasi, additional, Stenszky, János, additional, Virtanen, Annele, additional, Moisseev, Dmitri, additional, Kulmala, Markku, additional, Murray, Benjamin J., additional, Petäjä, Tuukka, additional, Möhler, Ottmar, additional, and Duplissy, Jonathan, additional

Published
2021
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33. Chemical composition of nanoparticles from α-pinene nucleation and the influence of isoprene and relative humidity at low temperature

Author

Caudillo, Lucía, Rörup, Birte, Heinritzi, Martin, Marie, Guillaume, Simon, Mario, Wagner, Andrea C., Müller, Tatjana, Granzin, Manuel, Amorim, Antonio, Ataei, Farnoush, Baalbaki, Rima, Bertozzi, Barbara, Brasseur, Zoé, Chiu, Randall, Chu, Biwu, Dada, Lubna, Duplissy, Jonathan, Finkenzeller, Henning, Gonzalez Carracedo, Loïc, He, Xu-Cheng, Hofbauer, Victoria, Kong, Weimeng, Lamkaddam, Houssni, Lee, Chuan P., Lopez, Brandon, Mahfouz, Naser G. A., Makhmutov, Vladimir, Manninen, Hanna E., Marten, Ruby, Massabò, Dario, Mauldin, Roy L., Mentler, Bernhard, Molteni, Ugo, Onnela, Antti, Pfeifer, Joschka, Philippov, Maxim, Piedehierro, Ana A., Schervish, Meredith, Scholz, Wiebke, Schulze, Benjamin, Shen, Jiali, Stolzenburg, Dominik, Stozhkov, Yuri, Surdu, Mihnea, Tauber, Christian, Tham, Yee Jun, Tian, Ping, Tomé, António, Vogt, Steffen, Wang, Mingyi, Wang, Dongyu S., Weber, Stefan K., Welti, André, Yonghong, Wang, Yusheng, Wu, Zauner-Wieczorek, Marcel, Baltensperger, Urs, El Haddad, Imad, Flagan, Richard C., Hansel, Armin, Höhler, Kristina, Kirkby, Jasper, Kulmala, Markku, Lehtipalo, Katrianne, Möhler, Ottmar, Saathoff, Harald, Volkamer, Rainer, Winkler, Paul M., Donahue, Neil M., Kürten, Andreas, and Curtius, Joachim

Subjects
Atmospheric Science
Abstract

The abstract is available here: https://uscholar.univie.ac.at/o:1597268

Published
2021

35. Supplementary material to &quot;Chemical composition of nanoparticles from α-pinene nucleation and the influence of isoprene and relative humidity at low temperature&quot;

Author

Caudillo, Lucía, primary, Rörup, Birte, additional, Heinritzi, Martin, additional, Marie, Guillaume, additional, Simon, Mario, additional, Wagner, Andrea C., additional, Müller, Tatjana, additional, Granzin, Manuel, additional, Amorim, Antonio, additional, Ataei, Farnoush, additional, Baalbaki, Rima, additional, Bertozzi, Barbara, additional, Brasseur, Zoé, additional, Chiu, Randall, additional, Chu, Biwu, additional, Dada, Lubna, additional, Duplissy, Jonathan, additional, Finkenzeller, Henning, additional, Gonzalez Carracedo, Loïc, additional, He, Xu-Cheng, additional, Hofbauer, Victoria, additional, Kong, Weimeng, additional, Lamkaddam, Houssni, additional, Lee, Chuan P., additional, Lopez, Brandon, additional, Mahfouz, Naser G. A., additional, Makhmutov, Vladimir, additional, Manninen, Hanna E., additional, Marten, Ruby, additional, Massabò, Dario, additional, Mauldin, Roy L., additional, Mentler, Bernhard, additional, Molteni, Ugo, additional, Onnela, Antti, additional, Pfeifer, Joschka, additional, Philippov, Maxim, additional, Piedehierro, Ana A., additional, Schervish, Meredith, additional, Scholz, Wiebke, additional, Schulze, Benjamin, additional, Shen, Jiali, additional, Stolzenburg, Dominik, additional, Stozhkov, Yuri, additional, Surdu, Mihnea, additional, Tauber, Christian, additional, Tham, Yee Jun, additional, Tian, Ping, additional, Tomé, António, additional, Vogt, Steffen, additional, Wang, Mingyi, additional, Wang, Dongyu S., additional, Weber, Stefan K., additional, Welti, André, additional, Yonghong, Wang, additional, Yusheng, Wu, additional, Zauner-Wieczorek, Marcel, additional, Baltensperger, Urs, additional, El Haddad, Imad, additional, Flagan, Richard C., additional, Hansel, Armin, additional, Höhler, Kristina, additional, Kirkby, Jasper, additional, Kulmala, Markku, additional, Lehtipalo, Katrianne, additional, Möhler, Ottmar, additional, Saathoff, Harald, additional, Volkamer, Rainer, additional, Winkler, Paul M., additional, Donahue, Neil M., additional, Kürten, Andreas, additional, and Curtius, Joachim, additional

