Search

Recent discovery of orbital currents in several material platforms including light element metals has opened new possibilities for exploring novel transport phenomena and applications to spin-orbitronic devices. These orbital currents, similar to spin currents, have the ability to generate torque on adjacent magnetic layers, opening a new avenue for efficient spintronic devices. However, separating spin and orbital currents has been one of the major challenges. Here, we show evidence for large conventional as well as unconventional spin and orbital currents in IrO$_2$ and disentangle them by crystal symmetry. We study the anisotropic spin and orbital Hall effects in IrO$_2$ (001), (100), and (111) orientations and find unconventional z-polarized orbital torques using angular spin torque ferromagnetic resonance of IrO$_2$/Ni heterostructures, which are in agreement regarding the relative signs with theoretical calculations of spin and orbital Hall conductivity. This work provides a promising route towards highly efficient low power spintronic and orbitronic devices in oxide heterostructures.

The emergence of anomalous Hall effects (AHE) in antiferromagnets presents an intriguing phenomenon with potential spintronic device applications due to their ultrafast switching dynamics. Mn3NiN antiperovskite stands out as a promising candidate owing to its noncollinear antiferromagnetism. In this study, we report a significant AHE observed in epitaxial Mn3NiN thin films below the N\'eel temperature, comparable to those observed in typical ferromagnets. Through a combination of magnetometry, neutron diffraction and ab-initio data analyses, we propose that the substantial AHE can be attributed to the non-vanishing Berry curvature arising from the {\Gamma}4g-type spin structure, coupled with uncompensated magnetic domains featuring a weak canted moment. This coupling, due to robust antiferromagnetic domains, enables deterministic detection and switching of AHE via the application of a magnetic field.

Unconventional spin-orbit torques arising from electric-field-generated spin currents in anisotropic materials have promising potential for spintronic applications, including for perpendicular magnetic switching in high-density memory applications. Here we determine all the independent elements of the spin torque conductivity tensor allowed by bulk crystal symmetries for the tetragonal conductor IrO2, via measurements of conventional (in plane) antidamping torques for IrO2 thin films in the high-symmetry (001) and (100) orientations. We then test that rotational transformations of this same tensor can predict both the conventional and unconventional anti-damping torques for IrO2 thin films in the lower-symmetry (101), (110), and (111) orientations, finding good agreement. The results confirm that spin-orbit torques from all these orientations are consistent with the bulk symmetries of IrO2, and show how simple measurements of conventional torques from high-symmetry orientations of anisotropic thin films can provide an accurate prediction of the unconventional torques from lower-symmetry orientations., Comment: Main text: 14 pages, 3 figures. Supporting Information: 19 pages, 10 figures, and 1 table

Recent theoretical predictions and experimental demonstrations of a large tunneling magnetoresistance (TMR) effect in antiferromagnetic (AFM) tunnel junctions (AFMTJs) offer a new paradigm for information technologies where the AFM N\`eel vector serves as a state variable. A large TMR is beneficial for the applications. Here, we predict the emergence of an extraordinary TMR (ETMR) effect in AFMTJs utilizing noncollinear AFM antiperovskite XNMn$_{3}$ (X = Ga, Sn,...) electrodes and a perovskite oxide ATiO$_{3}$ (A = Sr, Ba,...) barrier layer. The ETMR effect stems from the perfectly spin-polarized electronic states in the AFM antiperovskites that can efficiently tunnel through the low-decay-rate evanescent states of the perovskite oxide while preserving their spin state. Using an GaNMn$_{3}$/SrTiO$_{3}$/GaNMn$_{3}$ (001) AFMTJ as a representative example, we demonstrate a giant TMR ratio exceeding $10^{4}$% and originating from the ETMR effect. These results are promising for the efficient detection and control of the N\`eel vector in AFM spintronics.

