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Radiographic imaging is an omnipresent tool in basic research and applications in industry, material science and medical diagnostics. Often, the information contained in more than one modality can be valuable, but difficult to access simultaneously. This talk reviews developments in laser-plasma-accelerators for protons, electrons and x-rays from solid and gas targets for multimodal imaging. Laser-driven ion acceleration and x-ray generation have been investigated using tungsten micro-needle-targets at the Texas Petawatt laser [1]. The experiments and supporting numerical simulations reveal peaked proton spectra around 10 MeV with significant particle count and a strong keV level x-ray source. The source size for both has been measured to be in the few-µm range. Both sources were eventually applied to simultaneous radiographic imaging of biological and technological samples. In recent experiments at BELLA Center’s high repetition rate 100 TW dual-arm laser, steps were taken towards bi-modal x-ray and electron imaging of dynamic events such as hydrodynamic shocks, in which often both density and electro-magnetic fields are important quantities to measure. Here, a shock was driven by a 1 Joule, 200 ps laser focused in a 30 µm wide water jet. A laser wakefield accelerator was driven by a second 2 Joule, 40 fs laser in a gas-jet target, providing both 150 MeV electrons and broadband betatron x-rays up to ˜10 keV for projection imaging. This research aims to leverage unique properties readily available in laser plasma accelerators for applications. Specifically, the emission of pulsed, bright, multimodal bursts of radiation can open new ways in biological imaging (e.g., with ns-synchronized ions and x-rays) and in high-resolution diagnostics for high-energy density science (e.g., with fs-synchronized electrons and x-rays). [1] T. M. Ostermayr et al., “Laser-driven x-ray and proton micro-source and application to simultaneous single-shot bi-modal radiographic imaging,” Nat. Commun., vol. 11, no. 1, pp. 1–9, Dec. 2020. This work was supported by the DFG via the Cluster of Excellence Munich-Centre for Advanced Photonics (MAP) and Transregio SFB TR18. This work has been carried out within the framework of the EUROfusion Consortium and has received funding, through the ToIFE, from the European Union’s Horizon 2020 research and innovation program under grant agreement number 633053. The authors acknowledge funding by the Air Force Office of Scientific Research (AFOSR)(FA9550-14-1-0045, FA9550-17-1-0264). Work supported by DOE FES under grant DE-SC0020237. Work supported by US DOE NNSA DNN R&D, by Sc. HEP, by the Exascale Computing Project and by FES LaserNetUS under DOE Contract DE-AC02-05CH11231.

We present an online, non-destructive laser diagnostic capable of measuring the transverse position/pointing angle at focus of a 100-TW laser system using double-surface-coated wedged-mirror design for the final steering optic in the laser line.

This work examines pulses with orbital angular momentum and simulates the characterization of these pulses using STRIPED FISH, which correctly retrieves optical vortices and can be leveraged to provide deeper insight into laser plasma interactions.

Author(s): Isono, F; Van Tilborg, J; Barber, SK; Natal, J; Berger, C; Tsai, HE; Ostermayr, T; Gonsalves, A; Geddes, C; Esarey, E | Abstract: Controlling the delivery of multi-terawatt and petawatt laser pulses to final focus, both in position and angle, is critical to many laser applications such as optical guiding, laser-plasma acceleration, and laser-produced secondary radiation. We present an online, non-destructive laser diagnostic, capable of measuring the transverse position and pointing angle at focus. The diagnostic is based on a unique double-surface-coated wedged-mirror design for the final steering optic in the laser line, producing a witness beam highly correlated with the main beam. By propagating low-power kilohertz pulses to focus, we observed spectra of focus position and pointing angle fluctuations dominated by frequencies below 70 Hz. The setup was also used to characterize the excellent position and pointing angle correlation of the 1 Hz high-power laser pulses to this low-power kilohertz pulse train, opening a promising path to fast non-perturbative feedback concepts even on few-hertz-class high-power laser systems.