Published
2021
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36. Chemical composition of nanoparticles from α-pinene nucleation and the influence of isoprene and relative humidity at low temperature

Author

Caudillo, Lucía, primary, Rörup, Birte, additional, Heinritzi, Martin, additional, Marie, Guillaume, additional, Simon, Mario, additional, Wagner, Andrea C., additional, Müller, Tatjana, additional, Granzin, Manuel, additional, Amorim, Antonio, additional, Ataei, Farnoush, additional, Baalbaki, Rima, additional, Bertozzi, Barbara, additional, Brasseur, Zoé, additional, Chiu, Randall, additional, Chu, Biwu, additional, Dada, Lubna, additional, Duplissy, Jonathan, additional, Finkenzeller, Henning, additional, Gonzalez Carracedo, Loïc, additional, He, Xu-Cheng, additional, Hofbauer, Victoria, additional, Kong, Weimeng, additional, Lamkaddam, Houssni, additional, Lee, Chuan P., additional, Lopez, Brandon, additional, Mahfouz, Naser G. A., additional, Makhmutov, Vladimir, additional, Manninen, Hanna E., additional, Marten, Ruby, additional, Massabò, Dario, additional, Mauldin, Roy L., additional, Mentler, Bernhard, additional, Molteni, Ugo, additional, Onnela, Antti, additional, Pfeifer, Joschka, additional, Philippov, Maxim, additional, Piedehierro, Ana A., additional, Schervish, Meredith, additional, Scholz, Wiebke, additional, Schulze, Benjamin, additional, Shen, Jiali, additional, Stolzenburg, Dominik, additional, Stozhkov, Yuri, additional, Surdu, Mihnea, additional, Tauber, Christian, additional, Tham, Yee Jun, additional, Tian, Ping, additional, Tomé, António, additional, Vogt, Steffen, additional, Wang, Mingyi, additional, Wang, Dongyu S., additional, Weber, Stefan K., additional, Welti, André, additional, Yonghong, Wang, additional, Yusheng, Wu, additional, Zauner-Wieczorek, Marcel, additional, Baltensperger, Urs, additional, El Haddad, Imad, additional, Flagan, Richard C., additional, Hansel, Armin, additional, Höhler, Kristina, additional, Kirkby, Jasper, additional, Kulmala, Markku, additional, Lehtipalo, Katrianne, additional, Möhler, Ottmar, additional, Saathoff, Harald, additional, Volkamer, Rainer, additional, Winkler, Paul M., additional, Donahue, Neil M., additional, Kürten, Andreas, additional, and Curtius, Joachim, additional

Published
2021
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37. The seasonal cycle of ice-nucleating particles linked to the abundance of biogenic aerosol in boreal forests

Author

Schneider, Julia, primary, Höhler, Kristina, additional, Heikkilä, Paavo, additional, Keskinen, Jorma, additional, Bertozzi, Barbara, additional, Bogert, Pia, additional, Schorr, Tobias, additional, Umo, Nsikanabasi Silas, additional, Vogel, Franziska, additional, Brasseur, Zoé, additional, Wu, Yusheng, additional, Hakala, Simo, additional, Duplissy, Jonathan, additional, Moisseev, Dmitri, additional, Kulmala, Markku, additional, Adams, Michael P., additional, Murray, Benjamin J., additional, Korhonen, Kimmo, additional, Hao, Liqing, additional, Thomson, Erik S., additional, Castarède, Dimitri, additional, Leisner, Thomas, additional, Petäjä, Tuukka, additional, and Möhler, Ottmar, additional

Published
2021
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39. A full year of aerosol size distribution data from the central Arctic under an extreme positive Arctic Oscillation: Insights from the MOSAiC expedition.

