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28 results on '"D. Quénard"'

1. Chemical modelling of complex organic molecules with peptide-like bonds in star-forming regions

Author: Jonathan Holdship, Audrey Coutens, Izaskun Jiménez-Serra, Serena Viti, D. Quénard, AMOR 2017, Laboratoire d'Astrophysique de Bordeaux [Pessac] (LAB), and Université de Bordeaux (UB)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Bordeaux (UB)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)
Subjects: chemistry.chemical_classification, Physics, Astrochemistry, [SDU.ASTR.CO]Sciences of the Universe [physics]/Astrophysics [astro-ph]/Cosmology and Extra-Galactic Astrophysics [astro-ph.CO], 010308 nuclear & particles physics, FOS: Physical sciences, Astronomy and Astrophysics, Peptide, Activation energy, Star (graph theory), Astrophysics - Astrophysics of Galaxies, 01 natural sciences, Amino acid, Interstellar medium, Astrophysics - Solar and Stellar Astrophysics, chemistry, Space and Planetary Science, Computational chemistry, Astrophysics of Galaxies (astro-ph.GA), 0103 physical sciences, Molecule, Peptide bond, 010303 astronomy & astrophysics, Solar and Stellar Astrophysics (astro-ph.SR)
Abstract: Peptide bonds (N-C=O) play a key role in metabolic processes since they link amino acids into peptide chains or proteins. Recently, several molecules containing peptide-like bonds have been detected across multiple environments in the interstellar medium (ISM), growing the need to fully understand their chemistry and their role in forming larger pre-biotic molecules. We present a comprehensive study of the chemistry of three molecules containing peptide-like bonds: HNCO, NH$_2$CHO, and CH$_3$NCO. We also included other CHNO isomers (HCNO, HOCN), and C$_2$H$_3$NO isomers (CH$_3$OCN, CH$_3$CNO) to the study. We have used the \uclchem gas-grain chemical code and included in our chemical network all possible formation/destruction pathways of these peptide-like molecules recently investigated either by theoretical calculations or in laboratory experiments. Our predictions are compared to observations obtained toward the proto-star IRAS16293$-$2422 and the L1544 pre-stellar core. Our results show that some key reactions involving the CHNO and C$_2$H$_3$NO isomers need to be modified to match the observations. Consistently with recent laboratory findings, hydrogenation is unlikely to produce NH$_2$CHO on grain surfaces, while a combination of radical-radical surface reactions and gas-phase reactions is a better alternative. In addition, better results are obtained for NH$_2$CHO when a slightly higher activation energy of 25$\,$K is considered for the gas-phase reaction $\rm NH_2 + H_2CO \rightarrow NH_2CHO + H$. Finally, our modelling shows that the observed correlation between NH$_2$CHO and HNCO in star-forming regions may come from the fact that HNCO and NH$_2$CHO react to temperature in the same manner rather than from a direct chemical link between the two species., 18 pages, 5 figures, accepted for publication in MNRAS
Published: 2017
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2. Detection of methyl isocyanate (CH3NCO) in a solar-type protostar

Author: Leonardo Testi, R. Martín-Doménech, Victor M. Rivilla, D. Quénard, Jesús Martín-Pintado, and Izaskun Jiménez-Serra
Subjects: Physics, Range (particle radiation), 010308 nuclear & particles physics, Thermodynamic equilibrium, Abundance (chemistry), Comet, Analytical chemistry, FOS: Physical sciences, Astronomy and Astrophysics, Excitation temperature, Methyl isocyanate, 01 natural sciences, chemistry.chemical_compound, Astrophysics - Solar and Stellar Astrophysics, chemistry, Space and Planetary Science, 0103 physical sciences, Molecule, Protostar, Atomic physics, 010303 astronomy & astrophysics, Solar and Stellar Astrophysics (astro-ph.SR)
Abstract: We report the detection of the prebiotic molecule CH3NCO in a solar-type protostar, IRAS16293-2422 B. A significant abundance of this species on the surface of the comet 67P/Churyumov-Gerasimenko has been proposed, and it has recently been detected in hot cores around high-mass protostars. We observed IRAS16293-2422 B with ALMA in the 90 GHz to 265 GHz range, and detected 8 unblended transitions of CH3NCO. From our Local Thermodynamic Equilibrium analysis we derived an excitation temperature of 110+-19 K and a column density of (4.0+-0.3)x10^15 cm^-2 , which results in an abundance of
Published: 2017
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3. Seeds of Life in Space (SOLIS)

Author: C. Favre, C. Vastel, I. Jimenez-Serra, D. Quénard, P. Caselli, C. Ceccarelli, A. Chacón-Tanarro, F. Fontani, J. Holdship, Y. Oya, A. Punanova, N. Sakai, S. Spezzano, S. Yamamoto, R. Neri, A. López-Sepulcre, F. Alves, R. Bachiller, N. Balucani, E. Bianchi, L. Bizzocchi, C. Codella, E. Caux, M. De Simone, J. Enrique Romero, F. Dulieu, S. Feng, A. Jaber Al-Edhari, B. Lefloch, and J. Ospina-Zamudio
Published: 2020
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4. Modelling the 3D physical structure of astrophysical sources with gass

Author: Sandrine Bottinelli, Emmanuel Caux, D. Quénard, Institut de recherche en astrophysique et planétologie (IRAP), Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), and Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS)
Subjects: FOS: Physical sciences, 01 natural sciences, methods: numerical, Theoretical physics, Complex geometry, Physical structure, 0103 physical sciences, Radiative transfer, Code (cryptography), Instrumentation and Methods for Astrophysics (astro-ph.IM), 010303 astronomy & astrophysics, Solar and Stellar Astrophysics (astro-ph.SR), Astrophysics::Galaxy Astrophysics, Graphical user interface, Physics, [SDU.ASTR]Sciences of the Universe [physics]/Astrophysics [astro-ph], Molecular line, 010308 nuclear & particles physics, business.industry, Astronomy and Astrophysics, Grid, Astrophysics - Astrophysics of Galaxies, ISM: molecules, Computational physics, Interferometry, Astrophysics - Solar and Stellar Astrophysics, radiative transfer, [SDU]Sciences of the Universe [physics], Space and Planetary Science, Astrophysics of Galaxies (astro-ph.GA), Astrophysics - Instrumentation and Methods for Astrophysics, business
Abstract: International audience; The era of interferometric observations leads to the need of a more and more precise description of physical structures and dynamics of star-forming regions, from pre-stellar cores to protoplanetary discs. The molecular emission can be traced in multiple physical components such as infalling envelopes, outflows and protoplanetary discs. To compare with the observations, a precise and complex radiative transfer modelling of these regions is needed. We present gass (Generator of Astrophysical Sources Structure), a code that allows us to generate the three-dimensional (3D) physical structure model of astrophysical sources. From the gass graphical interface, the user easily creates different components such as spherical envelopes, outflows and discs. The physical properties of these components are modelled thanks to dedicated graphical interfaces that display various figures in order to help the user and facilitate the modelling task. For each component, the code randomly generates points in a 3D grid with a sample probability weighted by the molecular density. The created models can be used as the physical structure input for 3D radiative transfer codes to predict the molecular line or continuum emission. An analysis of the output hyper-spectral cube given by such radiative transfer code can be made directly in gass using the various post-treatment options implemented, such as calculation of moments or convolution with a beam. This makes gass well suited to model and analyse both interferometric and single-dish data. This paper is focused on the results given by the association of gass and lime, a 3D radiative transfer code, and we show that the complex geometry observed in star-forming regions can be adequately handled by gass+lime.
Published: 2017
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5. First detection of the pre-biotic molecule glycolonitrile (HOCH2CN) in the interstellar medium

Author: Rafa Martin-Domenech, Leonardo Testi, Jesús Martín-Pintado, D. Quénard, Shaoshan Zeng, Izaskun Jiménez-Serra, and Victor M. Rivilla
Subjects: Glycolonitrile, Physics, 010308 nuclear & particles physics, Abundance (chemistry), Pre biotic, FOS: Physical sciences, Astronomy and Astrophysics, Astrophysics, Astrophysics - Astrophysics of Galaxies, 01 natural sciences, Molecular physics, Interstellar medium, chemistry.chemical_compound, Astrophysics - Solar and Stellar Astrophysics, chemistry, 13. Climate action, Space and Planetary Science, Ionization, Astrophysics of Galaxies (astro-ph.GA), 0103 physical sciences, Protostar, Molecule, 010303 astronomy & astrophysics, Solar and Stellar Astrophysics (astro-ph.SR), Envelope (waves)
Abstract: Theories of a pre-RNA world suggest that glycolonitrile (HOCH$_2$CN) is a key species in the process of ribonucleotide assembly, which is considered as a molecular precursor of nucleic acids. In this Letter, we report the first detection of this pre-biotic molecule in the interstellar medium (ISM) by using ALMA data obtained at frequencies between 86.5$\,$GHz and 266.5$\,$GHz toward the Solar-type protostar IRAS16293-2422 B. A total of 15 unblended transitions of HOCH$_2$CN were identified. Our analysis indicates the presence of a cold (T$\rm _{ex}$=24$\pm$8$\,$K) and a warm (T$\rm _{ex}$=158$\pm$38$\,$K) component meaning that this molecule is present in both the inner hot corino and the outer cold envelope of IRAS16293 B. The relative abundance with respect to H$_2$ is (6.5$\pm$0.6)$\times$10$^{-11}$ and $\geq$(6$\pm$2)$\times$10$^{-10}$ for the warm and cold components respectively. Our chemical modelling seems to underproduce the observed abundance for both the warm and cold component under various values of the cosmic-ray ionisation rate ($\zeta$). Key gas phase routes for the formation of this molecule might be missing in our chemical network., Comment: 5 pages, 4 figures, 2 tables, accepted in Monthly Notices of the Royal Astronomical Society Letters
Published: 2019
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6. Astrochemical evolution along star formation: overview of the IRAM Large Program ASAI

