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Higgs and Goldstone modes manifest as fluctuations in the order parameter of system, offering insights into its phase transitions and symmetry properties. Exploring the dynamics of these collective excitations in a Rydberg atoms system advances various branches of condensed matter, particle physics, and cosmology. Here, we report an experimental signature of Higgs and Goldstone modes in a U(1) symmetry-broken Rydberg atomic gases. By constructing two probe fields to excite atoms, we observe the distinct phase and amplitude fluctuations of Rydberg atoms collective excitations under the particle-hole symmetry. Due to the van der Waals interactions between the Rydberg atoms, we detect a symmetric variance spectrum divided by the divergent regime and phase boundary, capturing the full dynamics of the additional Higgs and Goldstone modes. Studying the Higgs and Goldstone modes in Rydberg atoms allows us to explore fundamental aspects of quantum phase transitions and symmetry breaking phenomena, while leveraging the unique properties of these highly interacting systems to uncover new physics and potential applications in quantum simulation.

Study of phase transitions provide insights into how a many-body system behaves under different conditions, enabling us to understand the symmetry breaking, critical phenomena, and topological properties. Strong long-range interactions in highly excited Rydberg atoms create a versatile platform for exploring exotic emergent topological phases. Here, we report the experimental observation of dynamical topological phase transitions in cold Rydberg atomic gases under a microwave field driving. By measuring the system transmission curves while varying the probe intensity, we observe complex hysteresis trajectories characterized by distinct winding numbers as they cross the critical point. At the transition state, where the winding number flips, the topology of these hysteresis trajectories evolves into more non-trivial structures. The topological trajectories are shown to be robust against noise, confirming their rigidity in dynamic conditions. These findings contribute to the insights of emergence of complex dynamical topological phases in many-body systems.

The interactions between Rydberg atoms and microwave fields provide a valuable framework for studying the complex dynamics out of equilibrium, exotic phases, and critical phenomena in many-body physics. This unique interplay allows us to explore various regimes of nonlinearity and phase transitions. Here, we observe a phase transition from the state in the regime of bistability to that in multistability in strongly interacting Rydberg atoms by varying the microwave field intensity, accompanying with the breaking of Z3-symmetry. During the phase transition, the system experiences a hidden critical point, in which the multistable states are difficult to be identified. Through changing the initial state of system, we can identify a hidden multistable state and reveal a hidden trajectory of phase transition, allowing us to track to a hidden critical point. In addition, we observe multiple phase transitions in spectra, suggesting higher-order symmetry breaking. The reported results shed light on manipulating multistability in dissipative Rydberg atoms systems and hold promise in the applications of non-equilibrium many-body physics., Comment: 10 pages, 5 figures

The interplay between strong long-range interactions and the coherent driving contribute to the formation of complex patterns, symmetry, and novel phases of matter in many-body systems. However, long-range interactions may induce an additional dissipation channel, resulting in non-Hermitian many-body dynamics and the emergence of exceptional points in spectrum. Here, we report experimental observation of interaction-induced exceptional points in cold Rydberg atomic gases, revealing the breaking of charge-conjugation parity symmetry. By measuring the transmission spectrum under increasing and decreasing probe intensity, the interaction-induced hysteresis trajectories are observed, which give rise to non-Hermitian dynamics. We record the area enclosed by hysteresis loops and investigate the dynamics of hysteresis loops. The reported exceptional points and hysteresis trajectories in cold Rydberg atomic gases provide valuable insights into the underlying non-Hermitian physics in many-body systems, allowing us to study the interplay between long-range interactions and non-Hermiticity.

Detecting and controlling the chirality of materials play an essential role in exploring nature, providing new avenues for material creation, discrimination, and manipulation. In such tasks, chiral reagents are essential in defining or enhancing the chiral dichroism response. However, ignoring their influences on the symmetry of the medium hamper the ability to control and induce asymmetric synthesis. Here, we propose a simple but versatile chirality transfer method for synthesizing and manipulating the chirality of medium. The proposed method induces the dispersion of light in a neutral atomic system, allowing to deterministically and tunably control the chirality transfer using a helical field. First, we theoretically analyze the mechanism for this optically induced chirality transfer. Afterwards, we experimentally study the enantio-sensitive feature of the medium exposed to the auxiliary chiral field. This result can be suppressed or enhanced in a deterministic enantio-selection, opening up an efficient way to manipulate asymmetric synthesis., Comment: 16 pages, 6 figures

Crystal seeding enables a deeper understanding of phase behavior, leading to the development of methods for controlling and manipulating phase transitions in various applications such as materials synthesis, crystallization processes, and phase transformation engineering. How to seed a crystalline in time domain is an open question, which is of great significant and may provide an avenue to understand and control time-dependent quantum many-body physics. Here, we utilize a microwave pulse as a seed to induce the formation of a discrete time crystal in Floquet driven Rydberg atoms. In the experiment, the periodic driving on Rydberg states acts as a seeded crystalline order in subspace, which triggers the time-translation symmetry breaking across the entire ensemble. The behavior of the emergent time crystal is elaborately linked to alterations in the seed, such as the relative phase shift and the frequency difference, which result in phase dependent seeding and corresponding shift in periodicity of the time crystal, leading to embryonic synchronization. This result opens up new possibilities for studying and harnessing time-dependent quantum many-body phenomena, offering insights into the behavior of complex many-body systems under seeding.

