Search

We present an analysis method to search for exotic low-mass field (ELF) bursts generated during large energy astrophysical events such as supernovae, binary black hole or binary neutron star mergers, and fast radio bursts using the Global Network of Optical Magnetometers for Exotic physics searches (GNOME). In our model, the associated gravitational waves or electromagnetic signals herald the arrival of the ELF burst that interacts via coupling to the spin of fermions in the magnetometers. This enables GNOME to serve as a tool for multi-messenger astronomy. The algorithm employs a model-agnostic excess-power method to identify network-wide candidate events to be subjected to a model-dependent generalized likelihood-ratio test to determine their statistical significance. We perform the first search with this technique on GNOME data coincident with the binary black hole merger S200311bg detected by LIGO/Virgo on the 11th of March 2020 and find no significant events. We place the first lab-based limits on combinations of ELF production and coupling parameters.

Anti-quark nuggets (AQNs) have been suggested to solve the dark matter (DM) and the missing antimatter problem in the universe and have been proposed as an explanation of various observations. Their size is in the {\mu}m range and their density is about equal to the nuclear density with an expected flux of about $0.4 / km^2 / year$. For the typical velocity of DM constituents ($\sim$250 km/s), the solar system bodies act as highly performing gravitational lenses. Here we assume that DM streams or clusters are impinging, e.g., on the Earth, as it was worked out for DM axions and Weakly Interacting Massive Particles (WIMPs). Interestingly, in the LHC beam, unforeseen beam losses are triggered by so-called Unidentified Falling Objects (UFOs), which are believed to be constituted of dust particles with a size in the {\mu}m range and a density of several orders of magnitude lower than AQNs. Prezeau suggested that streaming DM constituents incident on the Earth should result in jet-like structures ("hairs") exiting the Earth, or a kind of caustics. Such ideas open novel directions in the search for DM. This work suggests a new analysis of the UFO results at the Large Hadron Collider (LHC), assuming that they are eventually, at least partly, due to AQNs. Firstly, a reanalysis of the existing data from the 4000 beam monitors since the beginning of the LHC is proposed, arguing that dust and AQNs should behave differently. The feasibility of this idea has been discussed with CERN accelerator people and potential collaborators., Comment: 4 pages

The $^{229}$Th nucleus has a long-lived isomeric state $A^*$ at 8.338(24) eV [Kraemer et al, Nature, \textbf{617}, 706 (2023)]. This state is connected to the ground state by an M1 transition. For a hydrogenlike Th ion in the $1s$ state the hyperfine structure splitting is about 0.7 eV. This means that the hyperfine interaction can mix the nuclear ground state with the isomeric state with a mixing coefficient $\beta$ about 0.03. If the electron is suddenly removed from this system, the nucleus will be left in the mixed state. The probability to find the nucleus in the isomeric state $A^*$ is equal to $\beta^2\sim 10^{-3}$. For the $2s$ state the effect is roughly two orders of magnitude smaller. An atom with a hole in the $1s$ or $2s$ shell is similar to the hydrogenlike atom, only the hole has a short lifetime $\tau$. After the hole is filled, there is a non-zero probability to find the nucleus in the $A^*$ state. Estimates of this probability are presented along with a discussion of possible experiments on Th-doped xenotime-type orthophosphate crystals and other broad band gap materials., Comment: 6 pages, 1 figure. V.2: Sec. IV and references added

Numerous observations suggest that there exist undiscovered beyond-the-Standard-Model particles and fields. Because of their unknown nature, these exotic particles and fields could interact with Standard Model particles in many different ways and assume a variety of possible configurations. Here we present an overview of the Global Network of Optical Magnetometers for Exotic physics searches (GNOME), our ongoing experimental program designed to test a wide range of exotic physics scenarios. The GNOME experiment utilizes a worldwide network of shielded atomic magnetometers (and, more recently, comagnetometers) to search for spatially and temporally correlated signals due to torques on atomic spins from exotic fields of astrophysical origin. We survey the temporal characteristics of a variety of possible signals currently under investigation such as those from topological defect dark matter (axion-like particle domain walls), axion-like particle stars, solitons of complex-valued scalar fields (Q-balls), stochastic fluctuations of bosonic dark matter fields, a solar axion-like particle halo, and bursts of ultralight bosonic fields produced by cataclysmic astrophysical events such as binary black hole mergers., Comment: 22 pages, 12 figures, submitted to Annalen der Physik