Author: E. Mendoza, Emmanuel Caux, José Cernicharo, Cécile Favre, Serena Viti, Kento Yoshida, Charlotte Vastel, Ana López-Sepulcre, Sylvie Cabrit, A. Fuente, E. Bianchi, Rafael Bachiller, Bertrand Lefloch, E. Roueff, Jonathan Holdship, Linda Podio, M. González-García, Cecilia Ceccarelli, Satoshi Yamamoto, T. Monfredini, Claudio Codella, A. I. Gómez-Ruiz, Nami Sakai, Nuria Marcelino, D. Quénard, Claudine Kahane, J. Ospina-Zamudio, Heloisa M. Boechat-Roberty, Mario Tafalla, Heidy M Quitián-Lara, Institut de Planétologie et d'Astrophysique de Grenoble (IPAG), Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Observatoire des Sciences de l'Univers de Grenoble (OSUG ), Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national des sciences de l'Univers (INSU - CNRS)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019]), Instituto de Ciencia de Materiales de Madrid (ICMM), Consejo Superior de Investigaciones Científicas [Madrid] (CSIC), foreign laboratories (FL), CERN [Genève], Univ Toulouse UPS, Ctr Etud Spatiale Rayonnements, F-31062 Toulouse 9, France, Centre Etud Spatiale Rayonnements Toulouse, Centre d'étude spatiale des rayonnements (CESR), Observatoire Midi-Pyrénées (OMP), Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Toulouse III - Paul Sabatier (UT3), Université Fédérale Toulouse Midi-Pyrénées, Instituto de Radio Astronomía Milimétrica, University College of London [London] (UCL), Centro de Investigaciones Energéticas Medioambientales y Tecnológicas [Madrid] (CIEMAT), INAF - Osservatorio Astrofisico di Arcetri (OAA), Istituto Nazionale di Astrofisica (INAF), Laboratoire d'Etude du Rayonnement et de la Matière en Astrophysique (LERMA (UMR_8112)), Sorbonne Université (SU)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Cergy Pontoise (UCP), Université Paris-Seine-Université Paris-Seine-Observatoire de Paris, Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL), Institut de biologie et chimie des protéines [Lyon] (IBCP), Université Claude Bernard Lyon 1 (UCBL), Université de Lyon-Université de Lyon-Centre National de la Recherche Scientifique (CNRS), Division of Clinical and Molecular Genetics, Shinshu University Hospital, Institut de Mathématiques de Jussieu (IMJ), Université Pierre et Marie Curie - Paris 6 (UPMC)-Université Paris Diderot - Paris 7 (UPD7)-Centre National de la Recherche Scientifique (CNRS), INAF - Osservatorio Astronomico di Bologna (OABO), Laboratoire d'Astrophysique de Grenoble (LAOG), Université Joseph Fourier - Grenoble 1 (UJF)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS), Consejo Superior de Investigaciones Científicas [Spain] (CSIC), Centre National d'Études Spatiales [Toulouse] (CNES)-Université Grenoble Alpes (UGA)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire des Sciences de l'Univers de Grenoble (OSUG), Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Joseph Fourier - Grenoble 1 (UJF)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes (UGA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Joseph Fourier - Grenoble 1 (UJF)-Centre National de la Recherche Scientifique (CNRS), Université Toulouse III - Paul Sabatier (UT3), Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS), Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, PSL Research University (PSL)-PSL Research University (PSL)-Université de Cergy Pontoise (UCP), Université Paris-Seine-Université Paris-Seine-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS), and Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université de Cergy Pontoise (UCP)
Subjects: Physics, [PHYS]Physics [physics], Solar System, Astrochemistry, 010308 nuclear & particles physics, Star formation, FOS: Physical sciences, Astronomy and Astrophysics, Astrophysics, 01 natural sciences, Astrophysics - Astrophysics of Galaxies, Article, Stars, 13. Climate action, Space and Planetary Science, Asteroid, Astrophysics of Galaxies (astro-ph.GA), 0103 physical sciences, Formation and evolution of the Solar System, [PHYS.ASTR]Physics [physics]/Astrophysics [astro-ph], 010303 astronomy & astrophysics, Chemical composition, ComputingMilieux_MISCELLANEOUS, Line (formation)
Abstract: Evidence is mounting that the small bodies of our Solar System, such as comets and asteroids, have at least partially inherited their chemical composition from the first phases of the Solar System formation. It then appears that the molecular complexity of these small bodies is most likely related to the earliest stages of star formation. It is therefore important to characterize and to understand how the chemical evolution changes with solar-type protostellar evolution. We present here the Large Program "Astrochemical Surveys At IRAM" (ASAI). Its goal is to carry out unbiased millimeter line surveys between 80 and 272 GHz of a sample of ten template sources, which fully cover the first stages of the formation process of solar-type stars, from prestellar cores to the late protostellar phase. In this article, we present an overview of the surveys and results obtained from the analysis of the 3 mm band observations. The number of detected main isotopic species barely varies with the evolutionary stage and is found to be very similar to that of massive star-forming regions. The molecular content in O- and C- bearing species allows us to define two chemical classes of envelopes, whose composition is dominated by either a) a rich content in O-rich complex organic molecules, associated with hot corino sources, or b) a rich content in hydrocarbons, typical of Warm Carbon Chain Chemistry sources. Overall, a high chemical richness is found to be present already in the initial phases of solar-type star formation., 19 pages, 7 figures, 5 Tables
Published: 2018
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7. Sulphur chemistry in the L1544 pre-stellar core

Author: Thomas H. G. Vidal, Valentine Wakelam, Rafael Bachiller, R. Le Gal, A. Andrianasolo, Charlotte Vastel, Cecilia Ceccarelli, Bertrand Lefloch, D. Quénard, Paola Caselli, Institut de recherche en astrophysique et planétologie (IRAP), Université Toulouse III - Paul Sabatier (UT3), Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées-Observatoire Midi-Pyrénées (OMP), Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS), AMOR 2018, Laboratoire d'Astrophysique de Bordeaux [Pessac] (LAB), Université de Bordeaux (UB)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Bordeaux (UB)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS), Institut de Planétologie et d'Astrophysique de Grenoble (IPAG), Centre National d'Études Spatiales [Toulouse] (CNES)-Université Grenoble Alpes (UGA)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire des Sciences de l'Univers de Grenoble (OSUG), Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Joseph Fourier - Grenoble 1 (UJF)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes (UGA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Joseph Fourier - Grenoble 1 (UJF)-Centre National de la Recherche Scientifique (CNRS), Institut de recherche en astrophysique et planétologie ( IRAP ), Université Paul Sabatier - Toulouse 3 ( UPS ) -Observatoire Midi-Pyrénées ( OMP ) -Centre National de la Recherche Scientifique ( CNRS ), Laboratoire d'Astrophysique de Bordeaux [Pessac] ( LAB ), Université de Bordeaux ( UB ) -Institut national des sciences de l'Univers ( INSU - CNRS ) -Centre National de la Recherche Scientifique ( CNRS ) -Université de Bordeaux ( UB ) -Institut national des sciences de l'Univers ( INSU - CNRS ) -Centre National de la Recherche Scientifique ( CNRS ), Institut de Planétologie et d'Astrophysique de Grenoble ( IPAG ), Observatoire des Sciences de l'Univers de Grenoble ( OSUG ), Université Joseph Fourier - Grenoble 1 ( UJF ) -Institut national des sciences de l'Univers ( INSU - CNRS ) -Centre National de la Recherche Scientifique ( CNRS ) -Université Grenoble Alpes ( UGA ) -Université Joseph Fourier - Grenoble 1 ( UJF ) -Institut national des sciences de l'Univers ( INSU - CNRS ) -Centre National de la Recherche Scientifique ( CNRS ) -Université Grenoble Alpes ( UGA ) -Centre National de la Recherche Scientifique ( CNRS ), Institut national des sciences de l'Univers (INSU - CNRS)-Université Toulouse III - Paul Sabatier (UT3), Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Centre National de la Recherche Scientifique (CNRS), Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Observatoire des Sciences de l'Univers de Grenoble (OSUG ), and Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national des sciences de l'Univers (INSU - CNRS)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019])
Subjects: Physics, [ PHYS.ASTR.SR ] Physics [physics]/Astrophysics [astro-ph]/Solar and Stellar Astrophysics [astro-ph.SR], Line-of-sight, Astrochemistry, 010308 nuclear & particles physics, Thermal desorption, FOS: Physical sciences, Astronomy and Astrophysics, Astrophysics, [ PHYS.ASTR.CO ] Physics [physics]/Astrophysics [astro-ph]/Cosmology and Extra-Galactic Astrophysics [astro-ph.CO], [PHYS.ASTR.SR]Physics [physics]/Astrophysics [astro-ph]/Solar and Stellar Astrophysics [astro-ph.SR], 01 natural sciences, Astrophysics - Astrophysics of Galaxies, Ion, Isotopomers, [PHYS.ASTR.CO]Physics [physics]/Astrophysics [astro-ph]/Cosmology and Extra-Galactic Astrophysics [astro-ph.CO], Pre-stellar core, Astrophysics - Solar and Stellar Astrophysics, Space and Planetary Science, Abundance (ecology), Astrophysics of Galaxies (astro-ph.GA), 0103 physical sciences, Radiative transfer, 010303 astronomy & astrophysics, Solar and Stellar Astrophysics (astro-ph.SR)
Abstract: The L1544 pre-stellar core has been observed as part of the ASAI IRAM 30m Large Program as well as follow-up programs. These observations have revealed the chemical richness of the earliest phases of low-mass star-forming regions. In this paper we focus on the twenty-one sulphur bearing species (ions, isotopomers and deuteration) that have been detected in this spectral-survey through fifty one transitions: CS, CCS, C3S, SO, SO2, H2CS, OCS, HSCN, NS, HCS+, NS+ and H2S. We also report the tentative detection (4 {\sigma} level) for methyl mercaptan (CH3SH). LTE and non-LTE radiative transfer modelling have been performed and we used the nautilus chemical code updated with the most recent chemical network for sulphur to explain our observations. From the chemical modelling we expect a strong radial variation for the abundances of these species, which mostly are emitted in the external layer where non thermal desorption of other species has previously been observed. We show that the chemical study cannot be compared to what has been done for the TMC-1 dark cloud, where the abundance is supposed constant along the line of sight, and conclude that a strong sulphur depletion is necessary to fully reproduce our observations of the prototypical pre-stellar core L1544., Comment: Accepted in MNRAS 2018 May 15. Received 2018 May 15; in original form 2018 January 30
Published: 2018
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8. 3D modelling of HCO$^+$ and its isotopologues in the low-mass proto-star IRAS16293$-$2422