Detecting microwave signals over a wide frequency range has numerous advantages as it enables simultaneous transmission of a large amount of information and access to more spectrum resources. This capability is crucial for applications such as microwave communication, remote sensing, and radar. However, conventional microwave receiving systems are limited by amplifiers and band-pass filters that can only operate efficiently in a specific frequency range. Typically, these systems can only process signals within a three-fold frequency range, which limits the data transfer bandwidth of the microwave communication systems. Developing novel atom-integrated microwave sensors, for example, radio frequency (RF)-chip coupled Rydberg atomic receiver, provides opportunities for a large working bandwidth of microwave sensing at the atomic level. Here, an ultra-wide dual-band RF sensing scheme is demonstrated by space-division multiplexing two RF-chip-integrated atomic receiver modules. The system can simultaneously receive dual-band microwave signals that span a frequency range exceeding 6 octaves (300 MHz and 24 GHz). This work paves the way for multi-band microwave reception applications within an ultra-wide range by RF-chip-integrated Rydberg atomic sensor., Comment: 11 pages, 5 figures

The identification of tipping points is essential for prediction of collapses or other sudden changes in complex systems. Applications include studies of ecology, thermodynamics, climatology, and epidemiology. However, detecting early signs of proximity to a tipping is made challenging by complexity and non-linearity. Strongly interacting Rydberg atom gases offer model systems that offer both complexity and non-linearity, including phase transition and critical slowing down. Here, via an external probe we observe prior warning of the proximity of a phase transition of Rydberg thermal gases. This warning signal is manifested as a deviation from linear growth of the variance with increasing probe intensity. We also observed the dynamics of the critical slowing down behavior versus different time scales, and atomic densities, thus providing insights into the study of a Rydberg atom system's critical behavior. Our experiment suggests that the full critical slowing down dynamics of strongly-interacting Rydberg atoms can be probed systematically, thus providing a benchmark with which to identify critical phenomena in quantum many-body systems.

Engineering a Terahertz (THz) frequency comb spectroscopy at atomic level advances the precisely measurement in spectroscopy and sensing. Current progresses on THz frequency comb rely on difference-frequency generation, optical parametric oscillation, and other methods. Generating a THz frequency comb poses challenges in source stability and achieving a narrow bandwidth, which traditional THz devices are difficult to achieve. Furthermore, accurately measuring the generated THz frequency comb necessitates a high-performance THz detector. Rydberg atoms are well-suited for electric field sensing due to their ultra-wide radio frequency transition energy levels, making them especially sensitive to external electric fields in the DC to THz bandwidth. However, there have been no reports about generating THz frequency comb spectroscopy at the atomic level until now. This work presents a THz frequency comb spectroscopy with Rydberg atoms, in which a Floquet comb-like transition is engineered through a time-periodic drive field. Our approach simplifies the setup required for THz frequency comb spectroscopy while extending the working bandwidth for Rydberg atomic sensors. The THz frequency comb spectroscopy at the atomic level reported in this article shows great potential for various applications in astronomy, remote sensing, spectral detection of biological samples, and other related fields.

Developing microwave electric field sensing based on Rydberg atom has received significant attention due to its unique advantages. However, achieving effective coupling between Rydberg atom and the microwave electric field in the sensing process is a challenging problem that greatly impacts the sensitivity. To address this, we propose the use of a microwave resonant cavity to enhance the effective coupling between the Rydberg atoms and the microwave electric field. In our experiment, we use a three-photon excitation scheme to prepare Rydberg atoms, make measurements of electric fields without and with a microwave cavity in which the vapor cell is put inside. Through experimental testing, we achieve an 18 dB enhancement of power sensitivity. The experiment shows an effective enhancement in electric field pulse signal detection. This result provides a promising direction for enhancing the sensitivity of Rydberg atomic electric field sensors and paves the way for their application in precision electric field measurements.

Efficient and tunable qubit unidirectional routers and spin-wave diodes play an important role in both classical and quantum information processing domains. Here, we reveal that multi-level neutral cold atoms can mediate both dissipative and coherent couplings. Interestingly, we investigate and practically implement this paradigm in experiments, successfully synthesizing a system with dual functionality as both a photonic qubit unidirectional router and a spin-wave diode. By manipulating the helicity of the field, we can effectively balance the coherence coupling and dissipative channel, thereby ensuring the unidirectional transfer of photonic qubits. The qubit fidelity exceeds 97.49%, and the isolation ratio achieves $16.8\pm0.11$ dB while the insertion loss is lower than 0.36 dB. Furthermore, we show that the spin-wave diode can effectively achieve unidirectional information transfer by appropriately setting the coherent coupling parameters. Our work not only provides new ideas for the design of extensive components in quantum networks, but also opens up new possibilities for non-Hermitian quantum physics, complex quantum networks, and unidirectional quantum information transfer., Comment: 7 pages, 4 figures