Relativistic electron beams driven by laser wakefield acceleration were utilized to produce ultrashort neutron sources. The experiment was carried out on the 38 fs, ∼0.5 J, 800 nm Ti:Sapphire laser in the 10 TW UT3 laser lab at University of Texas at Austin. The target gas was a high density pulsed gas jet composed of 90% He and 10% N2. The laser pulse with a peak intensity of 1.5 × 1018 W/cm2 interacted with the target to create a cylindrical plasma channel of 60 μm radius (FWHM) and 1.5 mm length (FWHM). Electron beams of ∼80 pC with the Gaussian energy distribution centered at 37 MeV and a width of 30 MeV (FWHM) were produced via laser wakefield acceleration. Neutron fluences of ∼2.4 × 106 per shot with hundreds of ps temporal length were generated through bremsstrahlung and subsequent photoneutron reactions in a 26.6 mm thick tungsten converter. Results were compared with those of simulations using EPOCH and GEANT4, showing agreement in electron spectrum, neutron fluence, neutron angular distribution and conversion rate. Keywords: Neutron source, LWFA, Photoneutron reaction, PACS Codes: 29.25.Dz, 52.38.Kd, 52.38.Ph, 52.59.-f

Physics of fluids 32(6), 066108 (2020). doi:10.1063/5.0005888, Density transition injection is an effective technique for controllably loading electrons into a trapped phase for laser plasma accelerators. One common technique to achieve the required fluid structure is to impinge a thin blade on the plume of a supersonic nozzle. Density transitions induced in this way are often assumed to be bow shocks and therefore sharp, but simulations and fluorescence measurements presented in this work show that in many cases of interest, the density transition accessible to a laser propagating transverse to the shock is an intercepting shock, and therefore, shock thickness and density vary with pressure, laser height, and blade position. The fluid dynamics of a supersonic nozzle impinged on by a thin, flat object are explored through simulations and relevant features are verified via planar laser-induced fluorescence measurements. The implications of the results for tuning electron beam injectors in laser plasma accelerators are discussed., Published by American Institute of Physics, [S.l.]

Supersonic gas jets produced by converging-diverging (C-D) nozzles are commonly used as targets for laser-plasma acceleration (LPA) experiments. A major point of interest for these targets is the gas density at the region of interaction where the laser ionizes the gas plume to create a plasma, providing the acceleration structure. Tuning the density profiles at this interaction region is crucial to LPA optimization. A "flat-top" density profile is desired at this line of interaction to control laser propagation and high energy electron acceleration, while a short high-density profile is often preferred for acceleration of lower-energy tightly-focused laser-plasma interactions. A particular design parameter of interest is the curvature of the nozzle's diverging section. We examine three nozzle designs with different curvatures: the concave "bell", straight conical and convex "trumpet" nozzles. We demonstrate that, at mm-scale distances from the nozzle exit, the trumpet and straight nozzles, if optimized, produce "flat-top" density profiles whereas the bell nozzle creates focused regions of gas with higher densities. An optimization procedure for the trumpet nozzle is derived and compared to the straight nozzle optimization process. We find that the trumpet nozzle, by providing an extra parameter of control through its curvature, is more versatile for creating flat-top profiles and its optimization procedure is more refined compared to the straight nozzle and the straight nozzle optimization process. We present results for different nozzle designs from computational fluid dynamics (CFD) simulations performed with the program ANSYS Fluent and verify them experimentally using neutral density interferometry., Comment: 14 pages, 16 figures, 5 tables

In this report, we demonstrate precise control of a laser plasma accelerator (LPA) through characterization of a shock-induced density downramp injector. Experiments systematically varied the shock injector profile, including shock angle, shock position, up-ramp width, and acceleration length. As a result, an electron beam that was highly tunable from 30 to 300 MeV with 8.5% energy spread, 1.5 mrad divergence and 0.35 mrad pointing fluctuation was produced. We also report the progress of a project focusing on demonstrating the crucial enablers of a compact LPA based MeV Thomson photon source in an integrated experiment and a dedicated 100 TW laser facility built at the Berkeley Lab Laser Accelerator (BELLA) Center, Lawrence Berkeley National Laboratory (LBNL).