Author: Emmanuel Caux, Valentine Wakelam, Sandrine Bottinelli, D. Quénard, Institut de recherche en astrophysique et planétologie (IRAP), Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS), AMOR 2018, Laboratoire d'Astrophysique de Bordeaux [Pessac] (LAB), Université de Bordeaux (UB)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Bordeaux (UB)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS), Institut national des sciences de l'Univers (INSU - CNRS)-Université Toulouse III - Paul Sabatier (UT3), Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées-Observatoire Midi-Pyrénées (OMP), and Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Centre National de la Recherche Scientifique (CNRS)
Subjects: [SDU.ASTR.CO]Sciences of the Universe [physics]/Astrophysics [astro-ph]/Cosmology and Extra-Galactic Astrophysics [astro-ph.CO], Star (game theory), FOS: Physical sciences, Astrophysics::Cosmology and Extragalactic Astrophysics, 01 natural sciences, 7. Clean energy, 0103 physical sciences, Gravitational collapse, Astrophysics::Solar and Stellar Astrophysics, 010303 astronomy & astrophysics, Solar and Stellar Astrophysics (astro-ph.SR), Astrophysics::Galaxy Astrophysics, Line (formation), Envelope (waves), Physics, Degree (graph theory), 010308 nuclear & particles physics, Ambipolar diffusion, Star formation, Astronomy and Astrophysics, Astrophysics - Astrophysics of Galaxies, Astrophysics - Solar and Stellar Astrophysics, Space and Planetary Science, Astrophysics of Galaxies (astro-ph.GA), Atomic physics, Low Mass
Abstract: Ions and electrons play an important role in various stages of the star formation process. By following the magnetic field of their environment and interacting with neutral species, they slow down the gravitational collapse of the proto-star envelope. This process (known as ambipolar diffusion) depends on the ionisation degree, which can be derived from the \hco abundance. We present a study of \hco and its isotopologues (H$^{13}$CO$^+$, HC$^{18}$O$^+$, DCO$^+$, and H$^{13}$CO$^+$) in the low-mass proto-star IRAS16293$-$2422. The structure of this object is complex, and the HCO$^+$ emission arises from the contribution of a young NW-SE outflow, the proto-stellar envelope and the foreground cloud. We aim at constraining the physical parameters of these structures using all the observed transitions. For the young NW-SE outflow, we derive $T_{\rm kin}=180-220$ K and $n({\rm H_2})=(4-7)\times10^6$ cm$^{-3}$ with an HCO$^+$ abundance of $(3-5)\times10^{-9}$. Following previous studies, we demonstrate that the presence of a cold ($T_{\rm kin}$$\leqslant$30 K) and low density ($n({\rm H_2})\leqslant1\times10^4$ cm$^{-3}$) foreground cloud is also necessary to reproduce the observed line profiles. We have used the gas-grain chemical code \textsc{nautilus} to derive the HCO$^+$ abundance profile across the envelope and the external regions where X(HCO$^+$)$\gtrsim1\times10^{-9}$ dominate the envelope emission. From this, we derive an ionisation degree of $10^{-8.9}\,\lesssim\,x(e)\,\lesssim\,10^{-7.9}$. The ambipolar diffusion timescale is $\sim$5 times the free-fall timescale, indicating that the magnetic field starts to support the source against gravitational collapse and the magnetic field strength is estimated to be $6-46 \mu$G., Comment: 17 pages, 10 figures, accepted for publication in MNRAS
Published: 2018
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9. Chemical modelling of N-bearing COMs in star-forming regions

Author: Serena Viti, Jonathan Holdship, Izaskun Jiménez-Serra, and D. Quénard
Subjects: Physics, Astrochemistry, Bearing (mechanical), Space and Planetary Science, law, Astronomy and Astrophysics, Astrophysics, Star (graph theory), law.invention
Abstract: The study of complex organic molecules, and more specifically those of prebiotic interest, is important to understand the chemical richness of star-forming regions. The chemistry of nitrogen bearing molecules such as formamide or methyl isocyanate is poorly constrained. We study different chemical pathways to form and destroy these molecules from both the gas phase and grain surface chemistry. From comparison with observations of four different relevant astrophysical regions, we show that both the gas phase and grain surface chemistry are required to explain the observed abundances of these species.
Published: 2017
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10. The fate of formamide in a fragmenting protoplanetary disc

Author: Izaskun Jiménez-Serra, Duncan Forgan, John D. Ilee, D. Quénard, Cassandra Hall, Ken Rice, European Research Council, University of St Andrews. St Andrews Centre for Exoplanet Science, and University of St Andrews. School of Physics and Astronomy
Subjects: Protoplanetary disks, 010504 meteorology & atmospheric sciences, NDAS, Library science, FOS: Physical sciences, Protoplanetary disk, 01 natural sciences, 0103 physical sciences, QB Astronomy, media_common.cataloged_instance, QD, European union, 010303 astronomy & astrophysics, Astrochemistry, QB, 0105 earth and related environmental sciences, media_common, Physics, Horizon (archaeology), European research, Astronomy and Astrophysics, QD Chemistry, Astrophysics - Astrophysics of Galaxies, 13. Climate action, Space and Planetary Science, Astrophysics of Galaxies (astro-ph.GA), Hydrodynamics, Partial support, formation [Planets and satellites]
Abstract: Recent high-sensitivity observations carried out with ALMA have revealed the presence of complex organic molecules (COMs) such as methyl cyanide (CH$_{\rm 3}$CN) and methanol (CH$_{\rm 3}$OH) in relatively evolved protoplanetary discs. The behaviour and abundance of COMs in earlier phases of disc evolution remains unclear. Here we combine a smoothed particle hydrodynamics simulation of a fragmenting, gravitationally unstable disc with a gas-grain chemical code. We use this to investigate the evolution of formamide (NH$_{\rm 2}$CHO), a pre-biotic species, in both the disc and in the fragments that form within it. Our results show that formamide remains frozen onto grains in the majority of the disc where the temperatures are $, Comment: 10 pages, 5 figures, accepted for publication in ApJ
Published: 2018
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11. Chemical modelling of glycolaldehyde and ethylene glycol in star-forming regions

Author: Serena Viti, Jonathan Holdship, M. T. Beltrán, Victor M. Rivilla, D. Quénard, Izaskun Jiménez-Serra, Audrey Coutens, J. M. C. Rawlings, AMOR 2018, Laboratoire d'Astrophysique de Bordeaux [Pessac] (LAB), Université de Bordeaux (UB)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Bordeaux (UB)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS), Atmospheric Physics Laboratory [UCL London], University College of London [London] (UCL), Centre Scientifique et Technique du Bâtiment (CSTB), Centro de Astrobiologia [Madrid] (CAB), and Instituto Nacional de Técnica Aeroespacial (INTA)-Consejo Superior de Investigaciones Científicas [Madrid] (CSIC)
Subjects: Physics, Glycolaldehyde, Astrochemistry, 010308 nuclear & particles physics, Methyl formate, Abundance (chemistry), [SDU.ASTR.CO]Sciences of the Universe [physics]/Astrophysics [astro-ph]/Cosmology and Extra-Galactic Astrophysics [astro-ph.CO], Radical, Analytical chemistry, FOS: Physical sciences, Astronomy and Astrophysics, 01 natural sciences, Astrophysics - Astrophysics of Galaxies, Luminosity, chemistry.chemical_compound, chemistry, Astrophysics - Solar and Stellar Astrophysics, 13. Climate action, Space and Planetary Science, Astrophysics of Galaxies (astro-ph.GA), Phase (matter), 0103 physical sciences, 010303 astronomy & astrophysics, Ethylene glycol, Solar and Stellar Astrophysics (astro-ph.SR)
Abstract: Glycolaldehyde (HOCH$_2$CHO) and ethylene glycol ((CH$_2$OH)$_2$) are two complex organic molecules detected in the hot cores and hot corinos of several star-forming regions. The ethylene glycol/glycolaldehyde abundance ratio seems to show an increase with the source luminosity. In the literature, several surface-chemistry formation mechanisms have been proposed for these two species. With the UCLCHEM chemical code, we explored the different scenarios and compared the predictions for a range of sources of different luminosities with the observations. None of the scenarios reproduce perfectly the trend. A better agreement is, however, found for a formation through recombination of two HCO radicals followed by successive hydrogenations. The reaction between HCO and CH$_2$OH could also contribute to the formation of glycolaldehyde in addition to the hydrogenation pathway. The predictions are improved when a trend of decreasing H$_2$ density within the core region with T $\geq$ 100 K as a function of luminosity, is included in the model. Destruction reactions of complex organic molecules in the gas phase would also need to be investigated, since they can affect the abundance ratios once the species have desorbed in the warm inner regions of the star-forming regions., Accepted in MNRAS
Published: 2017
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12. On the Nature of the Compact Sources in IRAS 16293–2422 Seen at Centimeter to Submillimeter Wavelengths

Author: Claire J. Chandler, D. Quénard, Sandrine Bottinelli, Emmanuel Caux, Paul T. P. Ho, Luis F. Rodríguez, Laurent Loinard, Crystal L. Brogan, Luis A. Zapata, Antonio Hernández-Gómez, Karl M. Menten, David J. Wilner, and Lee Hartmann
Subjects: Physics, Wavelength, Centimeter, Astrophysics - Solar and Stellar Astrophysics, Space and Planetary Science, Astrophysics of Galaxies (astro-ph.GA), FOS: Physical sciences, Astronomy, Astronomy and Astrophysics, Astrometry, Astrophysics - Astrophysics of Galaxies, Solar and Stellar Astrophysics (astro-ph.SR)
Abstract: We present multi-epoch continuum observations of the Class 0 protostellar system IRAS 16293-2422 taken with the Very Large Array (VLA) at multiple wavelengths between 7 mm and 15 cm (41 GHz down to 2 GHz), as well as single-epoch Atacama Large Millimeter/submillimeter Array (ALMA) continuum observations covering the range from 0.4 to 1.3 mm (700 GHz down to 230 GHz). The new VLA observations confirm that source A2 is a protostar driving episodic mass ejections, and reveal the complex relative motion between A2 and A1. The spectrum of component B can be described by a single power law ($S_\nu \propto \nu^{2.28}$) over the entire range from 3 to 700 GHz (10 cm down to 0.4 mm), suggesting that the emission is entirely dominated by dust even at $\lambda$ = 10 cm. Finally, the size of source B appears to increase with frequency up to 41 GHz, remaining roughly constant (at $0''.39$ $\equiv$ 55 AU) at higher frequencies. We interpret this as evidence that source B is a dusty structure of finite size that becomes increasingly optically thick at higher frequencies until, in the millimeter regime, the source becomes entirely optically thick. The lack of excess free-free emission at long wavelengths, combined with the absence of high-velocity molecular emission indicates that source B does not drive a powerful outflow, and might indicate that source B is at a particularly early stage of its evolution.
Published: 2019
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13. Seeds of Life in Space (SOLIS): I. Carbon-chain growth in the Solar-type protocluster OMC2-FIR4

