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1. Harmonisierung der GOME, SCIAMACHY und GOME-2 Ozonsäulendaten für die Untersuchung der Langzeittrends und deren Ursachen

Author

Chehade, Wissam, Burrows, John P., and Schrems, Otto

Subjects
SCIAMACHY, Ozone, GOME-2, ozone depleting substances (ODS), harmonisation, ozone trends, ddc:500, 500 Science, absorption cross section
Abstract

This thesis addresses the issue of the accurate measurements of ozone distributions in the atmosphere obtained from different satellite borne atmospheric chemistry spectrometers which represent a major need and pre-requisite for determining whether the atmospheric burden of ozone depleting substances (ODS) are reduced in accordance to the Montreal Protocol, and valuable for long-term trend analysis to detect a subsequent ozone recovery. A consolidated and homogeneous long term dataset requires a careful analysis of the relevant parameters used in the retrievals, one important parameter is the absorption cross section. This work presents the procedures followed to correct the ozone cross section data of SCIAMACHY and GOME-2 spectrometers starting from original raw data (optical density spectra). Using the available versions of SCIAMACHY and GOME-2 FM cross sections in the retrieval of total ozone from each satellite leads to an overestimation in the total ozone by 3-5% and 8-9% compared to collocated GOME data, respectively. The quality of the revised temperature-dependent ozone absorption cross sections is investigated over GOME-2 and SCIAMACHY's entire spectral range. The revised data agree well within 3% with other published ozone cross sections and preserve the correct temperature dependence in the Hartley, Huggins, Chappuis and Wulf bands as displayed by the literature data. SCIAMACHY's total ozone columns retrieved using the revised cross section data are shown to be within 1% compared to the ozone amounts retrieved routinely from SCIAMACHY, which uses Bogumil et al. (2003) data but adjusted with a scaling factor of 5.3% and a wavelength shift of 0.08 nm. The total ozone column retrieved from the GOME-2/MetOp-A satellite using the new cross section data is within 1% compared to the ozone amounts retrieved from the standard retrieval performed for GOME-2. The study also presents a long term statistical trend analysis of total ozone datasets obtained from various satellites. A multi-variate linear regression was applied to annual mean zonal mean data using various natural and anthropogenic explanatory variables that represent dynamical and chemical processes which modify global ozone distributions in a changing climate. The study investigated the magnitude and zonal distribution of the different atmospheric chemical and dynamical factors contributing to long-term total ozone changes. The regression model included the Equivalent Effective Stratospheric Chlorine (EESC), the 11 year solar cycle, the Quasi-Biennial Oscillation (QBO), stratospheric aerosol loading describing the effects from major volcanic eruptions, the El Nino/ Southern Oscillation (ENSO), the Arctic and Antarctic Oscillation, and accumulated eddy heat flux (EHF), the latter representing changes due to the Brewer Dobson circulation. The total ozone column dataset used here comprises the SBUV/TOMS/OMI merged data (1979 - 2012) MOD V8.0. The analysis explained most of the ozone variability. The results show that QBO dominates the ozone variability in the tropics (7 DU) while at higher latitudes, the dynamical indices, AO/AAO and eddy heat flux, have substantial influence on total ozone variations by up to 10 DU. ENSO signal are more evident in the Northern Hemisphere. EESC is found to be a main contributor to the long-term ozone decline and the trend changes after the end of 1990s. A positive significant trend in total ozone columns is found after 1997 (between 1 and 8.2DU/decade) which points at the slowing of ozone decline and the onset of ozone recovery. The EESC based trends are compared with the trends obtained from the statistical piecewise linear trend (PWLT or hockey stick) model to examine the differences between both approaches. The results do indicate that the positive PWLT turnaround trends are larger than indicated by the EESC trends, however, they agree within 2-sigma, thus demonstrating the success of the Montreal Protocol phasing out of the ozone depleting substances (ODS). A sensitivity study is carried out by comparing the regression results, using different satellite merged datasets as well as the ground based measurements (1979 - 2012) in the regression analysis in order to investigate the uncertainty in the long-term trends due to different ozone datasets and data versions. All the datasets show almost identical pre-turnaround trends before 1979 for both EESC and PWLT approaches while the positive trends after 1997 are greatly influenced by the short-term variability. In spite of that, all datasets agree within 2-sigma fit parameters.

