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Molecular tagging velocimetry (MTV) is a nonintrusive velocimetry technique based on laser spectroscopy. It is particularly effective in challenging gas flow conditions encountered in thermal hydraulics where particle-based methods such as particle image (or tracking) velocimetry do not perform well. The main principles for designing and operating this diagnostic are presented as well as a set of gases that have been identified as potential seeds. Two gases [H2O and nitrous oxide (N2O)] have been characterized extensively for thermodynamic conditions ranging from standard temperature and pressure to environments encountered in integral effects test (IET) facilities for high-temperature gas reactors. A flexible, modular, and transportable laser system has been designed and demonstrated with H2O and N2O seed gases. The laser system enables determining the optimum excitation wavelength, tracer concentration, and timing parameters. Velocity precision and thermodynamic domain of applicability are discussed for both tracers. The spectroscopic nature of the diagnostics enables one to perform first-principle uncertainty analysis, which makes it attractive for validating numerical models. Molecular tagging velocimetry is demonstrated for two flows. First, in blowdown tests with H2O seed, the unique laser system enables one of the largest dynamic ranges reported to date for velocimetry: 5000:1 (74 dB). N2O-MTV is then deployed in situ in an IET facility, i.e., the High-Temperature Test Facility at Oregon State University, during a depressurized conduction cooldown (DCC) event. Data enable researchers to gain insights into flow instabilities present during DCC. Thus, MTV shows a strong potential to gain a fundamental understanding of gas flows in nuclear thermal hydraulics and to provide validation data for numerical solvers. [ABSTRACT FROM AUTHOR]

A molecular tagging velocity (MTV) technique is developed to non-intrusively measure velocity in an integral effect test (IET) facility simulating a high temperature helium-cooled nuclear reactor in accident scenarios. In these scenarios, the velocities are expected to be low, on the order of 1 m/s or less, which forces special requirements on the MTV tracer selection. Nitrous oxide (N 2 O) is identified as a suitable seed gas to generate NO tracers capable of probing the flow over a large range of pressure, temperature, and flow velocity. The performance of N 2 O-MTV is assessed in the laboratory at temperature and pressure ranging from 295 to 781 K and 1 to 3 atm. MTV signal improves with a temperature increase, but decreases with a pressure increase. Velocity precision down to 0.004 m/s is achieved with a probe time of 40 ms at ambient pressure and temperature. Measurement precision is limited by tracer diffusion, and absorption of the tag laser beam by the seed gas. Processing by cross-correlation of single shot images with high signal-to-noise ratio reference images improves the precision by about 10% compared to traditional single shot image correlations. The instrument is then deployed to the IET facility. Challenges associated with heat, vibrations, safety, beam delivery, and imaging are addressed in order to successfully operate this sensitive instrument in-situ. Data are presented for an isothermal depressurized conduction cool-down. Velocity profiles from MTV reveal a complex flow transient driven by buoyancy, diffusion, and instability taking place over short (<1 s) and long (>30 min) time-scales at sub-meter per second speed. The precision of the in-situ results is estimated at 0.027, 0.0095, and 0.006 m/s for a probe time of 5, 15, and 35 ms, respectively.