Author

Boyer, Matthew, Aliaga, Diego, Pernov, Jakob Boyd, Angot, Hélène, Quéléver, Lauriane L. J., Dada, Lubna, Heutte, Benjamin, Dall'Osto, Manuel, Beddows, David C. S., Brasseur, Zoé, Beck, Ivo, Bucci, Silvia, Duetsch, Marina, Stohl, Andreas, Laurila, Tiia, Asmi, Eija, Massling, Andreas, Thomas, Daniel Charles, Nøjgaard, Jakob Klenø, and Tak Chan

Abstract

The Arctic environment is rapidly changing due to accelerated warming in the region. The warming trend is driving a decline in sea ice extent, which thereby enhances feedback loops in the surface energy budget in the Arctic. Arctic aerosols play an important role in the radiative balance, and hence the climate response, in the region; yet direct observations of aerosols over the Arctic Ocean are limited. In this study, we investigate the annual cycle in the aerosol particle number size distribution (PNSD), particle number concentration (PNC), and black carbon (BC) mass concentration in the central Arctic during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition. This is the first continuous, year-long dataset of aerosol PNSD ever collected over the sea ice in the central Arctic Ocean. We use a k-means cluster analysis, FLEXPART simulations, and inverse modeling to evaluate seasonal patterns and the influence of different source regions on the Arctic aerosol population. Furthermore, we compare the aerosol observations to land-based sites across the Arctic, using both long-term measurements and observations during the year of the MOSAiC expedition (2019 - 2020), to investigate interannual variability and to give context to the aerosol characteristics from within the central Arctic. Our analysis identifies that, overall, the central Arctic exhibits typical seasonal patterns of aerosols, including anthropogenic influence from Arctic Haze in winter and secondary aerosol processes in summer. The seasonal pattern corresponds with the global radiation, surface air temperature, and the timing of sea ice melting/freezing, which drives changes in transport patterns and secondary aerosol processes. In winter, the Norilsk region in Russia/Siberia was the dominant source of Arctic Haze signal in the PNSD and BC observations, which contributed to higher accumulation mode PNC and BC mass concentration in the central Arctic than at land-based observatories. We also show that the wintertime Arctic Oscillation (AO) phenomenon, which was reported to achieve a record-breaking positive phase during January - March 2020, explains the unusual timing and magnitude of Arctic Haze across the Arctic region compared to longer-term observations. In summer, the PNC of nucleation and Aitken mode aerosol is enhanced, but concentrations were notably lower in the central Arctic over the ice pack than at land-based sites further south. The analysis presented herein provides a current snapshot of Arctic aerosol processes in an environment that is characterized by rapid changes, which will be crucial for improving climate model predictions, understanding linkages between different environmental processes, and investigating the impacts of climate change in future Arctic aerosol studies. [ABSTRACT FROM AUTHOR]

Published
2022
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40. An intercomparison study of four different techniques for measuring the chemical composition of nanoparticles.

Author

Caudillo, Lucía, Surdu, Mihnea, Lopez, Brandon, Mingyi Wang, Thoma, Markus, Bräkling, Steffen, Buchholz, Angela, Simon, Mario, Wagner, Andrea C., Müller, Tatjana, Granzin, Manuel, Heinritzi, Martin, Amorim, Antonio, Bell, David M., Brasseur, Zoé, Dada, Lubna, Duplissy, Jonathan, Finkenzeller, Henning, Xu-Cheng He, and Lamkaddam, Houssni

