Search

The combination of a powerful and broadly applicable nuclear hyperpolarization technique with emerging (near-)zero-field modalities offer novel opportunities in a broad range of nuclear magnetic resonance spectroscopy and imaging applications, including biomedical diagnostics, monitoring catalytic reactions within metal reactors and many others. These are discussed along with a roadmap for future developments., Comment: 12 pages, 5 figures

Ultralight axion-like particles (ALPs) are well-motivated dark matter candidates introduced by theories beyond the standard model. However, the constraints on the existence of ALPs through existing laboratory experiments are hindered by their current sensitivities, which are usually weaker than astrophysical limits. Here, we demonstrate a new quantum sensor to search for ALPs in the mass range that spans about two decades from 8.3 feV to 744 feV. Our sensor makes use of hyperpolarized long-lived nuclear spins as a pre-amplifier that effectively enhances coherently oscillating axion-like dark-matter field by a factor of >100. Using spin-based amplifiers, we achieve an ultrahigh magnetic sensitivity of 18 fT/Hz$^{1/2}$, which is significantly better than state-of-the-art nuclear-spin magnetometers. Our experiment constrains the parameter space describing the coupling of ALPs to nucleons over our mass range, at 67.5 feV reaching $2.9\times 10^{-9}~\textrm{GeV}^{-1}$ ($95\%$ confidence level), improving over previous laboratory limits by at least five orders of magnitude. Our measurements also constrain the ALP-nucleon quadratic interaction and dark photon-nucleon interaction with new limits beyond the astrophysical ones, Comment: 8 pages, 4 figures

Deep neural networks (DNNs) are widely used in pattern-recognition tasks for which a human comprehensible, quantitative description of the data-generating process, e.g., in the form of equations, cannot be achieved. While doing so, DNNs often produce an abstract (entangled and non-interpretable) representation of the data-generating process. This is one of the reasons why DNNs are not extensively used in physics-signal processing: physicists generally require their analyses to yield quantitative information about the studied systems. In this article we use DNNs to disentangle components of oscillating time series, and recover meaningful information. We show that, because DNNs can find useful abstract feature representations, they can be used when prior knowledge about the signal-generating process exists, but is not complete, as it is particularly the case in "new-physics" searches. To this aim, we train our DNN on synthetic oscillating time series to perform two tasks: a regression of the signal latent parameters and signal denoising by an Autoencoder-like architecture. We show that the regression and denoising performance is similar to those of least-square curve fittings (LS-fit) with true latent parameters' initial guesses, in spite of the DNN needing no initial guesses at all. We then explore applications in which we believe our architecture could prove useful for time-series processing in physics, when prior knowledge is incomplete. As an example, we employ DNNs as a tool to inform LS-fits when initial guesses are unknown. We show that the regression can be performed on some latent parameters, while ignoring the existence of others. Because the Autoencoder needs no prior information about the physical model, the remaining unknown latent parameters can still be captured, thus making use of partial prior knowledge, while leaving space for data exploration and discoveries.

We report the results of an experimental search for ultralight axion-like dark matter in the mass range 162 neV to 166 neV. The detection scheme of our Cosmic Axion Spin Precession Experiment (CASPEr) is based on a precision measurement of $^{207}$Pb solid-state nuclear magnetic resonance in a polarized ferroelectric crystal. Axion-like dark matter can exert an oscillating torque on $^{207}$Pb nuclear spins via the electric-dipole moment coupling $g_d$, or via the gradient coupling $g_{\text{aNN}}$. We calibrated the detector and characterized the excitation spectrum and relaxation parameters of the nuclear spin ensemble with pulsed magnetic resonance measurements in a 4.4 T magnetic field. We swept the magnetic field near this value and searched for axion-like dark matter with Compton frequency within a 1 MHz band centered at 39.65 MHz. Our measurements place the upper bounds $|g_d|<9.5\times10^{-4}\,\text{GeV}^{-2}$ and $|g_{\text{aNN}}|<2.8\times10^{-1}\,\text{GeV}^{-1}$ (95% confidence level) in this frequency range. The constraint on $g_d$ corresponds to an upper bound of $1.0\times 10^{-21}\,\text{e}\cdot\text{cm}$ on the amplitude of oscillations of the neutron electric dipole moment, and $4.3\times 10^{-6}$ on the amplitude of oscillations of CP-violating $\theta$ parameter of quantum chromodynamics. Our results demonstrate the feasibility of using solid-state nuclear magnetic resonance to search for axion-like dark matter in the nano-electronvolt mass range.

