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In August 2017, a smoke plume from wildfires in British Columbia and the Northwest Territories recirculated and persisted over northern Canada for over two weeks. We compared a full‐factorial set of NASA Goddard Institute for Space Studies ModelE simulations of the plume to satellite retrievals of aerosol optical depth and carbon monoxide, finding that ModelE performance was dependent on the model configuration, and more so on the choice of injection height approach, aerosol scheme and biomass burning emissions estimates than to the choice of horizontal winds for nudging. In particular, ModelE simulations with free‐tropospheric smoke injection, a mass‐based aerosol scheme and comparatively high fire NOx emissions led to unrealistically high aerosol optical depth. Using paired simulations with and without fire emissions, we estimated that for 16 days over an 850,000 km2 region, the smoke decreased planetary boundary layer heights by between 253 and 547 m, decreased downward shortwave radiation by between 52 and 172 Wm−2, and decreased surface temperature by between 1.5°C and 4.9°C, the latter spanning an independent estimate from operational weather forecasts of a 3.7°C cooling. The strongest surface climate effects were for ModelE configurations with more detailed aerosol microphysics that led to a stronger first indirect effect. Plain Language Summary: Smoke from biomass burning is known to have effects on surface weather. We used the NASA GISS ModelE to estimate these effects for a large 2017 smoke plume over northern Canada that persisted for two weeks. We first found that the height of the smoke release at the source was the most important factor influencing agreement between ModelE and satellite retrievals of aerosols and carbon monoxide, and that specific, plausible configurations of the model led to unrealistically high aerosol amounts. By comparing simulations with and without fire, we estimated a 16‐day cooling over a 850,000 km2 region of between 1.5°C and 4.9°C, depending on the model configuration. Key Points: We captured the overall pattern and magnitude of a large 2017 smoke plume over Canada with the NASA GISS ModelEOf the sixteen plausible model configurations tested under a full‐factorial design, two with higher NOx emissions, free‐tropospheric smoke release and mass‐based aerosols led to unrealistically high aerosol optical depthOver an 850,000 km2 region, we estimated a 16‐day surface cooling of between 1.5°C and 4.9°C [ABSTRACT FROM AUTHOR]

The new TROPESS (TRopospheric Ozone and its Precursors from Earth System Sounding) profile retrievals of carbon monoxide (CO) from the Cross-track Infrared Sounder (CrIS) are evaluated against Measurement of Pollution in the Troposphere (MOPITT) CO version 9 data. Comparison results that were adjusted to common a priori constraints in the retrieval processes have improved agreement between the two data sets over direct comparisons. TROPESS-CrIS CO profiles are within 5 % of MOPITT but have higher concentrations in the lower troposphere and lower concentrations in the upper troposphere. For the intense western US wildfire events in September 2020, we compare CO fields simulated by the GISS climate model to the two satellite CO observations. We show intermediate steps of the comparison process to illustrate the evaluation of model simulations by deriving the "retrieved" model CO profiles as they would be observed by the satellite. This includes the application of satellite level-2 data along with their corresponding diagnostic operators provided in the TROPESS-CrIS and MOPITT products. The process allows a diagnosis of potential model improvements in modeling fire emissions and pollution transport. [ABSTRACT FROM AUTHOR]