Abstract

Currently, the complete chemical characterization of nanoparticles (<100 nm) represents an analytical challenge, since these particles are abundant in number but have negligible mass. Several methods for particle-phase characterization have been recently developed to better detect and infer more accurately the sources and fates of ultra-fine particles, but a detailed comparison of different approaches is missing. Here we report on the chemical composition of secondary organic aerosol (SOA) nanoparticles from experimental studies of α-pinene ozonolysis at -50 ºC, -30 ºC, and -10 ºC, and inter-compare the results measured by different techniques. The experiments were performed at the Cosmics Leaving OUtdoor Droplets (CLOUD) chamber at the European Organization for Nuclear Research (CERN). The chemical composition was measured simultaneously by four different techniques: 1) Thermal Desorption-Differential Mobility Analyzer (TD-DMA) coupled to a NO3 - chemical ionization-atmospheric-pressure-interface-time-of-flight (CI-APi-TOF) mass spectrometer, 2) Filter Inlet for Gases and AEROsols (FIGAERO) coupled to an I- high-resolution time-of-flight chemical-ionization mass spectrometer (HRToF-CIMS), 3) Extractive Electrospray Na+ Ionization time-of-flight mass spectrometer (EESI-TOF), and 4) Offline analysis of filters (FILTER) using Ultra-high-performance liquid chromatography (UHPLC) and heated electrospray ionization (HESI) coupled to an Orbitrap high-resolution mass spectrometer (HRMS). Intercomparison was performed by contrasting the observed chemical composition as a function of oxidation state and carbon number, by calculating the volatility and comparing the fraction of volatility classes, and by comparing the thermal desorption behavior (for the thermal desorption techniques: TD-DMA and FIGAERO) and performing positive matrix factorization (PMF) analysis for the thermograms. We found that the methods generally agree on the most important compounds that are found in the nanoparticles. However, they do see different parts of the organic spectrum. We suggest potential explanations for these differences: thermal decomposition, aging, sampling artifacts, etc. We applied PMF analysis and found insights of thermal decomposition in the TD-DMA and the FIGAERO. [ABSTRACT FROM AUTHOR]

Published
2022
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42. The seasonal cycle of ice-nucleating particles linked to the abundance of biogenic aerosol in boreal forests

Author

Schneider, Julia, primary, Höhler, Kristina, additional, Heikkilä, Paavo, additional, Keskinen, Jorma, additional, Bertozzi, Barbara, additional, Bogert, Pia, additional, Schorr, Tobias, additional, Umo, Nsikanabasi Silas, additional, Vogel, Franziska, additional, Brasseur, Zoé, additional, Wu, Yusheng, additional, Hakala, Simo, additional, Duplissy, Jonathan, additional, Moisseev, Dmitri, additional, Kulmala, Markku, additional, Adams, Michael P., additional, Murray, Benjamin J., additional, Korhonen, Kimmo, additional, Hao, Liqing, additional, Thomson, Erik S., additional, Castarède, Dimitri, additional, Leisner, Thomas, additional, Petäjä, Tuukka, additional, and Möhler, Ottmar, additional

Published
2020
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43. The seasonal cycle of biogenic ice-nucleating particles in a boreal forest environment

Author

Schneider, Julia, primary, Höhler, Kristina, additional, Heikkilä, Paavo, additional, Keskinen, Jorma, additional, Bertozzi, Barbara, additional, Schorr, Tobias, additional, Umo, Nsikanabasi, additional, Vogel, Franziska, additional, Brasseur, Zoé, additional, Wu, Yusheng, additional, Hakala, Simo, additional, Duplissy, Jonathan, additional, Petäjä, Tuukka, additional, Adams, Michael P., additional, Murray, Benjamin J., additional, Korhonen, Kimmo, additional, Thomson, Erik S., additional, Castarède, Dimitri, additional, Leisner, Thomas, additional, and Möhler, Ottmar, additional

Published
2020
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44. Synergistic HNO3–H2SO4–NH3 upper tropospheric particle formation.

Author

Wang, Mingyi, Xiao, Mao, Bertozzi, Barbara, Marie, Guillaume, Rörup, Birte, Schulze, Benjamin, Bardakov, Roman, He, Xu-Cheng, Shen, Jiali, Scholz, Wiebke, Marten, Ruby, Dada, Lubna, Baalbaki, Rima, Lopez, Brandon, Lamkaddam, Houssni, Manninen, Hanna E., Amorim, António, Ataei, Farnoush, Bogert, Pia, and Brasseur, Zoé

Abstract

New particle formation in the upper free troposphere is a major global source of cloud condensation nuclei (CCN)1–4. However, the precursor vapours that drive the process are not well understood. With experiments performed under upper tropospheric conditions in the CERN CLOUD chamber, we show that nitric acid, sulfuric acid and ammonia form particles synergistically, at rates that are orders of magnitude faster than those from any two of the three components. The importance of this mechanism depends on the availability of ammonia, which was previously thought to be efficiently scavenged by cloud droplets during convection. However, surprisingly high concentrations of ammonia and ammonium nitrate have recently been observed in the upper troposphere over the Asian monsoon region5,6. Once particles have formed, co-condensation of ammonia and abundant nitric acid alone is sufficient to drive rapid growth to CCN sizes with only trace sulfate. Moreover, our measurements show that these CCN are also highly efficient ice nucleating particles—comparable to desert dust. Our model simulations confirm that ammonia is efficiently convected aloft during the Asian monsoon, driving rapid, multi-acid HNO3–H2SO4–NH3 nucleation in the upper troposphere and producing ice nucleating particles that spread across the mid-latitude Northern Hemisphere.By performing experiments under upper tropospheric conditions, nitric acid, sulfuric acid and ammonia can form particles synergistically, at rates orders of magnitude faster than any two of the three components. [ABSTRACT FROM AUTHOR]

Published
2022
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45. Measurement report: Introduction to the HyICE-2018 campaign for measurements of ice nucleating particles in the Hyytiälä boreal forest.