Light scalar Dark Matter with scalar couplings to matter is expected within several scenarios to induce variations in the fundamental constants of nature. Such variations can be searched for, among other ways, via atomic spectroscopy. Sensitive atomic observables arise primarily due to possible changes in the fine-structure constant or the electron mass. Most of the searches to date have focused on slow variations of the constants (i.e. modulation frequencies $<$ 1 Hz). In a recent experiment \mbox{[Phys. Rev. Lett. 123, 141102 (2019)]} called WReSL (Weekend Relaxion-Search Laboratory), we reported on a direct search for rapid variations in the radio-frequency band. Such a search is particularly motivated within a class of relaxion Dark Matter models. We discuss the WReSL experiment, report on progress towards improved measurements of rapid fundamental constant variations, and discuss the planned extension of the work to molecules, in which rapid variations of the nuclear mass can be sensitively searched for., Comment: 15 pages, 4 figures

Numerous theories extending beyond the standard model of particle physics predict the existence of bosons that could constitute the dark matter (DM) permeating the universe. In the standard halo model (SHM) of galactic dark matter the velocity distribution of the bosonic DM field defines a characteristic coherence time $\tau_c$. Until recently, laboratory experiments searching for bosonic DM fields have been in the regime where the measurement time $T$ significantly exceeds $\tau_c$, so null results have been interpreted as constraints on the coupling of bosonic DM to standard model particles with a bosonic DM field amplitude $\Phi_0$ fixed by the average local DM density. However, motivated by new theoretical developments, a number of recent searches probe the regime where $T\ll\tau_c$. Here we show that experiments operating in this regime do not sample the full distribution of bosonic DM field amplitudes and therefore it is incorrect to assume a fixed value of $\Phi_0$ when inferring constraints on the coupling strength of bosonic DM to standard model particles. Instead, in order to interpret laboratory measurements (even in the event of a discovery), it is necessary to account for the stochastic nature of such a virialized ultralight field (VULF). The constraints inferred from several previous null experiments searching for ultralight bosonic DM were overestimated by factors ranging from 3 to 10 depending on experimental details, model assumptions, and choice of inference framework., Comment: Supplementary material was not compiled in previous version

The nature of dark matter, the invisible substance making up over $80\%$ of the matter in the Universe, is one of the most fundamental mysteries of modern physics. Ultralight bosons such as axions, axion-like particles or dark photons could make up most of the dark matter. Couplings between such bosons and nuclear spins may enable their direct detection via nuclear magnetic resonance (NMR) spectroscopy: as nuclear spins move through the galactic dark-matter halo, they couple to dark-matter and behave as if they were in an oscillating magnetic field, generating a dark-matter-driven NMR signal. As part of the Cosmic Axion Spin Precession Experiment (CASPEr), an NMR-based dark-matter search, we use ultralow-field NMR to probe the axion-fermion "wind" coupling and dark-photon couplings to nuclear spins. No dark matter signal was detected above background, establishing new experimental bounds for dark-matter bosons with masses ranging from $1.8\times 10^{-16}$ to $7.8\times 10^{-14}$ eV., Comment: 10 pages, 5 figures

We report the results of a search for axionlike dark matter using nuclear magnetic resonance (NMR) techniques. This search is part of the multi-faceted Cosmic Axion Spin Precession Experiment (CASPEr) program. In order to distinguish axionlike dark matter from magnetic fields, we employ a comagnetometry scheme measuring ultralow-field NMR signals involving two different nuclei ($^{13}$C and $^{1}$H) in a liquid-state sample of acetonitrile-2-$^{13}$C ($^{13}$CH$_{3}$CN). No axionlike dark matter signal was detected above background. This result constrains the parameter space describing the coupling of the gradient of the axionlike dark matter field to nucleons to be $g_{aNN}<6\times 10^{-5}$ GeV$^{-1}$ (95$\%$ confidence level) for particle masses ranging from $10^{-22}$ eV to $1.3\times10^{-17}$ eV, improving over previous laboratory limits for masses below $10^{-21}$ eV. The result also constrains the coupling of nuclear spins to the gradient of the square of the axionlike dark matter field, improving over astrophysical limits by orders of magnitude over the entire range of particle masses probed.

The Cosmic Axion Spin Precession Experiment (CASPEr) is a nuclear magnetic resonance experiment (NMR) seeking to detect axion and axion-like particles which could make up the dark matter present in the universe. We review the predicted couplings of axions and axion-like particles with baryonic matter that enable their detection via NMR. We then describe two measurement schemes being implemented in CASPEr. The first method, presented in the original CASPEr proposal, consists of a resonant search via continuous-wave NMR spectroscopy. This method offers the highest sensitivity for frequencies ranging from a few Hz to hundreds of MHz, corresponding to masses $ m_{\rm a} \sim 10^{-14}$--$10^{-6}$ eV. Sub-Hz frequencies are typically difficult to probe with NMR due to the diminishing sensitivity of magnetometers in this region. To circumvent this limitation, we suggest new detection and data processing modalities. We describe a non-resonant frequency-modulation detection scheme, enabling searches from mHz to Hz frequencies ($m_{\rm a} \sim 10^{-17}$--$10^{-14} $ eV), extending the detection bandwidth by three decades.