Search

Fusing small resource states into a larger, fully connected graph-state is essential for scalable photonic quantum computing. Theoretical analysis reveals that this can only be achieved when the success probability of the fusion gate surpasses a specific percolation threshold of 58.98% by using three-photon GHZ states as resource states. However, such an implementation of a fusion gate has never been experimentally realized before. Here, we successfully demonstrate a boosted fusion gate with a theoretical success probability of 75%, using deterministically generated auxiliary states. The success probability is experimentally measured to be 71.0(7)%. We further demonstrate the effectiveness of the boosted fusion gate by fusing two Bell states with a fidelity of 67(2)%. Our work paves a crucial path toward scalable linear optical quantum computing., Comment: 5 pages, 4 figures

Single-photon sources are essential for quantum networks, enabling applications ranging from quantum key distribution (QKD) to the burgeoning quantum internet. Despite the remarkable advancements, the current reliance of QKD on attenuated coherent (laser) light sources has imposed a fundamental limit on the secret key rate (SKR). This constraint is primarily attributable to the scarcity of single-photon components within coherent light, confined by an inherent upper bound of 1/e. Here, we report high-rate QKD using a high-efficiency single-photon source, enabling an SKR transcending the fundamental rate limit of coherent light. We developed an on-demand, bright semiconductor quantum-dot single-photon source with an efficiency of 0.71(2), exceeding the inherent bound of coherent light by approximately 2.87 dB. Implementing narrow-bandwidth filtering and random polarization modulation, we conducted a field QKD trial over a 14.6(1.1)-dB-loss free-space urban channel, achieving an SKR of 0.00108 bits per pulse. This surpasses the practical limit of coherent-light-based QKD by 2.53 dB. Our findings conclusively demonstrate the superior performance of nanotechnology-based single-photon sources over coherent light for QKD applications, marking a pivotal stride towards the realization of a global quantum internet., Comment: 22 pages, 5 figures, 1 Table

Bright, polarized, and high-purity single-photon sources in telecom wavelengths are crucial components in long-distance quantum communication, optical quantum computation and quantum networks. Semiconductor InAs/InP quantum dots (QDs) combined with photonic cavities provide a competitive path leading to optimal single-photon sources in this range. Here, we demonstrate a bright and polarized single-photon source operating in the telecom C-band based on an elliptical Bragg grating (EBG) cavity. With a significant Purcell enhancement of 5.25$\pm$0.05, the device achieves a polarization ratio of 0.986, single-photon purity of g^2 (0)=0.078$\pm$0.016 and single-polarized photon collection efficiency of ~ 24% at the first lens (NA=0.65) without blinking. These findings suggest that C-band QD-based single-photon sources are potential candidates for advancing quantum communication.

Photon loss is the biggest enemy for scalable photonic quantum information processing. This problem can be tackled by using quantum error correction, provided that the overall photon loss is below a threshold of 1/3. However, all reported on-demand and indistinguishable single-photon sources still fall short of this threshold. Here, by using tailor shaped laser pulse excitation on a high-quantum efficiency single quantum dot deterministically coupled to a tunable open microcavity, we demonstrate a high-performance source with a single-photon purity of 0.9795(6), photon indistinguishability of 0.986(16), and an overall system efficiency of 0.717(20), simultaneously. This source for the first time reaches the efficiency threshold for scalable photonic quantum computing. With this source, we further demonstrate 1.87(13) dB intensity squeezing, and consecutive 40-photon events with 1.67 mHz count rate.

In the quest to build general-purpose photonic quantum computers, fusion-based quantum computation has risen to prominence as a promising strategy. This model allows a ballistic construction of large cluster states which are universal for quantum computation, in a scalable and loss-tolerant way without feed-forward, by fusing many small n-photon entangled resource states. However, a key obstacle to this architecture lies in efficiently generating the required essential resource states on photonic chips. One such critical seed state that has not yet been achieved is the heralded three-photon Greenberger-Horne-Zeilinger (3-GHZ) state. Here, we address this elementary resource gap, by reporting the first experimental realization of a heralded dual-rail encoded 3-GHZ state. Our implementation employs a low-loss and fully programmable photonic chip that manipulates six indistinguishable single photons of wavelengths in the telecommunication regime. Conditional on the heralding detection, we obtain the desired 3-GHZ state with a fidelity 0.573+-0.024. Our work marks an important step for the future fault-tolerant photonic quantum computing, leading to the acceleration of building a large-scale optical quantum computer., Comment: Submitted. Comments are welcome!