Author: Rafael Bachiller, S. Spezzano, Jaime E. Pineda, Emmanuel Caux, Paola Caselli, Bertrand Lefloch, Piero Ugliengo, Yoko Oya, Audrey Coutens, Claudio Codella, Serena Viti, Claudine Kahane, Andy Pon, Jonathan Holdship, R. Neri, R. Choudhury, P. Hily-Blant, Patrice Theulé, Jacob C. Laas, Anton Vasyunin, Sandrine Bottinelli, A. Jaber Al-Edhari, Francesco Fontani, Izaskun Jiménez-Serra, Linda Podio, Felipe O. Alves, François Dulieu, Laurent Wiesenfeld, Cecilia Ceccarelli, D. Quénard, Satoshi Yamamoto, Cécile Favre, Ian R. Sims, Leonardo Testi, Vianney Taquet, Luca Bizzocchi, Nami Sakai, Ana López-Sepulcre, Albert Rimola, Nadia Balucani, E. Bianchi, Ana Chacón-Tanarro, Anna Punanova, Siyi Feng, C. Vastel, INAF - Osservatorio Astronomico di Brera (OAB), Istituto Nazionale di Astrofisica (INAF), Institut de Planétologie et d'Astrophysique de Grenoble (IPAG), Centre National d'Études Spatiales [Toulouse] (CNES)-Université Grenoble Alpes (UGA)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire des Sciences de l'Univers de Grenoble (OSUG), Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Joseph Fourier - Grenoble 1 (UJF)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes (UGA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Joseph Fourier - Grenoble 1 (UJF)-Centre National de la Recherche Scientifique (CNRS), Max Planck Institute for Extraterrestrial Physics (MPE), Max-Planck-Gesellschaft, Institut de Physique de Rennes (IPR), Université de Rennes 1 (UR1), Université de Rennes (UNIV-RENNES)-Université de Rennes (UNIV-RENNES)-Centre National de la Recherche Scientifique (CNRS), Università degli Studi di Perugia (UNIPG), Università degli Studi di Firenze [Firenze], Institut de recherche en astrophysique et planétologie (IRAP), Université Toulouse III - Paul Sabatier (UT3), Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées-Observatoire Midi-Pyrénées (OMP), Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS), INAF - Osservatorio Astrofisico di Arcetri (OAA), University College of London [London] (UCL), Laboratoire d'Etude du Rayonnement et de la Matière en Astrophysique (LERMA), École normale supérieure - Paris (ENS Paris)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, PSL Research University (PSL)-PSL Research University (PSL)-Université de Cergy Pontoise (UCP), Université Paris-Seine-Université Paris-Seine-Centre National de la Recherche Scientifique (CNRS), Universitat Autònoma de Barcelona [Barcelona] (UAB), Queen Mary University of London (QMUL), University of Western Ontario (UWO), RIKEN - Institute of Physical and Chemical Research [Japon] (RIKEN), Universiteit Leiden [Leiden], Physique des interactions ioniques et moléculaires (PIIM), Aix Marseille Université (AMU)-Centre National de la Recherche Scientifique (CNRS), Università degli studi di Torino (UNITO), Ural Federal University [Ekaterinburg] (UrFU), University of Electro-Communications [Tokyo] (UEC), Physique et Chimie du Milieu Interstellaire (PCMI) - Conseil National de la Recherche Scientifique (CNRS), Centre National d'Etudes Spatiales (CNES), LabeX Osug (Investissements d'avenir) [ANR10LABX56], Canadian Institute for Theoretical Astrophysics (CITA), European Research Council [PALs 320620], Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Observatoire des Sciences de l'Univers de Grenoble (OSUG ), Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national des sciences de l'Univers (INSU - CNRS)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019]), Università degli Studi di Firenze = University of Florence [Firenze] (UNIFI), Institut national des sciences de l'Univers (INSU - CNRS)-Université Toulouse III - Paul Sabatier (UT3), Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Centre National de la Recherche Scientifique (CNRS), LERMA Cergy (LERMA), Laboratoire d'Etude du Rayonnement et de la Matière en Astrophysique (LERMA (UMR_8112)), Sorbonne Université (SU)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Cergy Pontoise (UCP), Université Paris-Seine-Université Paris-Seine-Observatoire de Paris, Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Sorbonne Université (SU)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Cergy Pontoise (UCP), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL), Universitat Autònoma de Barcelona (UAB), Université de Rennes (UR)-Centre National de la Recherche Scientifique (CNRS), Università degli Studi di Perugia = University of Perugia (UNIPG), Università degli Studi di Firenze = University of Florence (UniFI), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS), Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université de Cergy Pontoise (UCP), Université Paris-Seine-Université Paris-Seine-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, Université Paris-Seine-Université Paris-Seine-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS), Universiteit Leiden, and Università degli studi di Torino = University of Turin (UNITO)
Subjects: 010504 meteorology & atmospheric sciences, radio lines ISM, CHEMICAL MODEL, chemistry.chemical_element, Flux, Astrophysics, 01 natural sciences, 7. Clean energy, star formation, MOLECULES, ISM molecules, ABUNDANCE RATIOS, FORMATION [STARS], 0103 physical sciences, Cluster (physics), CHAINS, 010303 astronomy & astrophysics, INTERSTELLAR MEDIUMS, ComputingMilieux_MISCELLANEOUS, Radio lines: ISM, 0105 earth and related environmental sciences, Line (formation), Physics, [PHYS]Physics [physics], EASTERN REGIONS, ISM: Molecules, Stars: Formation, Astronomy and Astrophysics, Space and Planetary Science, IONISATION RATES, Star formation, ISM [RADIO LINES], COSMIC RAYS, Galaxy, Interstellar medium, Stars, chemistry, 13. Climate action, MOLECULES [ISM], COSMOLOGY, IONIZATION, Molecular physics, [PHYS.ASTR]Physics [physics]/Astrophysics [astro-ph], Carbon, STARS
Abstract: The interstellar delivery of carbon atoms locked into molecules might be one of the key ingredients for the emergence of life. Cyanopolyynes are carbon chains delimited at their two extremities by an atom of hydrogen and a cyano group, meaning that they could be excellent reservoirs of carbon. The simplest member, HC3N, is ubiquitous in the galactic interstellar medium and found also in external galaxies. Thus, understanding the growth of cyanopolyynes in regions forming stars similar to our Sun, and what affects them, is particularly relevant. In the framework of the IRAM/NOEMA Large Program SOLIS (Seeds Of Life In Space), we have obtained a map of two cyanopolyynes, HC3N and HC5N, in the protocluster OMC-2 FIR4. Because our Sun is thought to be born in a rich cluster, OMC-2 FIR4 is one of the closest and best known representatives of the environment in which the Sun may have been born. We find a HC3N/HC5N abundance ratio across the source in the range 1..30, with the smallest values (≤10) in FIR5 and in the eastern region of FIR4. The ratios ≤10 can be reproduced by chemical models only if: (1) the cosmic-ray ionisation rate is ∼4× 10-14 s-1; (2) the gaseous elemental ratio C/O is close to unity; and (3) oxygen and carbon are largely depleted. The large is comparable to that measured in FIR4 by previous works and was interpreted as due to a flux of energetic (≥10 MeV) particles from embedded sources. We suggest that these sources could lie east of FIR4 and FIR5. A temperature gradient across FIR4, with T decreasing from east to west by about 10 K, could also explain the observed change in the HC3N/HC5N line ratio, without the need of a cosmic ray ionisation rate gradient. However, even in this case, a high constant cosmic-ray ionisation rate (of the order of 10s s-1) is necessary to reproduce the observations. © ESO 2017. European Research Council, ERC: PALs 320620 Centre National dâ Etudes Spatiales, CNES ANR10LABX56 Canadian Institute for Theoretical Astrophysics, ICAT Conseil National de la Recherche Scientifique, CNRS-L ★ Based on observations carried out under project number L15AA with the IRAM NOEMA Interferometer. IRAM is supported by INSU/CNRS (France), MPG (Germany) and IGN (Spain). ★★ The final IRAM data used in the paper (FITS format) are available at the CDS via anonymous ftp to cdsarc.u-strasbg.fr (130.79.128.5) or via http://cdsarc.u-strasbg.fr/viz-bin/qcat?J/A+A/605/A57 Acknowledgements. We thank the IRAM staff for their help in the data reduction. Many thanks to the anonymous referee for his/her constructive comments. This work was supported by the French program Physique et Chimie du Milieu In-terstellaire (PCMI) funded by the Conseil National de la Recherche Scientifique (CNRS) and Centre National d’Études Spatiales (CNES), and by a grant from LabeX Osug@2020 (Investissements d’avenir – ANR10LABX56). Partial salary support for A. Pon was provided by a Canadian Institute for Theoretical Astrophysics (CITA) National Fellowship. P.C., A. Punanova, A.C., and J.E.P. acknowledge support from the European Research Council (project PALs 320620). C.F. acknowledges founding from French space agency CNES.
Published: 2017
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14. Seeds of Life in Space (SOLIS). II. Formamide in protostellar shocks: Evidence for gas-phase formation

