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5. Propane oxidation on Pt-WO3/g -AL2O3 catalytic systems

Author

Silva M.A.Pereira da, Cardoso R.M., and Schmal M.

Subjects
Propane propane oxidation, Automotive automotive catalysts, lcsh:TP155-156, lcsh:Chemical engineering, equipment and supplies, Platinumplatinum-tungsten catalysts
Abstract

The oxidation of propane on was studied with Pt-xWO3/Al2O3 catalysts was studied ,by varying the concentration of tungsten sublayer. Thermal analysis and XRD in situ showed that the enrichment of tungsten at the surface is associated with the formation of HxWO3 bronze. FTIR results with C3H8 and O2 indicated that the catalyst surface properties and the interaction between W and Pt were modified. These modified surface complexes prevented the formation of acetates and formate species. The addition of W increased the activity of Pt/Al2O3 towards in C3H8 oxidation. Tungsten was the main responsible for the stability of the bimetallic catalysts in the presence of water.

Published
2003

8. Regional climate downscaling over Europe: perspectives from the EURO-CORDEX community

Author

Jacob, Daniela, Teichmann, Claas, Sobolowski, Stefan, Katragkou, Eleni, Anders, Ivonne, Belda, Michal, Benestad, Rasmus, Boberg, Fredrik, Buonomo, Erasmo, Cardoso, Rita M., Casanueva, Ana, Christensen, Ole B., Christensen, Jens Hesselbjerg, Coppola, Erika, De Cruz, Lesley, Davin, Edouard L., Dobler, Andreas, Domínguez, Marta, Fealy, Rowan, Fernandez, Jesus, Gaertner, Miguel Angel, García-Díez, Markel, Giorgi, Filippo, Gobiet, Andreas, Goergen, Klaus, Gómez-Navarro, Juan José, Alemán, Juan Jesús González, Gutiérrez, Claudia, Gutiérrez, José M., Güttler, Ivan, Haensler, Andreas, Halenka, Tomáš, Jerez, Sonia, Jiménez-Guerrero, Pedro, Jones, Richard G., Keuler, Klaus, Kjellström, Erik, Knist, Sebastian, Kotlarski, Sven, Maraun, Douglas, van Meijgaard, Erik, Mercogliano, Paola, Montávez, Juan Pedro, Navarra, Antonio, Nikulin, Grigory, de Noblet-Ducoudré, Nathalie, Panitz, Hans-Juergen, Pfeifer, Susanne, Piazza, Marie, Pichelli, Emanuela, Pietikäinen, Joni-Pekka, Prein, Andreas F., Preuschmann, Swantje, Rechid, Diana, Rockel, Burkhardt, Romera, Raquel, Sánchez, Enrique, Sieck, Kevin, Soares, Pedro M. M., Somot, Samuel, Srnec, Lidija, Sørland, Silje Lund, Termonia, Piet, Truhetz, Heimo, Vautard, Robert, Warrach-Sagi, Kirsten, Wulfmeyer, Volker, Climate Service Center Germany (GERICS), Helmholtz-Zentrum Geesthacht, Hamburg, Germany, NORCE Norwegian Research Centre, The Bjerknes Centre for Climate Research, Bergen, Norway, Department of Meteorology and Climatology, School of Geology, Aristotle University of Thessaloniki, Thessaloniki, Greece, Central Institute for Meteorology and Geodynamics (ZAMG), Vienna, Austria, Department of Atmospheric Physics, Faculty of Mathematics and Physics, Charles University, Prague, Czech Republic, The Norwegian Meteorological Institute, Oslo, Norway, Danish Meteorological Institute (DMI), Copenhagen, Denmark, School of Geography and the Environment, University of Oxford, Oxford, UK, Instituto Dom Luiz (IDL), Faculdade de Ciências, Universidade de Lisboa, Lisbon, Portugal, Meteorology Group, Department of Applied Mathematics and Computer Science, Universidad de Cantabria, Santander, Spain, Niels Bohr Institute, University of Copenhagen, Copenhagen, Denmark, International Centre for Theoretical Physics (ICTP), Trieste, Italy, Royal Meteorological Institute of Belgium (RMIB), Brussels, Belgium, Institute for Atmospheric and Climate Science, ETH Zurich, Zurich, Switzerland, Agencia Estatal de Meteorología, Madrid, Spain, ICARUS, Department of Geography, Maynooth