Quantum computing experiments are moving into a new realm of increasing size and complexity, with the short-term goal of demonstrating an advantage over classical computers. Boson sampling is a promising platform for such a goal, however, the number of involved single photons was up to five so far, limiting these small-scale implementations to a proof-of-principle stage. Here, we develop solid-state sources of highly efficient, pure and indistinguishable single photons, and 3D integration of ultra-low-loss optical circuits. We perform an experiment with 20 single photons fed into a 60-mode interferometer, and, in its output, sample over Hilbert spaces with a size of $10^{14}$ $-$over ten orders of magnitude larger than all previous experiments. The results are validated against distinguishable samplers and uniform samplers with a confidence level of 99.9%., Comment: 23 pages, 14 figures

Scalable quantum photonic architectures demand highly efficient, high-purity single-photon sources, which can be frequency matched via external tuning. We demonstrate a single-photon source based on an InAs quantum dot embedded in a micropillar resonator, which is frequency tunable via externally-applied stress. Our platform combines the advantages of a Bragg micropillar cavity and the piezo-strain-tuning technique enabling single photon spontaneous emission enhancement via the Purcell effect and quantum dot (QD) with tunable wavelength. Our optomechanical platform has been implemented by integration of semiconductor-based QD-micropillars on a piezoelectric substrate. The fabricated device exhibits spontaneous emission enhancement with a Purcell factor of 4.4$\pm$0.7 and allows for a pure triggered single-photon generation with $g^{(2)}(0)$ < 0.07 under resonant excitation. A quantum dot emission energy tuning range of 0.75 meV for 27 kV/cm applied to the piezo substrate has been achieved. Our results pave the way towards the scalable implementation of single-photon quantum photonic technologies using optoelectronic devices., Comment: 16 pages, 4 figures

An optimal single-photon source should deterministically deliver one and only one photon at a time, with no trade-off between the source's efficiency and the photon indistinguishability. However, all reported solid-state sources of indistinguishable single photons had to rely on polarization filtering which reduced the efficiency by 50%, which fundamentally limited the scaling of photonic quantum technologies. Here, we overcome this final long-standing challenge by coherently driving quantum dots deterministically coupled to polarization-selective Purcell microcavities--two examples are narrowband, elliptical micropillars and broadband, elliptical Bragg gratings. A polarization-orthogonal excitation-collection scheme is designed to minimize the polarization-filtering loss under resonant excitation. We demonstrate a polarized single-photon efficiency of 0.60+/-0.02 (0.56+/-0.02), a single-photon purity of 0.975+/-0.005 (0.991+/-0.003), and an indistinguishability of 0.975+/-0.006 (0.951+/-0.005) for the micropillar (Bragg grating) device. Our work provides promising solutions for truly optimal single-photon sources combining near-unity indistinguishability and near-unity system efficiency simultaneously., Comment: 28 pages, 16 figures. partial overlap with arXiv:1809.10992 which was unpublished

We report an experiment to test quantum interference, entanglement and nonlocality using two dissimilar photon sources, the Sun and a semiconductor quantum dot on the Earth, which are separated by 150 million kilometers. By making the otherwise vastly distinct photons indistinguishable all degrees of freedom, we observe time-resolved two-photon quantum interference with a raw visibility of 0.796(17), well above the 0.5 classical limit, providing the first evidence of quantum nature of thermal light. Further, using the photons with no common history, we demonstrate post-selected two-photon entanglement with a state fidelity of 0.826(24), and a violation of Bell's inequality by 2.20(6). The experiment can be further extended to a larger scale using photons from distant stars, and open a new route to quantum optics experiments at an astronomical scale., Comment: accepted version