Using 10 years of satellite‐borne radar and lidar observations coupled with a novel method for automated occlusion identification, composite transects of cloud and precipitation across occluded thermal ridges of extratropical cyclones are, for the first time, constructed. These composites confirm that occluded sectors are characterized by the most extensive cloud cover and heaviest precipitation in any of the frontal regions of the cyclone. Hydrometeor frequency in occluded sectors is sensitive to the cyclone's ascent strength but not to the mean precipitable water in the cyclone's environment. This result is in contrast to the strong relationships between hydrometeor frequency and both precipitable water and ascent strength as previously reported in warm frontal regions. In both hemispheres, cloud and precipitation increase with the maximum value of the equivalent potential temperature at 700 hPa within the occluded thermal ridge, until a threshold is reached. For very large values of maximum equivalent potential temperature, hydrometeors become less frequent while precipitation rates increase. It is suggested that this conjunction is a by‐product of an increase in the frequency of convection in those instances. While in the Northern Hemisphere occluded sectors exhibit deeper and wider cloud structures than their Southern Hemisphere counterparts, their hydrometeor occurrence frequencies are less. The differences in maximum equivalent potential temperature of the thermal ridges in both hemispheres does not appear to explain the more frequent hydrometeors in the Southern Hemisphere. These relationships offer new perspectives on the interplay between cloud processes and cyclone evolution, as well as new observational constraints for process evaluation of Earth system models. [ABSTRACT FROM AUTHOR]

Shifts in Southern Ocean (SO, 40–85°S) shortwave cloud feedback (SWFB) toward more positive values are the dominant contributor to higher effective climate sensitivity (ECS) in Coupled Model Intercomparison Project Phase 6 (CMIP6) models. To provide an observational constraint on the SO SWFB, we use a simplified physical model to connect SO SWFB with the response of column‐integrated liquid water mass (LWP) to warming and the susceptibility of albedo to LWP in 50 CMIP5 and CMIP6 GCMs. In turn, we predict the responses of SO LWP using a cloud‐controlling factor (CCF) model. The combination of the CCF model and radiative susceptibility explains about 50% of the variance in the GCM‐simulated SWFB in the SO. Observations of SW radiation fluxes, LWP, and CCFs from reanalysis are used to constrain the SO SWFB. Observations suggest a SO LWP increase in response to warming and albedo susceptibility to LWP that is on the lower end relative to GCMs. The overall constraint on the contribution of SO to global mean SWFB is −0.168 to +0.051 W m−2 K−1, relative to −0.277 to +0.270 Wm−2 K−1. In summary, observations suggest SO SWFB is less likely to be as extremely positive as predicted by some CMIP6 GCMs, but more likely to range from moderately negative to weakly positive. Plain Language Summary: Previous studies suggest that SO clouds reflect more sunlight in response to global warming and more strongly cool the planet ‐ a negative shortwave cloud feedback (SWFB). The SO SWFB in the latest generation of global climate models (GCMs) participating in the Coupled Model Intercomparison Project Phase 6 (CMIP6) has shifted toward more positive values, leading to the larger predicted temperature responses to greenhouse gas increases in these GCMs. In this study, we examine if this more positive SWFB is consistent with observations. We connect the effect of SO clouds on reflected sunlight with the predicted response of cloud liquid content to global warming. The linkage between cloud liquid water content and large‐scale meteorology is applied to predict this cloud liquid response. Satellite observations of reflected sunlight, cloud liquid, and observations of large‐scale meteorology are applied to constrain the SO SWFB for 50 CMIP5 and CMIP6 GCMs. The results suggest that SO cloud liquid will increase with warming around the average of predictions of 50 GCMs. Satellite records suggest that SO SWFB is moderately negative to weakly positive, instead of extremely positive or negative as suggested by some GCMs. Key Points: Southern Ocean liquid water path increased over the past two decades due to enhanced moisture convergenceEnhanced moisture convergence contributes to a negative cloud feedback in the Southern OceanAcross global climate models, the sensitivity of upwelling shortwave to cloud opposes the sensitivity of cloud to moisture convergence [ABSTRACT FROM AUTHOR]

The new TROPESS (TRopospheric Ozone and its Precursors from Earth System Sounding) profile retrievals of Carbon Monoxide (CO) from the Cross-track Infrared Sounder (CrIS) are evaluated against Measurement of Pollution in the Troposphere (MOPITT) CO Version 9 data. Comparison results that were adjusted to common a priori constraints in the retrieval processes have improved agreement between the two data sets over direct comparisons. CrIS CO profiles are within 5 % of MOPITT but have higher concentrations in the lower troposphere and lower concentrations in the upper troposphere. For the intense W. US wildfire events in September 2020, we compare GISS climate model simulated CO fields to the two satellite CO observations. We show intermediate steps of the comparison process to illustrate the evaluation of model simulations by deriving the "retrieved" model CO profiles as they would be observed by the satellite. This includes the application of satellite Level 2 data along with their corresponding diagnostic operators provided in the TROPESS and MOPITT products. The process allows a diagnosis of potential model improvements in modelling fire emissions and pollution transport. [ABSTRACT FROM AUTHOR]