Published
2014

2. Impact of ozone cross-section choice on WFDOAS total ozone retrieval applied to GOME, SCIAMACHY, and GOME-2 (1995-present)

Author

Weber, Mark, Chehade, Wissam, Gorshelev, Victor, Serdyuchenko, Anna, Spietz, Peter, and Weber, Mark

Subjects
absorption cross-section, spectroscopy, satellite, 500 Science, UV, SCIAMACHY, remote sensing, GOME-2, trace gas, DOAS, weighting function, ddc:500, GOME, retrieval
Abstract

Technical Note Issue 2 (January 2011) with updates from November 2013. A contribution to ACSO http://igaco-o3.fmi.fi/ACSO/. In this technical note we investigate how the choice of ozone cross-sections impact the WFDOAS (Weighting Function Differential Optical Absorption Spectroscopy) total ozone retrieval (Coldewey-Egbers et al., 2005) for the satellite instruments GOME, GOME-2, and SCIAMACHY.

Published
2013

3. State of the Climate in 2012

Author

Blunden, Jessica, Arndt, Derek S., Achberger, Christine, Ackerman, Stephen A., Albanil, Adelina, Alexander, P., Alfaro, Eric J., Allan, Rob, Alves, Lincoln M., Amador, Jorge A., Ambenje, Peter, Andrianjafinirina, Solonomenjanahary, Antonov, John, Aravequia, Jose A., Arendt, A., Arevalo, Juan, Ashik, I., Atheru, Zachary, Banzon, Viva, Baringer, Molly O., Barreira, Sandra, Barriopedro, David E., Beard, Grant, Becker, Andreas, Behrenfeld, Michael J., Bell, Gerald D., Benedetti, Angela, Bernhard, Germar, Berrisford, Paul, Berry, David I., Bhatt, U., Bidegain, Mario, Bindoff, Nathan, Bissolli, Peter, Blake, Eric S., Booneeady, Raj, Bosilovich, Michael, Box, J. E., Boyer, Tim, Braathen, Geir O., Bromwich, David H., Brown, R., Brown, L., Bruhwiler, Lori, Bulygina, Olga N., Burgess, D., Burrows, John, Calderon, Blanca, Camargo, Suzana J., Campbell, Jayaka, Cao, Y., Cappelen, J., Carrasco, Gualberto, Chambers, Don P., Chang A, L., Chappell, Petra, Chehade, Wissam, Cheliah, Muthuvel, Christiansen, Hanne H., Christy, John R., Ciais, Phillipe, Coelho, Caio A. S., Cogley, J. G., Colwell, Steve, Cross, J. N., Crouch, Jake, Cunningham, Stuart A., Dacic, Milan, Jeu, Richard A. M., Dekaa, Francis S., Demircan, Mesut, Derksen, C., Diamond, Howard J., Dlugokencky, Ed J., Dohan, Kathleen, Dolman, A. Johannes, Domingues, Catia M., Dong Shenfu, Dorigo, Wouter A., Drozdov, D. S., Duguay, Claude R., Dunn, Robert J. H., Duran-Quesada, Ana M., Dutton, Geoff S., Ehmann, Christian, Elkins, James W., Euscategui, Christian, Famiglietti, James S., Fang Fan, Fauchereau, Nicolas, Feely, Richard A., Fekete, Balazs M., Fenimore, Chris, Fioletov, Vitali E., Fogarty, Chris T., Fogt, Ryan L., Folland, Chris K., Foster, Michael J., Frajka-Williams, Eleanor, Franz, Bryan A., Frith, Stacey H., Frolov, I., Ganter, Catherine, Garzoli, Silvia, Geai, M. -L, Gerland, S., Gitau, Wilson, Gleason, Karin L., Gobron, Nadine, Goldenberg, Stanley B., Goni, Gustavo, Good, Simon A., Gottschalck, Jonathan, Gregg, Margarita C., Griffiths, Georgina, Grooss, Jens-Uwe, Guard, Charles Chip, Gupta, Shashi K., Hall, Bradley D., Halpert, Michael S., Harada, Yayoi, Hauri, C., Heidinger, Andrew K., Heikkila, Anu, Heim, Richard R., Heimbach, Patrick, Hidalgo, Hugo G., Hilburn, Kyle, Ho, Shu-Peng, Hobbs, Will R., Holgate, Simon, Hovsepyan, Anahit, Hu Zeng-Zhen, Hughes, P., Hurst, Dale F., Ingvaldsen, R., Inness, Antje, Jaimes, Ena, Jakobsson, Martin, James, Adamu I., Jeffries, Martin O., Johns, William E., Johnsen, Bjorn, Johnson, Gregory C., Johnson, Bryan, Jones, Luke T., Jumaux, Guillaume, Kabidi, Khadija, Kaiser, Johannes W., Kamga, Andre, Kang, Kyun-Kuk, Kanzow, Torsten O., Kao, Hsun-Ying, Keller, Linda M., Kennedy, John J., Key, J., Khatiwala, Samar, Pour, H. Kheyrollah, Kholodov, A. L., Khoshkam, Mahbobeh, Kijazi, Agnes, Kikuchi, T., Kim, B. -M, Kim, S. -J, Kimberlain, Todd B., Knaff, John A., Korshunova, Natalia N., Koskela, T., Kousky, Vernon E., Kramarova, Natalya, Kratz, David P., Krishfield, R., Kruger, Andries, Kruk, Michael C., Kumar, Arun, Lagerloef, Gary S. E., Lakkala, K., Lander, Mark A., Landsea, Chris W., Lankhorst, Matthias, Laurila, T., Lazzara, Matthew A., Lee, Craig, Leuliette, Eric, Levitus, Sydney, L Heureux, Michelle, Lieser, Jan, Lin, I-I, Liu, Y. Y., Liu, Y., Liu Hongxing, Liu Yanju, Lobato-Sanchez, Rene, Locarnini, Ricardo, Loeb, Norman G., Loeng, H., Long, Craig S., Lorrey, Andrew M., Luhunga, P., Lumpkin, Rick, Luo Jing-Jia, Lyman, John M., Macdonald, Alison M., Maddux, Brent C., Malekela, C., Manney, Gloria, Marchenko, S. S., Marengo, Jose A., Marotzke, Jochem, Marra, John J., Martinez-Gueingla, Rodney, Massom, Robert A., Mathis, Jeremy T., Mcbride, Charlotte, Mccarthy, Gerard, Mcvicar, Tim