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Following a sustainable development pathway designed to keep warming below 2 °C will benefit human health. We quantify premature deaths attributable to fine particulate matter (PM2.5) air pollution and heat exposures for China, South Asia, and the United States using projections from multiple climate models under high-and low-emission scenarios. Projected changes in premature deaths are typically dominated by population aging, primarily reflecting increased longevity leading to greater sensitivity to environmental risks. Changes in PM2.5 exposure typically have small impacts on premature deaths under a high-emission scenario but provide substantial benefits under a low-emission scenario. PM2.5-attributable deaths increase in South Asia throughout the century under both scenarios but shift to decreases by late century in China, and US values decrease throughout the century. In contrast, heat exposure increases under both scenarios and combines with population aging to drive projected increases in deaths in all countries. Despite population aging, combined PM2.5-and heat-related deaths decrease under the low-emission scenario by ~2.4 million per year by midcentury and ~2.9 million by century's end, with ~3% and ~21% of these reductions from heat, respectively. Intermodel variations in exposure projections generally lead to uncertainties of <40% except for US and China heat impacts. Health benefits of low emissions are larger from reduced heat exposure than improved air quality by the late 2090s in the United States. In contrast, in South and East Asia, the PM2.5-related benefits are largest throughout the century, and their valuation exceeds the cost of decarbonization, especially in China, over the next 30 y. [ABSTRACT FROM AUTHOR]

Over the CMIP6 historical period (1850–2014), aerosols provided the largest negative forcing compared to all other climate forcings via their ability to absorb or scatter solar radiation and alter clouds. Aerosols played an important role in counterbalancing warming by greenhouse gases (GHGs). Here we study aerosol forcing trends in the CMIP6 simulations of the NASA Goddard Institute for Space Studies (GISS) ocean‐atmosphere ModelE version 2.1 (GISS‐E2.1‐G) using a fully coupled atmospheric composition configuration, including interactive gas‐phase chemistry, and either an aerosol microphysical (MATRIX) or a mass‐based aerosol (OMA) module. Simulations of the CMIP6 historical period are analyzed as well as four Shared Socioeconomic Pathway (SSP) future scenarios for 2015–2100: SSP1‐2.6, SSP2‐4.5, SSP3‐7.0, and SSP5‐8.5. The main conclusion of this study is that aerosol forcing in the GISS model has reached its turning point, switching from globally increasing to a decreasing trend in the first decade of the 21st century. This result is robust, independent of which aerosol module or SSP scenario is used. Non‐linear aerosol‐cloud interactions dominate as a forcing agent over aerosol‐radiation interactions. Aerosols' ability to counterbalance GHG forcing on the global scale is today at a level comparable to that at the beginning of the last century. In the 1980s, the decade of largest global aerosol loads, aerosols balanced up to 80% of GHG forcing. As a consequence, global warming of the last decades, which is primarily driven by greenhouse gases, has been augmented by the effect of decreasing aerosol cooling in our model. By the end of this century, following the SSP scenarios, aerosols will only counterbalance 0%–20% of GHG forcing, depending on model and on scenario. Plain Language Summary: Climate change is the result of the aggregate effect of a number of individual forcing agents changing the radiative balance at the top of the atmosphere over time. As a result, if positive radiative forcings dominate over negative forcings, the Earth's surface warms. Over the historical period, since the pre‐industrial era, greenhouse gases (GHG) and aerosol have provided the largest positive and negative forcings, respectively. However, the relationship between GHG and aerosols have rapidly changed in the last decades, and future projections show much more dramatic dominance of GHG over aerosols. This study investigates the connection between emissions, atmospheric composition and climate forcing. We find that aerosols' ability to counterbalance GHG forcing reached its maximum effect in the 1980s, and that since the first decade of the 21st century, aerosol effects are globally on a decreasing trajectory. Reduced aerosol loads are important for health, but accelerate global warming, in the absence of concurrent GHG reductions. The results presented here are based upon the NASA GISS climate model, and the four future scenarios used. These scenarios are not intended as predictions, but represent a range of possible changes in atmospheric composition (including greenhouse gases) based on differing assumptions about future energy policies. Key Points: Aerosol forcing in the Goddard Institute for Space Studies model reached its turning point in the first decade of the 21st centuryNon‐linear aerosol‐cloud forcing dominates in magnitude over aerosol direct forcing and pinpoint the timing of the turning pointWithin the next 25 years, global aerosol forcing might balance only 0%–20% of greenhouse gas forcing, compared to 80% in 1980–1990 [ABSTRACT FROM AUTHOR]