University, Maynooth, Ireland, University of Castilla-La Mancha, Toledo, Spain, Centre for High-Performance Scientific Computing in Terrestrial Systems, Geoverbund ABC/J, Jülich, Germany, Regional Atmospheric Modeling Group, Department of Physics, University of Murcia, Murcia, Spain, Meteorology Group, Instituto de Física de Cantabria (CSIC-Universidad de Cantabria), Santander, Spain, Croatian Meteorological and Hydrological Service, Zagreb, Croatia, Met Office Hadley Centre, Exeter, UK, Chair of Atmospheric Processes, Brandenburg University of Technology Cottbus - Senftenberg, Cottbus, Germany, Swedish Meteorological and Hydrological Institute, Norrköping, Sweden, Meteorological Institute, University of Bonn, Bonn, Germany, Federal Office of Meteorology and Climatology MeteoSwiss, Zurich-Airport, Switzerland, Wegener Center for Climate and Global Change, University of Graz, Graz, Austria, Royal Netherlands Meteorological Institute (KNMI), De Bilt, The Netherlands, C.I.R.A., Capua, Italy, Centro Euro-Mediterraneo sui Cambiamenti Climatici (CMCC), Lecce, Italy, Laboratoire des Sciences du Climat et de l’Environnement, IPSL, Unité Mixte CEA-CNRS-UVSQ, Université Paris-Saclay, Gif-sur-Yvette cédex, France, Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology, Karlsruhe, Germany, Finnish Meteorological Institute (FMI), Helsinki, Finland, National Center for Atmospheric Research, Boulder, USA, Helmholtz-Zentrum Geesthacht, Geesthacht, Germany, CNRM, Université de Toulouse, Météo-France, CNRS, Toulouse, France, Department of Physics and Astronomy, Ghent University, Ghent, Belgium, Institute of Physics and Meteorology, University of Hohenheim, Stuttgart, Germany, Jacob D., Teichmann C., Sobolowski S., Katragkou E., Anders I., Belda M., Benestad R., Boberg F., Buonomo E., Cardoso R.M., Casanueva A., Christensen O.B., Christensen J.H., Coppola E., De Cruz L., Davin E.L., Dobler A., Dominguez M., Fealy R., Fernandez J., Gaertner M.A., Garcia-Diez M., Giorgi F., Gobiet A., Goergen K., Gomez-Navarro J.J., Aleman J.J.G., Gutierrez C., Gutierrez J.M., Guttler I., Haensler A., Halenka T., Jerez S., Jimenez-Guerrero P., Jones R.G., Keuler K., Kjellstrom E., Knist S., Kotlarski S., Maraun D., van Meijgaard E., Mercogliano P., Montavez J.P., Navarra A., Nikulin G., de Noblet-Ducoudre N., Panitz H.-J., Pfeifer S., Piazza M., Pichelli E., Pietikainen J.-P., Prein A.F., Preuschmann S., Rechid D., Rockel B., Romera R., Sanchez E., Sieck K., Soares P.M.M., Somot S., Srnec L., Sorland S.L., Termonia P., Truhetz H., Vautard R., Warrach-Sagi K., Wulfmeyer V., Electronics and Informatics, Physics, Universidad de Cantabria, Ministerio de Economía y Competitividad (España), CSIC-UC - Instituto de Física de Cantabria (IFCA), Ministerio de Ciencia, Innovación y Universidades (España), Agencia Estatal de Investigación (España), and European Commission

Subjects
IMPACTS, Climate Research, 010504 meteorology & atmospheric sciences, 0208 environmental biotechnology, Climate change, ENSEMBLE, 02 engineering and technology, Land cover, 01 natural sciences, Klimatforskning, COVER CHANGES, 11. Sustainability, ddc:330, Regional science, Adaptation (computer science), Temporal scales, TEMPERATURE, 0105 earth and related environmental sciences, MODEL DESCRIPTION, Global and Planetary Change, regional climate models, EURO-CORDEX, Land use, LAND-USE, FUTURE CHANGES, 15. Life on land, SIMULATIONS, 020801 environmental engineering, Earth system science, CORDEX, Geography, ddc:551.6, 13. Climate action, Earth and Environmental Sciences, MED-CORDEX, EURO-CORDEX, DAILY PRECIPITATION STATISTICS, Downscaling, Regional climate modelling, Regional climate models
Abstract