Author

Brasseur, Zoé, Castarède, Dimitri, Thomson, Erik S., Adams, Michael P., van Dusseldorp, Saskia Drossaart, Heikkilä, Paavo, Korhonen, Kimmo, Lampilahti, Janne, Paramonov, Mikhail, Schneider, Julia, Vogel, Franziska, Wu, Yusheng, Abbatt, Jonathan P. D., Atanasova, Nina S., Bamford, Dennis H., Bertozzi, Barbara, Boyer, Matthew, Brus, David, Daily, Martin I., and Fösig, Romy

Abstract

The formation of ice particles in Earth's atmosphere strongly influences the dynamics and optical properties of clouds and their impacts on the climate system. Ice formation in clouds is often triggered heterogeneously by ice nucleating particles (INPs) that represent a very low number of particles in the atmosphere. To date, many sources of INPs, such as mineral and soil dust, have been investigated and identified in the lower latitudes. Although less is known about the sources of ice nucleation at higher latitudes, efforts have been made to identify the sources of INPs in the Arctic and boreal environments. In this study, we investigate the INP emission potential from high latitude boreal forests. We introduce the HyICE-2018 measurement campaign conducted in the boreal forest of Hyytiälä, Finland between February and June 2018. The campaign utilized the infrastructure of the SMEAR II research station with additional instrumentation for measuring INPs to quantify the concentrations and sources of INPs in the boreal environment. In this contribution, we describe the measurement infrastructure and operating procedures during HyICE-2018 and we report results from specific time periods where INP instruments were run in parallel for inter-comparison purposes. Our results show that the suite of instruments deployed during HyICE-2018 reports consistent results and therefore lays the foundation for forthcoming results to be considered holistically. In addition, we compare the INP concentration we measured to INP parameterizations, and we show a very good agreement with the Tobo et al. (2013) parameterization developed from measurements conducted in a ponderosa pine forest ecosystem in Colorado, USA. [ABSTRACT FROM AUTHOR]

Published
2021
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46. Synergistic HNO3–H2SO4–NH3upper tropospheric particle formation

Author

Wang, Mingyi, Xiao, Mao, Bertozzi, Barbara, Marie, Guillaume, Rörup, Birte, Schulze, Benjamin, Bardakov, Roman, He, Xu-Cheng, Shen, Jiali, Scholz, Wiebke, Marten, Ruby, Dada, Lubna, Baalbaki, Rima, Lopez, Brandon, Lamkaddam, Houssni, Manninen, Hanna E., Amorim, António, Ataei, Farnoush, Bogert, Pia, Brasseur, Zoé, Caudillo, Lucía, De Menezes, Louis-Philippe, Duplissy, Jonathan, Ekman, Annica M. L., Finkenzeller, Henning, Carracedo, Loïc Gonzalez, Granzin, Manuel, Guida, Roberto, Heinritzi, Martin, Hofbauer, Victoria, Höhler, Kristina, Korhonen, Kimmo, Krechmer, Jordan E., Kürten, Andreas, Lehtipalo, Katrianne, Mahfouz, Naser G. A., Makhmutov, Vladimir, Massabò, Dario, Mathot, Serge, Mauldin, Roy L., Mentler, Bernhard, Müller, Tatjana, Onnela, Antti, Petäjä, Tuukka, Philippov, Maxim, Piedehierro, Ana A., Pozzer, Andrea, Ranjithkumar, Ananth, Schervish, Meredith, Schobesberger, Siegfried, Simon, Mario, Stozhkov, Yuri, Tomé, António, Umo, Nsikanabasi Silas, Vogel, Franziska, Wagner, Robert, Wang, Dongyu S., Weber, Stefan K., Welti, André, Wu, Yusheng, Zauner-Wieczorek, Marcel, Sipilä, Mikko, Winkler, Paul M., Hansel, Armin, Baltensperger, Urs, Kulmala, Markku, Flagan, Richard C., Curtius, Joachim, Riipinen, Ilona, Gordon, Hamish, Lelieveld, Jos, El-Haddad, Imad, Volkamer, Rainer, Worsnop, Douglas R., Christoudias, Theodoros, Kirkby, Jasper, Möhler, Ottmar, and Donahue, Neil M.