Aerosol-cloud interactions represent the leading uncertainty in our ability to infer climate sensitivity from the observational record. The forcing from changes in cloud albedo driven by increases in cloud droplet number (Nd) (the first indirect effect) is confidently negative and has narrowed its probable range in the last decade, but the sign and strength of forcing associated with changes in cloud macrophysics in response to aerosol (aerosol-cloud adjustments) remain uncertain. This uncertainty reflects our inability to accurately quantify variability not associated with a causal link flowing from the cloud microphysical state to cloud macrophysical state. Once variability associated with meteorology has been removed, covariance between the liquid water path averaged across cloudy and clear regions (LWP, here, characterizing the macrophysical state) and Nd (characterizing the microphysical) is the sum of two causal pathways linking Nd to LWP: Nd altering LWP (adjustments) and precipitation scavenging aerosol and thus depleting Nd. Only the former term is relevant to constraining adjustments, but disentangling these terms in observations is challenging. We hypothesize that the diversity of constraints on aerosol-cloud adjustments in the literature may be partly due to not explicitly characterizing covariance flowing from cloud to aerosol, and aerosol to cloud. Here, we restrict our analysis to the regime of extratropical clouds outside of low-pressure centers associated with cyclonic activity. Observations from MAC-LWP, and MODIS are compared to simulations in the MetOffice Unified Model (UM) GA7.1 (the atmosphere model of HadGEM3-GC3.1 and UKESM1). The meteorological predictors of LWP are found to be similar between the model and observations. There is also agreement with previous literature on cloud-controlling factors finding that increasing stability, moisture, and sensible heat flux enhance LWP, while increasing subsidence, and sea surface temperature decrease it. A simulation where cloud microphysics are insensitive to changes in Nd is used to characterize covariance between Nd and LWP that is induced by factors other than aerosol-cloud adjustments. By removing variability associated with meteorology and scavenging we infer the sensitivity of LWP to changes in Nd. Application of this technique to UM GA7.1 simulations reproduces the true model adjustment strength. Observational constraints developed using simulated covariability not induced by adjustments and observed covariability between Nd and LWP predict a 25-30 % overestimate by the UM GA7.1 in LWP change and a 30-35% overestimate in associated radiative forcing. [ABSTRACT FROM AUTHOR]

Extratropical cyclones provide a unique set of challenges and opportunities in understanding variability in cloudiness over the extratropics (poleward of 30°). We can gain insight into the shortwave cloud feedback from examining cyclone variability. Here we contrast global climate models (GCMs) with horizontal resolutions from 7 km up to hundreds of kilometers with Multi-Sensor Advanced Climatology Liquid Water Path (MAC-LWP) microwave observations of cyclone properties from the period 1992-2015. We find that inter-cyclone variability in both observations and models is strongly driven by moisture flux along the cyclone's warm conveyor belt (WCB). Stronger WCB moisture flux enhances liquid water path (LWP) within cyclones. This relationship is replicated in GCMs, although its strength varies substantially across models. In the southern hemisphere (SH) oceans 28-42% of the observed interannual variability in cyclone LWP may be explained by WCB moisture flux variability. This relationship is used to propose two cloud feedbacks acting within extratropical cyclones: a negative feedback driven by Clausius-Clapeyron increasing water vapor path (WVP), which enhances the amount of water vapor available to be fluxed into the cyclone; and a feedback moderated by changes in the life cycle and vorticity of cyclones under warming, which changes the rate at which existing moisture is imported into the cyclone. We show that changes in moisture flux drive can explain the observed trend in Southern Ocean cyclone LWP over the last two decades. Transient warming simulations show that the majority of the change in cyclone LWP can be explained by changes in WCB moisture flux, as opposed to changes in cloud phase. The variability within cyclone composites is examined to understand what cyclonic regimes the mixed phase cloud feedback is relevant to. At a fixed WCB moisture flux cyclone LWP increases with increasing SST in the half of the composite poleward of the low and decreases in the half equatorward of the low in both GCMs and observations. Cloud-top phase partitioning observed by the Atmospheric Infrared Sounder (AIRS) indicates that phase transitions may be driving increases in LWP in the poleward half of cyclones. [ABSTRACT FROM AUTHOR]