Higher-order and fractional discrete time crystals (DTCs) are exotic phases of matter where the discrete time translation symmetry is broken into higher-order and non-integer category. Generation of these unique DTCs has been widely studied theoretically in different systems. However, no current experimental methods can probe these higher-order and fractional DTCs in any quantum many-body systems. We demonstrate an experimental approach to observe higher-order and fractional DTCs in Floquet-driven Rydberg atomic gases. We have discovered multiple $n$-DTCs with integer values of $n$ = 2, 3, and 4, and others ranging up to 14, along with fractional $n$-DTCs with $n$ values beyond the integers. The system response can transition between adjacent integer DTCs, during which the fractional DTCs are investigated. Study of higher-order and fractional DTCs expands fundamental knowledge of non-equilibrium dynamics and is promising for discovery of more complex temporal symmetries beyond the single discrete time translation symmetry., Comment: Added references

A time crystal is an exotic phase of matter where time-translational symmetry is broken; this phase differs from the spatial symmetry breaking induced in crystals in space. Lots of experiments report the transition from a thermal equilibrium phase to time crystal phase. However, there is no experimental method to probe the bifurcation effect of distinct time crystals in quantum many-body systems. Here, in a driven and dissipative many-body Rydberg atom system, we observe multiple continuous dissipative time crystals and emergence of more complex temporal symmetries beyond the single time crystal phase. Bifurcation of time crystals in strongly interacting Rydberg atoms is observed; the process manifests as a transition from a time crystal state of long temporal order to one of short temporal order, or vice versa. By manipulating the driving field parameters, we observe the time crystal's bistability and a hysteresis loop. These investigations indicate new possibilities for control and manipulation of the temporal symmetries of non-equilibrium systems., Comment: Added references

Quantum many-body systems near phase transitions respond collectively to externally applied perturbations. We explore this phenomenon in a laser-driven dissipative Rydberg gas that is tuned to a bistable regime. Here two metastable phases coexist, which feature a low and high density of Rydberg atoms, respectively. The ensuing collective dynamics, which we monitor in situ, is characterized by stochastic collective jumps between these two macroscopically distinct many-body phases. We show that the statistics of these jumps can be controlled using a dual-tone microwave field. In particular, we find that the distribution of jump times develops peaks corresponding to subharmonics of the relative microwave detuning. Our study demonstrates the control of collective statistical properties of dissipative quantum many-body systems without the necessity of fine-tuning or of ultra cold temperatures. Such robust phenomena may find technological applications in quantum sensing and metrology.

Inherent spin angular momentum (SAM) and orbital angular momentum (OAM) which manifest as polarization and spatial degrees of freedom (DOF) of photons, hold a promise of large capability for applications in classical and quantum information processing. To enable these photonic spin and orbital dynamic properties strongly coupled with each other, Poincar\'{e} states have been proposed and offer advantages in data multiplexing, information encryption, precision metrology, and quantum memory. However, since the transverse size of Laguerre Gaussian beams strongly depends on their topological charge numbers $\left| l \right|$, it is difficult to store asymmetric Poincar\'{e} states due to the significantly different light-matter interaction for distinct spatial modes. Here, we experimentally realize the storage of perfect Poincar\'{e} states with arbitrary OAM quanta using the perfect optical vortex, in which 121 arbitrarily-selected perfect Poincar\'{e} states have been stored with high fidelity. The reported work has great prospects in optical communication and quantum networks for dramatically increased encoding flexibility of information.

Microwave sensing has important applications in areas such as data communication and remote sensing, so it has received much attention from international academia, industry, and governments. Atomic wireless sensing uses the strong response of the large electric dipole moment of a Rydberg atom to an external field to achieve precise measurement of a radio frequency (RF) electric field. This has advantages over traditional wireless sensing. The advantage of a Rydberg atom is its ultra-wide energy level transitions, which make it responsive to RF electric fields over a wide bandwidth. Here, we briefly review the progress of electric field measurement based on Rydberg atoms. The main contents include the properties of Rydberg atoms, measurement using Rydberg atoms, and experimental progress in electric field measurement in different bands. We show the different methods for detecting electric fields such as atomic superheterodyne, machine learning, and critically enhanced measurement. The development of Rydberg atomic measurement focuses on the advantages of Rydberg atomic sensing, especially compared with conventional microwave receivers. This is of major significance to developing Rydberg-based measurement in astronomy, remote sensing, and other fields., Comment: 16 pages, 10 figures

It is challenging to probe ergodicity breaking trends of a quantum many-body system when dissipation inevitably damages quantum coherence originated from coherent coupling and dispersive two-body interactions. Rydberg atoms provide a test bed to detect emergent exotic many-body phases and non-ergodic dynamics where the strong Rydberg atom interaction competes with and overtakes dissipative effects even at room temperature. Here we report experimental evidence of a transition from ergodic towards ergodic breaking dynamics in driven-dissipative Rydberg atomic gases. The broken ergodicity is featured by the long-time phase oscillation, which is attributed from the formation of Rydberg excitation clusters in limit cycle phases. The broken symmetry in the limit cycle is a direct manifestation of many-body interactions, which is verified by tuning atomic densities in our experiment. The reported result reveals that Rydberg many-body systems are a promising candidate to probe ergodicity breaking dynamics, such as limit cycles, and enable the benchmark of non-equilibrium phase transition.