R., Mears, Carl, Meier, W., Meinen, Christopher S., Menendez, Melisa, Merrifield, Mark A., Mitchard, Edward, Mitchum, Gary T., Montzka, Stephen A., Morcrette, Jean-Jacques, Mote, Thomas, Muehle, Jens, Muehr, Bernhard, Mullan, A. Brett, Mueller, Rolf, Nash, Eric R., Nerem, R. Steven, Newlin, Michele L., Newman, Paul A., Ng Ongolo, H., Nieto, Juan Jose, Nishino, S., Nitsche, Helga, Noetzli, Jeannette, Oberman, N. G., Obregon, Andre, Ogallo, Laban A., Oludhe, Christopher S., Omar, Mohamed I., Overland, James, Oyunjargal, Lamjav, Parinussa, Robert M., Park, Geun-Ha, Park, E-Hyung, David Berry, Pasch, Richard J., Pascual-Ramirez, Reynaldo, Pelto, Mauri S., Penalba, Olga, Peng, L., Perovich, Don K., Pezza, Alexandre B., Phillips, David, Pickart, R., Pinty, Bernard, Pitts, Michael C., Purkey, Sarah G., Quegan, Shaun, Quintana, Juan, Rabe, B., Rahimzadeh, Fatemeh, Raholijao, Nirivololona, Raiva, I., Rajeevan, Madhavan, Ramiandrisoa, Voahanginirina, Ramos, Alexandre, Ranivoarissoa, Sahondra, Rayner, Nick A., Rayner, Darren, Razuveav, Vyacheslav N., Reagan, James, Reid, Phillip, Renwick, James, Revedekar, Jayashree, Richter-Menge, Jacqueline, Rivera, Ingrid L., Robinson, David A., Rodell, Matthew, Romanovsky, Vladimir E., Ronchail, Josyane, Rosenlof, Karen H., Sabine, Christopher L., Salvador, Mozar A., Sanchez-Lugo, Ahira, Santee, Michelle L., Sasgen, I., Sawaengphokhai, P., Sayouri, Amal, Scambos, Ted A., Schauer, U., Schemm, Jae, Schlosser, P., Schmid, Claudia, Schreck, Carl, Semiletov, Igor, Send, Uwe, Sensoy, Serhat, Setzer, Alberto, Severinghaus, Jeffrey, Shakhova, Natalia, Sharp, M., Shiklomanov, Nicolai I., Siegel, David A., Silva, Viviane B. S., Silva, Frabricio D. S., Sima, Fatou, Simeonov, Petio, Simmonds, I., Simmons, Adrian, Skansi, Maria, Smeed, David A., Smethie, W. M., Smith, Adam B., Smith, Cathy, Smith, Sharon L., Smith, Thomas M., Sokolov, V., Srivastava, A. K., Stackhouse, Paul W., Stammerjohn, Sharon, Steele, M., Steffen, Konrad, Steinbrecht, Wolfgang, Stephenson, Tannecia, Su, J., Svendby, T., Sweet, William, Takahashi, Taro, Tanabe, Raymond M., Taylor, Michael A., Tedesco, Marco, Teng, William L., Thepaut, Jean-Noel, Thiaw, Wassila M., Thoman, R., Thompson, Philip, Thorne, Peter W., Timmermans, M. -L, Tobin, Skie, Toole, J., Trewin, Blair C., Trigo, Ricardo M., Trotman, Adrian, Tschudi, M., Wal, Roderik S. W., Werf, Guido R., Vautard, Robert, Vazquez, J. L., Vieira, Goncalo, Vincent, Lucie, Vose, Russ S., Wagner, Wolfgang W., Wahr, John, Walsh, J., Wang Junhong, Wang Chunzai, Wang, M., Wang Sheng-Hung, Wang Lei, Wanninkhof, Rik, Weaver, Scott, Weber, Mark, Werdell, P. Jeremy, Whitewood, Robert, Wijffels, Susan, Wilber, Anne C., Wild, J. D., Willett, Kate M., Williams, W., Willis, Joshua K., Wolken, G., Wong, Takmeng, Woodgate, R., Worthy, D., Wouters, B., Wovrosh, Alex J., Xue Yan, Yamada, Ryuji, Yin Zungang, Yu Lisan, Zhang Liangying, Zhang Peiqun, Zhao Lin, Zhao, J., Zhong, W., Ziemke, Jerry, Zimmermann, S., ICOS-ATC (ICOS-ATC), Laboratoire des Sciences du Climat et de l'Environnement [Gif-sur-Yvette] (LSCE), Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ), Laboratoire d'Océanographie et du Climat : Expérimentations et Approches Numériques (LOCEAN), Institut de Recherche pour le Développement (IRD)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Muséum national d'Histoire naturelle (MNHN)-Institut Pierre-Simon-Laplace (IPSL (FR_636)), École normale supérieure - Paris (ENS Paris), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris Diderot - Paris 7 (UPD7)-École polytechnique (X)-Centre National d'Études Spatiales [Toulouse] (CNES)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-École normale supérieure - Paris (ENS Paris), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris Diderot - Paris 7 (UPD7)-École polytechnique (X)-Centre National d'Études Spatiales [Toulouse] (CNES)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS), Extrèmes : Statistiques, Impacts et Régionalisation (ESTIMR), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS), Muséum national d'Histoire naturelle (MNHN)-Institut de Recherche pour le Développement (IRD)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Institut Pierre-Simon-Laplace (IPSL (FR_636)), École normale supérieure - Paris (ENS-PSL), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris Diderot - Paris 7 (UPD7)-École polytechnique (X)-Centre National d'Études Spatiales [Toulouse] (CNES)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-École normale supérieure - Paris (ENS-PSL), and Repositório da Universidade de Lisboa

