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The comprehension of quantum phase transitions (QPTs) is considered as a critical foothold in the field of many-body physics. Developing protocols to effectively identify and understand QPTs thus represents a key but challenging task for present quantum simulation experiments. Here, we establish a dynamical quench-interferometric framework to probe a zero-temperature QPT, which utilizes the evolved state by quenching the QPT Hamiltonian as input of a unitary interferometer. The metrological capability quantified by the quantum Fisher information captivatingly shows an unique peak in the vicinity of the quantum critical point, allowing us to probe the QPT without cooling the system to its ground state. We show that the probing can be implemented by extracting quantum fluctuations of the interferometric generator as well as parameter estimation uncertainty of the interferometric phase, and subsequently allows identifying the boundary of the phase diagram. Our results establish an important link between QPTs and quantum metrology, and enrich the toolbox of studying non-equilibrium many-body physics in current quantum simulators., Comment: Comments are welcome!

Ion-ion coupling over long distances represents a highly useful resource for quantum technologies, for example, to sympathetically cool or interconnect qubits in ion-based quantum-computing architectures. In this respect, the recently demonstrated wire-mediated ion-ion coupling stands due to the simplification of its trap layout and its prospects for deterministic entanglement. However, the strength of such coherent ion-wire-ion coupling is typically weak, hindering its practical utilization. Here, we propose a wire-mediated scheme for coherent ion-electron coupling. The scheme not only enables the sympathetic cooling of electrons via advanced ion-cooling techniques, but also allows to promote the effective ion-ion coupling strength by orders of magnitudes via electron mediation. Our work thus paves a way toward quantum information processing in ion-electron hybrid quantum systems., Comment: 14 pages, 6 figures

Entanglement, a hallmark of quantum mechanics, is a vital resource for quantum technologies. Generating highly entangled multipartite states is a key goal in current quantum experiments. We unveil a novel framework for understanding entanglement generation dynamics in Hamiltonian systems by quantum delocalization of an effective operator wavefunction on a correlation landscape. Our framework establishes a profound connection between the exponentially fast generation of multipartite entanglement, witnessed by the quantum Fisher information, and the linearly increasing asymptotics of hopping amplitudes governing the delocalization dynamics in Krylov space. We illustrate this connection using the paradigmatic Lipkin-Meshkov-Glick model and highlight potential signatures in chaotic Feingold-Peres tops. Our results provide a transformative tool for understanding and harnessing rapid entanglement production in complex quantum systems, providing a pathway for quantum enhanced technologies by large-scale entanglement.

Open systems possess unique potentials in high-precision sensing, yet the majority of previous studies rely on the spectral singularities known as exceptional points. Here we theoretically propose and experimentally demonstrate universal non-Hermitian sensing in the absence of exceptional points. The scheme makes use of the intrinsic sensitivity of a non-Hermitian probe to weak external fields, which can be understood as the direct consequence of non-Hermiticity. We confirm the basic mechanism by simulating the sensor-field dynamics using photon interferometry, and, as a concrete example, demonstrate the enhanced sensing of signals encoded in the setting angle of a wave plate. While the sensitivity of the probe is ultimately limited by the measurement noise, we find the non-Hermitian sensor showing superior performance under background noises that cannot be suppressed through repetitive measurements. Our experiment opens the avenue of enhanced sensing without exceptional points, complementing existing efforts aimed at harnessing the unique features of open systems.

The radical pair mechanism is an important model that may provide a basis for biological magnetoreception. To account for the high orientation precision of the real avian compass, P. J. Hore et al. proposed an intriguing phenomenon called quantum needle [Proc. Natl. Acad. Sci. 113, 4634 (2016)], where a spike-like feature emerges in the fractional yield signal. However, it is believed that quantum needle requires the radical pair lifetime to be longer than a few microseconds and thus poses stern challenges in realistic biological systems. Here, we exploit the optimization techniques and find a novel class of model system, which sustains much more prominent features of quantum needle and significantly relaxes the requirement for radical pair lifetime. Even more surprisingly, we find that the characteristics of quantum needle retain a narrow functional window around the geomagnetic field, which is absent in the previous model systems. Therefore, our work provides essential evidence for identifying the possible physical mechanism for quantum needle in chemical magnetoreception.

