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We report on the generation of ultrabroadband supercontinuum (SC) by filamentation of two optical-cycle, carrier-envelope phase-stable pulses at 2 μm in fused silica, sapphire, CaF₂ and YAG. The SC spectra extend from 450 nm to more than 2500 nm, and their particular shapes depend on dispersive properties of the materials. Prior to spectral super-broadening, we observe third-harmonic generation, which occurs in the condition of large phase and group velocity mismatch and consists of free and driven components. A double-peaked third-harmonic structure coexists with the SC pulse as demonstrated by the numerical simulations and verified experimentally. The SC pulses have stable carrier envelope phase with short-term rms fluctuations of ∼ 300 mrad, as simultaneously measured in YAG crystal by f-2f and f-3f interferometry, where the latter makes use of intrinsic third-harmonic generation.

We report on the generation of two optical-cycle, carrier-envelope phase-stable pulses with energy of 15 μJ at central wavelength of 2 μm. Pulses of 15 fs (2.3 optical cycles) duration are obtained by difference-frequency generation, which at the same time provides passive carrier-envelope phase stabilization, and noncollinear optical parametric amplification in beta-barium borate crystal, which is shown to provide broad phase-matching bandwidth if seeded by pulses in the 1.6-2.6 μm wavelength range. Pulse compression is achieved by means of a simple propagation through the optical setup and by precisely controlling the initial chirp of the pulses to be frequency downconverted.