One of the major difficulties in realizing a high-dimensional frequency converter for conventional optical vortex (COV) stems from the difference in ring diameter of COV modes with different topological charge numbers l. Here, we implement a high-dimensional frequency convertor for perfect optical vortex (POV) modes with invariant size through the four-wave mixing (FWM) process by utilizing Bessel-Gaussian beams instead of Laguerre-Gaussian beams. The measured conversion efficiency from 1530 nm to 795 nm is independent of l at least in subspace of {-6,...,6}, and the achieved conversion fidelities for two-dimensional (2D) superposed POV states exceed 97%. We further realize the frequency conversion of 3D, 5D and 7D superposition states with fidelities as high as 96.70%, 89.16% and 88.68%, respectively. The reported scheme is implemented in hot atomic vapor, it's also compatible with the cold atomic system and may find applications in high-capacity and long-distance quantum communication.

Building an efficient quantum memory in high-dimensional Hilbert spaces is one of the fundamental requirements for establishing high-dimensional quantum repeaters, where it offers many advantages over two-dimensional quantum systems, such as a larger information capacity and enhanced noise resilience. To date, there have been no reports about how to achieve an efficient high-dimensional quantum memory. Here, we experimentally realize a quantum memory that is operational in Hilbert spaces of up to 25 dimensions with a storage efficiency of close to 60%. The proposed approach exploits the spatial-mode-independent interaction between atoms and photons which are encoded in transverse size-invariant orbital angular momentum modes. In particular, our memory features uniform storage efficiency and low cross-talk disturbance for 25 individual spatial modes of photons, thus allowing storing arbitrary qudit states programmed from 25 eigenstates within the high-dimensional Hilbert spaces, and eventually contributing to the storage of a 25-dimensional qudit state. These results would have great prospects for the implementation of long-distance high-dimensional quantum networks and quantum information processing.

Infrared optical measurement has a wide range of applications in industry and science, but infrared light detectors suffer from high costs and inferior performance than visible light detectors. Four-wave mixing (FWM) process allows detection in the infrared range by detecting correlated visible light. We experimentally investigate the stimulated FWM process in a hot $^{85}$Rb atomic vapor cell, in which a weak infrared signal laser at $1530~$nm induces the FWM process and is amplified and converted into a strong FWM light at $780~$nm, the latter can be detected more easily. We find the optimized single- and two-photon detunings by studying the dependence of the frequency of input laser on the generated FWM light. What's more, the power gain increases rapidly as the signal intensity decreases, which is consistent with our theoretical analysis. As a result, the power gain can reach up to 500 at a signal laser power of $0.1~\mu$W and the number of detected photons increased by a factor of 250. Finally, we experimentally prove that our amplification process can work in a broad band in the frequency domain by exploring the response rate of our stimulated FWM process., Comment: 4 figures

The spectral properties of an interacting many-body system may display critical character and have potential applications in precision metrology. Here, we demonstrate such many-body enhanced metrology for microwave (MW) electric fields in a non-equilibrium Rydberg atomic gas. Near criticality the high sensitivity of Rydberg atoms to external MW electric fields, combined with many-body enhancement induces significant changes in the optical transmission. We quantify this behavior using the Fisher information. For continuous optical transmission at the critical point, the Fisher information is three orders of magnitude larger than in independent particle systems, the measured data provides an equivalent sensitivity of 49 nV/cm/$\textrm{Hz}^{1/2}$. The reported results constitute a milestone towards the application of many-body effects in precision metrology.

Rydberg atoms have great potential in electric field measurement and have an advantage with a large frequency bandwidth from the kHz to the THz scale. However, the sensitivity for measuring a weak MHz electric field signal is limited by the spectroscopic resolution, because the weak electric field induces only a small perturbation of the population and energy level shift of the Rydberg atoms. Here, we report highly sensitive measurement of a weak MHz electric field using electromagnetically induced transparency with Rydberg atoms in a thermal atomic system. Using the heterodyne method on a 30-MHz electric field, we successfully measure the minimum electric field strength to be \textcolor{black}{37.3 $\mathrm{\mu V/cm}$} with a sensitivity up to $-65$ dBm/Hz and a linear dynamic range over 65 dB. Additionally, we measure an amplitude-modulated signal and demodulate the signal with a fidelity over 98\%. This work extends the sensitivity of atomic sensors for measuring MHz electric fields, which advances atomic electric field-sensing technology., Comment: 6 pages, 4 figures