Efficient excitation of a single two-level system usually requires that the driving field is at the same frequency as the atomic transition. However, the scattered laser light in solid-state implementations can dominate over the single photons, imposing an outstanding challenge to perfect single-photon sources. Here, we propose a background-free method using a phase-locked dichromatic electromagnetic field with no spectral overlap with the optical transition for a coherent control of a two-level system, and we demonstrate this method experimentally with a single quantum dot embedded in a micropillar. Single photons generated by pi excitation show a purity of 0.988(1) and indistinguishability of 0.962(6). Further, the phase-coherent nature of the two-color excitation is captured by the resonance-fluorescence intensity dependence on the relative phase between the two pulses. Our two-color excitation method adds a useful toolbox to the study of atom-photon interaction, and the generation of spectrally isolated indistinguishable single photons., Comment: 17 pages, 5 figures, accepted for publication (2019)

Entangled photon sources with simultaneously near-unity heralding efficiency and indistinguishability are the fundamental elements for scalable photonic quantum technologies. We design and realize a degenerate entangled-photon source from an ultrafast pulsed laser pumped spontaneous parametric down-conversion (SPDC), which show simultaneously ~97% heralding efficiency and ~96% indistinguishability between independent single photons. Such a high-efficiency and frequency-uncorrelated SPDC source allows generation of the first 12-photon genuine entanglement with a state fidelity of 0.572(24). We further demonstrate a blueprint of scalable scattershot boson sampling using 12 SPDC sources and a 12*12-modes interferometer for three-, four-, and five-boson sampling, which yields count rates more than four orders of magnitudes higher than all previous SPDC experiments. Our work immediately enables high-efficiency implementations of multiplexing, scattershot boson sampling, and heralded creation of remotely entangled photons, opening up a promising pathway to scalable photonic quantum technologies., Comment: 17 pages, 5 figures. the make-SPDC-great-again paper

The key challenge to scalable optical quantum computing, boson sampling, and quantum metrology is sources of single photons with near-unity system efficiency and simultaneously near-perfect indistinguishability in all degrees of freedom (including spectral, temporal, spatial, and polarization). However, previous high-indistinguishability solid-state single-photon sources had to rely on polarization filtering that reduced the system efficiency by at least 50%. Here, we overcome this challenge by developing a new single-photon source based on a coherently driven quantum dot embedded in an elliptical micropillar. The asymmetric cavity lifts the polarization degeneracy into two orthogonal linearly polarized modes with a suitable energy separation. We design an excitation-collection scheme that allows the creation and collection of single photons with an indistinguishability of 0.976(1) and a degree of polarization of 91%. Our method provides a solution of combining near-unity system efficiency and indistinguishability compatible with background-free resonant excitation, and opens the way to truly optimal single-photon sources for scalable photonic quantum technologies., Comment: submitted for publication on 8 August 2018

Single photon sources, which are compatible with quantum memories are an important component of quantum networks. In this article, we show optical investigations on isolated GaAs/Al$_{0.25}$Ga$_{0.75}$As quantum dots grown via droplet epitaxy, which emit single photons on resonance with the Rb-87-D$_2$ line (780 nm). Under continuous wave resonant excitation conditions, we observe bright, clean and narrowband resonance fluorescence emission from such a droplet quantum dot. Furthermore, the second-order correlation measurement clearly demonstrates the single photon emission from this resonantly driven transition. Spectrally resolved resonance fluorescence of a similar quantum dot yields a linewidth as narrow as 660 MHz ($ 2.7~\mu eV $), which corresponds to a coherence time of 0.482 ns. The observed linewidth is the smallest reported so far for strain free GaAs quantum dots grown via the droplet method. We believe that this single photon source can be a prime candidate for applications in optical quantum networks., Comment: 11 pages

Boson sampling is a well-defined task that is strongly believed to be intractable for classical computers, but can be efficiently solved by a specific quantum simulator. However, an outstanding problem for large-scale experimental boson sampling is the scalability. Here we report an experiment on boson sampling with photon loss, and demonstrate that boson sampling with a few photons lost can increase the sampling rate. Our experiment uses a quantum-dot-micropillar single-photon source demultiplexed into up to seven input ports of a 16*16 mode ultra-low-loss photonic circuit, and we detect three-, four- and five-fold coincidence counts. We implement and validate lossy boson sampling with one and two photons lost, and obtain sampling rates of 187 kHz, 13.6 kHz, and 0.78 kHz for five-, six- and seven-photon boson sampling with two photons lost, which is 9.4, 13.9, and 18.0 times faster than the standard boson sampling, respectively. Our experiment shows an approach to significantly enhance the sampling rate of multiphoton boson sampling., Comment: 10 pages, 12 figures, submitted