Abstract

New particle formation in the upper free troposphere is a major global source of cloud condensation nuclei (CCN)1–4. However, the precursor vapours that drive the process are not well understood. With experiments performed under upper tropospheric conditions in the CERN CLOUD chamber, we show that nitric acid, sulfuric acid and ammonia form particles synergistically, at rates that are orders of magnitude faster than those from any two of the three components. The importance of this mechanism depends on the availability of ammonia, which was previously thought to be efficiently scavenged by cloud droplets during convection. However, surprisingly high concentrations of ammonia and ammonium nitrate have recently been observed in the upper troposphere over the Asian monsoon region5,6. Once particles have formed, co-condensation of ammonia and abundant nitric acid alone is sufficient to drive rapid growth to CCN sizes with only trace sulfate. Moreover, our measurements show that these CCN are also highly efficient ice nucleating particles—comparable to desert dust. Our model simulations confirm that ammonia is efficiently convected aloft during the Asian monsoon, driving rapid, multi-acid HNO3–H2SO4–NH3nucleation in the upper troposphere and producing ice nucleating particles that spread across the mid-latitude Northern Hemisphere.

Published
2022
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47. Interactions between the atmosphere, cryosphere, and ecosystems at northern high latitudes

Author

Barcelona Supercomputing Center, Boy, Michael, Thomson, Erik S., Acosta-Navarro, Juan C., Arnalds, Olafur, Batchvarova, Ekaterina, Bäck, Jaana, Berninger, Frank, Bilde, Merete, Brasseur, Zoé, Dagsson-Waldhauserova, Pavla, Castarède, Dimitri, Dalirian, Maryam, de Leeuw, Guerrit, Dragosics, Monika, Duplissy, Ella-Maria, Ekman, Annica M.L., Fang, Keyan, Gallet, Jean-Charles, Glasius, Marianne, Gryning, Sven-Erik, Grythe, Henrik, Hansson, Hans-Christen, Hansson, Margareta, Isaksson, Elisabeth, Iversen, Trond, Jonsdottir, Ingibjorg, Kasurinen, Ville, Kirkevag, Alf, Korhola, Atte, Krejci, Radovan, Kristjansson, Jon E., Lappalainen, Hanna K., Lauri, Antti, Lepparanta, Matti, Lihavainen, Heikki, Makkonen, Risto, Massling, Andreas, Meinander, Outi, Nilsson, E. Douglas, Olafsson, Haraldur, Pettersson, Jan B.C., Prisle, Nonne L., Riipinen, Ilona, Roldin, Pontus, Ruppel, Meri, Salter, Matthew, Sand, Maria, Seland, Oyvind, Seppa, Heikki, Skov, Henrik, Soares, Joana, Stohl, Andreas, Ström, Johan, Svensson, Jonas, Swieticki, Erik, Tabakova, Ksenia, Thorsteinsson, Throstur, Virkkula, Aki, Weyhenmeyer, Gesa A., Wu, Yesheng, Zieger, Paul, Kulmala, Markku, Barcelona Supercomputing Center, Boy, Michael, Thomson, Erik S., Acosta-Navarro, Juan C., Arnalds, Olafur, Batchvarova, Ekaterina, Bäck, Jaana, Berninger, Frank, Bilde, Merete, Brasseur, Zoé, Dagsson-Waldhauserova, Pavla, Castarède, Dimitri, Dalirian, Maryam, de Leeuw, Guerrit, Dragosics, Monika, Duplissy, Ella-Maria, Ekman, Annica M.L., Fang, Keyan, Gallet, Jean-Charles, Glasius, Marianne, Gryning, Sven-Erik, Grythe, Henrik, Hansson, Hans-Christen, Hansson, Margareta, Isaksson, Elisabeth, Iversen, Trond, Jonsdottir, Ingibjorg, Kasurinen, Ville, Kirkevag, Alf, Korhola, Atte, Krejci, Radovan, Kristjansson, Jon E., Lappalainen, Hanna K., Lauri, Antti, Lepparanta, Matti, Lihavainen, Heikki, Makkonen, Risto, Massling, Andreas, Meinander, Outi, Nilsson, E. Douglas, Olafsson, Haraldur, Pettersson, Jan B.C., Prisle, Nonne L., Riipinen, Ilona, Roldin, Pontus, Ruppel, Meri, Salter, Matthew, Sand, Maria, Seland, Oyvind, Seppa, Heikki, Skov, Henrik, Soares, Joana, Stohl, Andreas, Ström, Johan, Svensson, Jonas, Swieticki, Erik, Tabakova, Ksenia, Thorsteinsson, Throstur, Virkkula, Aki, Weyhenmeyer, Gesa A., Wu, Yesheng, Zieger, Paul, and Kulmala, Markku