Developing frequency combs spectral technologies has potential applications and prospects in the wide fields of cosmology, meteorology, and microwave measurement. Here, we demonstrate a Rydberg microwave frequency comb spectrometer via multiple-microwave field dressing, providing precise microwave measurement. The Rydberg microwave frequency comb spectrum provides a real-time and absolute frequency measurement with a range of 125 MHz and gives the relative phase of a single-frequency microwave signal. The reported experiment helps real-time sensing of an unknown microwave signal in a wide range using Rydberg atoms, which are vital for Rydberg-atom-based microwave metrology., Comment: 10 pages, 8 figures

The collective effect of large amounts of atoms exhibit an enhanced interaction between light and atoms. This holds great interest in quantum optics, and quantum information. When a collective excited state of a group of atoms during Rabi oscillation is varying, the oscillation exhibits rich dynamics. Here, we experimentally observe a size-reduction effect of the Rydberg collective state during Rabi oscillation in cold atomic dilute gases. The Rydberg collective state was first created by the Rydberg quantum memory, and we observed a decreased oscillation frequency effect by measuring the time traces of the retrieved light field amplitude, which exhibited chirped characteristics. This is caused by the simultaneous decay to the overall ground state and the overall loss of atoms. The observed oscillations are dependent on the effective Rabi frequency and detuning of the coupling laser, and the dephasing from inhomogeneous broadening. The reported results show the potential prospects of studying the dynamics of the collective effect of a large amount of atoms and manipulating a single-photon wave-packet based on the interaction between light and Rydberg atoms., Comment: 7 pages, 4 figures

Quantum memories are indispensible for establishing a long-distance quantum network. High-dimensional quantum memories enable a higher channel capacity compared to a quantum memory working in a two-dimensional space, and have a lower requirement for storage lifetime in the field of quantum coomunication. The photonic transverse spatial modes such as Laguerra-Gaussian modes orbital angular momentum (OAM) are ideal candidates for encoding high-dimensional information, because it can form an infinite-dimensional Hilbert space. Although the faithful storage of an OAM qubit or qutrit has been realized in pioneering works, the longest storage lifetime for the former is only in the order of a few microseconds, and hundreds of nano-seconds for the latter. Here we implement a quantum memory for OAM qubits and qutrits using a cold atomic ensemble, the experimental results clearly show that our memory can still beat the classical limit after a storage time of $400\mu s$,which is two orders of magnitude higher than the previous work. The retrieval efficiency at this time equals to $44\%$ of the value when the storage time is set to be $10\mu s$. Our work is very promising for establishing a high dimensional quantum network.

Recognition of multifrequency microwave (MW) electric fields is challenging because of the complex interference of multifrequency fields in practical applications. Rydberg atom-based measurements for multifrequency MW electric fields is promising in MW radar and MW communications. However, Rydberg atoms are sensitive not only to the MW signal but also to noise from atomic collisions and the environment, meaning that solution of the governing Lindblad master equation of light-atom interactions is complicated by the inclusion of noise and high-order terms. Here, we solve these problems by combining Rydberg atoms with deep learning model, demonstrating that this model uses the sensitivity of the Rydberg atoms while also reducing the impact of noise without solving the master equation. As a proof-of-principle demonstration, the deep learning enhanced Rydberg receiver allows direct decoding of the frequency-division multiplexed (FDM) signal. This type of sensing technology is expected to benefit Rydberg-based MW fields sensing and communication.

Photonic states encoded in spatial modes of paraxial light fields provide a promising platform for high-dimensional quantum information protocols and related studies, where several pioneering theoretical and experimental demonstrations have paved the path for future technologies. Crucially, critical issues encountered in free-space propagation still represent a major challenge. This is the case of asynchronous diffraction between spatial modes with different modal orders, which experience variations in their transverse structure upon free-space propagation. Here we address this issue by proposing an encoding method based on the use of Laguerre-Gaussian (LG) modes of the same modal order N to define a N + 1 dimensional space. Noteworthy, such modes endowed with orbital angular momentum (OAM) experience the same propagation aberrations featuring an identical Gouy phase and wavefront curvature. We demonstrate our proposal experimentally by using time-correlated-single-photon imaging combined with a digital propagation technique. Importantly, our technique allows to eliminate, without the use of imaging systems, all issues related to asynchronous diffraction, providing an accessible way to generate propagation-invariant OAM qudits for quantum optical protocols.

Abruptly autofocusing waves and associated ring-Airy (RA) beams are attracting increasing interest owing to their fascinating properties such as their ability of abruptly autofocusing to small F-number. Optical frequency conversion via nonlinear interactions can further expand their applications to new area, yet are rarely studied. In this work, we report the frequency conversion of RA beams via sum-frequency generation using perfect flattop and common Gauss beams as the pump beams. The nonlinear transformation of the spatial complex amplitude of the signal and associated influences on autofocusing behavior, under different conditions of interaction location (i.e., original, autofocusing, and Fourier planes) and pump structure, were systematically studied and experimentally investigated. This proof-of principle demonstration provides a general guideline to build the frequency interface for abruptly autofocusing waves and a reference for relevant studies involving nonlinear transformation of abruptly autofocusing waves., Comment: 12 pages, 8 figures