Subjects
[SDU.OCEAN]Sciences of the Universe [physics]/Ocean, Atmosphere, Atmospheric Science, 13. Climate action, Photosynthetically active radiation, Climate, Dynamics (mechanics), Data_FILES, Environmental science, Fraction (chemistry), 14. Life underwater, [SDU.ENVI]Sciences of the Universe [physics]/Continental interfaces, environment, Remote sensing
Abstract

For the first time in serveral years, the El Nino-Southern Oscillation did not dominate regional climate conditions around the globe. A weak La Ni a dissipated to ENSOneutral conditions by spring, and while El Nino appeared to be emerging during summer, this phase never fully developed as sea surface temperatures in the eastern conditions. Nevertheless, other large-scale climate patterns and extreme weather events impacted various regions during the year. A negative phase of the Arctic Oscillation from mid-January to early February contributed to frigid conditions in parts of northern Africa, eastern Europe, and western Asia. A lack of rain during the 2012 wet season led to the worst drought in at least the past three decades for northeastern Brazil. Central North America also experienced one of its most severe droughts on record. The Caribbean observed a very wet dry season and it was the Sahel's wettest rainy season in 50 years. Overall, the 2012 average temperature across global land and ocean surfaces ranked among the 10 warmest years on record. The global land surface temperature alone was also among the 10 warmest on record. In the upper atmosphere, the average stratospheric temperature was record or near-record cold, depending on the dataset. After a 30-year warming trend from 1970 to 1999 for global sea surface temperatures, the period 2000-12 had little further trend. This may be linked to the prevalence of La Ni a-like conditions during the 21st century. Heat content in the upper 700 m of the ocean remained near record high levels in 2012. Net increases from 2011 to 2012 were observed at 700-m to 2000-m depth and even in the abyssal ocean below. Following sharp decreases in to the effects of La Ni a, sea levels rebounded to reach records highs in 2012. The increased hydrological cycle seen in recent years continued, with more evaporation in drier locations and more precipitation in rainy areas. In a pattern that has held since 2004, salty areas of the ocean surfaces and subsurfaces were anomalously salty on average, while fresher areas were anomalously fresh. Global tropical cyclone activity during 2012 was near average, with a total of 84 storms compared with the 1981-2010 average of 89. Similar to 2010 and 2011, the North Atlantic was the only hurricane basin that experienced above-normal activity. In this basin, Sandy brought devastation to Cuba and parts of the eastern North American seaboard. All other basins experienced either near-or below-normal tropical cyclone activity. Only three tropical cyclones reached Category 5 intensity-all in Bopha became the only storm in the historical record to produce winds greater than 130 kt south of 7 N. It was also the costliest storm to affect the Philippines and killed more than 1000 residents. Minimum Arctic sea ice extent in September and Northern Hemisphere snow cover extent in June both reached new record lows. June snow cover extent is now declining at a faster rate (-17.6% per decade) than September sea ice extent (-13.0% per decade). Permafrost temperatures reached record high values in northernmost Alaska. A new melt extent record occurred on 11-12 July on the Greenland ice sheet; 97% of the ice sheet showed some form of melt, four times greater than the average melt for this time of year. The climate in Antarctica was relatively stable overall. The largest maximum sea ice extent since records begain in 1978 was observed in September 2012. In the stratosphere, warm air led to the second smallest ozone hole in the past two decades. Even so, the springtime ozone layer above Antarctica likely will not return to its early 1980s state until about 2060. Following a slight decline associated with the global 2 emissions from fossil fuel combustion and cement production reached a record 9.5 +/- 0.5 Pg C in 2011 and a new record of 9.7 +/- 0.5 Pg C is estimated for 2012. Atmospheric CO2 concentrations increased by 2.1 ppm in 2012, to 392.6 ppm. In spring 2012, 2 concentration exceeded 400 ppm at 7 of the 13 Arctic observation sites. Globally, other greenhouse gases including methane and nitrous oxide also continued to rise in concentration and the combined effect now represents a 32% increase in radiative forcing over a 1990 baseline. Concentrations of most ozone depleting substances continued to fall.

Published
2013
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4. State of the Climate in 2012 INTRODUCTION