We report a joint experimental and theoretical study of the interference properties of a single photon source based on a In(Ga)As quantum dot embedded in a quasi-planar GaAs-microcavity. Using resonant laser excitation with a pulse separation of 2 ns, we find near-perfect interference of the emitted photons, and a corresponding indistinguishability of $\mathcal{I} = (99.6\,^{+\,0.4}_{-\,1.4})\%$. For larger pulse separations, quasi-resonant excitation conditions, increasing pump power or with increasing temperature, the interference contrast is progressively and notably reduced. We present a systematic study of the relevant dephasing mechanisms, and explain our results in the framework of a microscopic model of our system. For strictly resonant excitation, we show that photon indistinguishability is independent of pump power, but strongly influenced by virtual phonon assisted processes which are not evident in excitonic Rabi oscillations., Comment: 12 pages, 6 figures

Quantum state transfer from flying photons to stationary matter qubits is an important element in the realization of quantum networks. Self-assembled semiconductor quantum dots provide a promising solid-state platform hosting both single photon and spin, with an inherent light-matter interface. Here, we develop a method to coherently and actively control the single-photon frequency bins in superposition using electro-optic modulators, and measure the spin-photon entanglement with a fidelity of $0.796\pm0.020$. Further, by Greenberger-Horne-Zeilinger-type state projection on the frequency, path and polarization degrees of freedom of a single photon, we demonstrate quantum state transfer from a single photon to a single electron spin confined in an InGaAs quantum dot, separated by 5 meters. The quantum state mapping from the photon's polarization to the electron's spin is demonstrated along three different axis on the Bloch sphere, with an average fidelity of $78.5\%$., Comment: Experiment finished in 2013, presented in QD2014 Pisa, under review in Phys. Rev. Lett

Monolayers of transition metal dichalcogenide materials emerged as a new material class to study excitonic effects in solid state, since they benefit from enormous coulomb correlations between electrons and holes. Especially in WSe2, sharp emission features have been observed at cryogenic temperatures, which act as single photon sources . Tight exciton localization has been assumed to induce an anharmonic excitation spectrum, however, the evidence of the hypothesis, namely the demonstration of a localized biexciton, is elusive. Here, we unambiguously demonstrate the existence of a localized biexciton in a monolayer of WSe2, which triggers an emission cascade of single photons. The biexciton is identified by its time-resolved photoluminescence, superlinearity and distinct polarization in micro-photoluminescence experiments. We evidence the cascaded nature of the emission process in a cross-correlation experiment, which yields a strong bunching behavior. Our work paves the way to a new generation of quantum optics experiments with two-dimensional semiconductors., Comment: 13 pages, 3 Figures

Atomic monolayers represent a novel class of materials to study localized and free excitons in two dimensions and to engineer optoelectronic devices based on their significant optical response. Here, we investigate the role of the substrate on the photoluminescense response of MoSe$_2$ and WSe$_2$ monolayers exfoliated either on SiO$_2$ or epitaxially grown InGaP substrates. In the case of MoSe$_2$, we observe a significant qualitative modification of the emission spectrum, which is widely dominated by the trion resonance on InGaP substrates. However, the effects of inhomogeneous broadening of the emission features are strongly reduced. Even more strikingly, in sheets of WSe$_2$, we could routinely observe emission lines from localized excitons with linewidths down to the resolution limit of 70\,$\mu$ eV. This is in stark contrast to reference samples featuring WSe$_2$ monolayers on SiO$_2$ surfaces, where the emission spectra from localized defects are widely dominated by spectral diffusion and blinking behaviour. Our experiment outlines the enormous potential of III-V-monolayer hybrid architectures to obtain high quality emission signals from atomic monolayers, which are straight forward to integrate into nanophotonic and integrated optoelectronic devices.