Author: Izaskun Jiménez-Serra, Ana Chacón-Tanarro, Claudine Kahane, Andy Pon, R. Neri, Yoko Oya, Patrice Theulé, Leonardo Testi, Audrey Coutens, Paola Caselli, Charlotte Vastel, Serena Viti, François Dulieu, Jaime E. Pineda, R. Choudhury, P. Hily-Blant, J. Ospina, Fanny Vazart, Vincenzo Barone, Ana López-Sepulcre, Ian R. Sims, Laurent Wiesenfeld, Claudio Codella, Anna Punanova, Sandrine Bottinelli, Vianney Taquet, Francesco Fontani, Jacob C. Laas, A. Jaber Al-Edhari, Linda Podio, Cecilia Ceccarelli, Satoshi Yamamoto, Nami Sakai, Felipe O. Alves, Rafael Bachiller, Emmanuel Caux, S. Spezzano, D. Quénard, Nadia Balucani, Siyi Feng, Cécile Favre, Luca Bizzocchi, Cristina Puzzarini, Bertrand Lefloch, Piero Ugliengo, Anton Vasyunin, Jonathan Holdship, Dimitrios Skouteris, Albert Rimola, E. Bianchi, Laboratoire d'Astrophysique de Grenoble (LAOG), Université Joseph Fourier - Grenoble 1 (UJF)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS), INAF - Osservatorio Astrofisico di Arcetri (OAA), Istituto Nazionale di Astrofisica (INAF), Università degli Studi di Perugia (UNIPG), INAF - Osservatorio Astronomico di Brera (OAB), Southern University of Science and Technology [Shenzhen] (SUSTech), Laboratoire d'Etude du Rayonnement et de la Matière en Astrophysique (LERMA), École normale supérieure - Paris (ENS Paris)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, PSL Research University (PSL)-PSL Research University (PSL)-Université de Cergy Pontoise (UCP), Université Paris-Seine-Université Paris-Seine-Centre National de la Recherche Scientifique (CNRS), Queen Mary University of London (QMUL), University College of London [London] (UCL), ESAB, Universitad polytecnica de Cataluna, University of Western Ontario (UWO), Max Planck Institute for Extraterrestrial Physics (MPE), Max-Planck-Gesellschaft, Institut de recherche en astrophysique et planétologie (IRAP), Université Toulouse III - Paul Sabatier (UT3), Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées-Observatoire Midi-Pyrénées (OMP), Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS), Institut de Planétologie et d'Astrophysique de Grenoble (IPAG), Centre National d'Études Spatiales [Toulouse] (CNES)-Université Grenoble Alpes (UGA)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire des Sciences de l'Univers de Grenoble (OSUG), Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Joseph Fourier - Grenoble 1 (UJF)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes (UGA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Joseph Fourier - Grenoble 1 (UJF)-Centre National de la Recherche Scientifique (CNRS), departament de Quimica, Universitat Autònoma de Barcelona [Barcelona] (UAB), RIKEN - Institute of Physical and Chemical Research [Japon] (RIKEN), Scuola Normale Superiore di Pisa (SNS), European Southern Observatory (ESO), Physique des interactions ioniques et moléculaires (PIIM), Aix Marseille Université (AMU)-Centre National de la Recherche Scientifique (CNRS), Università degli studi di Torino (UNITO), Codella, C., Ceccarelli, C., Caselli, P., Balucani, N., Barone, V., Fontani, F., Lefloch, B., Podio, L., Viti, S., Feng, S., Bachiller, R., Bianchi, E., Dulieu, F., Jiménez-Serra, I., Holdship, J., Neri, R., Pineda, J.E., Pon, A., Sims, I., Spezzano, S., Vasyunin, A.I., Alves, F., Bizzocchi, L., Bottinelli, S., Caux, E., Chacón-Tanarro, A., Choudhury, R., Coutens, A., Favre, C., Hily-Blant, P., Kahane, C., Jaber Al-Edhari, A., Laas, J., López-Sepulcre, A., Ospina, J., Oya, Y., Punanova, A., Puzzarini, C., Quenard, D., Rimola, A., Sakai, N., Skouteris, D., Taquet, V., Testi, L., Theulé, P., Ugliengo, P., Vastel, C., Vazart, F., Wiesenfeld, L., Yamamoto, S., Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Observatoire des Sciences de l'Univers de Grenoble (OSUG ), Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national des sciences de l'Univers (INSU - CNRS)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019]), Università degli Studi di Perugia = University of Perugia (UNIPG), Southern University of Science and Technology (SUSTech), LERMA Cergy (LERMA), Laboratoire d'Etude du Rayonnement et de la Matière en Astrophysique (LERMA (UMR_8112)), Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université de Cergy Pontoise (UCP), Université Paris-Seine-Université Paris-Seine-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, Université Paris-Seine-Université Paris-Seine-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS), Universitat Autònoma de Barcelona (UAB), Università degli studi di Torino = University of Turin (UNITO), Pineda, J. E., Vasyunin, A. I., Sorbonne Université (SU)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Cergy Pontoise (UCP), Université Paris-Seine-Université Paris-Seine-Observatoire de Paris, Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Sorbonne Université (SU)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Cergy Pontoise (UCP), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL), Institut national des sciences de l'Univers (INSU - CNRS)-Université Toulouse III - Paul Sabatier (UT3), Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Centre National de la Recherche Scientifique (CNRS), and Centre National de la Recherche Scientifique (CNRS)-Aix Marseille Université (AMU)
Subjects: Formamide, Abundance (chemistry), Direct evidence, Stars: formation, FOS: Physical sciences, Context (language use), Astrophysics, ISM: molecule, 01 natural sciences, chemistry.chemical_compound, 0103 physical sciences, Protostar, molecule [ISM], 010303 astronomy & astrophysics, ISM: jets and outflow, formation [Stars], ComputingMilieux_MISCELLANEOUS, Line (formation), Earth and Planetary Astrophysics (astro-ph.EP), ISM: individual objects: L1157-B1, ISM: jets and outflows, ISM: molecules, Astronomy and Astrophysics, Space and Planetary Science, Physics, [PHYS]Physics [physics], 010308 nuclear & particles physics, jets and outflow [ISM], individual objects: L1157-B1 [ISM], Astronomy and Astrophysic, Stars, chemistry, Millimeter, [PHYS.ASTR]Physics [physics]/Astrophysics [astro-ph], Astrophysics - Earth and Planetary Astrophysics
Abstract: Context: Modern versions of the Miller-Urey experiment claim that formamide (NH$_2$CHO) could be the starting point for the formation of metabolic and genetic macromolecules. Intriguingly, formamide is indeed observed in regions forming Solar-type stars as well as in external galaxies. Aims: How NH$_2$CHO is formed has been a puzzle for decades: our goal is to contribute to the hotly debated question of whether formamide is mostly formed via gas-phase or grain surface chemistry. Methods: We used the NOEMA interferometer to image NH$_2$CHO towards the L1157-B1 blue-shifted shock, a well known interstellar laboratory, to study how the components of dust mantles and cores released into the gas phase triggers the formation of formamide. Results: We report the first spatially resolved image (size $\sim$ 9", $\sim$ 2300 AU) of formamide emission in a shocked region around a Sun-like protostar: the line profiles are blueshifted and have a FWHM $\simeq$ 5 km s$^{-1}$. A column density of $N_{\rm NH_2CHO}$ = 8 $\times$ 10$^{12}$ cm$^{-1}$, and an abundance (with respect to H-nuclei) of 4 $\times$ 10$^{-9}$ are derived. We show a spatial segregation of formamide with respect to other organic species. Our observations, coupled with a chemical modelling analysis, indicate that the formamide observed in L1157-B1 is formed by gas-phase chemical process, and not on grain surfaces as previously suggested. Conclusions: The SOLIS interferometric observations of formamide provide direct evidence that this potentially crucial brick of life is efficiently formed in the gas-phase around Sun-like protostars., 7 pages, 1 table, 5 figures, A&A Letters, in press
Published: 2017
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15. High spectral resolution observations of HNC3 and HCCNC in the L1544 prestellar core

Author: Kentarou Kawaguchi, D. Quénard, Masatoshi Ohishi, H S P Müller, Bertrand Lefloch, Charlotte Vastel, Rafael Bachiller, Institut de recherche en astrophysique et planétologie (IRAP), Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS), Institut de Planétologie et d'Astrophysique de Grenoble (IPAG), Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Observatoire des Sciences de l'Univers de Grenoble (OSUG ), and Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national des sciences de l'Univers (INSU - CNRS)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019])
Subjects: Astrochemistry, 010504 meteorology & atmospheric sciences, FOS: Physical sciences, Astrophysics, 01 natural sciences, ISM: abundances, chemistry.chemical_compound, Abundance (ecology), 0103 physical sciences, Cyanoacetylene, Spectral resolution, 010303 astronomy & astrophysics, 0105 earth and related environmental sciences, Physics, astrochemistry, Late stage, Astronomy and Astrophysics, Astrophysics - Astrophysics of Galaxies, ISM: molecules, Pre-stellar core, chemistry, Space and Planetary Science, ISM: individual objects: L1544, [SDU]Sciences of the Universe [physics], Astrophysics of Galaxies (astro-ph.GA), Millimeter, line: identification
Abstract: HCCNC and HNC3 are less commonly found isomers of cyanoacetylene, HC3N, a molecule that is widely found in diverse astronomical sources. We want to know if HNC3 is present in sources other than the dark cloud TMC-1 and how its abundance is relative to that of related molecules. We used the ASAI unbiased spectral survey at IRAM 30m towards the prototypical prestellar core L1544 to search for HNC3 and HCCNC which are by-product of the HC3NH+ recombination, previously detected in this source. We performed a combined analysis of published HNC3 microwave rest frequencies with thus far unpublished millimeter data because of issues with available rest frequency predictions. We determined new spectroscopic parameters for HNC3, produced new predictions and detected it towards L1544. We used a gas-grain chemical modelling to predict the abundances of N-species and compare with the observations. The modelled abundances are consistent with the observations, considering a late stage of the evolution of the prestellar core. However the calculated abundance of HNC3 was found 5-10 times higher than the observed one. The HC3N, HNC3 and HCCNC versus HC3NH+ ratios are compared in the TMC-1 dark cloud and the L1544 prestellar core., Comment: Accepted in MNRAS letters. 5 pages plus 2 additional pages for the on-line material
Published: 2017
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16. The ALMA Frontier Fields Survey - II. Multiwavelength Photometric analysis of 1.1mm continuum sources in Abell 2744, MACSJ0416.1-2403 and MACSJ1149.5+2223

Author: P. Troncoso-Iribarren, Larry Bradley, G. Brammer, Xingxing Huang, N. Padilla, Edo Ibar, Hugo Messias, R. Kneissl, C. Romero-Cañizales, Nicolas Laporte, Leopoldo Infante, Franz E. Bauer, Timo Anguita, Richard S. Ellis, R. Demarco, R. Pello, A. M. Muñoz Arancibia, Adi Zitrin, Harold Francke, Neil M. Nagar, W. Zheng, Anton M. Koekemoer, Manuel Aravena, J. González-López, M. Carrasco, Holland C. Ford, Marc Postman, D. Quénard, Ezequiel Treister, E. Villard, Seock-Sam Kim, R. J. Bouwens, L. F. Barrientos, R. Carvajal, Dan Coe, Institut de recherche en astrophysique et planétologie (IRAP), Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), and Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS)
Subjects: submillimeter: galaxies, FOS: Physical sciences, Astrophysics, Astrophysics::Cosmology and Extragalactic Astrophysics, 01 natural sciences, infrared: galaxies, [PHYS.ASTR.CO]Physics [physics]/Astrophysics [astro-ph]/Cosmology and Extra-Galactic Astrophysics [astro-ph.CO], Photometry (optics), Spitzer Space Telescope, galaxies: high-redshift, 0103 physical sciences, Astrophysics::Solar and Stellar Astrophysics, 010303 astronomy & astrophysics, ComputingMilieux_MISCELLANEOUS, Astrophysics::Galaxy Astrophysics, Photometric redshift, radio continuum: galaxies, Luminous infrared galaxy, Physics, Very Large Telescope, 010308 nuclear & particles physics, Astronomy and Astrophysics, Astrophysics - Astrophysics of Galaxies, Redshift, Galaxy, galaxies: photometry, Abell 2744, Space and Planetary Science, Astrophysics of Galaxies (astro-ph.GA), Astrophysics::Earth and Planetary Astrophysics, galaxies: distances and redshifts
Abstract: [abridged] The Hubble and Spitzer Space Telescope surveys of the Frontier Fields (FF) provide extremely deep images around six massive, strong-lensing clusters of galaxies. The ALMA FF survey aims to cover the same fields at 1.1mm, with maps reaching (unlensed) sensitivities of $$5$\sigma$) sources in the first three FF clusters observed by ALMA, based on data from Hubble and Spitzer, the VLT and Herschel. We measure the total photometry in all available bands and determine the photometric redshifts and the physical properties of the counterparts via SED-fitting. In particular, we carefully estimate the FIR photometry using 1.1mm priors to limit the misidentification of blended FIR counterparts, which strongly affect some flux estimates in previous FIR catalogs. We identify robust near-infrared (NIR) counterparts for all 11 sources with K$_s$ detection, the majority of which are quite red, with eight having $F814W-K_s\gtrsim 4$ and five having $F160W-[4.5]\gtrsim3$. From the FIR point of view, all our objects have $z_{phot}$$\sim$1--3, whereas based on the optical SED one object prefers a high-$z$ solution ($z\geq\ $7). Five objects among our sample have spectroscopic redshifts from the GLASS survey for which we can reproduce their SEDs with existing templates. This verification confirms the validity of our photometric redshift methodology. The mean redshift of our sample is $z_{phot}$=1.99$\pm$0.27. All 1.1mm selected objects are massive (10.0$ \approx$1.6) and high dust contents (8.1 $, Comment: 18 pages, 11 figures, accepted for publication in A&A
Published: 2017
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17. Detection of the HC$_3$NH$^+$ and HCNH$^+$ ions in the L1544 pre-stellar core

