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The significance of mass spectrometry lies in its unparalleled ability to accurately identify and quantify molecules in complex samples, providing invaluable insights into molecular structures and interactions. Here, we leverage diamond nanostructures as highly sensitive mass sensors by utilizing a self-excitation mechanism under an electron beam in a conventional scanning electron microscope (SEM). The diamond molecular balance (DMB) exhibits an exceptional mass resolution of 0.36 MDa, based on its outstanding mechanical quality factor and frequency stability, along with an extensive dynamic range from MDa to TDa. This positions the DMB at the forefront of molecular balances operating at room temperature. Notably, the DMB demonstrates its ability to measure the mass of a single bacteriophage T4 by precisely locating the analyte on the device. These findings highlight the groundbreaking potential of the DMB as a revolutionary tool for mass spectrometry at room temperature., Comment: 16 pages, 4 figures

Variational quantum eigensolver (VQE), which combines quantum systems with classical computational power, has been arisen as a promising candidate for near-term quantum computing applications. However, the experimental resources such as the number of measurements to implement VQE rapidly increases as the Hamiltonian problem size grows. Applying entanglement measurements to reduce the number of measurement setups has been proposed to address this issue, however, entanglement measurements themselves can introduce additional resource demands. Here, we apply entanglement measurements to the photonic VQE utilizing polarization and path degrees of freedom of a single-photon. In our photonic VQE, entanglement measurements can be deterministically implemented using linear optics, so it takes full advantage of introducing entanglement measurements without additional experimental demands. Moreover, we show that such a setup can mitigate errors in measurement apparatus for a certain Hamiltonian., Comment: Comments are welcome

We demonstrate integrated photonic circuits for quantum devices using sputtered polycrystalline aluminum nitride (AlN) on insulator. The on-chip AlN waveguide directional couplers, which are one of the most important components in quantum photonics, are fabricated and show the output power splitting ratios from 50:50 to 99:1. The polarization beam splitters with an extinction ratio of more than 10 dB are also realized from the AlN directional couplers. Using the fabricated AlN waveguide beam splitters, we observe the Hong-Ou-Mandel interference with a visibility of 91.7 +(-) 5.66 %., Comment: 9 pages, 4 figures

Engineering a strongly interacting uniform qubit cluster would be a major step towards realizing a scalable quantum system for quantum sensing, and a node-based qubit register. For a solid-state system that uses a defect as a qubit, various methods to precisely position defects have been developed, yet the large-scale fabrication of qubits within the strong coupling regime at room temperature continues to be a challenge. In this work, we generate nitrogen vacancy (NV) color centers in diamond with sub-10 nm scale precision by using a combination of nanoscale aperture arrays (NAAs) with a high aspect ratio of 10 and a secondary E-beam hole pattern used as an ion-blocking mask. We perform optical and spin measurements on a small cluster of NV spins and statistically investigate the effect of the NAAs during an ion-implantation process. We discuss how this technique is effective for constructing a scalable system., Comment: 18 pages, 5 figures

We report the experimental resource-efficient implementation of the variational quantum eigensolver (VQE) using four-dimensional photonic quantum states of single-photons. The four-dimensional quantum states are implemented by utilizing polarization and path degrees of freedom of a single-photon. Our photonic VQE is equipped with the quantum error mitigation (QEM) protocol that efficiently reduces the effects of Pauli noise in the quantum processing unit. We apply our photonic VQE to estimate the ground state energy of He--H$^{+}$ cation. The simulation and experimental results demonstrate that our resource-efficient photonic VQE can accurately estimate the bond dissociation curve, even in the presence of large noise in the quantum processing unit., Comment: 16 pages, 8 figures. Comments are welcome