Evaluating multicomponent climate change mitigation strategies requires knowledge of the diverse direct and indirect effects of emissions. Methane, ozone, and aerosols are linked through atmospheric chemistry so that emissions of a single pollutant can affect several species. We calculated atmospheric composition changes, historical radiative forcing, and forcing per unit of emission due to aerosol and tropospheric ozone precursor emissions in a coupled composition-climate model. We found that gas-aerosol interactions substantially alter the relative importance of the various emissions. In particular, methane emissions have a larger impact than that used in current carbon-trading schemes or in the Kyoto Protocol Thus, assessments of multigas mitigation policies, as well as any separate efforts to mitigate warming from short-lived pollutants, should include gas-aerosol interactions. [ABSTRACT FROM AUTHOR]

Observed trends in tropospheric ozone, an important air pollutant and short‐lived climate forcer (SLCF), are estimated using available surface and ozonesonde profile data for 1993–2019, using a coherent methodology, and compared to modeled trends (1995–2015) from the Arctic Monitoring Assessment Program SLCF 2021 assessment. Increases in observed surface ozone at Arctic coastal sites, notably during winter, and concurrent decreasing trends in surface carbon monoxide, are generally captured by multi‐model median trends. Wintertime increases are also estimated in the free troposphere at most Arctic sites, with decreases during spring months. Winter trends tend to be overestimated by the multi‐model medians. Springtime surface ozone increases in northern coastal Alaska are not simulated while negative springtime trends in northern Scandinavia are not always reproduced. Possible reasons for observed changes and model performance are discussed including decreasing precursor emissions, changing ozone dry deposition, and variability in large‐scale meteorology. Plain Language Summary: The Arctic is warming much faster than the rest of the globe due to increases in carbon dioxide, and other trace constituents like ozone, also an air pollutant. However, improved understanding is needed about long‐term changes or trends in Arctic tropospheric ozone. A coherent methodology is used to identify trends in surface and regular profile measurements over the last 20–30 years, and results from six chemistry‐climate models. Increases in observed ozone are found at the surface and in the free troposphere during winter in the high Arctic. Paradoxically, decreases in nitrogen oxide emissions at mid‐latitudes appear to be leading to increases in ozone during winter, but associated increases in Arctic tropospheric ozone tend to be overestimated in the models. Increases are also found at the surface in northern Alaska during spring but not reproduced by the models. The causes are unknown but could be related to changes in local sources or sinks of Arctic ozone or in large‐scale weather patterns. Declining mid‐latitude emissions, or increased dry deposition to northern forests, may explain negative surface ozone trends over northern Scandinavia in spring that are not always captured by the models. Further work is needed to understand changes in Arctic tropospheric ozone. Key Points: Coherent ozone trend analysis methodology applied to multi‐decade, pan‐Arctic surface and ozonesonde datasets and multi‐model mediansIncreasing winter Arctic tropospheric ozone overestimated by models in the free troposphere, and spring surface changes not capturedSpring (summer) decreases (increases) in observed ozone throughout the troposphere, not always simulated by models [ABSTRACT FROM AUTHOR]