Scalar-field dark matter models imply small oscillations of fundamental constants. These oscillations could result in observable variations of the magnetic field in a permanent magnet. We propose an experiment for detection of this type of dark matter through searches of oscillations of magnetic field of permanent magnets with a SQUID magnetometer or a low-noise radiofrequency amplifier. We show that this experiment may have comparable sensitivity to leading experiments searching for variations of fundamental constants in the range of frequencies from a few Hz to about 1 MHz. We also discuss applicability of the approach of variations of fundamental constants for accounting for the interaction with scalar dark matter., Comment: 9 pages, 1 figure

Axions are well-motivated dark matter candidates with simple cosmological production mechanisms. They were originally introduced to solve the strong CP problem, but also arise in a wide range of extensions to the Standard Model. This Snowmass white paper summarizes axion phenomenology and outlines next-generation laboratory experiments proposed to detect axion dark matter. There are vibrant synergies with astrophysical searches and advances in instrumentation including quantum-enabled readout, high-Q resonators and cavities and large high-field magnets. This white paper outlines a clear roadmap to discovery, and shows that the US is well-positioned to be at the forefront of the search for axion dark matter in the coming decade., Comment: restore and expand author list

The last decade has seen unprecedented effort in dark matter model building at all mass scales coupled with the design of numerous new detection strategies. Transformative advances in quantum technologies have led to a plethora of new high-precision quantum sensors and dark matter detection strategies for ultralight ($<10\,$eV) bosonic dark matter that can be described by an oscillating classical, largely coherent field. This white paper focuses on searches for wavelike scalar and vector dark matter candidates., Comment: Snowmass 2021 White Paper

A possible implication of an ultralight dark matter (UDM) field interacting wibeginth the Standard Model (SM) degrees of freedom is oscillations of fundamental constants. Here, we establish direct experimental bounds on the coupling of an oscillating UDM field to the up, down, and strange quarks and to the gluons, for oscillation frequencies between 10 Hz and 10^8 Hz. We employ spectroscopic experiments that take advantage of the dependence of molecular transition frequencies on the nuclear masses. Our results apply to previously unexplored frequency bands, and improve on existing bounds at frequencies > 5 MHz. We identify a sector of UDM - SM coupling space where the bounds from Equivalence Principle tests may be challenged by next-generation experiments of the present kind., Comment: 23 pages,9 figures

We report measurements of isotope shifts for the five spinless Yb isotopes on the $6s^2\,^1\textrm{S}_0 \rightarrow 5d6s\,^1\textrm{D}_2$ transition using Doppler-free two-photon spectroscopy. We combine these data with existing measurements on two transitions in Yb$^+$ [Phys. Rev. Lett. 125, 123002 (2020)], where deviation from King-plot linearity showed hints of a new bosonic force carrier at the 3$\sigma$ level. The combined data strongly reduces the significance of the new-physics signal. We show that the observed nonlinearity in the joint Yb/Yb$^+$ King-plot analysis can be accounted for by the deformation of the Yb nuclei., Comment: Minor changes

We discuss how molecule-based searches offer complementary probes to study the violation of fundamental symmetries. These experiments have the potential to probe not only the electron EDM, but also hadronic CPV phenomena. Future experimental developments will offer generic sensitivity to probe flavor neutral sources of both leptonic and hadronic CPV at scales of $\geq$ 100 TeV, and flavor changing CPV at scales of $\geq$ 1000 TeV.

This article is the second in a pair of articles on the topic of the generation of a two-color artificial star (which we term a "laser photometric ratio star," or LPRS) of de-excitation light from neutral sodium atoms in the mesosphere, for use in precision telescopic measurements in astronomy and atmospheric physics, and more specifically for the calibration of measurements of dark energy using type Ia supernovae. The two techniques respectively described in both this and the previous article would each generate an LPRS with a precisely 1:1 ratio of yellow (589/590 nm) photons to near-infrared (819/820 nm) photons produced in the mesosphere. Both techniques would provide novel mechanisms for establishing a spectrophotometric calibration ratio of unprecedented precision, from above most of Earth's atmosphere, for upcoming telescopic observations across astronomy and atmospheric physics. The technique described in this article has the advantage of producing a much brighter (specifically, brighter by approximately a factor of 1000) LPRS, using lower-power (<30 W average power) lasers, than the technique using a single 500 W average power laser described in the first article of this pair. However, the technique described here would require polarization filters to be installed into the telescope camera in order to sufficiently remove laser atmospheric Rayleigh backscatter from telescope images, whereas the technique described in the first article would only require more typical wavelength filters in order to sufficiently remove laser Rayleigh backscatter., Comment: The first article in this pair of articles is at arXiv:2001.10958 . This article has 15 pages and 3 figures. Both articles are published in MNRAS