Author(s): Swanson, KK; Tsai, HE; Barber, SK; Lehe, R; Mao, HS; Steinke, S; Van Tilborg, J; Nakamura, K; Geddes, CGR; Schroeder, CB; Esarey, E; Leemans, WP | Abstract: Control of the properties of laser-plasma-accelerated electron beams that were injected along a shock-induced density downramp through precision tailoring of the density profile was demonstrated using a 1.8 J, 45 fs laser interacting with a mm-scale gas jet. The effects on the beam spatial profile, steering, and absolute energy spread of the density region before the shock and tilt of the shock were investigated experimentally and with particle-in-cell simulations. By adjusting these density parameters, the electron beam quality was controlled and improved while the energy (30-180 MeV) and energy spread (2-11 MeV) were independently tuned. Simple models that are in good agreement with the experimental results are proposed to explain these relationships, advancing the understanding of downramp injection. This technique allows for high-quality electron beams with percent-level energy spread to be tailored based on the application.

Single-shot, charge-dependent emittance measurements of electron beams generated by a laser plasma accelerator (LPA) reveal that shock-induced density down-ramp injection produces beams with normalized emittances a factor of 2 smaller than beams produced via ionization injection. Such a comparison is made possible by the tunable LPA setup, which allows electron beams with nearly identical central energy and peak spectral charge density to be produced using the two distinct injection mechanisms. Parametric measurements of this type are essential for the development of LPA-based applications which ultimately require high charge density and low emittance.

Previous work has demonstrated the use of a plasma mirror (PM), after a laser-plasma accelerator (LPA), for generating Compton γ-rays by retro-reflecting the spent laser pulse into the just-accelerated electrons. Here, we investigate the use of a PM to stimulate Compton backscatter (CBS) by retro-reflecting a spent pulse from the Texas Petawatt (TPW) laser after it has driven a cm-scale, GeV LPA. A comparative analysis between the electron and CBS pointing and divergence reveals strong agreement, from shot-to-shot, suggesting a reliable, non-invasive extension for GeV-beam metrology. Our observations confirm the self-aligning PM method is scalable to GeV LPAs, while also suggesting a technique with unique advantages and a robustness that can potentially be exploited for investigations of nonlinear Compton backscatter from ultralow divergence, GeV electrons using the Texas Petawatt Laser.

Author(s): Van Tilborg, J; Barber, SK; Tsai, HE; Swanson, KK; Steinke, S; Geddes, CGR; Gonsalves, AJ; Schroeder, CB; Esarey, E; Bulanov, SS; Bobrova, NA; Sasorov, PV; Leemans, WP | Abstract: Active plasma lenses have attracted interest in novel accelerator applications due to their ability to provide large-field-gradient (short focal length), tunable, and radially symmetric focusing for charged particle beams. However, if the discharge current is not flowing uniformly as a function of radius, one can expect a radially varying field gradient as well as potential emittance degradation. We have investigated this experimentally for a 1-mm-diameter active plasma lens. The measured near-axis field gradient is approximately 35% larger than expected for a uniform current distribution, and at overfocusing currents ring-shaped electron beams are observed. These observations are explained by simulations.

Compact, high-quality photon sources at MeV energies are being developed based on Laser-Plasma Accelerators (LPAs), and these sources at the same time provide precision diagnostics of beam evolution to support LPA development. We review design of experiments and laser capabilities to realize a photon source, integrating LPA acceleration for compactness, control of scattering to increase photon flux, and electron deceleration to mitigate beam dump size. These experiments are developing a compact photon source system with the potential to enable new monoenergetic photon applications currently restricted by source size, including nuclear nonproliferation. Diagnostic use of the energy-angle spectra of Thomson scattered photons is presented to support development of LPAs to meet the needs of advanced high yield/low-energy-spread photon sources and future high energy physics colliders.