Vectorial structured light with spatially varying amplitude, phase, and polarization is reshaping many areas of modern optics, including nonlinear optics, as diverse parametric processes can be used to explore interactions between such complex vector fields, extending the frontiers of optics to new physical phenomena. However, the most basic nonlinear application, i.e., frequency conversion, still remains challenging for vectorial structured light since parametric processes are polarization dependent, leading to a change in the spatial topological structure of signals. In this work, to break this fundamental limit, we propose a novel conformal frequency conversion scheme that allows to maintain the full spatial structure of vectorial structured light in the conversion; and systematically examine its spatial polarization independence based on non-degenerate sum-frequency generation with type-0 phase matching. This proof-of-principle demonstration paves the way for a wide range of applications requiring conformal frequency conversion, and, particularly, to implement frequency interfaces with multimodal communication channels, high-dimensional quantum states, and polarization-resolved upconversion imaging., Comment: 15 pages with 10 figures

It is increasingly important to understand the spatial dynamics of epidemics. While there are numerous mathematical models of epidemics, there is a scarcity of physical systems with sufficiently well-controlled parameters to allow quantitative model testing. It is also challenging to replicate the macro non-equilibrium effects of complex models in microscopic systems. In this work, we demonstrate experimentally a physics analog of epidemic spreading using optically driven non-equilibrium phase transitions in strongly interacting Rydberg atoms. Using multiple laser beams we can impose any desired spatial structure. We observe spatially localized phase transitions and their interplay in different parts of the sample. These phase transitions simulate the outbreak of an infectious disease in multiple locations, as well as the dynamics towards herd immunity and endemic state in different regimes. The reported results indicate that Rydberg systems are versatile enough to model complex spatial-temporal dynamics., Comment: 22 pages, 10 figures

Long-lived storage of arbitrary transverse multimodes is important for establishing a high-channel-capacity quantum network. Most of the pioneering works focused on atomic diffusion as the dominant impact on the retrieved pattern in an atom-based memory. In this work, we demonstrate that the unsynchronized Larmor precession of atoms in the inhomogeneous magnetic field dominates the distortion of the pattern stored in a cold-atom-based memory. We find that this distortion effect can be eliminated by applying a strong uniform polarization magnetic field. By preparing atoms in magnetically insensitive states, the destructive interference between different spin-wave components is diminished, and the stored localized patterns are synchronized further in a single spin-wave component; then, an obvious enhancement in preserving patterns for a long time is obtained. The reported results are very promising for studying transverse multimode decoherence in storage and high-dimensional quantum networks in the future., Comment: 5 figures

Engineering vector spatial modes of photons is an important approach for manipulating high-dimension photonic states in various quantum optical experiments. In this work, we demonstrate generation of heralded single photons with well-defined vector spatial modes by using a self-locking polarizing interferometer comprising a spatial light modulator. Specifically, it is shown that, by carefully tailoring and compensating spatial and temporal amplitudes of manipulated photons, one can exactly convert ultrafast single photons into desired spin-orbit states with extremely high purity. This compact and robust device provides a versatile way for not only generation, but also manipulation and characterization of arbitrary photonic spin-orbit states.

In analog to counterparts widely used in electronic circuits, all optical non-reciprocal devices are basic building blocks for both classical and quantum optical information processing. Approaching the fundamental limit of such devices, where the propagation of a single photon exhibits a good non-reciprocal characteristic, requires an asymmetric strong coupling between a single photon and a matter. Unfortunately it has been not realized yet. Here, we propose and experimentally realize a quantum non-reciprocity device with low optical losses and a high isolation of larger than 14 dB based on the cold atoms. Besides, the non-reciprocal transmission of a quantum qubit and non-reciprocal quantum storage of a true single photon are also realized. All results achieved would be very promising in building up quantum non-reciprocal devices for quantum networks., Comment: The concept of quantum non-reciprocity is not suitable in this manuscript

Cavity-free optical nonreciprocity components, which have an inherent strong asymmetric interaction between the forward- and backward-propagation direction of the probe field, are key to produce such as optical isolators and circulators. According to the proposal presented by Xia et al., [Phys. Rev. Lett. 121, 203602 (2018)], we experimentally build a device that uses cross-Kerr nonlinearity to achieve a cavity-free optical isolator and circulator. Its nonreciprocal behavior arises from the thermal motion of N-type configuration atoms, which induces a strong chiral cross-Kerr nonlinear response for the weak probe beam. We obtain a two-port optical isolator for up to 20 dB of isolation ratio in a specially designed Sagnac interferometer. The distinct propagation directions of the weak probe field determine its cross-phase shift and transmission, by which we demonstrate the accessibility of a four-port optical circulator., Comment: 5 pages, 3 figures

The long-range interaction between Rydberg-excited atoms endows a medium with large optical nonlinearity. Here, we demonstrate an optical switch to operate on a single photon from an entangled photon pair under a Rydberg electromagnetically induced transparency configuration. With the presence of the Rydberg blockade effect, we switch on a gate field to make the atomic medium nontransparent thereby absorbing the single photon emitted from another atomic ensemble via the spontaneous four-wave mixing process. In contrast to the case without a gate field, more than 50% of the photons sent to the switch are blocked, and finally achieve an effective single-photon switch. There are on average 1-2 gate photons per effective blockade sphere in one gate pulse. This switching effect on a single entangled photon depends on the principal quantum number and the photon number of the gate field. Our experimental progress is significant in the quantum information process especially in controlling the interaction between Rydberg atoms and entangled photon pairs., Comment: 9 pages, 8 figures