Astrophysical observations indicate that there is roughly five times more dark matter in the Universe than ordinary baryonic matter, with an even larger amount of the Universe's energy content due to dark energy. So far, the microscopic properties of these dark components have remained shrouded in mystery. In addition, even the five percent of ordinary matter in our Universe has yet to be understood, since the Standard Model of particle physics lacks any consistent explanation for the predominance of matter over antimatter. Inspired by these central problems of modern physics, we present here a direct search for interactions of antimatter with dark matter, and place direct constraints on the interaction of ultra-light axion-like particles $-$ one of the dark-matter candidates $-$ and antiprotons. If antiprotons exhibit a stronger coupling to these dark-matter particles than protons, such a CPT-odd coupling could provide a link between dark matter and the baryon asymmetry in the Universe. We analyse spin-flip resonance data acquired with a single antiproton in a Penning trap [Smorra et al., Nature 550, 371 (2017)] in the frequency domain to search for spin-precession effects from ultra-light axions with a characteristic frequency governed by the mass of the underlying particle. Our analysis constrains the axion-antiproton interaction parameter $f_a/C_{\overline{p}}$ to values greater than $0.1$ to $0.6$ GeV in the mass range from $2 \times 10^{-23}$ to $4 \times 10^{-17}\,$eV/$c^2$, improving over astrophysical antiproton bounds by up to five orders of magnitude. In addition, we derive limits on six combinations of previously unconstrained Lorentz-violating and CPT-violating terms of the non-minimal Standard Model Extension., Comment: 26 pages, 7 figures, including supplementary information

Nitrogen-vacancy (NV) centers in diamond have shown promise as inherently localized electric-field sensors, capable of detecting individual charges with nanometer resolution. Working with NV ensembles, we demonstrate that a detailed understanding of the internal electric field environment enables enhanced sensitivity in the detection of external electric fields. We follow this logic along two complementary paths. First, using excitation tuned near the NV's zero-phonon line, we perform optically detected magnetic resonance (ODMR) spectroscopy at cryogenic temperatures in order to precisely measure the NV center's excited-state susceptibility to electric fields. In doing so, we demonstrate that the characteristically observed contrast inversion arises from an interplay between spin-selective optical pumping and the NV centers' local charge distribution. Second, motivated by this understanding, we propose and analyze a novel scheme for optically-enhanced electric-field sensing using NV ensembles; we estimate that our approach should enable order of magnitude improvements in the DC electric-field sensitivity., Comment: 6+10 pages, 3+6 figures

The largest uncertainty on measurements of dark energy using type Ia supernovae is presently due to systematics from photometry; specifically to the relative uncertainty on photometry as a function of wavelength in the optical spectrum. We show that a precise constraint on relative photometry between the visible and near-infrared can be achieved in upcoming surveys (such as in LSST at the Vera C. Rubin Observatory) via a mountaintop-located laser source tuned to the 342.78 nm vacuum excitation wavelength of neutral sodium atoms. Using a high-power (500 W) laser modified from laser guide star studies, this excitation will produce an artificial star (which we term a "laser photometric ratio star," or LPRS) of de-excitation light in the mesosphere that is observable from the ground at approximately 20 magnitude (i.e., well within the expected single-image magnitude limit of LSST) at wavelengths in vacuum of 589.16 nm, 589.76 nm, 818.55 nm, and 819.70 nm, with the sum of the numbers of 589.16 nm and 589.76 nm photons produced by this process equal to the sum of the numbers of 818.55 nm and 819.70 nm photons, establishing a precise calibration ratio between, for example, the LSST r and z filters. This technique can thus provide a novel mechanism for establishing a spectrophotometric calibration ratio of unprecedented precision, from above most of the Earth's atmosphere, for upcoming telescopic observations across astronomy and atmospheric physics. This article is the first in a pair of articles on this topic. The second article of the pair describes an alternative technique to achieve a similar, but brighter, LPRS than the technique described in this paper, by using two mountaintop-located lasers, at optical frequencies approximately 4 GHz away from resonances at wavelengths in vacuum of 589.16 nm and 819.71 nm respectively., Comment: The second article in this pair of articles is at arXiv:2010.08683 . This article has 14 pages & 7 figures. Both articles are published in MNRAS. This most recent arXiv version fixes a minor error in the caption of Figure 4

