1. Numerical analysis of hydrogen recombination on a vertical flat plate catalyst
- Author
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Dae-Hyun Kim, Youngsu Na, and Dong-Wook Oh
- Subjects
Passive autocatalytic recombiner ,Hydrogen recombination ,Computational fluid dynamics ,Catalyst plate ,Technology - Abstract
This study conducts a computational fluid dynamics (CFD) analysis to assess passive autocatalytic recombiners (PARs) for mitigating hydrogen risks in severe accidents. We modeled hydrogen-air mixtures' thermal-fluid dynamics and chemical reactions, comparing single-step reaction rate models with detailed chemical mechanisms on platinum-coated catalyst plates. Results indicate that the simplified single-step model accurately predicts hydrogen recombination on Pt surfaces. Incorporating radiative heat transfer was essential; neglecting it led to significant overestimations of catalyst plate temperatures and hydrogen removal rates. While CFD results aligned with experimental trends from the REKO-3 apparatus, discrepancies arose due to overestimated recombination rates. These findings highlight the importance of precise chemical and thermal modeling in optimizing PAR design, enhancing hydrogen reduction efficiency, and minimizing auto-ignition risks. The validated CFD model offers valuable guidance for improving hydrogen removal efficiency of PARs during severe accidents.
- Published
- 2025
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