Point defects in crystals provide important building blocks for quantum applications. To initialize, control, and read-out their quantum states, an efficient optical interface for addressing defects with photons is required. However, conventional confocal fluorescence microscopy with high refractive index crystals has limited photon collection efficiency and spatial resolution. Here, we demonstrate high resolution, high contrast imaging for defects qubits using microsphere-assisted confocal microscopy. A microsphere provides an excellent optical interface for point defects with a magnified virtual image that improves spatial resolution up to ~${\lambda}$/5 as well as an optical signal-to-noise ratio by four times. These features enable individual optical addressing of single photons and single spins of spatially-unresolved defects in conventional confocal microscopy with improved signal contrast. The combined optical tweezers show the possibility of positioning or scanning the microspheres for deterministic coupling and wide-field imaging of defects. The approach does not require any complicated fabrication and additional optical system but uses simple micro-optics off-the-shelf. From these distinctive advantages of the microspheres, our approach can provide an efficient way for imaging and addressing closely-spaced defects with higher resolution and sensitivity., Comment: 20 pages, 5 figures

Multiparty quantum communication provides delightful applications including quantum cryptographic communication and quantum secret sharing. Measurement-Device-Independent (MDI) quantum communication based on the Greenberg-Horne-Zeilinger (GHZ) state measurement provides a practical way to implement multiparty quantum communication. With the standard spatially localized GHZ state measurement, however, information can be imbalanced among the communication parties that can cause significant problems in multiparty cryptographic communication. Here, we propose an equitable multiparty quantum communication where information balance among the communication parties is achieved without a trusted third party. Our scheme is based on the GHZ state measurement which is not spatially localized but implemented in a way that all the distant communication parties symmetrically participate. We also verify the feasibility of our scheme by presenting the proof-of-principle experimental demonstration of informationally balanced three-party quantum communication using weak coherent pulses., Comment: Ask the authors for the supplemental materials

A quantum state transformation can be generally approximated by single- and two-qubit gates. This, however, does not hold with noisy intermediate-scale quantum technologies due to the errors appearing in the gate operations, where errors of two-qubit gates such as controlled-NOT and SWAP operations are dominated. In this work, we present a cost efficient single-copy certification for a realization of a two-qubit gate in the presence of depolarization noise, where it is aimed to identify if the realization is noise-free, or not. It is shown that entangled resources such as entangled states and a joint measurement are not necessary for the purpose, i.e., a noise-free two-qubit gate is not needed to certify an implementation of a two-qubit gate. A proof-of-principle demonstration is presented with photonic qubits., Comment: 9 pages. arXiv admin note: text overlap with arXiv:1812.02087

One of the common conceptions of nature, typically derived from the experiences with classical systems, is that attributes of the matter coexist with the substance. In the quantum regime, however, the quantum particle itself and its physical property may be in spatial separation, known as the quantum Cheshire cat effect. While there have been several reports to date on the observation of the quantum Cheshire cat effect, all such experiments are based on first-order interferometry and destructive projection measurement, thus allowing simple interpretation due to measurement-induced disturbance and also subject to trivial interpretation based on classical waves. In this work, we report a genuine experimental observation of the quantum Cheshire cat effect with noninvasive weak quantum measurement as originally proposed. The use of the weak-measurement probe has allowed us to identify the location of the single-photon and that of the disembodied polarization state in a quantum interferometer. We furthermore elucidate the paradox of the quantum Cheshire cat effect as quantum interference of the transition amplitudes for the photon and the polarization state which are directly obtained from the measurement outcomes or the weak values.

Reference-Frame-Independent Quantum Key Distribution (RFI-QKD) provides a practical way to generate secret keys between two remote parties without sharing common reference frames. On the other hand, Measurement-Device-Independent QKD (MDI-QKD) offers high level of security as it immunes against all the quantum hacking attempts to the measurement devices. The combination of these two QKD protocols, i.e., RFI-MDI-QKD, is one of the most fascinating QKD protocols since it holds both advantages of practicality and security. For further practicality of RFI-MDI-QKD, it is beneficial to reduce the implementation complexity. Here, we have shown that RFI-MDI-QKD can be implemented using fewer quantum states than those of its original proposal. We found that, in principle, the number of quantum states for one of the parties can be reduced from six to three without compromising security. Comparing to the conventional RFI-MDI-QKD where both parties should transmit six quantum states, it significantly simplifies the implementation of the QKD protocol. We also verify the feasibility of the scheme with the proof-of-principle experiment., Comment: A few revision has been made during the publication process