We numerically study a method to increase the photon return flux of continuous-wave laser guide stars using one-dimensional atomic cooling principles. The method relies on chirping the laser towards higher frequencies following the change in velocity of sodium atoms due to recoil, which raises atomic populations available for laser excitation within the Doppler distribution. The efficiency of this effect grows with the average number of atomic excitations between two atomic collisions in the mesosphere. We find the parameters for maximizing the return flux and evaluate the performance of chirping for operation at La Palma. According to our simulations, the optimal chirp rate lies between 0.8-1.0 MHz/$\mu$s and an increase in the fluorescence of the sodium guide star up to 60% can be achieved with current 20 W-class guide star lasers.

Nuclear spin ensembles in diamond are promising candidates for quantum sensing applications, including rotation sensing. Here we perform a characterization of the optically detected nuclear-spin transitions associated with the 14N nuclear spin within diamond nitrogen vacancy (NV) centers. We observe nuclear-spin-dependent fluorescence with the contrast of optically detected 14N nuclear Rabi oscillations comparable to that of the NV electron spin. Using Ramsey spectroscopy, we investigate the temperature and magnetic-field dependence of the nuclear spin transitions in the 77.5-420 K and 350-675 G range, respectively. The nuclear quadrupole coupling constant Q was found to vary with temperature T yielding d|Q|/dT=-35.0(2) Hz/K at T=297 K. The temperature and magnetic field dependencies reported here are important for quantum sensing applications such as rotation sensing and potentially for applications in quantum information processing., Comment: Main text: 6 pages, 4 figures. Supplemental Information: 3 pages, 3 figures

The interaction of standard model's particles with the axionic Dark Matter field may generate oscillating nuclear electric dipole moments (EDMs), oscillating nuclear Schiff moments and oscillating nuclear magnetic quadrupole moments (MQMs) with a frequency corresponding to the axion's Compton frequency. Within an atom or a molecule an oscillating EDM, Schiff moment or MQM can drive transitions between atomic or molecular states. The excitation events can be detected, for example, via subsequent fluorescence or photoionization. Here we calculate the rates of such transitions. If the nucleus has octupole deformation or quadrupole deformation then the transition rate due to Schiff moment and MQM can be up to $10^{-16}$ transition per molecule per year. In addition, an MQM-induced transition may be of M2-type, which is useful for the elimination of background noise since M2-type transitions are suppressed for photons., Comment: 10 pages

We report on studies of simultaneous continuous-wave mirrorless lasing on multiple optical transitions, realized by pumping hot cesium vapor with laser light resonant with the 6$S_{1/2}\rightarrow 8$P$_{3/2}$ transition. The multiplicity of decay paths for the excited atoms to their ground state is responsible for the emergence of lasing in a number of transitions, observed here in at least seven wavelengths in the infrared (IR), and at two wavelengths in the blue. We study the properties of the fields generated in the cesium vapor, such as optical power, directionality and optical linewidth., Comment: 5 pages, 4 figures

Among the prominent candidates for dark matter are bosonic fields with small scalar couplings to the Standard-Model particles. Several techniques are employed to search for such couplings and the current best constraints are derived from tests of gravity or atomic probes. In experiments employing atoms, observables would arise from expected dark-matter-induced oscillations in the fundamental constants of nature. These studies are primarily sensitive to underlying particle masses below $10^{-14}$ eV. We present a method to search for fast oscillations of fundamental constants using atomic spectroscopy in cesium vapor. We demonstrate sensitivity to scalar interactions of dark matter associated with a particle mass in the range $8\cdot10^{-11}$ to $4\cdot 10^{-7}$ eV. In this range our experiment yields constraints on such interactions, which within the framework of an astronomical-size dark matter structure, are comparable with, or better than, those provided by experiments probing deviations from the law of gravity., Comment: 8 pages, 7 figures

