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Coherent quantum systems are a key resource for emerging quantum technology. Solid-state spin systems are of particular importance for compact and scalable devices. However, interaction with the solid-state host degrades the coherence properties. The negatively-charged silicon vacancy center in diamond is such an example. While spectral properties are outstanding, with optical coherence protected by the defects symmetry, the spin coherence is susceptible to rapid orbital relaxation limiting the spin dephasing time. A prolongation of the orbital relaxation time is therefore of utmost urgency and has been tackled by operating at very low temperatures or by introducing large strain. However, both methods have significant drawbacks, the former requires use of dilution refrigerators and the latter affects intrinsic symmetries. Here, a novel method is presented to prolong the orbital relaxation with a locally modified phonon density of states in the relevant frequency range, by restricting the diamond host to below 100 nm. The method works at liquid Helium temperatures of few Kelvin and in the low-strain regime.

Quantum random number generation is a key ingredient for quantum cryptography and fundamental quantum optics and could advance Monte-Carlo simulations and machine learning. An established generation scheme is based on single photons impinging on a beam splitter. Here, we experimentally demonstrate quantum random number generation solely based on the spontaneous emission process in combination with the symmetric emission profile of a dipole aligned orthogonal to the laboratory frame. The demonstration builds on defect centers in hexagonal boron nitride and benefits from the ability to manipulate and align the emission directionality. We prove the randomness in the correlated photon detection events making use of the NIST randomness test suite and show that the randomness remains for two independently emitting defect centers. The scheme can be extended to random number generation by coherent single photons with potential applications in solid-state based quantum communication at room temperature., Comment: 7 pages, 4 figures

Coherent exchange of single photons is at the heart of applied Quantum Optics. The negatively-charged silicon vacancy center in diamond is among most promising sources for coherent single photons. Its large Debye-Waller factor, short lifetime and extraordinary spectral stability is unique in the field of solid-state single photon sources. However, the excitation and detection of individual centers requires high numerical aperture optics which, combined with the need for cryogenic temperatures, puts technical overhead on experimental realizations. Here, we investigate a hybrid quantum photonics platform based on silicon-vacancy center in nanodiamonds and metallic bullseye antenna to realize a coherent single-photon interface that operates efficiently down to low numerical aperture optics with an inherent resistance to misalignment.

Spin-based quantum photonics promise to realize distributed quantum computing and quantum networks. The performance depends on efficient entanglement distribution, where the efficiency can be boosted by means of cavity quantum electrodynamics. The central challenge is the development of compact devices with large spin-photon coupling rates and high operation bandwidth. Photonic crystal cavities comprise strong field confinement but put high demands on accurate positioning of an atomic system in the mode field maximum. Color center in diamond, and in particular the negatively-charged Silicon-Vacancy center, emerged as a promising atom-like systems. Large spectral stability and access to long-lived, nuclear spin memories enabled elementary demonstrations of quantum network nodes including memory-enhanced quantum communication. In a hybrid approach, we deterministically place SiV$^-$-containing nanodiamonds inside one hole of a one-dimensional, free-standing, Si$_3$N$_4$-based photonic crystal cavity and coherently couple individual optical transitions to the cavity mode. We optimize the light-matter coupling by utilizing two-mode composition, waveguiding, Purcell-enhancement and cavity resonance tuning. The resulting photon flux is increased by more than a factor of 14 as compared to free-space. The corresponding lifetime shortening to below 460 ps puts the potential operation bandwidth beyond GHz rates. Our results mark an important step to realize quantum network nodes based on hybrid quantum photonics with SiV$^-$- center in nanodiamonds.

Quantum emitters in hexagonal Boron Nitride (hBN) were recently reported to hol a homogeneous linewidth according to the Fourier-Transform limit up to room temperature. This unusual observation was traced back to decoupling from in-plane phonon modes which can arise if the emitter is located between two planes of the hBN host material. In this work, we investigate the origins for the mechanical decoupling. Improved sample preparation enabled a reduced background and a 70-fold decrease of spectral diffusion which was so far the major drawback of defect center in hBN and allowed us to reveal a gap in the electron-phonon spectral density for low phonon frequencies. This decoupling from phonons persists at room temperature and explains the observed Fourier Transform limited lines up to 300K. Furthermore, we investigate the dipole emission directionality and show a preferred photon emission through the side of the hBN flakes supporting the claim for an out-of-plane distortion of the defect center. Our work lays the foundation to a deeper understanding of the underlying physics for the persistence of Fourier-Transform limit lines up to room temperature. It furthermore provides a description on how to identify the mechanically isolated emitter within the large number of defect centers in hBN. Therefore, it paves the way for quantum optics applications with defect centers in hBN at room temperature., Comment: 9 pages, 5 figures

Hybrid quantum photonics combines classical photonics with quantum emitters in a postprocessing step. It facilitates to link ideal quantum light sources to optimized photonic platforms. Optical cavities enable to harness the Purcell-effect boosting the device efficiency. Here, we postprocess a free-standing, crossed-waveguide photonic crystal cavity based on Si$_3$N$_4$ with SiV$^-$ center in nanodiamonds. We develop a routine that holds the capability to optimize all degrees of freedom of the evanescent coupling term utilizing AFM nanomanipulation. After a few optimization cycles we resolve the fine-structure of individual SiV$^-$ centers and achieve a Purcell enhancement of more than 4 on individual optical transitions, meaning that four out of five spontaneously emitted photons are channeled into the photonic device. Our work opens up new avenues to construct efficient quantum photonic devices., Comment: 7 pages, 4 figures. Nanophotonics (2020)

Optical coupling enables intermediate- and long-range interactions between distant quantum emitters. Such interaction may be the basic element in bottom-up approaches of coupled spin systems or for integrated quantum photonics and quantum plasmonics. Here, we prepare nanodiamonds carrying single, negatively-charged silicon-vacancy centers for evanescent optical coupling with access to all degrees of freedom by means of atomic force nanomanipulation. The color centers feature excellent optical properties, comparable to silicon-vacancy centers in bulk diamond, resulting in a resolvable fine structure splitting, a linewidth close to the Fourier-Transform limit under resonant excitation and a good polarization contrast. We determine the orbital relaxation time $T_{1}$ of the orbitally split ground states and show that all optical properties are conserved during translational nanomanipulation. Furthermore, we demonstrate the rotation of the nanodiamonds. In contrast to the translational operation, the rotation leads to a change in polarization contrast. We utilize the change in polarization contrast before and after nanomanipulation to determine the rotation angle. Finally, we evaluate the likelihood for indistinguishable, single photon emission of silicon-vacancy centers located in different nanodiamonds. Our work enables ideal evanescent, optical coupling of distant nanodiamonds containing silicon-vacancy centers with applications in the realization of quantum networks, quantum repeaters or complex quantum systems., Comment: 15 pages, 4 figures