Quantum key distribution (QKD) networks constitute promising solutions for secure communication. Beyond conventional point-to-point QKD, we developed 1xN QKD network systems with a sub-ns resolution optical path length compensation scheme. With a practical plug-and-play QKD architecture and compact timing control modules based on a field programmable gate array (FPGA), we achieved long term stable operation of a 1x64 QKD network system. Using this architecture, 64 users can simultaneously share secret keys with one server, without using complex software algorithms and expensive hardware. We demonstrated the working of a 1x4 QKD network system using the fiber network of a metropolitan area., Comment: To be published in Photonics Research

Entanglement among multiple particles is a keystone for not only fundamental research on quantum information but also various practical quantum information applications. In particular, W state has attracted a lot of attention due to the robustness against particle loss and the applications in multiparty quantum communication. However, it is challenging to generate photonic W state with large number of photons since N-photon W state requires superposition among N probability amplitudes. In this paper, we propose an efficient linear optical scheme to generate N-photon W state via quantum erasure. The success probability of our protocol polynomially decreases as the number of photons increase. We also discuss the experimental feasibility of our protocol, and anticipate that one can efficiently generate tens of photonic W state with our scheme using currently available quantum photonics technologies., Comment: Comments are welcome. A few references are added

Different nonlocal quantum correlations of entanglement, steering and Bell nonlocality are defined with the help of local hidden state (LHS) and local hidden variable (LHV) models. Considering their unique roles in quantum information processing, it is of importance to understand the individual nonlocal quantum correlation as well as their relationship. Here, we investigate the effects of amplitude damping decoherence on different nonlocal quantum correlations. In particular, we have theoretically and experimentally shown that the entanglement sudden death phenomenon is distinct from those of steering and Bell nonlocality. In our scenario, we found that all the initial states present sudden death of steering and Bell nonlocality, while only some of the states show entanglement sudden death. These results suggest that the environmental effect can be different for different nonlocal quantum correlations, and thus, it provides distinct operational interpretations of different quantum correlations., Comment: 9 pages, 4 figures including appendix

In free-space quantum key distribution (QKD) between moving parties, e.g., free-space QKD via satellite, the reference frame rotation and fluctuation degrades the performance of QKD. Reference-frame-independent QKD (RFI-QKD) provides a simple but efficient way to overcome this problem. While there has been a number of theoretical and experimental studies on RFI-QKD, the experimental verification of the robustness of RFI-QKD over other QKD protocols under the reference frame rotation and fluctuation is still missing. Here, we have constructed a free-space QKD system which can implement BB84, six-state, and RFI-QKD protocols, and compared their performances under the reference frame rotation and fluctuation. With the theoretical analysis and experimental data, we have successfully verified the robustness of RFI-QKD protocol over other QKD protocols in the presence of reference frame rotation and fluctuation., Comment: 6 pages, 4 figures

Bell state measurement (BSM) plays crucial roles in photonic quantum information processing. The standard linear optical BSM is based on Hong-Ou-Mandel interference where two photons meet and interfere at a beamsplitter (BS). However, a generalized two-photon interference is not based on photon-photon interaction, but interference between two-photon probability amplitudes. Therefore, it might be possible to implement BSM without interfering photons at a BS. Here, we investigate a linear optical BSM scheme which does not require two photon overlapping at a BS. By unleashing the two photon coexistence condition, it can be symmetrically divided into two parties. The symmetrically dividable property suggests informationally symmetrical BSM between remote parties without a third party. We also present that our BSM scheme can be used for Bell state preparation between remote parties without a third party. Since our BSM scheme can be easily extended to multiple photons, it can be useful for various quantum communication applications.