Author

Achberger, Christine, Ackerman, Stephen A., Albanil, Adelina, Alexander, P., Alfaro, Eric J., Allan, Rob, Alves, Lincoln M., Amador, Jorge A., Ambenje, Peter, Andrianjafinirina, Solonomenjanahary, Antonov, John, Aravequia, Jose A., Arendt, A., Arevalo, Juan, Arndt, Derek S., Ashik, I., Atheru, Zachary, Banzon, Viva, Baringer, Molly O., Barreira, Sandra, Barriopedro, David E., Beard, Grant, Becker, Andreas, Behrenfeld, Michael J., Bell, Gerald D., Benedetti, Angela, Bernhard, Germar, Berrisford, Paul, Berry, David I., Bhatt, U., Bidegain, Mario, Bindoff, Nathan, Bissolli, Peter, Blake, Eric S., Blunden, Jessica, Booneeady, Raj, Bosilovich, Michael, Box, J. E., Boyer, Tim, Braathen, Geir O., Bromwich, David H., Brown, R., Brown, L., Bruhwiler, Lori, Bulygina, Olga N., Burgess, D., Burrows, John, Calderon, Blanca, Camargo, Suzana J., Campbell, Jayaka, Cao, Y., Cappelen, J., Carrasco, Gualberto, Chambers, Don P., Chang A, L., Chappell, Petra, Chehade, Wissam, Cheliah, Muthuvel, Christiansen, Hanne H., Christy, John R., Ciais, Phillipe, Coelho, Caio A. S., Cogley, J. G., Colwell, Steve, Cross, J. N., Crouch, Jake, Cunningham, Stuart A., Dacic, Milan, Jeu, Richard A. M., Dekaa, Francis S., Demircan, Mesut, Derksen, C., Diamond, Howard J., Dlugokencky, Ed J., Dohan, Kathleen, Dolman, A. Johannes, Domingues, Catia M., Dong Shenfu, Dorigo, Wouter A., Drozdov, D. S., Duguay, Claude R., Dunn, Robert J. H., Duran-Quesada, Ana M., Dutton, Geoff S., Ehmann, Christian, Elkins, James W., Euscategui, Christian, Famiglietti, James S., Fang Fan, Fauchereau, Nicolas, Feely, Richard A., Fekete, Balazs M., Fenimore, Chris, Fioletov, Vitali E., Fogarty, Chris T., Fogt, Ryan L., Folland, Chris K., Foster, Michael J., Frajka-Williams, Eleanor, Franz, Bryan A., Frith, Stacey H., Frolov, I., Ganter, Catherine, Garzoli, Silvia, Geai, M. -L, Gerland, S., Gitau, Wilson, Gleason, Karin L., Gobron, Nadine, Goldenberg, Stanley B., Goni, Gustavo, Good, Simon A., Gottschalck, Jonathan, Gregg, Margarita C., Griffiths, Georgina, Grooss, Jens-Uwe, Guard, Charles Chip, Gupta, Shashi K., Hall, Bradley D., Halpert, Michael S., Harada, Yayoi, Hauri, C., Heidinger, Andrew K., Heikkila, Anu, Heim, Richard R., Heimbach, Patrick, Hidalgo, Hugo G., Hilburn, Kyle, Ho, Shu-Peng, Hobbs, Will R., Holgate, Simon, Hovsepyan, Anahit, Hu Zeng-Zhen, Hughes, P., Hurst, Dale F., Ingvaldsen, R., Inness, Antje, Jaimes, Ena, Jakobsson, Martin, James, Adamu I., Jeffries, Martin O., Johns, William E., Johnsen, Bjorn, Johnson, Gregory C., Johnson, Bryan, Jones, Luke T., Jumaux, Guillaume, Kabidi, Khadija, Kaiser, Johannes W., Kamga, Andre, Kang, Kyun-Kuk, Kanzow, Torsten O., Kao, Hsun-Ying, Keller, Linda M., Kennedy, John J., Key, J., Khatiwala, Samar, Pour, H. Kheyrollah, Kholodov, A. L., Khoshkam, Mahbobeh, Kijazi, Agnes, Kikuchi, T., Kim, B. -M, Kim, S. -J, Kimberlain, Todd