Density transition injection is an effective technique for controllably loading electrons into a trapped phase for laser-plasma accelerators. One common technique to achieve this fluid phenomenon is to impinge a thin blade on the plume of a supersonic nozzle. 2-D simulations show that the density transition accessible to a transverse laser is produced by a rapid re-expansion of the high pressure region behind the initial bow shock, and not by the bow shock produced by the blade, as is commonly thought. This pressure mismatched re-expansion generates compression waves that could coalesce into shock-fronts as they interact with the surrounding ambient gas. This has consequences when interpreting the electron injection mechanism. In the simulations presented here, the fluid dynamics of a supersonic nozzle impinged on by a thin, flat object is explored, along with the implications for electron beam injectors in laser-plasma accelerators.

In this paper, we demonstrate a highly tunable, controlled-injection laser-plasma accelerator (LPA) through systematically varying parameters of a density shock injector. Beam energy, energy spread, charge and pointing can be controlled in the range of 50−300 MeV, with

We report production of a self-injected, collimated (8 mrad divergence), 600 pC bunch of electrons with energies up to 350 MeV from a petawatt laser-driven plasma accelerator in a plasma of electron density ne = 1017 cm−3, an order of magnitude lower than previous self-injected laser-plasma accelerators. The energy of the focused drive laser pulse (150 J, 150 fs) was distributed over several hot spots. Simulations show that these hot spots remained independent over a 5 cm interaction length, and produced weakly nonlinear plasma wakes without bubble formation capable of accelerating pre-heated (~1 MeV) plasma electrons up to the observed energies. The required pre-heating is attributed tentatively to pre-pulse interactions with the plasma.

Electrically discharged active plasma lenses (APLs) are actively pursued in compact high-brightness plasma-based accelerators due to their high-gradient, tunable, and radially symmetric focusing properties. In this manuscript, the APL is experimentally compared with a conventional quadrupole triplet, highlighting the favorable reduction in the energy dependence (chromaticity) in the transport line. Through transport simulations, it is explored how the non-uniform radial discharge current distribution leads to beam-integrated emittance degradation and a charge density reduction at focus. However, positioning an aperture at the APL entrance will significantly reduce emittance degradation without additional loss of charge in the high-quality core of the beam. An analytical model is presented that estimates the emittance degradation from a short beam driving a longitudinally varying wakefield in the APL. Optimizing laser plasma accelerator operation is discussed where emittance degradation from the non-unifor...

Author(s): Barber, SK; Van Tilborg, J; Schroeder, CB; Lehe, R; Tsai, HE; Swanson, KK; Steinke, S; Nakamura, K; Geddes, CGR; Benedetti, C; Esarey, E; Leemans, WP | Abstract: Laser plasma accelerators (LPA) offer an exciting possibility to deliver high energy, high brightness electrons beams in drastically smaller distance scales than is typical for conventional accelerators. As such, LPAs draw considerable attention as potential drivers for next generation light sources and for a compact linear collider. In order to asses the viability of an LPA source for a particular application, the brightness of the source should be properly characterized. In this paper, we present charge dependent transverse emittance measurements of LPA sources using both ionization injection and shock induced density down ramp injection, with the latter delivering smaller transverse emittances by a factor of two when controlling for charge density. The single shot emittance method is described in detail with a discussion on limitations related to second order transport effects. The direct role of space charge is explored through a series of simulations and found to be consistent with experimental observations.

The injection physics in a shock-induced density down-ramp injector was characterized, demonstrating precise control of a laser-plasma accelerator (LPA). Using a jet-blade assembly, experiments systematically varied the shock injector profile, including shock angle, shock position, up-ramp width, and acceleration length. Our work demonstrates that beam energy, energy spread, and pointing can be controlled by adjusting these parameters. As a result, an electron beam that was highly tunable from 25 to 300 MeV with 8% energy spread (ΔEFWHM/E), 1.5 mrad divergence, and 0.35 mrad pointing fluctuation was produced. Particle-in-cell simulation characterized how variation in the shock angle and up-ramp width impacted the injection process. This highly controllable LPA represents a suitable, compact electron beam source for LPA applications such as Thomson sources and free-electron lasers.