Despite continuous improvements in microwave sensors and retrieval algorithms, our understanding of precipitation uncertainty is quite limited, due primarily to inconsistent findings in studies that compare satellite estimates toin situobservations over different parts of the world. This study seeks to characterize the temporal and spatial properties of uncertainty in the Tropical Rainfall Measuring Mission Microwave Imager surface rainfall product over tropical ocean basins. Two uncertainty analysis frameworks are introduced to qualitatively evaluate the properties of uncertainty under a hierarchy of spatiotemporal data resolutions. The first framework (i.e. ‘climate method’) demonstrates that, apart from random errors and regionally dependent biases, a large component of the overall precipitation uncertainty is manifested in cyclical patterns that are closely related to large-scale atmospheric modes of variability. By estimating the magnitudes of major uncertainty sources independently, the climate method is able to explain 45–88% of the monthly uncertainty variability. The percentage is largely resolution dependent (with the lowest percentage explained associated with a 1° × 1° spatial/1 month temporal resolution, and highest associated with a 3° × 3° spatial/3 month temporal resolution). The second framework (i.e. ‘weather method’) explains regional mean precipitation uncertainty as a summation of uncertainties associated with individual precipitation systems. By further assuming that self-similar recurring precipitation systems yield qualitatively comparable precipitation uncertainties, the weather method can consistently resolve about 50% of the daily uncertainty variability, with only limited dependence on the regions of interest. [ABSTRACT FROM PUBLISHER]

The Multi-Sensor Advanced Climatology of Liquid Water Path (MAC-LWP), an updated and enhanced version of the University of Wisconsin (UWisc) cloud liquid water path (CLWP) climatology, currently provides 29 years (1988 - 2016) of monthly gridded (1°) oceanic CLWP information constructed using Remote Sensing Systems (RSS) inter-calibrated 0.25°-resolution retrievals. Satellite sources include SSM/I, TMI, AMSR-E, WindSat, SSMIS, AMSR-2 and GMI. To mitigate spurious CLWP trends, the climatology is corrected for drifting satellite overpass times by simultaneously solving for the monthly average CLWP and monthly-mean diurnal cycle. In addition to a longer record and six additional satellite products, major enhancements relative to the UWisc climatology include updating the input to version 7 RSS retrievals, a correction for a CLWP bias (based on matchups to clear-sky MODIS scenes), and the construction of a total (cloud+rain) liquid water path (TLWP) record for use in analyses of columnar liquid water in raining clouds. Because the microwave emission signal from cloud water is similar to that of precipitation-sized hydrometeors, greater uncertainty in the CLWP record is expected in regions of substantial precipitation. Therefore, the TLWP field can also be used as a quality-control screen, where uncertainty increases as the ratio of CLWP to TLWP decreases. For regions where confidence in CLWP is highest (i.e. CLWP:TLWP > 0.8), systematic differences in MAC CLWP relative to UWisc CLWP range from -15% (e.g. global oceanic stratocumulus decks) to +5-10% (e.g. portions of the higher-latitudes, storm tracks, and shallower convection regions straddling the ITCZ). The dataset is currently hosted at the Goddard Earth Science Data and Information Services Center (http://disc.sci.gsfc.nasa.gov).