Nonlocal quantum correlation is at the heart of bizarre nature of quantum physics. While there are various classes of nonlocal quantum correlation, steerability of a quantum state by local measurements provides unique operational features. Here, we theoretically and experimentally investigate the hidden quantum steerability. In particular, we find that there are initially unsteerable states which can reveal the steerability by using local filters on individual quantum systems. It is remarkable that a certain set of local filters are more effective on revealing steerability than Bell nonlocality whereas there exists another set of filters that is more effective on revealing Bell nonlocality than steerability. Finally, we present a counter-intuitive result that mixed states originating from non-maximally pure entangled states can have hidden steerability while the mixed state from a maximally pure entangled state fails to show steerability., Comment: The manuscript has been updated to the published version

Photon anti-bunching, measured via the Hanbury-Brown-Twiss experiment, is one of the key signatures of quantum light and is tied to sub-Poissonian photon number statistics. Recently, it has been reported that photon anti-bunching or conditional sub-Poissonian photon number statistics can be obtained via second-order interference of mutually incoherent weak lasers and heralding based on photon counting. Here, we report theoretical analysis on the limits of manipulating conditional photon statistics via interference of weak lasers. It is shown that conditional photon number statistics can become super-Poissonian in such a scheme. We, however, demonstrate explicitly that it cannot become sub-Poissonian, i.e., photon anti-bunching cannot be obtained in such a scheme. We point out that incorrect results can be obtained if one does not properly account for seemingly negligible higher-order photon number expansions of the coherent state., Comment: 9 pages, 4 figures

Reference-Frame-Independent quantum key distribution (RFI-QKD) is known to be robust against slowly varying reference frames. However, other QKD protocols such as BB84 can also provide secrete keys if the speed of the relative motion of the reference frames is slow enough. While there has been a few studies to quantify the speed of the relative motion of the reference frames in RFI- QKD, it is not yet clear if RFI-QKD provides better performance than other QKD protocols under this condition. Here, we analyze and compare the security of RFI-QKD and BB84 protocol in the presence of the relative motion of the reference frames. In order to compare their security in real world implementation, we also consider the QKD protocols with decoy state method. Our analysis shows that RFI-QKD provides more robustness than BB84 protocol against the relative motion of the reference frames., Comment: 6 pages, 3 figures, comments and suggestions are welcome

We report investigation on quantum discord in classical second-order interference. In particular, we theoretically show that a bipartite state with D = 0.311 of discord can be generated via classical second-order interference. We also experimentally verify the theory by obtaining D = 0.197 +- 0.060 of non-zero discord state. Together with the fact that non-classicalities originated from physical constraints and information theoretic perspectives are not equivalent, this result provides an insight to understand the nature of quantum discord., Comment: 8 pages, 5 figures

We developed a countermeasure against blinding attacks on low-noise detectors with a background noise cancellation scheme in quantum key distribution (QKD) systems. Background noise cancellation includes self-differencing and balanced avalanche photon diode (APD) schemes and is considered a promising solution for low-noise APDs, which are critical components in high-performance QKD systems. However, its vulnerability to blinding attacks has been recently reported. In this work, we propose a new countermeasure that prevents this potential security loophole from being used in detector blinding attacks. An experimental QKD setup is implemented and various tests are conducted to verify the feasibility and performance of the proposed method. The obtained measurement results show that the proposed scheme successfully detects occurring blinding-attack-based hacking attempts., Comment: 10 pages, 11 figures, 1 table

Entanglement is known to be an essential resource for many quantum information processes. However, it is now known that some quantum features may be acheived with quantum discord, a generalized measure of quantum correlation. In this paper, we study how quantum discord, or more specifically, the measures of entropic discord and geometric discord are affected by the influence of amplitude damping decoherence. We also show that a protocol deploying weak measurement and quantum measurement reversal can effectively protect quantum discord from amplitude damping decoherence, enabling to distribute quantum correlation between two remote parties in a noisy environment., Comment: 7 pages, 3 figures

Quantum key distribution (QKD) gaurantees unconditional communication security based on the laws of quantum physics. However, practical QKD suffers from a number of quantum hackings due to the device imperfections. From the security standpoint, measurement-device-independent quantum key distribution (MDI-QKD) is in the limelight since it eliminates all the possible loopholes in detection. Due to active control units for mode matching between the photons from remote parties, however, the implementation of MDI-QKD is highly impractical. In this article, we propose a novel method in which the indistinguishability issue is resolved without any active control unit. By introducing Plug-and-Play (P&P) concept into MDI-QKD, the indistinguishability between photons can naturally be guaranteed. We show the feasibility of P&P MDI-QKD with a proof-of-principle experiment., Comment: 7 pages, 5 figures