Decoherence and imperfect control are crucial challenges for quantum technologies. Common protection strategies rely on noise temporal autocorrelation, which is not optimal if other correlations are present. We develop and demonstrate experimentally a strategy that utilizes the cross-correlation of two noise sources. We achieve a tenfold coherence time extension by destructive interference of cross-correlated noise, improve control fidelity, and surpass the state-of-the-art sensitivity for high frequency quantum sensing, significantly expanding the applicability of noise protection strategies., Comment: Main: 5 pages, 5 figures; SM: 16 pages, 10 figures

Reaching a given target quantum state with high fidelity and fast operation speed close to the quantum limit represents an important goal in quantum information science. Here, we experimentally demonstrate superadiabatic quantum driving to achieve population transfer in a three-level solid-state spin system. Starting from traditional stimulated Raman adiabatic passage (STIRAP), our approach implements superadiabatic corrections to the STIRAP Hamiltonians with several paradigmatic pulse shapes. It requires no need of intense microwave pulses or long transfer times and shows enhanced robustness over pulse imperfections. These results might provide a useful tool for quantum information processing and coherent manipulations of quantum systems., Comment: 8 pages, 7 figures

The electric dipole moment (EDM) plays a crucial role in determining the interaction strength of an atom with electric fields, making it paramount to quantum technologies based on coherent atomic control. We propose a scheme for engineering the potential in a Paul trap to realize a two-level quantum system with a giant EDM formed by the motional states of a trapped electron. We show that, under realistic experimental conditions, the EDM can significantly exceed the ones attainable with Rydberg atoms. Furthermore, we show that such artificial atomic dipoles can be efficiently initialized, readout, and coherently controlled, thereby providing a potential platform for quantum technologies such as ultrahigh-sensitivity electric-field sensing., Comment: 7 pages, 4 5 figures + 26 pages Supplemental Material. Comments are welcome

In a solid-state spin system, we experimentally demonstrate a protocol for quantum-state population transfer with an improved efficiency compared to traditional stimulated Raman adiabatic passage (STIRAP). Using the ground-state triplet of the nitrogen-vacancy center in diamond, we show that the required evolution time for high-fidelity state transfer can be reduced by almost one order of magnitude. Furthermore, we establish an improved robustness against frequency detuning caused by magnetic noise as compared to STIRAP. These results provide a powerful tool for coherent spin manipulation in the context of quantum sensing and quantum computation., Comment: 8 pages, 6 figures

NV center is one of the most promising platforms in the field of quantum sensing. Magnetometry based on NV center, especially, has achieved a concrete development in regions of biomedicine and medical diagnostics. Improving the sensitivity of NV center sensor under wide inhomogeneous broadening and filed amplitude drift is one crucial issue of continuous concern, which relies on the coherent control of NV center with higher average fidelity. Quantum optimal control (QOC) methods provide access to this target, nevertheless the high time consumption of current methods due to the large number of needful sample points as well as the complexity of the parameter space has hindered their usability. In this paper we propose the Bayesian estimation phase-modulated (B-PM) method to tackle this problem. In the case of state transforming of NV center ensemble, the B-PM method reduces the time consumption by more than $90\%$ compared to the conventional standard Fourier base (SFB) method while increasing the average fidelity from $0.894$ to $0.905$. In AC magnetometry scenery, the optimized control pulse given by B-PM method achieves a eight-fold extension of the coherence time $T_2$ compared to rectangular $\pi$ pulse. Similar application can be made in other sensing situations. As a general algorithm, the B-PM method can be further extended to open- and closed-loop optimization of complex systems based on a variety of quantum platforms.

Quantum sensing is considered to be one of the most promising subfields of quantum information to deliver practical quantum advantages in real-world applications. However, its impressive capabilities, including high sensitivity, are often hindered by the limited quantum resources available. Here, we incorporate the expected information gain (EIG) and techniques such as accelerated computation into Bayesian experimental design (BED) in order to use quantum resources more efficiently. A simulated nitrogen-vacancy center in diamond is used to demonstrate real-time operation of the BED. Instead of heuristics, the EIG is used to choose optimal control parameters in real-time. Moreover, combining the BED with accelerated computation and asynchronous operations, we find that up to a tenfold speed-up in absolute time cost can be achieved in sensing multiple surrounding C13 nuclear spins. Our work explores the possibilities of applying the EIG to BED-based quantum-sensing tasks and provides techniques useful to integrate BED into more generalized quantum sensing systems.