Nowadays the most intriguing features of wave particle complementarity of single photon is exemplified by the famous Wheeler's delayed choice experiment in linear optics, nuclear magnetic resonance and integrated photonic device systems. Studying the wave particle behavior in light and matter interaction at single photon level is challenging and interesting, which gives how single photons complement in light and matter interaction. Here, we demonstrate a Wheeler's delayed choice experiment in an interface of light and atomic memory, in which the cold atomic memory makes the heralded single photon divided into a superposition of atomic collective excitation and leaked pulse, thus acting as memory beam splitters. We observe the morphing behavior between particle and wave of a heralded single photon by changing the relative proportion of quantum random number generator, the second memory efficiency, and the relative storage time of two memories. The reported results exhibit the complementarity behavior of single photon under the interface of light atom interaction., Comment: 7 pages, 5 figures; comments welcome

The complex interactions between orbital angular momentum (OAM) light and atoms are particularly intriguing in the areas of quantum optics and quantum information science. Building a versatile high-dimensional quantum network needs broad spiral-bandwidth for preparing higher-quanta OAM mode and resolving the bandwidth mismatch in spatial space and etc. Here, we experimentally demonstrate a broad spiral-bandwidth quantum interface between photon and memory. Through twisted fields of the writing and reading, the correlated OAM distribution between photon and memory is significantly broadened. This broad spiral-bandwidth quantum interface could be spanned in multiplexing regime and could work in high-quanta scenario with capability of |l|=30, and we demonstrate the entanglement within 2-D subspace with a fidelity of 80.5\text{\textpm}4.8\% for high l. Such state-of-the-art technology to freely control the spatial distribution of OAM memory is very helpful to construct high-dimensional quantum networks and provides a benchmark in the field of actively developing methods to engineer OAM single photon from matters., Comment: 8 pages, 6 figures

The Einstein Podolsky Rosen (EPR) entangled quantum state is of special importance not only for fundamental research in quantum mechanics, but also for information processing in the field of quantum information. Previous EPR entangled state demonstrations were constructed with photons of equal phase wave fronts. More complex scenarios with structured wave fronts have not been investigated. Here, we report the first experimental demonstration of EPR entanglement for photon pairs carrying orbital angular momentum (OAM) information, resulting in an OAM embedded EPR entangled state. We measured the dynamics of the dependence of the ghost interference on relative phase under projection. In addition, the reconstructed matrix in the OAM and EPR position momentum spaces shows a specific hyper entanglement in high dimension., Comment: 22pages, 4 figures

Precise measurements are the key to advances in all fields of science. Quantum entanglement shows higher sensitivity than achievable by classical methods. Most physical quantities including position, displacement, distance, angle, and optical path length can be obtained by optical phase measurements. Reducing the photon wavelength of the interferometry can further enhance the optical path length sensitivity and imaging resolution. By quantum frequency up conversion, we realized a short wavelength two photon number entangled state. Nearly perfect Hong Ou Mandel interference is achieved after both 1547-nm photons are up converted to 525 nm. Optical phase measurement of two photon entanglement state yields a visibility greater than the threshold to surpass the standard quantum limit. These results offer new ways for high precision quantum metrology using short wavelength quantum entanglement number state., Comment: coments are welcome, manuscript under review

Are quantum states real? This most fundamental question in quantum mechanics has not yet been satisfactorily resolved, although its realistic interpretation seems to have been rejected by various delayed-choice experiments. Here, to address this long-standing issue, we present a quantum twisted double-slit experiment. By exploiting the subluminal feature of twisted photons, the real nature of a photon during its time in flight is revealed for the first time. We found that photons' arrival times were inconsistent with the states obtained in measurements but agreed with the states during propagation. Our results demonstrate that wavefunctions describe the realistic existence and evolution of quantum entities rather than a pure mathematical abstraction providing a probability list of measurement outcomes. This finding clarifies the long-held misunderstanding of the role of wavefunctions and their collapse in the evolution of quantum entities., Comment: Comments are welcome.12 pages, 5 figures

Multi-photon entangled states play a crucial role in quantum information applications such as secure quantum communication, scalable computation, and high-precision quantum metrology. Quantum memory for entangled states is a key component of quantum repeaters, which are indispensable in realizing quantum communications. Storing a single photon or an entangled photon has been realized through different protocols. However, there has been no report demonstrating whether a multi-photon state can be stored in any physical system or not. Here, we report on the experimental storage of a two-photon NOON state in a cold atomic ensemble. Quantum interference measured before and after storage clearly shows that the properties of the two-photon NOON state are preserved during storage. Our experiment completes the first step towards storing a multi-photon entangled state., Comment: comments are welcome