We report an experimental-computational study of the optical properties of plasma mirrors (PMs) at the incident laser frequency when irradiated directly at relativistic intensity (1e18 < I_0 < 1e19 W/cm^2) by near-normally incident (4 degree), high-contrast, 30 fs, 800 nm laser pulses. We find that such relativistic PMs are highly reflective (0.6 to 0.8), and focus a significant fraction of reflected light to intensity as large as 10I_0 at distance f as small 25 microns from the PM, provided that pre-pulses do not exceed 1e14 W/cm^2 prior to 20 ps before arrival of the main pulse peak. Particle-in-cell simulations show that focusing results from denting of the reflecting surface by light pressure combined with relativistic transparency, and that reflectivity and f can be adjusted by controlling pre-plasma length L over the range 0.5 < L < 3 microns. Pump-probe reflectivity measurements show the PM's focusing properties evolve on a ps time scale., 11 pages, 10 figures

We measure the evolution history of terawatt-laser driven plasma wakefields in the nonlinear bubble regime using an all-optical frequency-domain streak camera (FDSC) technique. The longitudinal profiles of the plasma “bubble” at different propagation distances within a 3 mm long ionized helium gas target are imaged in single shots, illustrating formation, propagation and coalescence of the bubble. 3D particle-in-cell (PIC) simulations validate the observed density-dependent bubble evolution, and correlate it with generation of a quasi-monoenergetic ∼ 100 MeV electron beam. To visualize petawatt-laser- or e-beam driven plasma wakefields, FDSC is extended to multi-object-plane imaging (MOPI) to measure evolution of wakefield transverse profiles over acceleration distance up to ∼ 1 m in a single shot.

We demonstrate the first tunable Compton backscatter (CBS) x-ray source based on the combination of a laser wakefield accelerator (LWFA) and a plasma mirror (PM). A thin plastic film near the gas jet exit efficiently retro-reflects the LWFA driving pulse with relativistic intensity into oncoming electrons to produce CBS x-rays without detectable bremsstrahlung background. The X-ray central energy is tunable from 75 KeV to 200 KeV by tuning the LWFA e-beam central energy. These CBS x-rays have angular divergence of 10-20 mrad, 50 % (FWHM) energy spread, and 2×107 photons per shot. Photon conversion efficiency from laser to X-rays is 6×10−12, the highest yet demonstrated among LWFA-based monoenergetic Compton sources. Particle-in-cell simulations of the interaction of the LWFA drive pulse with the PM elucidate the scattering process.

By using an axicon lens in conjunction with the ignitor-heater scheme, a 1.2-cm-long high-quality plasma waveguide is generated efficiently, which can extend the range of laser-plasma interaction much beyond the limit of Rayleigh range

We visualize ps-time-scale evolution of an electron density bubble--a wake structure created in atmospheric density plasma by an intense ultrashort laser pulse--from the phase "streak" that the bubble imprints onto a probe pulse that crosses its path obliquely. Phase streaks, recovered in one shot using frequency-domain interferometric techniques, reveal the formation, propagation, and coalescence of the bubble within a 3 mm long ionized helium gas target. 3D particle-in-cell simulations validate the observed density-dependent bubble evolution, and correlate it with the generation of a quasimonoenergetic ∼ 100 MeV electron beam. The results provide a basis for understanding optimized electron acceleration at a plasma density n(e) ≈ 2 × 10(19) cm(-3), inefficient acceleration at lower density, and dephasing limits at higher density.

We visualize formation, propagation and collapse of laser-driven plasma bubbles using a single-shot frequency domain streak camera, thereby identifying bubble dynamics that optimize electron injection and acceleration.

Laser-plasma accelerators of only a centimetre’s length have produced nearly monoenergetic electron bunches with energy as high as 1 GeV. Scaling these compact accelerators to multi-gigaelectronvolt energy would open the prospect of building X-ray free-electron lasers and linear colliders hundreds of times smaller than conventional facilities, but the 1 GeV barrier has so far proven insurmountable. Here, by applying new petawatt laser technology, we produce electron bunches with a spectrum prominently peaked at 2 GeV with only a few per cent energy spread and unprecedented sub-milliradian divergence. Petawatt pulses inject ambient plasma electrons into the laser-driven accelerator at much lower density than was previously possible, thereby overcoming the principal physical barriers to multi-gigaelectronvolt acceleration: dephasing between laser-driven wake and accelerating electrons and laser pulse erosion. Simulations indicate that with improvements in the laser-pulse focus quality, acceleration to nearly 10 GeV should be possible with the available pulse energy., Laser-plasma accelerators can produce high-energy electron bunches over just a few centimetres of distance, offering possible table-top accelerator capabilities. Wang et al. break the current 1 GeV barrier by applying a petawatt laser to accelerate electrons nearly monoenergetically up to 2 GeV.