B., Knaff, John A., Korshunova, Natalia N., Koskela, T., Kousky, Vernon E., Kramarova, Natalya, Kratz, David P., Krishfield, R., Kruger, Andries, Kruk, Michael C., Kumar, Arun, Lagerloef, Gary S. E., Lakkala, K., Lander, Mark A., Landsea, Chris W., Lankhorst, Matthias, Laurila, T., Lazzara, Matthew A., Lee, Craig, Leuliette, Eric, Levitus, Sydney, L Heureux, Michelle, Lieser, Jan, Lin, I-I, Liu, Y. Y., Liu, Y., Liu Hongxing, Liu Yanju, Lobato-Sanchez, Rene, Locarnini, Ricardo, Loeb, Norman G., Loeng, H., Long, Craig S., Lorrey, Andrew M., Luhunga, P., Lumpkin, Rick, Luo Jing-Jia, Lyman, John M., Macdonald, Alison M., Maddux, Brent C., Malekela, C., Manney, Gloria, Marchenko, S. S., Marengo, Jose A., Marotzke, Jochem, Marra, John J., Martinez-Gueingla, Rodney, Massom, Robert A., Mathis, Jeremy T., Mcbride, Charlotte, Mccarthy, Gerard, Mcvicar, Tim R., Mears, Carl, Meier, W., Meinen, Christopher S., Menendez, Melisa, Merrifield, Mark A., Mitchard, Edward, Mitchum, Gary T., Montzka, Stephen A., Morcrette, Jean-Jacques, Mote, Thomas, Muehle, Jens, Muehr, Bernhard, Mullan, A. Brett, Mueller, Rolf, Nash, Eric R., Nerem, R. Steven, Newlin, Michele L., Newman, Paul A., Ng Ongolo, H., Nieto, Juan Jose, Nishino, S., Nitsche, Helga, Noetzli, Jeannette, Oberman, N. G., Obregon, Andre, Ogallo, Laban A., Oludhe, Christopher S., Omar, Mohamed I., Overland, James, Oyunjargal, Lamjav, Parinussa, Robert M., Park, Geun-Ha, Park, E-Hyung, Parker, David, Pasch, Richard J., Pascual-Ramirez, Reynaldo, Pelto, Mauri S., Penalba, Olga, Peng, L., Perovich, Don K., Pezza, Alexandre B., Phillips, David, Pickart, R., Pinty, Bernard, Pitts, Michael C., Purkey, Sarah G., Quegan, Shaun, Quintana, Juan, Rabe, B., Rahimzadeh, Fatemeh, Raholijao, Nirivololona, Raiva, I., Rajeevan, Madhavan, Ramiandrisoa, Voahanginirina, Ramos, Alexandre, Ranivoarissoa, Sahondra, Rayner, Nick A., Rayner, Darren, Razuveav, Vyacheslav N., Reagan, James, Reid, Phillip, Renwick, James, Revedekar, Jayashree, Richter-Menge, Jacqueline, Rivera, Ingrid L., Robinson, David A., Rodell, Matthew, Romanovsky, Vladimir E., Ronchail, Josyane, Karen Rosenlof, Sabine, Christopher L., Salvador, Mozar A., Sanchez-Lugo, Ahira, Santee, Michelle L., Sasgen, I., Sawaengphokhai, P., Sayouri, Amal, Scambos, Ted A., Schauer, U., Schemm, Jae, Schlosser, P., Schmid, Claudia, Schreck, Carl, Semiletov, Igor, Send, Uwe, Sensoy, Serhat, Setzer, Alberto, Severinghaus, Jeffrey, Shakhova, Natalia, Sharp, M., Shiklomanov, Nicolai I., Siegel, David A., Silva, Viviane B. 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5. Harmonisation of the GOME, SCIAMACHY, and GOME-2 total ozone data records for a better understanding of long-term trends and their causes