Abstract

The Nordic Centre of Excellence CRAICC (Cryosphere–Atmosphere Interactions in a Changing Arctic Climate), funded by NordForsk in the years 2011–2016, is the largest joint Nordic research and innovation initiative to date, aiming to strengthen research and innovation regarding climate change issues in the Nordic region. CRAICC gathered more than 100 scientists from all Nordic countries in a virtual centre with the objectives of identifying and quantifying the major processes controlling Arctic warming and related feedback mechanisms, outlining strategies to mitigate Arctic warming, and developing Nordic Earth system modelling with a focus on short-lived climate forcers (SLCFs), including natural and anthropogenic aerosols. The outcome of CRAICC is reflected in more than 150 peer-reviewed scientific publications, most of which are in the CRAICC special issue of the journal Atmospheric Chemistry and Physics. This paper presents an overview of the main scientific topics investigated in the centre and provides the reader with a state-of-the-art comprehensive summary of what has been achieved in CRAICC with links to the particular publications for further detail. Faced with a vast amount of scientific discovery, we do not claim to completely summarize the results from CRAICC within this paper, but rather concentrate here on the main results which are related to feedback loops in climate change–cryosphere interactions that affect Arctic amplification., The CRAICC team acknowledges the following institutions for financial support: the Finnish Cultural Foundation grant, Markku Kulmala “International Working Groups”; Russian mega-grant no. 11.G34.31.0048 (University of Nizhny Novgorod); Academy of Finland contracts 259537, 257411, and 254195; Beautiful Beijing (Finland–China collaboration project) funded by TEKES; Nordforsk CRAICC-PEEX (amendment to contract 26060); CRAICC-CRUCIAL (project no. 81257); Icelandic Research Fund (Rannis) grant no. 152248- 051; Danish Environmental Protection Agency with means from the Dancea fund for environmental support to the Arctic region (M 112 002700); the Villum Foundation; the Carlsberg Foundation (project 009_1_0515); COST1303 (TOPROF); COST ES1404 (HarmoSnow); and the Pan-Eurasian Experiment (PEEX). The development and use of NorESM1 was supported by the Norwegian Research Council through the projects Earth-Clim (207711/E10), EVA (grant no. 229771), NOTUR (nn2345k), and NorStore (ns2345k) and through the Nordic Centre of Excellence eSTICC (57001) and the EU H2020 project CRESCENDO (grant no. 641816). The CRAICC team also thanks Rogier Floors for providing Fig. 8 and Christoph Münkel for Fig. 9. The authors and entire CRAICC community would like to thank and acknowledge the work and inspiration of Jon Egill Kristjansson, whose life was cut short during these collaborations. Jon Egill Kristjansson is deeply missed, but his scientific legacy continues., Peer Reviewed, Postprint (published version)