Author: Rafael Bachiller, P. Hily-Blant, Charlotte Vastel, Bertrand Lefloch, D. Quénard, Cecilia Ceccarelli, Institut de recherche en astrophysique et planétologie (IRAP), Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS), Institut de Planétologie et d'Astrophysique de Grenoble (IPAG), Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Observatoire des Sciences de l'Univers de Grenoble (OSUG ), and Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national des sciences de l'Univers (INSU - CNRS)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019])
Subjects: Astrochemistry, molecular data, Thermodynamic equilibrium, Ionic bonding, FOS: Physical sciences, 01 natural sciences, Ion, TheoryofComputation_ANALYSISOFALGORITHMSANDPROBLEMCOMPLEXITY, 0103 physical sciences, Radiative transfer, Spectral resolution, 010303 astronomy & astrophysics, Hyperfine structure, Solar and Stellar Astrophysics (astro-ph.SR), Physics, [SDU.ASTR]Sciences of the Universe [physics]/Astrophysics [astro-ph], 010308 nuclear & particles physics, astrochemistry, Astronomy and Astrophysics, Astrophysics - Astrophysics of Galaxies, Pre-stellar core, Astrophysics - Solar and Stellar Astrophysics, Space and Planetary Science, radiative transfer, [SDU]Sciences of the Universe [physics], Astrophysics of Galaxies (astro-ph.GA), Atomic physics, line: identification
Abstract: The L1544 pre-stellar core was observed as part of the ASAI (Astrochemical Surveys At IRAM) Large Program. We report the first detection in a pre-stellar core of the HCNH$^+$ and HC$_3$NH$^+$ ions. The high spectral resolution of the observations allows to resolve the hyperfine structure of HCNH$^+$. Local thermodynamic equilibrium analysis leads to derive a column density equal to (2.0$\pm$0.2)$\times$10$^{13}$cm$^{-2}$ for HCNH$^+$ and (1.5$\pm$0.5)$\times$10$^{11}$cm$^{-2}$ for HC$_3$NH$^+$. We also present non-LTE analysis of five transitions of HC$_3$N, three transitions of H$^{13}$CN and one transition of HN$^{13}$C, all of them linked to the chemistry of HCNH$^+$ and HC$_3$NH$^+$. We computed for HC$_3$N, HCN, and HNC a column density of (2.0$\pm$0.4)$\times$10$^{13}$cm$^{-2}$, (3.6$\pm$0.9)$\times10^{14}$cm$^{-2}$, and (3.0$\pm$1.0)$\times$10$^{14}$cm$^{-2}$, respectively. We used the gas-grain chemical code Nautilus to predict the abundances all these species across the pre-stellar core. Comparison of the observations with the model predictions suggests that the emission from HCNH$^+$ and HC$_3$NH$^+$ originates in the external layer where non-thermal desorption of other species was previously observed. The observed abundance of both ionic species ([HCNH$^+$]$\,\simeq3\times10^{-10}$ and [HC$_3$NH$^+$]$\,\simeq[1.5-3.0]\times10^{-12}$, with respect to H$_2$) cannot be reproduced at the same time by the chemical modelling, within the error bars of the observations only. We discuss the possible reasons for the discrepancy and suggest that the current chemical models are not fully accurate or complete. However, the modelled abundances are within a factor of three consistent with the observations, considering a late stage of the evolution of the pre-stellar core, compatible with previous observations., Comment: Accepted for publication in MNRAS, 13 pages, 9 figures
Published: 2017
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18. Seeds Of Life In Space (SOLIS): The Organic Composition Diversity at 300-1000 au Scale in Solar-type Star-forming Regions

Author: R. Choudhury, Emmanuel Caux, Felipe O. Alves, Jacob C. Laas, Albert Rimola, François Dulieu, Satoshi Yamamoto, Charlotte Vastel, Francesco Fontani, Serena Viti, Anton Vasyunin, Leonardo Testi, E. Bianchi, Jonathan Holdship, Ana Chacón-Tanarro, Nami Sakai, P. Hily-Blant, J. Ospina, Sandrine Bottinelli, Claudine Kahane, Andy Pon, D. Quénard, Bertrand Lefloch, Piero Ugliengo, Laurent Wiesenfeld, Ana López-Sepulcre, R. Neri, Rafael Bachiller, Cecilia Ceccarelli, Jaime E. Pineda, Claudio Codella, Vianney Taquet, Cécile Favre, Paola Caselli, Anna Punanova, A. Jaber Al-Edhari, Patrice Theulé, Linda Podio, S. Spezzano, Luca Bizzocchi, Yoko Oya, Audrey Coutens, Siyi Feng, Nadia Balucani, Ian R. Sims, Izaskun Jiménez-Serra, Institut de Planétologie et d'Astrophysique de Grenoble (IPAG), Centre National d'Études Spatiales [Toulouse] (CNES)-Université Grenoble Alpes (UGA)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire des Sciences de l'Univers de Grenoble (OSUG), Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Joseph Fourier - Grenoble 1 (UJF)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes (UGA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Joseph Fourier - Grenoble 1 (UJF)-Centre National de la Recherche Scientifique (CNRS), Max Planck Institute for Extraterrestrial Physics (MPE), Max-Planck-Gesellschaft, INAF - Osservatorio Astronomico di Brera (OAB), Istituto Nazionale di Astrofisica (INAF), INAF - Osservatorio Astrofisico di Arcetri (OAA), Queen Mary University of London (QMUL), University College of London [London] (UCL), Institut de recherche en astrophysique et planétologie (IRAP), Université Toulouse III - Paul Sabatier (UT3), Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées-Observatoire Midi-Pyrénées (OMP), Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS), Università degli Studi di Perugia (UNIPG), Università degli Studi di Firenze [Firenze], Laboratoire d'Etude du Rayonnement et de la Matière en Astrophysique (LERMA), École normale supérieure - Paris (ENS Paris)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, PSL Research University (PSL)-PSL Research University (PSL)-Université de Cergy Pontoise (UCP), Université Paris-Seine-Université Paris-Seine-Centre National de la Recherche Scientifique (CNRS), University of Western Ontario (UWO), Universitat Autònoma de Barcelona [Barcelona] (UAB), RIKEN - Institute of Physical and Chemical Research [Japon] (RIKEN), Institut de Physique de Rennes (IPR), Université de Rennes 1 (UR1), Université de Rennes (UNIV-RENNES)-Université de Rennes (UNIV-RENNES)-Centre National de la Recherche Scientifique (CNRS), Physique des interactions ioniques et moléculaires (PIIM), Aix Marseille Université (AMU)-Centre National de la Recherche Scientifique (CNRS), Università degli studi di Torino (UNITO), Ural Federal University [Ekaterinburg] (UrFU), Centre National de la Recherche Scientifique (CNRS), University of Electro-Communications [Tokyo] (UEC), European Research Council (ERC) [320620, 741002], French program Physique et Chimie du Milieu Interstellaire (PCMI) - Conseil National de la Recherche Scientifique (CNRS), Centre National dEtudes Spatiales (CNES), Italian Ministero dell'Istruzione, Universita e Ricerca, through the grant Progetti Premiali iALMA [CUP C52I13000140001], Canadian Institute for Theoretical Astrophysics (CITA) National Fellowship, STFC [ST/L004801, ST/M004139], Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Observatoire des Sciences de l'Univers de Grenoble (OSUG ), Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national des sciences de l'Univers (INSU - CNRS)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019]), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS), Università degli Studi di Perugia = University of Perugia (UNIPG), Università degli Studi di Firenze = University of Florence (UniFI), LERMA Cergy (LERMA), Laboratoire d'Etude du Rayonnement et de la Matière en Astrophysique (LERMA (UMR_8112)), Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université de Cergy Pontoise (UCP), Université Paris-Seine-Université Paris-Seine-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, Université Paris-Seine-Université Paris-Seine-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS), Universitat Autònoma de Barcelona (UAB), Université de Rennes (UR)-Centre National de la Recherche Scientifique (CNRS), Università degli studi di Torino = University of Turin (UNITO), Centre National d'Études Spatiales [Toulouse] (CNES)-Observatoire des Sciences de l'Univers de Grenoble (OSUG ), Institut national des sciences de l'Univers (INSU - CNRS)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Institut National de Recherche pour l’Agriculture, l’Alimentation et l’Environnement (INRAE)-Université Grenoble Alpes (UGA)-Météo-France -Institut national des sciences de l'Univers (INSU - CNRS)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Institut National de Recherche pour l’Agriculture, l’Alimentation et l’Environnement (INRAE)-Université Grenoble Alpes (UGA)-Météo-France, Max-Planck-Institut fur Extraterrestrische Physik, Giessenbachstrasse 1, D-85748 Garching, Germany, INAF-Osservatorio Astrofisico di Arcetri (INAF-OAA), Institut de RadioAstronomie Millimétrique (IRAM), Department of Physics and Astronomy, University College London, Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Université Fédérale Toulouse Midi-Pyrénées-Météo-France -Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS), Observatorio Astronómico Nacional, Observatorio de Madrid, Alfonso XII (OAN), École normale supérieure - Paris (ENS-PSL), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, Université Paris sciences et lettres (PSL)-Université de Cergy Pontoise (UCP), Molécules dans l'Univers, Laboratoire d'Etude du Rayonnement et de la Matière en Astrophysique et Atmosphères (LERMA (UMR_8112)), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-CY Cergy Paris Université (CY)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-CY Cergy Paris Université (CY), University of AL-Muthanna, College of Science, Physics Department, AL-Muthanna, Iraq, Department of Physics, University of Tokyo, Departament de Quimica, Universitat Autonoma de Barcelona, E-08193 Bellaterra, Spain, RIKEN The Institute of Physical and Chemical Research, Institut national des sciences de l'Univers (INSU - CNRS)-Université Toulouse III - Paul Sabatier (UT3), Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Centre National de la Recherche Scientifique (CNRS), Università degli Studi di Firenze = University of Florence [Firenze] (UNIFI), Sorbonne Université (SU)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Cergy Pontoise (UCP), Université Paris-Seine-Université Paris-Seine-Observatoire de Paris, Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Sorbonne Université (SU)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Cergy Pontoise (UCP), and Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)
Subjects: radio lines ISM, FOS: Physical sciences, Scale (descriptive set theory), Astrophysics, Type (model theory), Star (graph theory), Space (mathematics), ISM: clouds, 01 natural sciences, ISM: abundances, Spectral line, ISM molecules, Abundance (ecology), ISM: molecules, radio lines: ISM, Astronomy and Astrophysics, Space and Planetary Science, 0103 physical sciences, 14. Life underwater, 010303 astronomy & astrophysics, ISM abundances, Solar and Stellar Astrophysics (astro-ph.SR), ComputingMilieux_MISCELLANEOUS, Physics, [PHYS]Physics [physics], 010308 nuclear & particles physics, Astrophysics - Astrophysics of Galaxies, Interstellar medium, ISM clouds, Astrophysics - Solar and Stellar Astrophysics, 13. Climate action, Astrophysics of Galaxies (astro-ph.GA), Molecular physics, [PHYS.ASTR]Physics [physics]/Astrophysics [astro-ph], Order of magnitude
Abstract: Complex organic molecules have been observed for decades in the interstellar medium. Some of them might be considered as small bricks of the macromolecules at the base of terrestrial life. It is hence particularly important to understand organic chemistry in Solar-like star forming regions. In this article, we present a new observational project: SOLIS (Seeds Of Life In Space). This is a Large Project at the IRAM-NOEMA interferometer, and its scope is to image the emission of several crucial organic molecules in a sample of Solar-like star forming regions in different evolutionary stage and environments. Here, we report the first SOLIS results, obtained from analysing the spectra of different regions of the Class 0 source NGC1333-IRAS4A, the protocluster OMC-2 FIR4, and the shock site L1157-B1. The different regions were identified based on the images of formamide (NH2CHO) and cyanodiacetylene (HC5N) lines. We discuss the observed large diversity in the molecular and organic content, both on large (3000-10000 au) and relatively small (300-1000 au) scales. Finally, we derive upper limits to the methoxy fractional abundance in the three observed regions of the same order of magnitude of that measured in few cold prestellar objects, namely ~10^-12-10^-11 with respect to H2 molecules., Comment: Accepted for publication on The Astrophysical Journal
Published: 2017
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19. History of the solar-type protostar IRAS 16293–2422 as told by the cyanopolyynes