We discuss the possibility of creating novel research tools by producing and storing highly relativistic beams of highly ionised atoms in the CERN accelerator complex, and by exciting their atomic degrees of freedom with lasers to produce high-energy photon beams. Intensity of such photon beams would be by several orders of magnitude higher than offered by the presently operating light sources, in the particularly interesting gamma-ray energy domain of 0.1-400 MeV. In this energy range, the high-intensity photon beams can be used to produce secondary beams of polarised electrons, polarised positrons, polarised muons, neutrinos, neutrons and radioactive ions. New research opportunities in a wide domain of fundamental and applied physics can be opened by the Gamma Factory scientific programme based on the above primary and secondary beams., Comment: 12 pages; presented by W. Placzek at the XXV Cracow Epiphany Conference on Advances in Heavy Ion Physics, 8-11 January 2019, Cracow, Poland

We present a detailed description of experimental studies of the parity violation effect in an isotopic chain of atomic ytterbium (Yb), whose results were reported in a recent Letter [Antypas et al., Nat. Phys. 15, 120 (2019)]. We discuss the principle of these measurements, made on the Yb 6s$^2$ $^1$S$_0 \rightarrow $5d6s $^3$D$_1$ optical transition at 408 nm, describe the experimental apparatus, and give a detailed account of our studies of systematic effects in the experiment. Our results offer the first direct observation of the isotopic variation in the atomic parity violation effect, a variation which is in agreement with the prediction of the Standard Model. These measurements are used to constrain electron-proton and electron-neutron interactions, mediated by a light $Z'$ boson., Comment: 24 pages, 17 figures, 5 tables

We estimate the relative contribution of nuclear structure and new physics couplings to the parity non-conserving spin-independent effects in atomic systems, for both single isotopes and isotopic ratios. General expressions are presented to assess the sensitivity of isotopic ratios to neutron skins and to couplings beyond standard model at tree level. The specific coefficients for these contributions are calculated assuming Fermi distribution for proton and neutron nuclear densities for isotopes of Cs, Ba, Sm, Dy, Yb, Pb, Fr, and Ra. The present work aims to provide a guide to the choice of the best isotopes and pairs of isotopes for conducting atomic PNC measurements., Comment: 11 pages, 2 figures, 3 tables

We present a technique for generating light in an arbitrary polarization state. The technique is based on interference of two orthogonally polarized light beams, whose amplitudes and phases are controlled with a Mach-Zehnder inteferometer with acousto-optic modulators (AOMs) placed in each arm. We demonstrate that via control over amplitudes, phases, and frequencies of acoustic waves driving the AOMs, any polarization state can be synthesized. In particular, we demonstrate generation of linearly polarized light, whose polarization plane continuously rotates at a rate from 1~kHz to 1~MHz. Such light finds applications in science (e.g., investigations of Bloch-Siegert effect) and technology (optically-pumped magnetometers).

The Global Network of Optical Magnetometers to search for Exotic physics (GNOME) is a network of geographically separated, time-synchronized, optically pumped atomic magnetometers that is being used to search for correlated transient signals heralding exotic physics. The GNOME is sensitive to nuclear- and electron-spin couplings to exotic fields from astrophysical sources such as compact dark-matter objects (for example, axion stars and domain walls). Properties of the GNOME sensors such as sensitivity, bandwidth, and noise characteristics are studied in the present work, and features of the network's operation (e.g., data acquisition, format, storage, and diagnostics) are described. Characterization of the GNOME is a key prerequisite to searches for and identification of exotic physics signatures., Comment: 45 pages, 16 figures, 2 tables

Atoms and molecules can serve as sensitive probes of a possible variation of the fine structure constant $\alpha$ and electron-to-proton mass ratio $\mu$. Two types of sensitivity coefficients are often used to quantify and compare the sensitivity of different species to the variation of fundamental constants. The dimensionless coefficients $K$ are related to the fractional sensitivity, while dimensional factors $q$ are related to the absolute sensitivity. Here we discuss several common errors and misconceptions regarding these coefficients that frequently appear in the literature., Comment: 3 pages

In certain laboratory experiments the production and/or detection of axions is due to the photon-axion transformations in a strong magnetic field. This process is coherent, and the rate of the transformation is proportional to the length $l$ and magnitude $B$ of the magnetic field squared, $\sim l^2B^2$. In the present paper, we consider coherent production of axions due to the forward scattering of photons on atoms or molecules. This process may be represented as being due to an effective electromagnetic field which converts photons to axions. We present analytical expressions for such effective magnetic and electric fields induced by resonant atomic M0 and M1 transitions, as well as give some numerical estimates for these fields. The corresponding experiments would allow one to measure the electron-axion coupling constant $g_{ae}$ in the same way as the photon-axion coupling $g_{a\gamma}$ is studied., Comment: 6 pages