The Earth's climate is rapidly changing. Over the past centuries, aerosols, via their ability to absorb or scatter solar radiation and alter clouds, played an important role in counterbalancing some of the greenhouse gas (GHG) caused global warming. The multicentury anthropogenic aerosol cooling effect prevented present‐day climate from reaching even higher surface air temperatures and subsequent more dramatic climate impacts. Trends in aerosol concentrations and optical depth show that in many polluted regions such as Europe and the United States, aerosol precursor emissions decreased back to levels of the 1950s. More recent polluting countries such as China may have reached a turning point in recent years as well, while India still follows an upward trend. Here we study aerosol trends in the Coupled Model Intercomparison Project Phase 6 (CMIP6) simulations of the GISS ModelE2.1 climate model using a fully coupled atmosphere composition configuration, including interactive gas‐phase chemistry and either an aerosol microphysical (MATRIX) or a mass‐based (One‐Moment Aerosol, OMA) aerosol module. Results show that whether global aerosol radiative forcing is already declining depends on the aerosol scheme used. Using the aerosol microphysical scheme, where the aerosol system reacts more strongly to the trend in sulfur dioxide (SO2) emissions, global peak direct aerosol forcing was reached in the 1980s, whereas the mass‐based scheme simulates peak direct aerosol forcing around 2010. Plain Language Summary: The National Aeronautics and Space Administration (NASA) Earth system model, GISS ModelE2.1, has released new interactive composition climate simulations from 1850 to 2014 into the Coupled Model Intercomparison Project Phase 6 (CMIP6) Diagnosis, Evaluation, and Characterization of Klima protocol archive. The GISS model includes two different schemes to simulate aerosols in the atmosphere, driven by natural and anthropogenic emissions. The two aerosol schemes differ by degree of complexity. One model better resolves aerosol microphysical processes, while the other model has more detailed chemistry regarding secondary organic aerosol formation. The models simulate different trends in aerosol radiative forcing. An evaluation with satellite data between 2001 and 2014 demonstrates that the model with more detailed aerosol microphysics has reached maximal aerosol direct forcing in the 1980s and is since on a decreasing global forcing trajectory. This has implications for using the trends over recent decades as predictive for greenhouse‐gas related changes in the future. Key Points: A discussion is presented of the AMIP aerosol simulations for the years 1850 to 2014 of the GISS ModelE2.1 for CMIP6, using two different aerosol schemesThe detailed treatment of aerosol microphysical processes greatly impacts aerosol forcing and forcing trendsOne model suggests that Earth has already exceeded the maximum negative forcing effects of anthropogenic aerosol in the 1980s [ABSTRACT FROM AUTHOR]

Societal benefits from climate change mitigation accrue via multiple pathways. We examine the US impacts of emission changes on several factors that are affected by both climate and air quality responses. Nationwide benefits through midcentury stem primarily from air quality improvements, which are realized rapidly, and include human health, labor productivity, and crop yield benefits. Benefits from reduced heat exposure become large around 2060, thereafter often dominating over those from improved air quality. Monetized benefits are in the tens of trillions of dollars for avoided deaths and tens of billions for labor productivity and crop yield increases and reduced hospital expenditures. Total monetized benefits this century are dominated by health and are much larger than in previous analyses due to improved understanding of the human health impacts of exposure to both heat and air pollution. Benefit-cost ratios are therefore much larger than in prior studies, especially those that neglected clean air benefits. Specifically, benefits from clean air exceed costs in the first decade, whereas benefits from climate alone exceed costs in the latter half of the century. Furthermore, monetized US benefits largely stem from US emissions reductions. Increased emphasis on the localized, near-term air quality-related impacts would better align policies with societal benefits and, by reducing the mismatch between perception of climate as a risk distant in space and time and the need for rapid action to mitigate long-term climate change, might help increase acceptance of mitigation policies. [ABSTRACT FROM AUTHOR]