Van der Waals (vdW) assembly allows controlling symmetry of two-dimensional (2D) materials that determines their physical properties. Especially interesting is the recently demonstrated breaking inversion symmetry by polar layer stacking to realize novel electronic, magnetic, and transport properties of 2D vdW materials switchable by induced electric polarization. Here, based on symmetry analyses and density-functional calculations, we explore the emergence of the anomalous Hall effect (AHE) in antiferromagnetic MnBi2Te4 films assembled by polar layer stacking. We demonstrate that breaking PT symmetry in an MnBi2Te4 bilayer makes this 2D material magnetoelectric and produces a spontaneous AHE switchable by electric polarization. We find that reversable polarization at one of the interfaces in a three-layer MnBi2Te4 film drives a metal-insulator transition, as well as switching between an AHE and quantum AHE (QAHE). Finally, we predict that engineering an interlayer polarization in a three-layer MnBi2Te4 film allows converting MnBi2Te4 from a trivial insulator to a Chern insulator. Overall, our work emphasizes the emergence of quantum-transport phenomena in 2D vdW antiferromagnets by polar layer stacking, which do not exist in this material in the bulk or bulk-like thin-film forms.

Ferromagnets are known to support spin-polarized currents that control various spin-dependent transport phenomena useful for spintronics. On the contrary, fully compensated antiferromagnets are expected to support only globally spin-neutral currents. Here, we demonstrate that these globally spin-neutral currents can represent the N\'eel spin currents, i.e. staggered spin currents flowing through different magnetic sublattices. The N\'eel spin currents emerge in antiferromagnets with strong intra-sublattice coupling (hopping) and drive the spin-dependent transport phenomena such as tunneling magnetoresistance (TMR) and spin-transfer torque (STT) in antiferromagnetic tunnel junctions (AFMTJs). Using RuO$_{2}$ and Fe$_{4}$GeTe$_{2}$ as representative antiferromagnets, we predict that the N\'eel spin currents with a strong staggered spin-polarization produce a sizable field-like STT capable of the deterministic switching of the N\'eel vector in the associated AFMTJs. Our work uncovers the previously unexplored potential of fully compensated antiferromagnets and paves a new route to realize the efficient writing and reading of information for antiferromagnetic spintronics.

Antiferromagnetic (AFM) spintronics has emerged as a subfield of spintronics driven by the advantages of antiferromagnets producing no stray fields and exhibiting ultrafast magnetization dynamics. The efficient method to detect an AFM order parameter, known as the N\'eel vector, by electric means is critical to realize concepts of AFM spintronics. Here, we demonstrate that non-collinear AFM metals, such as Mn3Sn, exhibit a momentum dependent spin polarization which can be exploited in AFM tunnel junctions to detect the N\'eel vector. Using first-principles calculations based on density functional theory, we predict a tunneling magnetoresistance (TMR) effect as high as 300% in AFM tunnel junctions with Mn3Sn electrodes, where the junction resistance depends on the relative orientation of their N\'eel vectors and exhibits four non-volatile resistance states. We argue that the spin-split band structure and the related TMR effect can also be realized in other non-collinear AFM metals like Mn3Ge, Mn3Ga, Mn3Pt, and Mn3GaN. Our work provides a robust method for detecting the N\'eel vector in non-collinear antiferromagnets via the TMR effect, which may be useful for their application in AFM spintronic devices.

Spin-polarized currents play a key role in spintronics. Recently, it has been found that antiferromagnets with a non-spin-degenerate band structure can efficiently spin-polarize electric currents, even though their net magnetization is zero. Among the antiferromagnetic metals with magnetic space group symmetry supporting this functionality, the noncollinear antiferromagnetic antiperovskites ANMn$_3$ (A = Ga, Ni, Sn, and Pt) are especially promising. This is due to their high N\'eel temperatures and a good lattice match to perovskite oxide substrates, offering possibilities of high structural quality heterostructures based on these materials. Here, we investigate the spin polarization of antiferromagnetic ANMn$_3$ metals using first-principles density functional theory calculations. We find that the spin polarization of the longitudinal currents in these materials is comparable to that in widely used ferromagnetic metals, and thus can be exploited in magnetic tunnel junctions and spin transfer torque devices. Moreover, for certain film growth directions, the out-of-plane transverse spin currents with a giant charge-to-spin conversion efficiency can be achieved, implying that the ANMn$_3$ antiperovskites can be used as efficient spin sources. These properties make ANMn$_3$ compounds promising for application in spintronics.