Author: A. Jaber Al-Edhari, Emmanuel Caux, François Lique, Nadia Balucani, Alexandre Faure, D. Quénard, Claudine Kahane, Serena Viti, Laurent Wiesenfeld, E. Mendoza, Bertrand Lefloch, Cecilia Ceccarelli, Institut de Planétologie et d'Astrophysique de Grenoble (IPAG), Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Observatoire des Sciences de l'Univers de Grenoble (OSUG ), Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national des sciences de l'Univers (INSU - CNRS)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019]), Università degli Studi di Perugia (UNIPG), Institut de recherche en astrophysique et planétologie (IRAP), Institut national des sciences de l'Univers (INSU - CNRS)-Université Toulouse III - Paul Sabatier (UT3), Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées-Observatoire Midi-Pyrénées (OMP), Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Centre National de la Recherche Scientifique (CNRS), Laboratoire Ondes et Milieux Complexes (LOMC), Centre National de la Recherche Scientifique (CNRS)-Université Le Havre Normandie (ULH), Normandie Université (NU)-Normandie Université (NU), Centro de Investigaciones Energéticas Medioambientales y Tecnológicas [Madrid] (CIEMAT), Centre National d'Études Spatiales [Toulouse] (CNES)-Université Grenoble Alpes (UGA)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire des Sciences de l'Univers de Grenoble (OSUG), Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Joseph Fourier - Grenoble 1 (UJF)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes (UGA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Joseph Fourier - Grenoble 1 (UJF)-Centre National de la Recherche Scientifique (CNRS), Univ Toulouse UPS, Ctr Etud Spatiale Rayonnements, F-31062 Toulouse 9, France, Centre Etud Spatiale Rayonnements Toulouse, Neurobiologie de l'apprentissage, de la mémoire et de la communication (NAMC), Université Paris-Sud - Paris 11 (UP11)-Centre National de la Recherche Scientifique (CNRS), Université Le Havre Normandie (ULH), Normandie Université (NU)-Normandie Université (NU)-Centre National de la Recherche Scientifique (CNRS), Centre Scientifique et Technique du Bâtiment (CSTB Saint Martin d'Hères), Centre Scientifique et Technique du Bâtiment (CSTB), Università degli Studi di Perugia = University of Perugia (UNIPG), Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), and Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS)
Subjects: Astrochemistry, 010504 meteorology & atmospheric sciences, FOS: Physical sciences, Context (language use), Astrophysics, 01 natural sciences, Spectral line, IRAS 16293-2422, chemistry.chemical_compound, Abundances - ISM, 0103 physical sciences, Cyanoacetylene, Protostar, 010303 astronomy & astrophysics, Solar and Stellar Astrophysics (astro-ph.SR), ComputingMilieux_MISCELLANEOUS, 0105 earth and related environmental sciences, Physics, [PHYS]Physics [physics], Cyanopolyyne, Molecular cloud, Astrochemistry - ISM, Individual objects, Astronomy and Astrophysics, Space and Planetary Science, Astrophysics - Astrophysics of Galaxies, Interstellar medium, chemistry, Astrophysics - Solar and Stellar Astrophysics, 13. Climate action, [SDU]Sciences of the Universe [physics], Astrophysics of Galaxies (astro-ph.GA)
Abstract: Cyanopolyynes are chains of carbon atoms with an atom of hydrogen and a CN group on either side. They are detected almost everywhere in the ISM, as well as in comets. In the past, they have been used to constrain the age of some molecular clouds, since their abundance is predicted to be a strong function of time. We present an extensive study of the cyanopolyynes distribution in the solar-type protostar IRAS16293-2422 based on TIMASSS IRAM-30m observations. The goals are (i) to obtain a census of the cyanopolyynes in this source and of their isotopologues; (ii) to derive how their abundance varies across the protostar envelope; and (iii) to obtain constraints on the history of IRAS16293-2422. We detect several lines from HC3N and HC5N, and report the first detection of DC3N, in a solar-type protostar. We found that the HC3N abundance is roughly constant (~1.3x10^(-11)) in the outer cold envelope of IRAS16293-2422, and it increases by about a factor 100 in the inner region where Tdust>80K. The HC5N has an abundance similar to HC3N in the outer envelope and about a factor of ten lower in the inner region. The HC3N abundance derived in the inner region, and where the increase occurs, also provide strong constraints on the time taken for the dust to warm up to 80K, which has to be shorter than ~10^3-10^4yr. Finally, the cyanoacetylene deuteration is about 50\% in the outer envelope and, Accepted for publication in A&A
Published: 2017
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20. MULTI-EPOCH VLA OBSERVATIONS OF IRAS 16293-2422B AND THE MODELING OF ITS CONTINUUM EMISSION

Author: A. Hernández-Gómez, D. Quénard, L. Loinard, and E. Caux
Subjects: Física, Astronomía y Matemáticas
Published: 2017

21. Detectability of deuterated water in prestellar cores

Author: Cecilia Ceccarelli, Charlotte Vastel, Paola Caselli, Vianney Taquet, D. Quénard, Institut de recherche en astrophysique et planétologie (IRAP), Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS), Institut de Planétologie et d'Astrophysique de Grenoble (IPAG), Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Observatoire des Sciences de l'Univers de Grenoble (OSUG ), and Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national des sciences de l'Univers (INSU - CNRS)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019])
Subjects: Astrochemistry, Opacity, FOS: Physical sciences, Context (language use), Astrophysics, 7. Clean energy, 01 natural sciences, ISM: abundances, 0103 physical sciences, Radiative transfer, Protostar, 010303 astronomy & astrophysics, Solar and Stellar Astrophysics (astro-ph.SR), Line (formation), Physics, [SDU.ASTR]Sciences of the Universe [physics]/Astrophysics [astro-ph], 010308 nuclear & particles physics, Star formation, astrochemistry, Astronomy and Astrophysics, Planetary system, ISM: molecules, Astrophysics - Solar and Stellar Astrophysics, 13. Climate action, Space and Planetary Science, ISM: individual objects: L1544, [SDU]Sciences of the Universe [physics], line: identification
Abstract: Water is an important molecule in the chemical and thermal balance of dense molecular gas, but knowing its history through-out the various stages of the star formation is a fundamental problem. Its molecular deuteration provides us with a crucial clue to its formation history. H$_2$O has recently been detected for the first time towards the prestellar core L1544 with the Herschel Space Observatory with a high spectral resolution (HIFI instrument). Prestellar cores provide the original reservoir of material from which future planetary systems are built, but few observational constraints exist on the formation of water and none on its deuteration before the collapse starts and a protostar forms at the centre. We report on new APEX observations of the ground state 1$_{0,1}$-0$_{0,0}$ HDO transition at 464 GHz towards the prestellar core L1544. The line is undetected, and we present an extensive study of the conditions for its detectability in cold and dense cloud cores. The water and deuterated water abundances have been estimated using an advanced chemical model simplified for the limited number of reactions or processes that are active in cold regions (< 15 K). We use the LIME radiative transfer code to compute the expected intensity and profile of both H$_2$O and HDO lines and compare them with the observations. We present several ad hoc profiles that best-fit the observations and compare the profiles with results from an astrochemical modelling, coupling gas phase and grain surface chemistry. Our comparison between observations, radiative transfer, and chemical modelling shows the limits of detectability for singly deuterated water, through the ground-state transitions 1$_{0,1}$-0$_{0,0}$ and 1$_{1,1}$-0$_{0,0}$ at 464.9 and 893.6 GHz, respectively, with both single-dish telescope and interferometric observations., 8 pages, 6 figures
Published: 2016
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22. Dust in the Reionization Era: ALMA Observations of a z = 8.38 Gravitationally Lensed Galaxy