Simulations of the CMIP6 historical period 1850–2014, characterized by the emergence of anthropogenic climate drivers like greenhouse gases, are presented for different configurations of the NASA Goddard Institute for Space Studies (GISS) Earth System ModelE2.1. The GISS‐E2.1 ensembles are more sensitive to greenhouse gas forcing than their CMIP5 predecessors (GISS‐E2) but warm less during recent decades due to a forcing reduction that is attributed to greater longwave opacity in the GISS‐E2.1 pre‐industrial simulations. This results in an atmosphere less sensitive to increases in opacity from rising greenhouse gas concentrations, demonstrating the importance of the base climatology to forcing and forced climate trends. Most model versions match observed temperature trends since 1979 from the ocean to the stratosphere. The choice of ocean model is important to the transient climate response, as found previously in CMIP5 GISS‐E2: the model that more efficiently exports heat to the deep ocean shows a smaller rise in tropospheric temperature. Model sea level rise over the historical period is traced to excessive drawdown of aquifers to meet irrigation demand with a smaller contribution from thermal expansion. This shows how fully coupled models can provide indirect observational constraints upon forcing, in this case, constraining irrigation rates with observed sea level changes. The overall agreement of GISS‐E2.1 with observed trends is familiar from evaluation of its predecessors, as is the conclusion that these trends are almost entirely anthropogenic in origin. Plain Language Summary: Measurements show clear evidence of warming over the twentieth century and up to the present day. Our anticipation of future change comes from computer models of climate. These are based upon well‐established physical principles like Newton's laws of motion and radiative transfer theory; the models are closely related to those used for weather forecasting. We can never predict the weather on a particular day, 50 years in the future, but we can calculate whether that future decade will be warmer than our present climate. Part of our confidence in such a forecast comes from testing a climate model's ability to reproduce warming and other changes measured over the past century. We use observations of atmospheric composition and the sunlight received by our planet to calculate how the model responds to their changes. The climate model of the NASA Goddard Institute for Space Studies, GISS‐E2.1, closely follows changes measured in the ocean and atmosphere as the concentrations of greenhouse gases and other pollutants rise. This agreement suggests that future warming by greenhouse gases will be reliably predicted by GISS‐E2.1. This suggests that the warming we already experience is due to our consumption of fossil fuels that has led to the increase of carbon dioxide and other greenhouse gases in the atmosphere over the past two centuries. Key Points: Tropospheric warming and ocean heat uptake by 2014 are smaller in GISS‐E2.1 and closer to observed trends than in its CMIP5 predecessorGISS‐E2.1 climate sensitivity is higher than in CMIP5 GISS‐E2, but forcing by greenhouse gases is smallerAtmospheric trends vary among model configurations with the storage of heat beneath the thermocline [ABSTRACT FROM AUTHOR]

This paper describes the GISS‐E2.1 contribution to the Coupled Model Intercomparison Project, Phase 6 (CMIP6). This model version differs from the predecessor model (GISS‐E2) chiefly due to parameterization improvements to the atmospheric and ocean model components, while keeping atmospheric resolution the same. Model skill when compared to modern era climatologies is significantly higher than in previous versions. Additionally, updates in forcings have a material impact on the results. In particular, there have been specific improvements in representations of modes of variability (such as the Madden‐Julian Oscillation and other modes in the Pacific) and significant improvements in the simulation of the climate of the Southern Oceans, including sea ice. The effective climate sensitivity to 2 × CO2 is slightly higher than previously at 2.7–3.1°C (depending on version) and is a result of lower CO2 radiative forcing and stronger positive feedbacks. Plain Language Summary: This paper describes the latest iteration of the National Aeronautics and Space Administration (NASA) Goddard Institute for Space Studies (GISS) climate model, which will be used for understanding historical climate change and to make projections for the future. We compare the model output to a wide range of observations over the recent era (1979–2014) and show that there has been a significant increase in how well the model performs compared to the previous version from 2014, particularly in the Southern Ocean, though some persistent biases remain. The model has a temperature response to the increase of carbon dioxide that is slightly higher than previous versions but is well within the range expected from observational and past climate constraints. Key Points: GISS‐E2.1 is an updated climate model version for use within the CMIP6 projectAtmospheric composition is calculated consistently in all model versionsResults demonstrate a significant improvement in skill in a climate model without changes to atmospheric resolution [ABSTRACT FROM AUTHOR]