Author

Chehade, Wissam and Chehade, Wissam

Abstract

This thesis addresses the issue of the accurate measurements of ozone distributions in the atmosphere obtained from different satellite borne atmospheric chemistry spectrometers which represent a major need and pre-requisite for determining whether the atmospheric burden of ozone depleting substances (ODS) are reduced in accordance to the Montreal Protocol, and valuable for long-term trend analysis to detect a subsequent ozone recovery. A consolidated and homogeneous long term dataset requires a careful analysis of the relevant parameters used in the retrievals, one important parameter is the absorption cross section. This work presents the procedures followed to correct the ozone cross section data of SCIAMACHY and GOME-2 spectrometers starting from original raw data (optical density spectra). Using the available versions of SCIAMACHY and GOME-2 FM cross sections in the retrieval of total ozone from each satellite leads to an overestimation in the total ozone by 3-5% and 8-9% compared to collocated GOME data, respectively. The quality of the revised temperature-dependent ozone absorption cross sections is investigated over GOME-2 and SCIAMACHY's entire spectral range. The revised data agree well within 3% with other published ozone cross sections and preserve the correct temperature dependence in the Hartley, Huggins, Chappuis and Wulf bands as displayed by the literature data. SCIAMACHY's total ozone columns retrieved using the revised cross section data are shown to be within 1% compared to the ozone amounts retrieved routinely from SCIAMACHY, which uses Bogumil et al. (2003) data but adjusted with a scaling factor of 5.3% and a wavelength shift of 0.08 nm. The total ozone column retrieved from the GOME-2/MetOp-A satellite using the new cross section data is within 1% compared to the ozone amounts retrieved from the standard retrieval performed for GOME-2. The study also presents a long term statistical trend analysis of total ozone datasets obtained from various