In a recently demonstrated quantum-state tomography scheme [Phys. Rev. Lett. 124, 010405 (2020)], a random control field is locally applied to a multipartite system to reconstruct the full quantum state of the system through single-observable measurements. Here, we analyze the robustness of such a tomography scheme against measurement errors. We characterize the sensitivity to measurement errors using the logarithm of the condition number of a linear system that fully describes the tomography process. Using results from random matrix theory we derive the scaling law of the logarithm of this condition number with respect to the system size when Haar-random evolutions are considered. While this expression is independent on how Haar randomness is created, we also perform numerical simulations to investigate the temporal behavior of the robustness for two specific quantum systems that are driven by a single random control field. Interestingly, we find that before the mean value of the logarithm of the condition number as a function of the driving time asymptotically approaches the value predicted for a Haar-random evolution, it reaches a plateau whose length increases with the system size., Comment: 10 pages, 4 figures

Surpassing the standard quantum limit and even reaching the Heisenberg limit using quantum entanglement, represents the Holy Grail of quantum metrology. However, quantum entanglement is a valuable resource that does not come without a price. The exceptional time overhead for the preparation of large-scale entangled states raises disconcerting concerns about whether the Heisenberg limit is fundamentally achievable. Here we find a universal speed limit set by the Lieb-Robinson light cone for the quantum Fisher information growth to characterize the metrological potential of quantum resource states during their preparation. Our main result establishes a strong precision limit of quantum metrology accounting for the complexity of many-body quantum resource state preparation and reveals a fundamental constraint for reaching the Heisenberg limit in a generic many-body lattice system with bounded one-site energy. It enables us to identify the essential features of quantum many-body systems that are crucial for achieving the quantum advantage of quantum metrology, and brings an interesting connection between many-body quantum dynamics and quantum metrology., Comment: 7 pages, 3 figures + supplementary information (14 pages)

Recently, we find a physical limit on energy consumption of quantum metrology, and demonstrate that it essentially arises from the erasure of quantum Fisher information (QFI) which determines the best achievable measurement precision. Here, we provide more details in order to further elaborate the essence of this principle.

Quantum metrology is deeply connected to quantum geometry, through the fundamental notion of quantum Fisher information. Inspired by advances in topological matter, it was recently suggested that the Berry curvature and Chern numbers of band structures can dictate strict lower bounds on metrological properties, hence establishing a strong connection between topology and quantum metrology. In this work, we provide a first experimental verification of such topological bounds, by performing optimal quantum multi-parameter estimation and achieving the best possible measurement precision. By emulating the band structure of a Chern insulator, we experimentally determine the metrological potential across a topological phase transition, and demonstrate strong enhancement in the topologically non-trivial regime. Our work opens the door to metrological applications empowered by topology, with potential implications for quantum many-body systems., Comment: 6 pages, 4 figures + 13 pages (SI), comments are welcome

The nitrogen-vacancy (NV) center spin represents an appealing candidate for quantum information processing. Besides the widely used microwave control, its coherent manipulation may also be achieved using laser as mediated by the excited energy levels. Nevertheless, the multiple levels of the excited state of NV center spin make the coherent transition process become complex and may affect the fidelity of coherent manipulation. Here, we adopt the strategy of optimal quantum control to accelerate coherent state transfer in the ground state manifold of NV center spin using laser. The results demonstrate improved performance in both the speed and the fidelity of coherent state transfer which will be useful for optical control of NV center spin in diamond.

The features of topological physics can manifest in a variety of physical systems in distinct ways. Periodically driven systems, with the advantage of high flexibility and controllability, provide a versatile platform to simulate many topological phenomena and may lead to novel phenomena that can not be observed in the absence of driving. Here we investigate the influence of realistic experimental noise on the realization of a two-level system under a two-frequency drive that induces topologically nontrivial band structure in the two-dimensional Floquet space. We propose a dynamical decoupling scheme that sustains the topological phase transition overcoming the influence of dephasing. Therefore, the proposal would facilitate the observation of topological frequency conversion in the solid state spin system, e.g. NV center in diamond., Comment: 9 pages, 6 figures

The heat dissipation in quantum metrology represents not only an unavoidable problem towards practical applications of quantum sensing devices but also a fundamental relationship between thermodynamics and quantum metrology. However, a general thermodynamic principle which governs the rule of energy consumption in quantum metrology, similar to Landauer's principle for heat dissipation in computations, has remained elusive. Here, we establish such a physical principle for energy consumption in order to achieve a certain level of measurement precision in quantum metrology, and show that it is intrinsically determined by the erasure of quantum Fisher information. The principle provides a powerful tool to investigate the advantage of quantum resources, not only in measurement precision but also in energy efficiency. It also serves as a bridge between thermodynamics and various fundamental physical concepts related in quantum physics and quantum information theory., Comment: Comments are welcome