Author: Nicolas Laporte, Richard S. Ellis, Ismael Perez-Fournon, D. Quénard, Guido Roberts-Borsani, Roser Pello, Frédéric Boone, Alina Streblyanska, Franz E. Bauer, Institut de recherche en astrophysique et planétologie ( IRAP ), Université Paul Sabatier - Toulouse 3 ( UPS ) -Observatoire Midi-Pyrénées ( OMP ) -Centre National de la Recherche Scientifique ( CNRS ), Institut de recherche en astrophysique et planétologie (IRAP), Université Toulouse III - Paul Sabatier (UT3), Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées-Observatoire Midi-Pyrénées (OMP), Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS), Institut national des sciences de l'Univers (INSU - CNRS)-Université Toulouse III - Paul Sabatier (UT3), and Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Centre National de la Recherche Scientifique (CNRS)
Subjects: submillimeter: galaxies, Stellar mass, [ PHYS.ASTR ] Physics [physics]/Astrophysics [astro-ph], Astrophysics::Cosmology and Extragalactic Astrophysics, Astrophysics, 01 natural sciences, Spectral line, galaxies: high-redshift, 0103 physical sciences, galaxies: formation, Astrophysics::Solar and Stellar Astrophysics, 010303 astronomy & astrophysics, Reionization, Astrophysics::Galaxy Astrophysics, Photometric redshift, Physics, 010308 nuclear & particles physics, Astrophysics::Instrumentation and Methods for Astrophysics, Astronomy and Astrophysics, Atacama Large Millimeter Array, early universe, Galaxy, Redshift, Abell 2744, Space and Planetary Science, galaxies: star formation, Astrophysics::Earth and Planetary Astrophysics, [PHYS.ASTR]Physics [physics]/Astrophysics [astro-ph], galaxies: evolution
Abstract: International audience; We report on the detailed analysis of a gravitationally lensed Y-band dropout, A2744_YD4, selected from deep Hubble Space Telescope imaging in the Frontier Field cluster Abell 2744. Band 7 observations with the Atacama Large Millimeter/submillimeter Array (ALMA) indicate the proximate detection of a significant 1 mm continuum flux suggesting the presence of dust for a star-forming galaxy with a photometric redshift of $z\simeq 8$. Deep X-SHOOTER spectra confirms the high-redshift identity of A2744_YD4 via the detection of Lyα emission at a redshift z = 8.38. The association with the ALMA detection is confirmed by the presence of [O iii] 88 μm emission at the same redshift. Although both emission features are only significant at the 4σ level, we argue their joint detection and the positional coincidence with a high-redshift dropout in the Hubble Space Telescope images confirms the physical association. Analysis of the available photometric data and the modest gravitational magnification ($\mu \simeq 2$) indicates A2744_YD4 has a stellar mass of ∼2 × 10(9) ${M}_{\odot }$, a star formation rate of ∼20 ${M}_{\odot }$ yr(−)(1) and a dust mass of ∼6 × 10(6) ${M}_{\odot }$. We discuss the implications of the formation of such a dust mass only $\simeq 200\,\mathrm{Myr}$ after the onset of cosmic reionization.
Published: 2017
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23. Modeling the physical structure of star-forming regions with LIME, a 3D radiative transfer code

Author: Emmanuel Caux, Sandrine Bottinelli, and D. Quénard
Subjects: Physics, Physical structure, Space and Planetary Science, General Engineering, engineering, Code (cryptography), Radiative transfer, Astronomy and Astrophysics, Star (graph theory), engineering.material, Line (formation), Lime, Computational physics
Abstract: The ability to predict line emission is crucial in order to make a comparison with observations. From LTE to full radiative transfer codes, the goal is always to derive the most accurately possible the physical properties of the source. Non-LTE calculations can be very time consuming but are needed in most of the cases since many studied regions are far from LTE.
Published: 2015
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24. HCO+and N2H+as ionisation tracers in the low-mass protostar IRAS16293-2422

Author: Emmanuel Caux, Sandrine Bottinelli, and D. Quénard
Subjects: Physics, Space and Planetary Science, Chemical physics, Ionization, General Engineering, Protostar, Molecule, Astronomy and Astrophysics, Electron, Astrophysics, Low Mass, Organic molecules, Ion
Abstract: Ionisation in the molecular environment of star-forming regions gives important clues on the chemical processes that take place in the environment of a young protostar. Ionisation can be traced with molecules like HCO+ and N2 H+ and it regulates the formation of larger molecules such as complex organic molecules (COMs). The ionisation degree can also play an important role in the free-fall timescale of the protostar since it prevents the neutral material to collapse through collisions with ions and electrons bound to the magnetic field of the central protostar.
Published: 2015
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25. Transferts conductifs et radiatifs dans les matériaux du bâtiment : état de l’art et progrès récents

Author: F. Olive, H. Sallée, D. Giraud, B. Chevalier, and D. Quénard
Subjects: Materials Chemistry, Metals and Alloys, Physical and Theoretical Chemistry, Condensed Matter Physics
Published: 1999
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26. Phosphorus-bearing molecules in the Galactic Center

Author: Sergio Martín, Izaskun Jiménez-Serra, S. Viti, Rebeca Aladro, Jesús Martín-Pintado, Jairo Armijos-Abendaño, D. Quénard, Francesco Fontani, Shaoshan Zeng, M. A. Requena-Torres, M. T. Beltrán, Victor M. Rivilla, and Denise Riquelme
Subjects: Physics, 010504 meteorology & atmospheric sciences, Star formation, Molecular cloud, Phosphorus, Galactic Center, FOS: Physical sciences, chemistry.chemical_element, Astronomy and Astrophysics, Cosmic ray, Astrophysics, Radiation, 01 natural sciences, Astrophysics - Astrophysics of Galaxies, Interstellar medium, chemistry, 13. Climate action, Space and Planetary Science, Astrophysics of Galaxies (astro-ph.GA), 0103 physical sciences, Molecule, 010303 astronomy & astrophysics, 0105 earth and related environmental sciences
Abstract: Phosphorus (P) is one of the essential elements for life due to its central role in biochemical processes. Recent searches have shown that P-bearing molecules (in particular PN and PO) are present in star-forming regions, although their formation routes remain poorly understood. In this Letter, we report observations of PN and PO towards seven molecular clouds located in the Galactic Center, which are characterized by different types of chemistry. PN is detected in five out of seven sources, whose chemistry is thought to be shock-dominated. The two sources with PN non-detections correspond to clouds exposed to intense UV/X-rays/cosmic-ray radiation. PO is detected only towards the cloud G+0.693$-$0.03, with a PO/PN abundance ratio of $\sim$1.5. We conclude that P-bearing molecules likely form in shocked gas as a result of dust grain sputtering, while are destroyed by intense UV/X-ray/cosmic ray radiation., 5 pages, 3 figures, 2 tables, accepted for publication in MNRAS Letters

27. Dust in the Reionization Era: ALMA Observations of a z = 8.38 Gravitationally Lensed Galaxy.

Author: N. Laporte, R. S. Ellis, F. Boone, F. E. Bauer, D. Quénard, G. W. Roberts-Borsani, R. Pelló, I. Pérez-Fournon, and A. Streblyanska
Published: 2017
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28. Astrochemical evolution along star formation: Overview of the IRAM Large Program ASAI.

Author: Lefloch B, Bachiller R, Ceccarelli C, Cernicharo J, Codella C, Fuente A, Kahane C, López-Sepulcre A, Tafalla M, Vastel C, Caux E, González-García M, Bianchi E, Gómez-Ruiz A, Holdship J, Mendoza E, Ospina-Zamudio J, Podio L, Quénard D, Roueff E, Sakai N, Viti S, Yamamoto S, Yoshida K, Favre C, Monfredini T, Quitián-Lara HM, Marcelino N, Boechat-Roberty HM, and Cabrit S
Abstract: Evidence is mounting that the small bodies of our Solar System, such as comets and asteroids, have at least partially inherited their chemical composition from the first phases of the Solar System formation. It then appears that the molecular complexity of these small bodies is most likely related to the earliest stages of star formation. It is therefore important to characterize and to understand how the chemical evolution changes with solar-type protostellar evolution. We present here the Large Program "Astrochemical Surveys At IRAM" (ASAI). Its goal is to carry out unbiased millimeter line surveys between 80 and 272 GHz of a sample of ten template sources, which fully cover the first stages of the formation process of solar-type stars, from prestellar cores to the late protostellar phase. In this article, we present an overview of the surveys and results obtained from the analysis of the 3 mm band observations. The number of detected main isotopic species barely varies with the evolutionary stage and is found to be very similar to that of massive star-forming regions. The molecular content in O- and C- bearing species allows us to define two chemical classes of envelopes, whose composition is dominated by either a) a rich content in O-rich complex organic molecules, associated with hot corino sources, or b) a rich content in hydrocarbons, typical of Warm Carbon Chain Chemistry sources. Overall, a high chemical richness is found to be present already in the initial phases of solar-type star formation.
Published: 2018
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28 results on '"D. Quénard"'

1. Chemical modelling of complex organic molecules with peptide-like bonds in star-forming regions

2. Detection of methyl isocyanate (CH3NCO) in a solar-type protostar

3. Seeds of Life in Space (SOLIS)

4. Modelling the 3D physical structure of astrophysical sources with gass

5. First detection of the pre-biotic molecule glycolonitrile (HOCH2CN) in the interstellar medium

6. Astrochemical evolution along star formation: overview of the IRAM Large Program ASAI

7. Sulphur chemistry in the L1544 pre-stellar core

8. 3D modelling of HCO$^+$ and its isotopologues in the low-mass proto-star IRAS16293$-$2422

9. Chemical modelling of N-bearing COMs in star-forming regions

10. The fate of formamide in a fragmenting protoplanetary disc

11. Chemical modelling of glycolaldehyde and ethylene glycol in star-forming regions

12. On the Nature of the Compact Sources in IRAS 16293–2422 Seen at Centimeter to Submillimeter Wavelengths

13. Seeds of Life in Space (SOLIS): I. Carbon-chain growth in the Solar-type protocluster OMC2-FIR4

14. Seeds of Life in Space (SOLIS). II. Formamide in protostellar shocks: Evidence for gas-phase formation

15. High spectral resolution observations of HNC3 and HCCNC in the L1544 prestellar core

16. The ALMA Frontier Fields Survey - II. Multiwavelength Photometric analysis of 1.1mm continuum sources in Abell 2744, MACSJ0416.1-2403 and MACSJ1149.5+2223

17. Detection of the HC$_3$NH$^+$ and HCNH$^+$ ions in the L1544 pre-stellar core

18. Seeds Of Life In Space (SOLIS): The Organic Composition Diversity at 300-1000 au Scale in Solar-type Star-forming Regions

19. History of the solar-type protostar IRAS 16293–2422 as told by the cyanopolyynes

20. MULTI-EPOCH VLA OBSERVATIONS OF IRAS 16293-2422B AND THE MODELING OF ITS CONTINUUM EMISSION

21. Detectability of deuterated water in prestellar cores

22. Dust in the Reionization Era: ALMA Observations of a z = 8.38 Gravitationally Lensed Galaxy

23. Modeling the physical structure of star-forming regions with LIME, a 3D radiative transfer code

24. HCO+and N2H+as ionisation tracers in the low-mass protostar IRAS16293-2422

25. Transferts conductifs et radiatifs dans les matériaux du bâtiment : état de l’art et progrès récents

26. Phosphorus-bearing molecules in the Galactic Center

27. Dust in the Reionization Era: ALMA Observations of a z = 8.38 Gravitationally Lensed Galaxy.

28. Astrochemical evolution along star formation: Overview of the IRAM Large Program ASAI.

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28 results on '"D. Quénard"'

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