6. Harmonisation of the GOME, SCIAMACHY, and GOME-2 total ozone data records for a better understanding of long-term trends and their causes

Author

Chehade, Wissam and Chehade, Wissam

Abstract

This thesis addresses the issue of the accurate measurements of ozone distributions in the atmosphere obtained from different satellite borne atmospheric chemistry spectrometers which represent a major need and pre-requisite for determining whether the atmospheric burden of ozone depleting substances (ODS) are reduced in accordance to the Montreal Protocol, and valuable for long-term trend analysis to detect a subsequent ozone recovery. A consolidated and homogeneous long term dataset requires a careful analysis of the relevant parameters used in the retrievals, one important parameter is the absorption cross section. This work presents the procedures followed to correct the ozone cross section data of SCIAMACHY and GOME-2 spectrometers starting from original raw data (optical density spectra). Using the available versions of SCIAMACHY and GOME-2 FM cross sections in the retrieval of total ozone from each satellite leads to an overestimation in the total ozone by 3-5% and 8-9% compared to collocated GOME data, respectively. The quality of the revised temperature-dependent ozone absorption cross sections is investigated over GOME-2 and SCIAMACHY's entire spectral range. The revised data agree well within 3% with other published ozone cross sections and preserve the correct temperature dependence in the Hartley, Huggins, Chappuis and Wulf bands as displayed by the literature data. SCIAMACHY's total ozone columns retrieved using the revised cross section data are shown to be within 1% compared to the ozone amounts retrieved routinely from SCIAMACHY, which uses Bogumil et al. (2003) data but adjusted with a scaling factor of 5.3% and a wavelength shift of 0.08 nm. The total ozone column retrieved from the GOME-2/MetOp-A satellite using the new cross section data is within 1% compared to the ozone amounts retrieved from the standard retrieval performed for GOME-2. The study also presents a long term statistical trend analysis of total ozone datasets obtained from various

7. Harmonisation of the GOME, SCIAMACHY, and GOME-2 total ozone data records for a better understanding of long-term trends and their causes

Author

Chehade, Wissam and Chehade, Wissam

Abstract

This thesis addresses the issue of the accurate measurements of ozone distributions in the atmosphere obtained from different satellite borne atmospheric chemistry spectrometers which represent a major need and pre-requisite for determining whether the atmospheric burden of ozone depleting substances (ODS) are reduced in accordance to the Montreal Protocol, and valuable for long-term trend analysis to detect a subsequent ozone recovery. A consolidated and homogeneous long term dataset requires a careful analysis of the relevant parameters used in the retrievals, one important parameter is the absorption cross section. This work presents the procedures followed to correct the ozone cross section data of SCIAMACHY and GOME-2 spectrometers starting from original raw data (optical density spectra). Using the available versions of SCIAMACHY and GOME-2 FM cross sections in the retrieval of total ozone from each satellite leads to an overestimation in the total ozone by 3-5% and 8-9% compared to collocated GOME data, respectively. The quality of the revised temperature-dependent ozone absorption cross sections is investigated over GOME-2 and SCIAMACHY's entire spectral range. The revised data agree well within 3% with other published ozone cross sections and preserve the correct temperature dependence in the Hartley, Huggins, Chappuis and Wulf bands as displayed by the literature data. SCIAMACHY's total ozone columns retrieved using the revised cross section data are shown to be within 1% compared to the ozone amounts retrieved routinely from SCIAMACHY, which uses Bogumil et al. (2003) data but adjusted with a scaling factor of 5.3% and a wavelength shift of 0.08 nm. The total ozone column retrieved from the GOME-2/MetOp-A satellite using the new cross section data is within 1% compared to the ozone amounts retrieved from the standard retrieval performed for GOME-2. The study also presents a long term statistical trend analysis of total ozone datasets obtained from various

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