An amendment to this paper has been published and can be accessed via a link at the top of the paper. [ABSTRACT FROM AUTHOR]

Observations of climate change during the CMIP5 extended historical period (1850-2012) are compared to trends simulated by six versions of the NASA Goddard Institute for Space Studies ModelE2 Earth System Model. The six models are constructed from three versions of the ModelE2 atmospheric general circulation model, distinguished by their treatment of atmospheric composition and the aerosol indirect effect, combined with two ocean general circulation models, HYCOM and Russell. Forcings that perturb the model climate during the historical period are described. Five-member ensemble averages from each of the six versions of ModelE2 simulate trends of surface air temperature, atmospheric temperature, sea ice and ocean heat content that are in general agreement with observed trends, although simulated warming is slightly excessive within the past decade. Only simulations that include increasing concentrations of long-lived greenhouse gases match the warming observed during the twentieth century. Differences in twentieth-century warming among the six model versions can be attributed to differences in climate sensitivity, aerosol and ozone forcing, and heat uptake by the deep ocean. Coupled models with HYCOM export less heat to the deep ocean, associated with reduced surface warming in regions of deepwater formation, but greater warming elsewhere at high latitudes along with reduced sea ice. All ensembles show twentieth-century annular trends toward reduced surface pressure at southern high latitudes and a poleward shift of the midlatitude westerlies, consistent with observations. [ABSTRACT FROM AUTHOR]

Abstract: Fire emissions associated with tropical land use change and maintenance influence atmospheric composition, air quality, and climate. In this study, we explore the effects of representing fire emissions at daily versus monthly resolution in a global composition-climate model. We find that simulations of aerosols are impacted more by the temporal resolution of fire emissions than trace gases such as carbon monoxide or ozone. Daily-resolved datasets concentrate emissions from fire events over shorter time periods and allow them to more realistically interact with model meteorology, reducing how often emissions are concurrently released with precipitation events and in turn increasing peak aerosol concentrations. The magnitude of this effect varies across tropical ecosystem types, ranging from smaller changes in modeling the low intensity, frequent burning typical of savanna ecosystems to larger differences when modeling the short-term, intense fires that characterize deforestation events. The utility of modeling fire emissions at a daily resolution also depends on the application, such as modeling exceedances of particulate matter concentrations over air quality guidelines or simulating regional atmospheric heating patterns. [Copyright &y& Elsevier]

We present a description of the ModelE2 version of the Goddard Institute for Space Studies (GISS) General Circulation Model (GCM) and the configurations used in the simulations performed for the Coupled Model Intercomparison Project Phase 5 (CMIP5). We use six variations related to the treatment of the atmospheric composition, the calculation of aerosol indirect effects, and ocean model component. Specifically, we test the difference between atmospheric models that have noninteractive composition, where radiatively important aerosols and ozone are prescribed from precomputed decadal averages, and interactive versions where atmospheric chemistry and aerosols are calculated given decadally varying emissions. The impact of the first aerosol indirect effect on clouds is either specified using a simple tuning, or parameterized using a cloud microphysics scheme. We also use two dynamic ocean components: the Russell and HYbrid Coordinate Ocean Model (HYCOM) which differ significantly in their basic formulations and grid. Results are presented for the climatological means over the satellite era (1980-2004) taken from transient simulations starting from the preindustrial (1850) driven by estimates of appropriate forcings over the 20th Century. Differences in base climate and variability related to the choice of ocean model are large, indicating an important structural uncertainty. The impact of interactive atmospheric composition on the climatology is relatively small except in regions such as the lower stratosphere, where ozone plays an important role, and the tropics, where aerosol changes affect the hydrological cycle and cloud cover. While key improvements over previous versions of the model are evident, these are not uniform across all metrics. [ABSTRACT FROM AUTHOR]

