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The Stark effect provides a powerful method to shift the spectra of molecules, atoms and electronic transitions in general, becoming one of the simplest and most straightforward way to tune the frequency of quantum emitters by means of a static electric field. At the same time, in order to reduce the emitter sensitivity to charge noise, inversion symmetric systems are typically designed, providing a stable emission frequency, with a quadratic-only dependence on the applied field. However, such nonlinear behaviour might reflect in correlations between the tuning ability and unwanted spectral fluctuations. Here, we provide experimental evidence of this trend, using molecular quantum emitters in the solid state cooled down to liquid helium temperatures. We finally combine the electric field generated by electrodes, which results parallel to the molecule induced dipole, to optically excite long-lived charge states, acting in the perpendicular direction. Based on the anisotropy of the molecule's polarizability, our two-dimensional control of the local electric field allows not only to tune the emitter's frequency but also to sensibly suppress the spectral instabilities associated to field fluctuations.

We study the quantum dynamics in response to time-dependent external potentials of the edge modes of a small fractional quantum Hall fluid composed of few particles on a lattice in a bosonic Laughlin-like state at filling {\nu} = 1/2. We show that the nonlinear chiral Luttinger liquid theory provides a quantitatively accurate description even for the small lattices that are available in state-of-the-art experiments, away from the continuum limit. Experimentally-accessible data related to the quantized value of the bulk transverse Hall conductivity are identified both in the linear and the non-linear response to an external excitation. The strong nonlinearity induced by the open boundaries is responsible for sizable quantum blockade effects, leading to the generation of nonclassical states of the edge modes., Comment: 4+15 pages

In this tutorial review, we briefly discuss the role that the Jaynes-Cummings model occupies in present-day research in cavity quantum electrodynamics with a particular focus on the so-called ultrastrong coupling regime. We start by critically analyzing the various approximations required to distill such a simple model from standard quantum electrodynamics. We then discuss how many of those approximations can, and often have been broken in recent experiments. The consequence of these failures has been the need to abandon the Jaynes-Cummings model for more complex models. In this, the quantum Rabi model has the most prominent role and we will rapidly survey its rich and peculiar phenomenology. We conclude the paper by showing how the Jaynes-Cummings model still plays a crucial role even in non-perturbative light-matter coupling regimes., Comment: Included in the special issue 'The Jaynes-Cummings Model: 60 Years and Still Counting'

We theoretically study how the peculiar properties of the vacuum state of an ultra-strongly coupled system can affect basic light-matter interaction processes. In this unconventional electromagnetic environment, an additional emitter no longer couples to the bare cavity photons, but rather to the polariton modes emerging from the ultra-strong coupling. As such, the effective light-matter interaction strength is sensitive to the properties of the distorted vacuum state. Different interpretations of our predictions in terms of modified quantum fluctuations in the vacuum state and of radiative reaction in classical electromagnetism are critically discussed. Whereas our discussion is focused on the experimentally most relevant case of intersubband polaritons in semiconductor devices, our framework is fully general and applies to generic material systems., Comment: Revised version in extensive regular article

We study the open relaxation dynamics of an asymmetric dipole that is ultrastrongly coupled to a single electromagnetic cavity mode. By using a thermalizing master equation for the whole interacting system we derive a phase diagram of the Liouvillian gap. It emerges that the ultrastrong coupling inhibits the system relaxation toward the equilibrium state due to an exponential suppression of the dipole tunneling rate. However, we find that polaronic multi-photon resonances restore fast relaxation by a cavity-mediated dipole resonant tunneling process. Aside of the numerical evidences, we develop a fully analytical description by diagonalizing the Rabi model through a generalized rotating-wave approximation, valid in the so-called polaron frame. The relaxation physics of such ultrastrong-coupling systems is then reduced to a multi-photon polaron version of the standard text-book dressed states picture. At the end we discuss an extension to a multi-well dipole that can set the basis of a cascaded resonant tunnelling setup in the ultrastrong coupling regime.

We study light-matter interactions in the bulk of a two-dimensional photonic lattice system, where photons are subject to the combined effect of a synthetic magnetic field and an orthogonal synthetic electric field. In this configuration, chiral waveguide modes appear in the bulk region of the lattice, in direct analogy to transverse Hall currents in electronic systems. By evaluating the non-Markovian dynamics of emitters that are coupled to those modes, we identify critical coupling conditions, under which the shape of the spontaneously emitted photons becomes almost fully symmetric. Combined with a directional, dispersionless propagation, this property enables a complete reabsorption of the photon by another distant emitter, without relying on any time-dependent control. We show that this mechanism can be generalized to arbitrary in-plane synthetic potentials, thereby enabling flexible realizations of re-configurable networks of quantum emitters with arbitrary chiral connectivity.