We report on measurements of atomic parity violation, made on a chain of ytterbium isotopes with mass numbers A=170, 172, 174, and 176. In the experiment, we optically excite the 6s2 1S0 -> 5d6s 3D1 transition in a region of crossed electric and magnetic fields, and observe the interference between the Stark- and weak-interaction-induced transition amplitudes, by making field reversals that change the handedness of the coordinate system. This allows us to determine the ratio of the weak-interaction-induced electric-dipole (E1) transition moment and the Stark-induced E1 moment. Our measurements, which are at the 0.5% level of accuracy for three of the four isotopes measured, allow a definitive observation of the isotopic variation of the weak-interaction effects in an atom, which is found to be consistent with the prediction of the Standard Model. In addition, our measurements provide information about an additional Z' boson., Comment: 19 pages, 4 figures, 2 tables

Detection schemes for the quantum chromodynamics axions and other axion-like particles in light-shining-through-a-wall (LSW) experiments are based on the conversion of these particles into photons in a magnetic field. An alternative scheme may involve the detection via a resonant atomic or molecular transition induced by resonant axion absorption. The signal obtained in this process is second order in the axion-electron interaction constant but may become first order if we allow interference between the axion-induced transition amplitude and the transition amplitude induced by the electromagnetic radiation that produces the axions., Comment: 12 pages, 4 figures, 3 tables

Understanding the effect of vibrations on the relaxation process of individual spins is crucial for implementing nano systems for quantum information and quantum metrology applications. In this work, we present a theoretical microscopic model to describe the spin-lattice relaxation of individual electronic spins associated to negatively charged nitrogen-vacancy centers in diamond, although our results can be extended to other spin-boson systems. Starting from a general spin-lattice interaction Hamiltonian, we provide a detailed description and solution of the quantum master equation of an electronic spin-one system coupled to a phononic bath in thermal equilibrium. Special attention is given to the dynamics of one-phonon processes below 1 K where our results agree with recent experimental findings and analytically describe the temperature and magnetic-field scaling. At higher temperatures, linear and second-order terms in the interaction Hamiltonian are considered and the temperature scaling is discussed for acoustic and quasi-localized phonons when appropriate. Our results, in addition to confirming a $T^5$ temperature dependence of the longitudinal relaxation rate at higher temperatures, in agreement with experimental observations, provide a theoretical background for modeling the spin-lattice relaxation at a wide range of temperatures where different temperature scalings might be expected.

An overview of our experimental program to search for axion and axion-like-particle (ALP) dark matter using nuclear magnetic resonance (NMR) techniques is presented. An oscillating axion field can exert a time-varying torque on nuclear spins either directly or via generation of an oscillating nuclear electric dipole moment (EDM). Magnetic resonance techniques can be used to detect such an effect. The first-stage experiments explore many decades of ALP parameter space beyond the current astrophysical and laboratory bounds. It is anticipated that future versions of the experiments will be sensitive to the axions associated with quantum chromodynamics (QCD) having masses $\lesssim 10^{-9}~{\rm eV}/c^2$., Comment: 9 pages, 4 figures

Light (pseudo-)scalar fields are promising candidates to be the dark matter in the Universe. Under certain initial conditions in the early Universe and/or with certain types of self-interactions, they can form compact dark-matter objects such as axion stars or Q-balls. Direct encounters with such objects can be searched for by using a global network of atomic magnetometers. It is shown that for a range of masses and radii not ruled out by existing observations, the terrestrial encounter rate with axion stars or Q-balls can be sufficiently high (at least once per year) for a detection. Furthermore, it is shown that a global network of atomic magnetometers is sufficiently sensitive to pseudoscalar couplings to atomic spins so that a transit through an axion star or Q-ball could be detected over a broad range of unexplored parameter space., Comment: 8 pages, 3 figures

This article reviews recent developments in tests of fundamental physics using atoms and molecules, including the subjects of parity violation, searches for permanent electric dipole moments, tests of the CPT theorem and Lorentz symmetry, searches for spatiotemporal variation of fundamental constants, tests of quantum electrodynamics, tests of general relativity and the equivalence principle, searches for dark matter, dark energy and extra forces, and tests of the spin-statistics theorem. Key results are presented in the context of potential new physics and in the broader context of similar investigations in other fields. Ongoing and future experiments of the next decade are discussed., Comment: 121 pages, 24 figures. This version fixes Figs. 16 and 18