A spatial light modulator (SLM) is one of the most useful and convenient device to generate structural light beams such as twisted light and complexed images used in modern optical science. The unbounded dimension of twisted light makes it promising in harnessing information carrying ability of a single photon, which greatly enhances the channel capacity in optical communications. We perform a detail theoretical study of the birth, evolution and reverse transformation of twisted light generated from a phase-only SLM based on diffraction theory, analytical expressions are obtained to show the special evolution behaviors of the light beam with the propagation distance. Beam intensity distributions calculated theoretically are in well agreement with experimental observations. Our findings clearly reveal how twisted light gradually emerges from a Gaussian spatial shape to a ring shape, and also the ring shape will gradually evolve to a quasi-Gaussian shape conversely, in the reverse transformation. These results will provide guidelines for using SLM in many optical experiments and OAM-mode multiplexing in optical communications., Comment: primary manscript, comments are welcome

Silicon-on-chip (SOI) photonic circuit is the most promising platform for scalable quantum information technology for its low loss, small footprint, CMOS-compatible and telecom communications techniques compatible. Multiple multiplexed entanglement sources include: energy-time, time-bin and polarization entangled sources based on 1-cm length single silicon nanowire, all these sources are compatible with (100GHz) dense-wave-division-multiplexing (DWDM) system. Different methods such as two photon interference pattern, Bell-Inequality and quantum state tomography are used to characterize the quality of these entangled sources. Multiple entanglements are generated over more than 5 channel pairs with high raw (net) visibilities around 97% (100%). The emission spectral brightness of these entangled sources reaches 4.2*105 /(s.nm.mW). The quality of the photon pair generated in continuous and pulse pump regimes are compared. High qualities of these multiplexed entanglement sources make them very promising to be used in future minimized quantum communication and computation systems., Comment: Accepted by Physical Review Applied

Quantum communication provides an absolute security advantage, and it has been widely developed over the past 30 years. As an important branch of quantum communication, quantum secure direct communication (QSDC) promotes high security and instantaneousness in communication through directly transmitting messages over a quantum channel. The full implementation of a quantum protocol always requires the ability to control the transfer of a message effectively in the time domain; thus, it is essential to combine QSDC with quantum memory to accomplish the communication task. In this paper, we report the experimental demonstration of QSDC with state-of-the-art atomic quantum memory for the first time in principle. We used the polarization degrees of freedom of photons as the information carrier, and the fidelity of entanglement decoding was verified as approximately 90%. Our work completes a fundamental step toward practical QSDC and demonstrates a potential application for long-distance quantum communication in a quantum network., Comment: To appear in PRL

The Einstein-Podolsky-Rosen (EPR) entanglement is of special importance not only for fundamental research in quantum mechanics, but also for quantum information processing. Establishing EPR entanglement between two memory systems, such as atomic ensembles, nitrogen-vacancy centers, and rare-earth-ion-doped solids is promising for realizing spatial-multimode based quantum communication, quantum computation, and quantum imaging. To date, there have been few reports on realizing EPR entanglement between physical systems in true position and momentum. Here we describe successfully establishing such entanglement between two separated atomic ensembles by using quantum storage. We clearly prove the existence of EPR entanglement in position and momentum between two memories by demonstrating the satisfying of the inseparability criterion with the aid of quantum ghost-imaging and ghost-interference experiments.

Optical fields with orbital angular momentum (OAM) interact with medium have many remarkable properties with its unique azimuthal phase, showing many potential applications in high capacity information processing, high precision measurement etc. The dephasing mechanics of optical fields with OAM in an interface between light and matter plays a vital role in many areas of physics. In this work, we study the transverse azimuthal dephasing of OAM spin wave in a hot atomic gas via OAM storage. The transverse azimuthal phase difference between the control and probe beams is mapped onto the spin wave, which essentially results in dephasing of atomic spin wave. The dephasing of OAM spin wave can be controlled by the parameters of OAM topological charge and beam waist. Our results are helpful for studying OAM light interaction with matter, maybe hold a promise in OAM-based quantum information processing., Comment: 11 pages, 4 figures, original manuscript, comments welcome

Abstract Far-from equilibrium dynamics that lead to self-organization are highly relevant to complex dynamical systems not only in physics, but also in life-, earth-, and social sciences. It is challenging however to find systems with sufficiently controllable parameters that allow quantitatively modelling of emergent properties. Here, we study a non-equilibrium phase transition and observe signatures of self-organized criticality in a dilute thermal vapour of atoms optically excited to strongly interacting Rydberg states. Electromagnetically induced transparency (EIT) provides excellent control over the population dynamics and enables high-resolution probing of the driven-dissipative dynamics, which also exhibits phase bistability. Increased sensitivity compared to previous work allows us to reconstruct the complete phase diagram including in the vicinity of the critical point. We observe that interaction-induced energy shifts and enhanced decay only occur in one of the phases above a critical Rydberg population. This limits the application of generic mean-field models, however a modified, threshold-dependent approach is in qualitative agreement with experimental data. Near threshold, we observe self-organized dynamics in the form of population jumps that return the density to a critical value., Comment: 15 pages, 11 figures, comments welcome