We address the fundamental question whether or not it is possible to achieve conditions under which the coupling of a single dipole to a strongly confined electromagnetic vacuum can result in non-perturbative corrections to the dipole's ground state. To do so we consider two simplified, but otherwise rather generic cavity QED setups, which allow us to derive analytic expressions for the total ground state energy and to distinguish explicitly between purely electrostatic and genuine vacuum-induced contributions. Importantly, this derivation takes the full electromagnetic spectrum into account while avoiding any ambiguities arising from an ad-hoc mode truncation. Our findings show that while the effect of confinement per se is not enough to result in substantial vacuum-induced corrections, the presence of high-impedance modes, such as plasmons or engineered LC resonances, can drastically increase these effects. Therefore, we conclude that with appropriately designed experiments it is at least in principle possible to access a regime where light-matter interactions become non-perturbative., Comment: 20 pages, 10 figures

We analyse the effect of a strong perpendicular magnetic field on an intersubband transition in a disordered doped quantum well strongly coupled to an optical cavity. The magnetic field changes the lineshape of the intersubband optical transition due to the interface roughness of the quantum well from a Lorentzian to a Gaussian one. In this regime, a novel form of magnetic-field-induced cavity protection sets in, which strongly reduces the polariton linewidth to the cavity contribution only. Implications of our results for fundamental studies of nonlinear polariton dynamics and for technological applications to polariton lasers are finally highlighted.

We theoretically investigate the effect of optical-force-mediated interactions onto the quantum dynamics of a pair of dielectric nanospheres optically trapped in two neighboring optical tweezers. Thanks to the interference between the tweezer beams and the elastically scattered light by the other nanosphere, the effective inter nanosphere coupling can reach the ultrastrong coupling regime. Experimentally accessible signatures of the entangled nature of the quantum ground state are highlighted, including entanglement witnesses based on position/momentum correlation functions and a sizable dynamical Casimir excitation upon a fast modulation of the tweezer's properties., Comment: We found a flaw in the main physical assumptions. Despite the math is correct, the article arrives to false predictions

We study light-matter interactions in two dimensional photonic systems in the presence of a spatially homogeneous synthetic magnetic field for light. Specifically, we consider one or more two-level emitters located in the bulk region of the lattice, where for increasing magnetic field the photonic modes change from extended plane waves to circulating Landau levels. This change has a drastic effect on the resulting emitter-field dynamics, which becomes intrinsically non-Markovian and chiral, leading to the formation of strongly coupled Landau-photon polaritons. The peculiar dynamical and spectral properties of these quasi-particles can be probed with state-of-the-art photonic lattices in the optical and the microwave domain and may find various applications for the quantum simulation of strongly interacting topological models.

The structure of solids and their phases is mainly determined by static Coulomb forces while the coupling of charges to the dynamical, i.e., quantized degrees of freedom of the electromagnetic field plays only a secondary role. Recently, it has been speculated that this general rule can be overcome in the context of cavity quantum electrodynamics (QED), where the coupling of dipoles to a single field mode can be dramatically enhanced. Here we present a first exact analysis of the ground states of a dipolar cavity QED system in the non-perturbative coupling regime, where electrostatic and dynamical interactions play an equally important role. Specifically, we show how strong and long-range vacuum fluctuations modify the states of dipolar matter and induce novel phases with unusual properties. Beyond a purely fundamental interest, these general mechanisms can be important for potential applications, ranging from cavity-assisted chemistry to quantum technologies based on ultrastrongly coupled circuit QED systems., Comment: 25 pages, 5 figures (+ 5 in Appendix)

We study the thermodynamic properties of a system of two-level dipoles that are coupled ultrastrongly to a single cavity mode. By using exact numerical and approximate analytical methods, we evaluate the free energy of this system at arbitrary interaction strengths and discuss strong-coupling modifications of derivative quantities such as the specific heat or the electric susceptibility. From this analysis we identify the lowest-order cavity-induced corrections to those quantities in the collective ultrastrong coupling regime and show that for even stronger interactions the presence of a single cavity mode can strongly modify extensive thermodynamic quantities of a large ensemble of dipoles. In this non-perturbative coupling regime we also observe a significant shift of the ferroelectric phase transition temperature and a characteristic broadening and collapse of the black-body spectrum of the cavity mode. Apart from a purely fundamental interest, these general insights will be important for identifying potential applications of ultrastrong-coupling effects, for example, in the field of quantum chemistry or for realizing quantum thermal machines., Comment: 16 pages, 7 figures

We revisit the derivation of Rabi- and Dicke-type models, which are commonly used for the study of quantum light-matter interactions in cavity and circuit QED. We demonstrate that the validity of the two-level approximation, which is an essential step in this derivation, depends explicitly on the choice of gauge once the system enters the ultrastrong coupling regime. In particular, while in the electric dipole gauge the two-level approximation can be performed as long as the Rabi frequency remains much smaller than the energies of all higher-lying levels, it can dramatically fail in the Coulomb gauge, even for systems with an extremely anharmonic spectrum. We extensively investigate this phenomenon both in the single-dipole (Rabi) and multi-dipole (Dicke) case, and considering the specific examples of dipoles confined by double-well and by square-well potentials, and of circuit QED systems with flux qubits coupled to an LC resonator., Comment: See also related independent work arxiv:1805.06356

We study a generic cavity-QED system where a set of (artificial) two-level dipoles is coupled to the electric field of a single-mode LC resonator. This setup is used to derive a minimal quantum mechanical model for cavity QED, which accounts for both dipole-field and direct dipole-dipole interactions. The model is applicable for arbitrary coupling strengths and allows us to extend the usual Dicke model into the non-perturbative regime of QED, where the dipole-field interaction can be associated with an effective finestructure constant of order unity. In this regime, we identify three distinct classes of normal, superradiant and subradiant vacuum states and discuss their characteristic properties and the transitions between them. Our findings reconcile many of the previous, often contradictory predictions in this field and establish a common theoretical framework to describe ultrastrong coupling phenomena in a diverse range of cavity-QED platforms.