Ensembles of nitrogen-vacancy (NV) centers in diamond are widely used as AC magnetometers. While such measurements are usually performed using standard (XY) dynamical decoupling (DD) protocols at room temperature, we study the sensitivities achieved by utilizing various DD protocols, for measuring magnetic AC fields at frequencies in the 10-250 kHz range, at room temperature and 77 K. By performing measurements on an isotopically pure $^{12}$C sample, we find that the Carr-Purcell-Meiboom-Gill (CPMG) protocol, which is not robust against pulse imperfections, is less efficient for magnetometry than robust XY-based sequences. The concatenation of a standard XY-based protocol may enhance the sensitivities only for measuring high-frequency fields, for which many ($> 500$) DD pulses are necessary and the robustness against pulse imperfections is critical. Moreover, we show that cooling is effective only for measuring low-frequency fields (~10 kHz), for which the experiment time apporaches $T_1$ at a small number of applied DD pulses.

The magnetic signature of an urban environment is investigated using a geographically distributed network of fluxgate magnetometers deployed in and around Berkeley, California. The system hardware and software are described and results from initial operation of the network are reported. The sensors sample the vector magnetic field with a 4 kHz resolution and are sensitive to fluctuations below 0.1 $\textrm{nT}/\sqrt{\textrm{Hz}}$. Data from separate stations are synchronized to around $\pm100$ $\mu{s}$ using GPS and computer system clocks. Data from all sensors are automatically uploaded to a central server. Anomalous events, such as lightning strikes, have been observed. A wavelet analysis is used to study observations over a wide range of temporal scales up to daily variations that show strong differences between weekend and weekdays. The Bay Area Rapid Transit (BART) is identified as the most dominant signal from these observations and a superposed epoch analysis is used to study and extract the BART signal. Initial results of the correlation between sensors are also presented., Comment: 20 pages, 14 figures

We report on progress towards performing precision measurements of parity violation in Yb, in which the theoretical prediction for a strong weak-interaction-induced effect in the 6s^{2} ^{1}S_{0} \rightarrow 5d6s ^{3}D_{1} optical transition at 408 nm has already been confirmed, with a measurement of the effect at the \approx 10 % level of accuracy. With a new atomic-beam apparatus offering enhanced sensitivity, we are aiming at precisely determining the parity violation observable in Yb, which will allow us to probe the distributions of neutrons in different isotopes, investigate physics beyond the Standard Model, as well as to study intra-nucleus weak interactions, through an observation of the anapole moment of Yb nuclei with nonzero spin. We present the experimental principle employed to probe atomic parity violation, describe our new apparatus, and discuss the attained experimental sensitivity as well as the methods for characterizing systematics in these measurements.

We demonstrate nuclear magnetic resonance (NMR) spectroscopy of picoliter-volume solutions with a nanostructured diamond chip. Using optical interferometric lithography, diamond surfaces were nanostructured with dense, high-aspect-ratio nanogratings, enhancing the surface area by more than a factor of 15 over mm^2 regions of the chip. The nanograting sidewalls were doped with nitrogen-vacancy (NV) centers so that more than 10 million NV centers in a (25 micrometer)^2 laser spot are located close enough to the diamond surface (5 nm) to detect the NMR spectrum of 1 pL of fluid lying within adjacent nanograting grooves. The platform was used to perform 1H and 19F NMR spectroscopy at room temperature in magnetic fields below 50 mT. Using a solution of CsF in glycerol, we demonstrate that 4 +/- 2 x 10^12 19F spins in a 1 pL volume, can be detected with a signal-to-noise ratio of 3 in 1 s integration. This represents nearly two orders of magnitude improvement in concentration sensitivity over previous NV and picoliter NMR studies., Comment: 7 pages, 6 figures (main text) + 11 pages, 7 figures, 5 tables (Supplemental)

We present an experimental and theoretical study of the optically detected magnetic resonance signals for ensembles of negatively charged nitrogen-vacancy (NV) centers in 13C isotopically enriched single-crystal diamond. We observe four broad transition peaks with superimposed sharp features at zero magnetic field and study their dependence on applied magnetic field. A theoretical model that reproduces all qualitative features of these spectra is developed. Understanding the magnetic-resonance spectra of NV centers in isotopically enriched diamond is important for emerging applications in nuclear magnetic resonance., Comment: 5 pages, 3 figures