Background: Tropospheric ozone and black carbon (BC), a component of fine particulate matter (PM ≤ 2.5 μm in aerodynamic diameter; PM2.5), are associated with premature mortality and they disrupt global and regional climate. Objectives: We examined the air quality and health benefits of 14 specific emission control measures targeting BC and methane, an ozone precursor, that were selected because of their potential to reduce the rate of climate change over the next 20–40 years. Methods: We simulated the impacts of mitigation measures on outdoor concentrations of PM2.5 and ozone using two composition-climate models, and calculated associated changes in premature PM2.5‑ and ozone-related deaths using epidemiologically derived concentration–response functions. Results: We estimated that, for PM2.5 and ozone, respectively, fully implementing these measures could reduce global population-weighted average surface concentrations by 23–34% and 7–17% and avoid 0.6–4.4 and 0.04–0.52 million annual premature deaths globally in 2030. More than 80% of the health benefits are estimated to occur in Asia. We estimated that BC mitigation measures would achieve approximately 98% of the deaths that would be avoided if all BC and methane mitigation measures were implemented, due to reduced BC and associated reductions of nonmethane ozone precursor and organic carbon emissions as well as stronger mortality relationships for PM2.5 relative to ozone. Although subject to large uncertainty, these estimates and conclusions are not strongly dependent on assumptions for the concentration–response function. Conclusions: In addition to climate benefits, our findings indicate that the methane and BC emission control measures would have substantial co-benefits for air quality and public health worldwide, potentially reversing trends of increasing air pollution concentrations and mortality in Africa and South, West, and Central Asia. These projected benefits are independent of carbon dioxide mitigation measures. Benefits of BC measures are underestimated because we did not account for benefits from reduced indoor exposures and because outdoor exposure estimates were limited by model spatial resolution. [ABSTRACT FROM AUTHOR]

Tropospheric ozone and black carbon (BC) contribute to both degraded air quality and global warming. We considered ~400 emission control measures to reduce these pollutants by using current technology and experience. We identified 14 measures targeting methane and BC emissions that reduce projected global mean warming ~0.5°C by 2050. This strategy avoids 0.7 to 4.7 million annual premature deaths from outdoor air pollution and increases annual crop yields by 30 to 135 million metric tons due to ozone reductions in 2030 and beyond. Benefits of methane emissions reductions are valued at $700 to $5000 per metric ton, which is well above typical marginal abatement costs (less than $250). The selected controls target different sources and influence climate on shorter time scales than those of carbon dioxide--reduction measures. Implementing both substantially reduces the risks of crossing the 2°C threshold. [ABSTRACT FROM AUTHOR]