Published
2019

48. Interactions between the atmosphere, cryosphere, and ecosystems at northern high latitudes

Author

Boy, Michael, primary, Thomson, Erik S., additional, Acosta Navarro, Juan-C., additional, Arnalds, Olafur, additional, Batchvarova, Ekaterina, additional, Bäck, Jaana, additional, Berninger, Frank, additional, Bilde, Merete, additional, Brasseur, Zoé, additional, Dagsson-Waldhauserova, Pavla, additional, Castarède, Dimitri, additional, Dalirian, Maryam, additional, de Leeuw, Gerrit, additional, Dragosics, Monika, additional, Duplissy, Ella-Maria, additional, Duplissy, Jonathan, additional, Ekman, Annica M. L., additional, Fang, Keyan, additional, Gallet, Jean-Charles, additional, Glasius, Marianne, additional, Gryning, Sven-Erik, additional, Grythe, Henrik, additional, Hansson, Hans-Christen, additional, Hansson, Margareta, additional, Isaksson, Elisabeth, additional, Iversen, Trond, additional, Jonsdottir, Ingibjorg, additional, Kasurinen, Ville, additional, Kirkevåg, Alf, additional, Korhola, Atte, additional, Krejci, Radovan, additional, Kristjansson, Jon Egill, additional, Lappalainen, Hanna K., additional, Lauri, Antti, additional, Leppäranta, Matti, additional, Lihavainen, Heikki, additional, Makkonen, Risto, additional, Massling, Andreas, additional, Meinander, Outi, additional, Nilsson, E. Douglas, additional, Olafsson, Haraldur, additional, Pettersson, Jan B. C., additional, Prisle, Nønne L., additional, Riipinen, Ilona, additional, Roldin, Pontus, additional, Ruppel, Meri, additional, Salter, Matthew, additional, Sand, Maria, additional, Seland, Øyvind, additional, Seppä, Heikki, additional, Skov, Henrik, additional, Soares, Joana, additional, Stohl, Andreas, additional, Ström, Johan, additional, Svensson, Jonas, additional, Swietlicki, Erik, additional, Tabakova, Ksenia, additional, Thorsteinsson, Throstur, additional, Virkkula, Aki, additional, Weyhenmeyer, Gesa A., additional, Wu, Yusheng, additional, Zieger, Paul, additional, and Kulmala, Markku, additional

Published
2019
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49. The seasonal cycle of ice-nucleating particles linked to the abundance of biogenic aerosol in boreal forests.

Author

Schneider, Julia, Höhler, Kristina, Heikkilä, Paavo, Keskinen, Jorma, Bertozzi, Barbara, Bogert, Pia, Schorr, Tobias, Umo, Nsikanabasi Silas, Vogel, Franziska, Brasseur, Zoé, Wu, Yusheng, Hakala, Simo, Duplissy, Jonathan, Moisseev, Dmitri, Kulmala, Markku, Adams, Michael P., Murray, Benjamin J., Korhonen, Kimmo, Hao, Liqing, and Thomson, Erik S.

Abstract

Ice-nucleating particles (INPs) trigger the formation of cloud ice crystals in the atmosphere. Therefore, they strongly influence cloud microphysical and optical properties, as well as precipitation and the life cycle of clouds. Improving weather forecasting and climate projection requires an appropriate formulation of atmospheric INP concentrations. This remains challenging, as the global INP distribution and variability depend on a variety of aerosol types and sources, and neither their short-term variability nor their long-term seasonal cycles are well covered by continuous measurements. Here, we provide the first year-long set of observations with a pronounced INP seasonal cycle in a boreal forest environment. Besides the observed seasonal cycle in INP concentrations with a minimum in wintertime and maxima in early and late summer, we also provide indications for a seasonal variation in the prevalent INP type. We show that the seasonal dependency of INP concentrations and prevalent INP types is most likely driven by the abundance of biogenic aerosol. As current parameterizations do not reproduce this variability, we suggest a new parameterization approach, which considers the seasonal variation of INP concentrations. For this, we use the ambient air temperature as a proxy for the season which affects the source strength of biogenic emissions and by that the INP abundance over the boreal forest areas. Furthermore, we provide new INP parameterizations based on the Ice Nucleation Active Surface Site (INAS) approach, which specifically describes the ice nucleation activity of boreal aerosols particles prevalent in different seasons. Our results characterize the boreal forest as an important but variable INP source and provide new perspectives to describe these new findings in atmospheric models. [ABSTRACT FROM AUTHOR]

Published
2020
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50. The seasonal cycle of ice-nucleating particles linked to the abundance of biogenic aerosol in boreal forests

Author

Schneider, Julia, Höhler, Kristina, Heikkilä, Paavo, Keskinen, Jorma, Bertozzi, Barbara, Bogert, Pia, Schorr, Tobias, Umo, Nsikanabasi Silas, Vogel, Franziska, Brasseur, Zoé, Wu, Yusheng, Hakala, Simo, Duplissy, Jonathan, Moisseev, Dmitri, Kulmala, Markku, Adams, Michael P., Murray, Benjamin J., Korhonen, Kimmo, Hao, Liqing, Thomson, Erik S., Castarède, Dimitri, Leisner, Thomas, Petäjä, Tuukka, and Möhler, Ottmar

Subjects
Ice nucleating particles, 13. Climate action, 15. Life on land, Field experiment

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