Electron self-injection into a laser-plasma accelerator (LPA) driven by the Texas Petawatt (TPW) laser is reported at plasma densities 1.7 - 6.2 × 1017 cm−3. Energy and charge of the electron beam, ranging from 0.5 GeV to 2 GeV and tens to hundreds of pC, respectively, depended strongly on laser beam quality and plasma density. Angular beam divergence was consistently around 0.5 mrad (FWHM), while shot-to-shot pointing fluctuations were limited to ±1.4 mrad rms. Betatron x-rays with tens of keV photon energy are also clearly observed.

We globally optimize a terawatt-laser-driven wakefield accelerator by systematically varying laser and target parameters to achieve 100 MeV electrons, 10% energy spread, 100 pC charge, 4 mrad divergence and 10 mrad pointing fluctuation with ∼100% reproducibility, thereby meeting conditions for producing ∼106 200 keV X-ray photons/pulse by inverse Compton scatter.

We report electron acceleration to 1.25 GeV by petawatt-laser-driven wakefield acceleration at plasma density 5×1017 cm3. Electron beams are dark-current-free, quasi-monoenergetic, highly collimated (

We accelerate electrons beyond 2 GeV by driving plasma of density ~4×10^17 cm^-3 with 150 fs, 150 J pulses from the Texas Petawatt Laser. The best beams are dark-current-free with sub-milliradian divergence.

We report observation of electron self-injection and acceleration in a plasma accelerator driven by the Texas petawatt laser at 1017 cm−3 plasma density, an order of magnitude lower density than previous self-injected laser-plasma accelerators.

An optical-field-ionization EUV laser with prepulse-controlled nanoplasma expansion in a cluster gas jet was demonstrated. Pd-like xenon lasing at 41.8-nm with 100 nJ/pulse and 5-mrad divergence was achieved, indicating near-saturation amplification.

An optical-field-ionization soft x-ray laser using a clustered gas jet was demonstrated. Pd-like xenon lasing at 41.8 nm with 95-nJ pulse energy and 5.2-mrad divergence was achieved, indicating near-saturation amplification. By using a prepulse to control the expansion of ionized clusters, it was found that the microscopic uniformity of the plasma is essential for efficient lasing. In addition, the optimal atom density for maximum lasing reported previously is verified to result from the tradeoff between large gain coefficient and short gain length due to ionization-induced refraction.

By using deflectometry of a longitudinal probe pulse and reflective interferometry of a transverse probe pulse to resolve the spatiotemporal distribution of the preformed plasma, we characterize and control the plasma density distribution near the target surface for the development of solid-target x-ray lasers. We show that the use of prepulses in an ignitor-heater scheme can increase the scale length of the preformed plasma and how the effect varies with target materials. Many important issues crucial to x-ray lasing such as electron density distribution, electron temperature, and the optimal timing between pumping pulses can be resolved with these methods.

By utilizing the intensity- and duration-dependent heating and expansion rate of nanoplasma to generate a transient transverse gradient of the refractive index, prepulse controlled laser-beam propagation is demonstrated. The dynamical response of the macroscopic optical refractive index is traced back to the microscopic polarizability of nanoplasmas experimentally, in accordance with hydrodynamic nanoplasma models. In particular, the delay between the prepulse and the main pulse for maximum Rayleigh scattering is found to be longer than that for maximum x-ray emission, supporting the more refined one-dimensional self-consistent hydrodynamic nanoplasma model.

We identify three regimes of correlated GeV-electron/keV-betatron-x-ray generation by a laser-plasma accelerator driven by the Texas Petawatt laser, and relate them to variations in strength of blowout, injection geometry and beam loading.

We generate a collimated (