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The landscape of ultrafast structured light pulses has recently evolved driven by the capability of high-order harmonic generation (HHG) to up-convert orbital angular momentum (OAM) from the infrared to the extreme-ultraviolet (EUV) spectral regime. Accordingly, HHG has been proven to produce EUV vortex pulses at the femtosecond timescale. Here we demonstrate the generation of attosecond vortex pulse trains, i.e. a succession of attosecond pulses with a helical wavefront, resulting from the synthesis of a comb of EUV high-order harmonics with the same OAM. By driving HHG with a polarization tilt-angle fork grating, two spatially separated circularly polarized high-order harmonic beams with order-independent OAM are created. Our work opens the route towards attosecond-resolved OAM light-matter interactions., Comment: Main text (1-14 pages) and supplemental material (14-16 pages)

Vigorous efforts to harness the topological properties of light have enabled a multitude of novel applications. Translating the applications of structured light to higher spatial and temporal resolutions mandates their controlled generation, manipulation, and thorough characterization in the short-wavelength regime. Here, we resort to high-order harmonic generation (HHG) in a noble gas to upconvert near-infrared (IR) vector, vortex, and vector-vortex driving beams that are tailored respectively in their Spin Angular Momentum (SAM), Orbital Angular Momentum (OAM), and simultaneously in their SAM and OAM. We show that HHG enables the controlled generation of extreme-ultraviolet (EUV) vector beams exhibiting various spatially-dependent polarization distributions, or EUV vortex beams with a highly twisted phase. Moreover, we demonstrate the generation of EUV vector-vortex beams (VVB) bearing combined characteristics of vector and vortex beams. We rely on EUV wavefront sensing to unambiguously affirm the topological charge scaling of the HHG beams with the harmonic order. Interestingly, our work shows that HHG allows for a synchronous controlled manipulation of SAM and OAM. These EUV structured beams bring in the promising scenario of their applications at nanometric spatial and sub-femtosecond temporal resolutions using a table-top harmonic source., Comment: 13 pages, 6 figures

We present a phase retrieval algorithm for dispersion scan (d-scan), inspired by ptychography, which is capable of characterizing multiple mutually-incoherent ultrafast pulses (or modes) in a pulse train simultaneously from a single d-scan trace. In addition, a form of Newton's method is employed as a solution to the square root problem commonly encountered in second harmonic pulse measurement techniques. Simulated and experimental phase retrievals of both single-mode and multi-mode d-scan traces are shown to demonstrate the accuracy and robustness of the algorithm., Comment: 17 pages, 8 figures

Vacuum ultraviolet (VUV) light is critical for the study of molecules and materials, but the generation of femtosecond pulses in the VUV region at high repetition rates has proven difficult. Here, we demonstrate the efficient generation of VUV light at MHz repetition rates using highly cascaded four-wave mixing processes in a negative-curvature hollow-core fiber. Both even and odd order harmonics are generated up to the 15th harmonic (69 nm, 18.0 eV), with high energy resolution of ~40 meV. In contrast to direct high harmonic generation, this highly cascaded harmonic generation process requires lower peak intensity and therefore can operate at higher repetition rates, driven by a robust ~10 W fiber-laser system in a compact setup. Additionally, we present numerical simulations that explore the fundamental capabilities and spatiotemporal dynamics of highly cascaded harmonic generation. This VUV source can enhance the capabilities of spectroscopies of molecular and quantum materials, such as photoionization mass spectrometry and time , angle , and spin-resolved photoemission., Comment: 9 pages, 4 figures. Submitted to Optica (OSA)

Here we introduce three-dimensional single-shot ptychography (3DSSP). 3DSSP leverages an additional constraint unique to the single-shot geometry to deconvolve multiple 2D planes of a 3D object. Numeric simulations and analytic calculations demonstrate that 3DSSP reconstructs multiple planes in an extended 3D object with a minimum separation consistent with the depth of field for a conventional microscope. We experimentally demonstrate 3DSSP by reconstructing orthogonal hair strands axially separated by 5 mm. Three-dimensional single-shot ptychography provides a pathway towards volumetric imaging of dynamically evolving systems on ultrafast timescales., Comment: 7 pages, 5 figures

Few-cycle pulsed laser technology highlights the need for control and stabilization of the carrier-envelope phase (CEP) for applications requiring shot-to-shot timing and phase consistency. This general requirement has been achieved successfully in a number of free space and fiber lasers via feedback and feed-forward methods. Expanding upon existing results, we demonstrate CEP stabilization through the feed-forward method applied to a SESAM mode-locked Er:Yb:glass laser at 1.55 um with a measured ultralow timing jitter of 2.9 as (1 Hz - 3 MHz) and long-term stabilization over a duration of eight hours. Single-digit attosecond stabilization at telecom wavelengths opens a new direction in applications requiring ultra-stable frequency and time precision such as high-resolution spectroscopy and fiber timing networks., Comment: 4 pages, 4 figures, submitted to Optics Letters

The interaction of intense mid-infrared laser fields with atoms and molecules leads to a range of new opportunities, from the production of bright, coherent radiation in the soft x-ray range to imaging molecular structures and dynamics with attosecond temporal and sub-angstrom spatial resolution. However, all these effects, which rely on laser-driven recollision of an electron removed by the strong laser field and the parent ion, suffer from the rapidly increasing role of the magnetic field component of the driving pulse: the associated Lorentz force pushes the electrons off course in their excursion and suppresses all recollision-based processes, including high harmonic generation, elastic and inelastic scattering. Here we show how the use of two non-collinear beams with opposite circular polarizations produces a forwards ellipticity which can be used to monitor, control, and cancel the effect of the Lorentz force. This arrangement can thus be used to re-enable recollision-based phenomena in regimes beyond the long-wavelength breakdown of the dipole approximation, and it can be used to observe this breakdown in high-harmonic generation using currently-available light sources.

We investigate the problem of shaping radially symmetric annular beams into desired intensity patterns along the optical axis. Within the Fresnel approximation, we show that this problem can be expressed in a variational form equivalent to the one arising in phase retrieval. Using the uncertainty principle we prove rigorous lower bounds on the functional that capture how the various physical parameters in the problem determine the accuracy of the beam shaping. We also use the method of stationary phase to construct a natural ansatz for a minimizer in the short wavelength limit. We illustrate the implications of our results by applying the method of stationary phase coupled with the Gerchberg-Saxton algorithm to beam shaping problems arising in remote delivery of beams and pulses., Comment: 34 Pages, 6 figures, 1 appendix; revised figures and discussion