The authors simulate transient twentieth-century climate in the Goddard Institute for Space Studies (GISS) GCM, with aerosol and ozone chemistry fully coupled to one another and to climate including a full dynamic ocean. Aerosols include sulfate, black carbon (BC), organic carbon, nitrate, sea salt, and dust. Direct and BC-snow-albedo radiative effects are included. Model BC and sulfur trends agree fairly well with records from Greenland and European ice cores and with sulfur deposition in North America; however, the model underestimates the sulfur decline at the end of the century in Greenland. Global BC effects peak early in the century (1940s); afterward the BC effects decrease at high latitudes of the Northern Hemisphere but continue to increase at lower latitudes. The largest increase in aerosol optical depth occurs in the middle of the century (1940s--80s) when sulfate forcing peaks and causes global dimming. After this, aerosols decrease in eastern North America and northern Eurasia leading to regional positive forcing changes and brightening. These surface forcing changes have the correct trend but are too weak. Over the century, the net aerosol direct effect is −−0.41 W m−−2, the BC-albedo effect is −−0.02 W m−−2, and the net ozone forcing is ++0.24 W m−−2. The model polar stratospheric ozone depletion develops, beginning in the 1970s. Concurrently, the sea salt load and negative radiative flux increase over the oceans around Antarctica. Net warming over the century is modeled fairly well; however, the model fails to capture the dynamics of the observed midcentury cooling followed by the late century warming. Over the century, 20%% of Arctic warming and snow--ice cover loss is attributed to the BC-albedo effect. However, the decrease in this effect at the end of the century contributes to Arctic cooling. To test the climate responses to sulfate and BC pollution, two experiments were branched from 1970 that removed all pollution sulfate or BC. Averaged over 1970--2000, the respective radiative forcings relative to the full experiment were ++0.3 and −−0.3 W m−−2; the average surface air temperature changes were ++0.2°° and −−0.03°°C. The small impact of BC reduction on surface temperature resulted from reduced stability and loss of low-level clouds. [ABSTRACT FROM AUTHOR]

Global temperatures are known to have varied over the past 1500 years, but the spatial patterns have remained poorly defined. We used a global climate proxy network to reconstruct surface temperature patterns over this interval. The Medieval period is found to display warmth that matches or exceeds that of the past decade in some regions, but which falls well below recent levels globally. This period is marked by a tendency for La Niña--like conditions in the tropical Pacific. The coldest temperatures of the Little Ice Age are observed over the interval 1400 to 1700 C.E., with greatest cooling over the extratropical Northern Hemisphere continents. The patterns of temperature change imply dynamical responses of climate to natural radiative forcing changes involving El Niño and the North Atlantic Oscillation-Arctic Oscillation. [ABSTRACT FROM AUTHOR]

A full description of the ModelE version of the Goddard Institute for Space Studies (GISS) atmospheric general circulation model (GCM) and results are presented for present-day climate simulations (ca. 1979). This version is a complete rewrite of previous models incorporating numerous improvements in basic physics, the stratospheric circulation, and forcing fields. Notable changes include the following: the model top is now above the stratopause, the number of vertical layers has increased, a new cloud microphysical scheme is used, vegetation biophysics now incorporates a sensitivity to humidity, atmospheric turbulence is calculated over the whole column, and new land snow and lake schemes are introduced. The performance of the model using three configurations with different horizontal and vertical resolutions is compared to quality-controlled in situ data, remotely sensed and reanalysis products. Overall, significant improvements over previous models are seen, particularly in upper-atmosphere temperatures and winds, cloud heights, precipitation, and sea level pressure. Data–model comparisons continue, however, to highlight persistent problems in the marine stratocumulus regions. [ABSTRACT FROM AUTHOR]

The profound changes in global SO2 emissions over the last decades have affected atmospheric composition on a regional and global scale with large impact on air quality, atmospheric deposition and the radiative forcing of sulfate aerosols. Reproduction of historical atmospheric pollution levels based on global aerosol models and emission changes is crucial to prove that such models are able to predict future scenarios. Here, we analyze consistency of trends in observations of sulfur components in air and precipitation from major regional networks and estimates from six different global aerosol models from 1990 until 2015. There are large interregional differences in the sulfur trends consistently captured by the models and observations, especially for North America and Europe. Europe had the largest reductions in sulfur emissions in the first part of the period while the highest reduction came later in North America and East Asia. The uncertainties in both the emissions and the representativity of the observations are larger in Asia. However, emissions from East Asia clearly increased from 2000 to 2005 followed by a decrease, while in India a steady increase over the whole period has been observed and modelled. The agreement between a bottom-up approach, which uses emissions and process-based chemical transport models, with independent observations gives an improved confidence in the understanding of the atmospheric sulfur budget. [ABSTRACT FROM AUTHOR]