Deterministic techniques enabling the implementation and engineering of bright and coherent solid-state quantum light sources are key for the reliable realization of a next generation of quantum devices. Such a technology, at best, should allow one to significantly scale up the number of implemented devices within a given processing time. In this work, we discuss a possible technology platform for such a scaling procedure, relying on the application of nanoscale quantum dot imaging to the pillar microcavity architecture, which promises to combine very high photon extraction efficiency and indistinguishability. We discuss the alignment technology in detail, and present the optical characterization of a selected device which features a strongly Purcell-enhanced emission output. This device, which yields an extraction efficiency of $\eta=(49\pm4)~\%$, facilitates the emission of photons with $(94\pm2.7)~\%$ indistinguishability., Comment: 8 pages, 5 figures. arXiv admin note: text overlap with arXiv:1512.07453

Boson sampling is considered as a strong candidate to demonstrate the quantum computational supremacy over classical computers. However, previous proof-of-principle experiments suffered from small photon number and low sampling rates owing to the inefficiencies of the single-photon sources and multi-port optical interferometers. Here, we develop two central components for high-performance boson sampling: robust multi-photon interferometers with 0.99 transmission rate, and actively demultiplexed single-photon sources from a quantum-dot-micropillar with simultaneously high efficiency, purity and indistinguishability. We implement and validate 3-, 4-, and 5-photon boson sampling, and achieve sampling rates of 4.96 kHz, 151 Hz, and 4 Hz, respectively, which are over 24,000 times faster than the previous experiments, and over 220 times faster than obtaining one sample through calculating the matrices permanent using the first electronic computer (ENIAC) and transistorized computer (TRADIC) in the human history. Our architecture is feasible to be scaled up to larger number of photons and with higher rate to race against classical computers, and might provide experimental evidence against the Extended Church-Turing Thesis., Comment: Revised for clarity. More information added. This work kick-starts a race against classical computers using photonic machines. A different version will appear in Nature Photonics

Boson sampling is a problem intractable for classical computers, but can be naturally solved on a specialized photonic quantum simulator which requires less resources than building a universal quantum computer. The biggest challenge to implement boson sampling with a large number of photons has been the lack of reliable single-photon sources. Here we demonstrate a scalable architecture of boson sampling using a solid-state single-photon source with simultaneously high efficiency, purity, and indistinguishability. The single photons are time-bin encoded and interfered in an electrically programmable loop-based network. We implement and validate boson sampling with input three and four single photons, and track the dynamical multi-photon evolution inside the circuit. With further refinement of the system efficiency, our approach may be feasible to be scaled up to >20-boson sampling to outperform classical computers, and thus provide experimental evidence against the Extended Church-Turing Thesis., Comment: 12 pages, 4 figures, additional references added

The implementation and engineering of bright and coherent solid state quantum light sources is key for the realization of both on chip and remote quantum networks. Despite tremendous efforts for more than 15 years, the combination of these two key prerequisites in a single, potentially scalable device is a major challenge. Here, we report on the observation of bright and coherent single photon emission generated via pulsed, resonance fluorescence conditions from a single quantum dot (QD) deterministically centered in a micropillar cavity device via cryogenic optical lithography. The brightness of the QD fluorescence is greatly enhanced on resonance with the fundamental mode of the pillar, leading to an overall device efficiency of $\eta=(74\pm4)~\%$ for a single photon emission as pure as $g^{(2)}(0)=0.0092\pm0.0004$. The combination of large Purcell enhancement and resonant pumping conditions allows us to observe a two-photon wave packet overlap up to $\nu=(88\pm3)~\%$, Comment: submitted