The European CORDEX (EURO-CORDEX) initiative is a large voluntary effort that seeks to advance regional climate and Earth system science in Europe. As part of the World Climate Research Programme (WCRP) - Coordinated Regional Downscaling Experiment (CORDEX), it shares the broader goals of providing a model evaluation and climate projection framework and improving communication with both the General Circulation Model (GCM) and climate data user communities. EURO-CORDEX oversees the design and coordination of ongoing ensembles of regional climate projections of unprecedented size and resolution (0.11° EUR-11 and 0.44° EUR-44 domains). Additionally, the inclusion of empirical-statistical downscaling allows investigation of much larger multi-model ensembles. These complementary approaches provide a foundation for scientific studies within the climate research community and others. The value of the EURO-CORDEX ensemble is shown via numerous peer-reviewed studies and its use in the development of climate services. Evaluations of the EUR-44 and EUR-11 ensembles also show the benefits of higher resolution. However, significant challenges remain. To further advance scientific understanding, two flagship pilot studies (FPS) were initiated. The first investigates local-regional phenomena at convection-permitting scales over central Europe and the Mediterranean in collaboration with the Med-CORDEX community. The second investigates the impacts of land cover changes on European climate across spatial and temporal scales. Over the coming years, the EURO-CORDEX community looks forward to closer collaboration with other communities, new advances, supporting international initiatives such as the IPCC reports, and continuing to provide the basis for research on regional climate impacts and adaptation in Europe., S.S. acknowledges the support of NOTUR/NORSTORE projects NN9280K/NS9001K and the Research Council of Norway and its basic institute support of the strategic project on Climate Services. E.K. acknowledges the support of the Greek Research & Technology Network (GRNET) for provision of technical support and facilities (HPC-ARIS). L.S. and I.G. acknowledge the support of Croatian Science Foundation project CARE (2831) and Ministry of Environment and Energy project TF/HR/P3-M1-O1-0101 (www.prilagodba-klimi.hr). J. F. acknowledges support from the Spanish R+D Programme through grant INSIGNIA (CGL2016-79210-R), co-funded by ERDF/FEDER, and the Altamira Supercomputer at Instituto de Física de Cantabria (IFCA-CSIC), member of the Spanish Supercomputing Network. P.T. acknowledges support from the Belgian Science Policy (BELSPO) within the CORDEX.be (BR/143/A2) project, and the VSC (Flemish Supercomputer Center), funded by the Research Foundation - Flanders (FWO) and the Flemish Government – department EWI.M.A.G. acknowledges support from the Spanish R+D Programme through grants CGL2013-47261-R and CGL2017-89583-R, co-funded by the European Regional Development Fund. RF acknowledges support provided by ICHEC (Irish Centre for High End Computing) and the Irish Environmental Protection Agency. K.G. and S.K. gratefully acknowledge the computing time granted through JARA-HPC on the supercomputers JUROPA and JURECA at Forschungszentrum Jülich. M.B. and T.H. acknowledge support by The Ministry of Education, Youth and Sports from the Large Infrastructures for Research, Experimental Development and Innovations project “IT4Innovations National Supercomputing Center – LM2015070” and the INTER-EXCELLENCE program LTT17007, and support by Charles University from the PROGRES Q16 program. We acknowledge the approval and support of the two Flagship Pilot Studies (the FPS on Convective phenomena at high resolution over Europe and the Mediterranean and the FPS on Land Use and Climate Across Scales) by WRCP CORDEX. We thank Merja Tölle for providing simulation CCLM5-0-9-JLU as contribution to the CORDEX-FPS “Convective phenomena at high resolution over Europe and the Mediterranean”. D. M., M.P., and H.T. gratefully acknowledge the support received via the projects HighEnd:Extremes, SPIRIT, and reclip:convex, funded by the Austrian Climate Research Programme (ACRP) of the Klima- und Energiefonds (nos. B368608, B960272, and B769999, respectively), as well as the Jülich Supercomputing Centre (JSC) for compute time on JURECA through the grant JJSC39 and the Vienna Scientific Cluster (VSC) through the grants 70992 and 71193.

Published
2020

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