Simulating quantum phenomena in extreme spacetimes in the laboratory represents a powerful approach to explore fundamental physics in the interplay of quantum field theory and general relativity. Here we propose to simulate the movement of a Dirac particle propagating with a superluminal velocity caused by the emergent Alcubierre warp drive spacetime using trapped ions. We demonstrate that the platform allows observing the tilted lightcone that manifests as a superluminal velocity, which is in agreement with the prediction of general relativity. Furthermore, the Zitterbewegung effect arising from relativistic quantum mechanics persists with the superluminal propagation and is experimentally measurable. The present scheme can be extended to simulate the Dirac equation in other exotic curved spacetimes, thus provides a versatile tool to gain insights into the fundamental limit of these extreme spacetimes.

Optomechanical systems offer unique opportunities to explore macroscopic quantum state and related fundamental problems in quantum mechanics. Here, we propose a quantum optomechanical system involving exchange interaction between spin angular momentum of light and a torsional oscillator. We demonstrate that this system allows coherent control of the torsional quantum state of a torsional oscillator on the single photon level, which facilitates efficient cooling and squeezing of the torsional oscillator. Furthermore, the torsional oscillator with a macroscopic length scale can be prepared in Schr\"odinger cat-like state. Our work provides a platform to verify the validity of quantum mechanics in macroscopic systems on the micrometer and even centimeter scale., Comment: 5 pages + 14 pages of appendices, 9 figures

The quantum Fisher information (QFI) represents a fundamental concept in quantum physics. On the one hand, it quantifies the metrological potential of quantum states in quantum-parameter-estimation measurements. On the other hand, it is intrinsically related to the quantum geometry and multipartite entanglement of many-body systems. Here, we explore how the QFI can be estimated via randomized measurements, an approach which has the advantage of being applicable to both pure and mixed quantum states. In the latter case, our method gives access to the sub-quantum Fisher information, which sets a lower bound on the QFI. We experimentally validate this approach using two platforms: a nitrogen-vacancy center spin in diamond and a 4-qubit state provided by a superconducting quantum computer. We further perform a numerical study on a many-body spin system to illustrate the advantage of our randomized-measurement approach in estimating multipartite entanglement, as compared to quantum state tomography. Our results highlight the general applicability of our method to general quantum platforms, including solid-state spin systems, superconducting quantum computers and trapped ions, hence providing a versatile tool to explore the essential role of the QFI in quantum physics., Comment: 11 pages, 6 figures, comments are welcome

We present a method for the direct measurement of the Wigner characteristic function of a thermalizing harmonic oscillator that is completely inaccessible for control or measurement. The strategy employs a recently proposed probe-measurement-based scheme [Phys. Rev. Lett. 122, 110406 (2019)] which relies on the pulsed control of a two-level probe. We generalize this scheme to the case of a nonunitary time evolution of the target harmonic oscillator, describing its thermalization through contact to a finite-temperature environment, given in the form of a Lindblad master equation. This generalization is achieved using a superoperator formalism and yields analytical expressions for the direct measurement of the characteristic function, accounting for the decoherence during the measurement process., Comment: 13 pages, 4 figures

Quantum optimal control represents a powerful technique to enhance the performance of quantum experiments by engineering the controllable parameters of the Hamiltonian. However, the computational overhead for the necessary optimization of these control parameters drastically increases as their number grows. We devise a novel variant of a gradient-free optimal-control method by introducing the idea of phase-modulated driving fields, which allows us to find optimal control fields efficiently. We numerically evaluate its performance and demonstrate the advantages over standard Fourier-basis methods in controlling an ensemble of two-level systems showing an inhomogeneous broadening. The control fields optimized with the phase-modulated method provide an increased robustness against such ensemble inhomogeneities as well as control-field fluctuations and environmental noise, with one order of magnitude less of average search time. Robustness enhancement of single quantum gates is also achieved by the phase-modulated method. Under environmental noise, an XY-8 sequence constituted by optimized gates prolongs the coherence time by $50\%$ compared with standard rectangular pulses in our numerical simulations, showing the application potential of our phase-modulated method in improving the precision of signal detection in the field of quantum sensing., Comment: 13 pages, 11 figures

Precise spectroscopy of oscillating fields plays significant roles in many fields. Here, we propose an experimentally feasible scheme to measure the frequency of a fast-oscillating field using a single-qubit sensor. By invoking a stable classical clock, the signal phase correlations between successive measurements enable us to extract the target frequency with extremely high precision. In addition, we integrate dynamical decoupling technique into the framework to suppress the influence of slow environmental noise. Our framework is feasible with a variety of atomic and single solid-state-spin systems within the state-of-the-art experimental capabilities as a versatile tool for quantum spectroscopy.