The control of spin-dependent properties by voltage, not involving magnetization switching, has significant advantages for low-power spintronics. Here, we predict that the interfacial crystal Hall effect (ICHE) can serve for this purpose. We show that the ICHE can occur in heterostructures composed of compensated antiferromagnetic metals and non-magnetic insulators due to reduced symmetry at the interface, and it can be made reversible if the antiferromagnet is layered symmetrically between two identical ferroelectric layers. We explicitly demonstrate this phenomenon using density functional theory calculations for three material systems: MnBi$_{2}$Te$_{4}$/GeI$_{2}$ and topological In$_{2}$Te$_{3}$/MnBi$_{2}$Te$_{4}$/In$_{2}$Te$_{3}$ van der Waals heterostructures, and GeTe/Ru$_{2}$MnGe/GeTe heterostructure composed of three-dimensional materials. We show that all three systems reveal a sizable ICHE, while the latter two exhibit a quantum ICHE and ICHE, respectively, reversible with ferroelectric polarization. Our proposal opens an alternative direction for voltage controlled spintronics and offers not yet explored possibilities for functional devices by heterostructure design.

Antiferromagnetic (AFM) spintronics exploits the N\'eel vector as a state variable for novel spintronic devices. Recent studies have shown that the field-like and antidamping spin-orbit torques (SOT) can be used to switch the N\'eel vector in antiferromagnets with proper symmetries. However, the precise detection of the N\'eel vector remains a challenging problem. In this letter, we predict that the nonlinear anomalous Hall effect (AHE) can be used to detect the N\'eel vector in most compensated antiferromagnets supporting the antidamping SOT. We show that the magnetic crystal group symmetry of these antiferromagnets combined with spin-orbit coupling produce a sizable Berry curvature dipole and hence the nonlinear AHE. As a specific example, we consider half-Heusler alloy CuMnSb, which N\'eel vector can be switched by the antidamping SOT. Based on density functional theory calculations, we show that the nonlinear AHE in CuMnSb results in a measurable Hall voltage under conventional experimental conditions. The strong dependence of the Berry curvature dipole on the N\'eel vector orientation provides a new detection scheme of the N\'eel vector based on the nonlinear AHE. Our predictions enrich the material platform for studying non-trivial phenomena associated with the Berry curvature and broaden the range of materials useful for AFM spintronics.

The anomalous Hall effect (AHE) is a well-known fundamental property of ferromagnetic metals, commonly associated with the presence of a net magnetization. Recently, an AHE has been discovered in non-collinear antiferromagnetic (AFM) metals. Driven by non-vanishing Berry curvature of AFM materials with certain magnetic space group symmetry, anomalous Hall conductivity (AHC) is very sensitive to the specific type of magnetic ordering. Here, we investigate the appearance of AHC in antiperovskite GaNMn$_{3}$ as a representative of broader materials family ANMn$_{3}$ (A is a main group element), where different types of non-collinear magnetic ordering can emerge. Using symmetry analyses and first-principles density-functional theory calculations, we show that with almost identical band structure, the nearly degenerate non-collinear AFM $\Gamma_{5g}$ and $\Gamma_{4g}$ phases of GaNMn$_{3}$ have zero and finite AHC, respectively. In a non-collinear ferrimagnetic $M$-1 phase, GaNMn$_{3}$ exhibits a large AHC due to the presence of a sizable net magnetic moment. In the non-collinear antiperovskite magnets, transitions between different magnetic phases, exhibiting different AHC states, can be produced by doping, strain, or spin transfer torque, which makes these materials promising for novel spintronic applications.

Topological antiferromagnetic (AFM) spintronics is an emerging field of research, which exploits the N\'eel vector to control the topological electronic states and the associated spin-dependent transport properties. A recently discovered N\'eel spin-orbit torque has been proposed to electrically manipulate Dirac band crossings in antiferromagnets; however, a reliable AFM material to realize these properties in practice is missing. Here, we predict that room temperature AFM metal MnPd$_{2}$ allows the electrical control of the Dirac nodal line by the N\'eel spin-orbit torque. Based on first-principles density functional theory calculations, we show that reorientation of the N\'eel vector leads to switching between the symmetry-protected degenerate state and the gapped state associated with the dispersive Dirac nodal line at the Fermi energy. The calculated spin Hall conductivity strongly depends on the N\'eel vector orientation and can be used to experimentally detect the predicted effect using a proposed spin-orbit torque device. Our results indicate that AFM Dirac nodal line metal MnPd$_{2}$ represents a promising material for topological AFM spintronics.