We propose a new method to search for hypothetical scalar particles that have feeble interactions with Standard-Model particles. In the presence of massive bodies, these interactions produce a non-zero Yukawa-type scalar-field magnitude. Using radio-frequency spectroscopy data of atomic dysprosium, as well as atomic clock spectroscopy data, we constrain the Yukawa-type interactions of a scalar field with the photon, electron, and nucleons for a range of scalar-particle masses corresponding to length scales $ > 10$ cm. In the limit as the scalar-particle mass $m_\phi \to 0$, our derived limits on the Yukawa-type interaction parameters are: $\Lambda_\gamma \gtrsim 8 \times 10^{19}$ GeV, $\Lambda_e \gtrsim 1.3 \times 10^{19}$ GeV, and $\Lambda_N \gtrsim 6 \times 10^{20}$ GeV. Our measurements also constrain combinations of interaction parameters, which cannot otherwise be probed with traditional anomalous-force measurements. We suggest further measurements to improve on the current level of sensitivity., Comment: 7 pages, 2 figures

Experiments searching for exotic spin-dependent interactions typically employ magnetic shielding between the source of the exotic field and the interrogated spins. We explore the question of what effect magnetic shielding has on detectable signals induced by exotic fields. Our general conclusion is that for common experimental geometries and conditions, magnetic shields should not significantly reduce sensitivity to exotic spin-dependent interactions, especially when the technique of comagnetometry is used. However, exotic fields that couple to electron spin can induce magnetic fields in the interior of shields made of a soft ferro- or ferrimagnetic material. This induced magnetic field must be taken into account in the interpretation of experiments searching for new spin-dependent interactions and raises the possibility of using a flux concentrator inside magnetic shields to amplify exotic spin-dependent signals., Comment: 8 pages, 5 figures

The use of anti-relaxation coatings in alkali vapor cells yields substantial performance improvements by reducing the probability of spin relaxation in wall collisions by several orders of magnitude. Some of the most effective anti-relaxation coating materials are alpha-olefins, which (as in the case of more traditional paraffin coatings) must undergo a curing period after cell manufacturing in order to achieve the desired behavior. Until now, however, it has been unclear what physicochemical processes occur during cell curing, and how they may affect relevant cell properties. We present the results of nondestructive Raman-spectroscopy and magnetic-resonance investigations of the influence of alkali metal vapor (Cs or K) on an alpha-olefin, 1-nonadecene coating the inner surface of a glass cell. It was found that during the curing process, the alkali metal catalyzes migration of the carbon-carbon double bond, yielding a mixture of cis- and trans-2-nonadecene., Comment: 5 pages, 6 figures

A dichroic atomic vapor laser lock (DAVLL) system exploiting buffer-gas-filled millimeter-scale vapor cells is presented. This system offers similar stability as achievable with conventional DAVLL system using bulk vapor cells, but has several important advantages. In addition to its compactness, it may provide continuous stabilization in a multi-gigahertz range around the optical transition. This range may be controlled either by changing the temperature of the vapor or by application of a buffer gas under an appropriate pressure. In particular, we experimentally demonstrate the ability of the system to lock the laser frequency between two hyperfine components of the $^{85}$Rb ground state or as far as 16 GHz away from the closest optical transition., Comment: 11 pages, 7 figures. Published in Review of Scientific Instruments 2016

We present results of our research on two-field (two-frequency) microwave spectroscopy in nitrogen-vacancy (NV-) color centers in a diamond. Both fields are tuned to transitions between the spin sublevels of the NV- ensemble in the 3A2 ground state (one field has a fixed frequency while the second one is scanned). Particular attention is focused on the case where two microwaves fields drive the same transition between two NV- ground state sublevels (ms=0 -> ms=+1). In this case, the observed spectra exhibit a complex narrow structure composed of three Lorentzian resonances positioned at the pump-field frequency. The resonance widths and amplitudes depend on the lifetimes of the levels involved in the transition. We attribute the spectra to coherent population oscillations induced by the two nearly degenerate microwave fields, which we have also observed in real time. The observations agree well with a theoretical model and can be useful for investigation of the NV relaxation mechanisms., Comment: 17 pages