Quantum criticality, as a fascinating quantum phenomenon, may provide significant advantages for quantum sensing. Here we propose a dynamic framework for quantum sensing with a family of Hamiltonians that undergo quantum phase transitions (QPT). By giving the formalism of the quantum Fisher information (QFI) for quantum sensing based on critical quantum dynamics, we demonstrate its divergent feature when approaching the critical point. We illustrate the basic principle and the details of experimental implementation using quantum Rabi model. The framework is applicable to a variety of examples and does not rely on the stringent requirement for particular state preparation or adiabatic evolution. It is expected to provide a route towards the implementation of criticality-enhanced quantum sensing.

The quantum Cram\'er-Rao bound sets a fundamental limit on the accuracy of unbiased parameter estimation in quantum systems, relating the uncertainty in determining a parameter to the inverse of the quantum Fisher information. We experimentally demonstrate near saturation of the quantum Cram\'er-Rao bound in the phase estimation of a solid-state spin system, provided by a nitrogen-vacancy center in diamond. This is achieved by comparing the experimental uncertainty in phase estimation with an independent measurement of the related quantum Fisher information. The latter is independently extracted from coherent dynamical responses of the system under weak parametric modulations, without performing any quantum-state tomography. While optimal parameter estimation has already been observed for quantum devices involving a limited number of degrees of freedom, our method offers a versatile and powerful experimental tool to explore the Cram\'er-Rao bound and the quantum Fisher information in systems of higher complexity, as relevant for quantum technologies.

Quantum sensing exploits fundamental features of quantum system to achieve highly efficient measurement of physical quantities. Here, we propose a strategy to realize a single-qubit pseudo-Hermitian sensor from a dilated two-qubit Hermitian system. The pseudo-Hermitian sensor exhibits divergent susceptibility in dynamical evolution that does not necessarily involve exceptional point. We demonstrate its potential advantages to overcome noises that cannot be averaged out by repetitive measurements. The proposal is feasible with the state-of-art experimental capability in a variety of qubit systems, and represents a step towards the application of non-Hermitian physics in quantum sensing., Comment: 6 pages, 3 figure, comments are welcome

Single-qubit measurements are typically insufficient for inferring arbitrary quantum states of a multi-qubit system. We show that if the system can be fully controlled by driving a single qubit, then utilizing a local random pulse is almost always sufficient for complete quantum-state tomography. Experimental demonstrations of this principle are presented using a nitrogen-vacancy (NV) center in diamond coupled to a nuclear spin, which is not directly accessible. We report the reconstruction of a highly entangled state between the electron and nuclear spin with fidelity above 95%, by randomly driving and measuring the NV-center electron spin only. Beyond quantum-state tomography, we outline how this principle can be leveraged to characterize and control quantum processes in cases where the system model is not known., Comment: 9 pages, 6 figures

Topological charge pumping represents an important quantum phenomenon that shows the fundamental connection to the topological properties of dynamical systems. Here, we introduce a pumping process in a spin-dependent double-well optical lattice with glide symmetry. In the dynamic process, the glide symmetry protects the band touching points and topological properties of the system are characterised by the non-Abelian Berry curvature. By engineering suitable form of interaction between different spin components, the model not only demonstrates topological phase transition, but also shows hybridisation between the spatial and temporal domain with novel topological features captured by the Wilson line along the synthetic directions. Our work provides a new model based on ultracold atoms towards the implementation of versatile topological matters and topological phenomena., Comment: 5 pages, 3 figures

One of the key challenges for the implementation of scalable quantum information processing is the design of scalable architectures that support coherent interaction and entanglement generation between distant quantum systems. We propose a nanotube double quantum dot spin transducer that allows to achieve steady-state entanglement between nitrogen-vacancy center spins in diamond with spatial separations over micrometers. The distant spin entanglement further enables us to design a scalable architecture for solid-state quantum information processing based on a hybrid platform consisting of nitrogen-vacancy centers and carbon-nanotube double quantum dots., Comment: 13 pages, 7 figures