Resonant excitation of solid state quantum emitters has the potential to deterministically excite a localized exciton while ensuring a maximally coherent emission. In this work, we demonstrate the coherent coupling of an exciton localized in a lithographically positioned, site-controlled semiconductor quantum dot to an external resonant laser field. For strong continuous-wave driving we observe the characteristic Mollow triplet and analyze the Rabi splitting and sideband widths as a function of driving strength and temperature. The sideband widths increase linearly with temperature and the square of the driving strength, which we explain via coupling of the exciton to longitudinal acoustic phonons. We also find an increase of the Rabi splitting with temperature, which indicates a temperature induced delocalization of the excitonic wave function resulting in an increase of the oscillator strength. Finally, we demonstrate coherent control of the exciton excited state population via pulsed resonant excitation and observe a damping of the Rabi oscillations with increasing pulse area, which is consistent with our exciton-photon coupling model. We believe that our work outlines the possibility to implement fully scalable platforms of solid state quantum emitters. The latter is one of the key prerequisites for more advanced, integrated nanophotonic quantum circuits., Comment: accepted for publication in Optica

We report on the observation of bright emission of single photons under pulsed resonance fluorescence conditions from a single quantum dot (QD) in a micropillar cavity. The brightness of the QD fluorescence is greatly enhanced via the coupling to the fundamental mode of a micropillar, allowing us to determine a single photon extraction efficiency of $(20.7\pm0.8)~\%$ per linear polarization basis. This yields an overall extraction efficiency of $(41.4\pm1.5)~\%$ in our device. We observe the first Rabi-oscillation in a weakly coupled quantum dot-micropillar system under coherent pulsed optical excitation, which enables us to deterministically populate the excited QD state. In this configuration, we probe the single photon statistics of the device yielding $g^{(2)}(0)=0.072\pm0.011$ at a QD-cavity detuning of $75~\mu$eV., Comment: accepted for publication in Optics Express

Single quantum emitters (SQEs) are at the heart of quantum optics and photonic quantum information technologies. To date, all demonstrated solid-state single-photon sources are confined in three-dimensional materials. Here, we report a new class of SQEs based on excitons that are spatially localized by defects in two-dimensional tungsten-diselenide monolayers. The optical emission from these SQEs shows narrow linewidths of ~0.13 meV, about two orders of magnitude smaller than that of delocalized valley excitons. Second-order correlation measurements reveal strong photon anti-bunching, unambiguously establishing the single photon nature of the emission. The SQE emission shows two non-degenerate transitions, which are cross-linearly polarized. We assign this fine structure to two excitonic eigen-modes whose degeneracy is lifted by a large ~0.71 meV coupling, likely due to the electron-hole exchange interaction in presence of anisotropy. Magneto-optical measurements also reveal an exciton g-factor of ~8.7, several times larger than that of delocalized valley excitons. In addition to their fundamental importance, establishing new SQEs in 2D quantum materials could give rise to practical advantages in quantum information processing, such as efficient photon extraction and high integratability and scalability., Comment: 19 pages, 10 figures, including supplementary information

We demonstrate deterministic and robust generation of pulsed resonance fluorescence single photons from a single InGaAs quantum dot using the method of rapid adiabatic passage. Comparative study is performed with transform-limited, negatively chirped and positively chirped pulses, identifying the last one to be the most robust against fluctuation of driving strength. The generated single photons are background free, have a vanishing two-photon emission probability of 0.3% and a raw (corrected) two-photon Hong-Ou-Mandel interference visibility of 97.9% (99.5%), reaching a precision that places single photons at the threshold for fault-tolerant surface-code quantum computing. The single-photon source can be readily scaled up to multi-photon entanglement and used for quantum metrology, boson sampling and linear optical quantum computing., Comment: 5 pages, 4 figures, submitted

We investigate temperature-dependent resonance fluorescence spectra obtained from a single self-assembled quantum dot. A decrease of the Mollow triplet sideband splitting is observed with increasing temperature, an effect we attribute to a phonon-induced renormalisation of the driven dot Rabi frequency. We also present first evidence for a non-perturbative regime of phonon coupling, in which the expected linear increase in sideband linewidth as a function of temperature is cancelled by the corresponding reduction in Rabi frequency. These results indicate that dephasing in semiconductor quantum dots may be less sensitive to changes in temperature than expected from a standard weak-coupling analysis of phonon effects., Comment: Close to published version, new figure and minor changes to the text. 5 pages, 3 figures

Single photon sources based on semiconductor quantum dots offer distinct advantages for quantum information, including a scalable solid-state platform, ultrabrightness, and interconnectivity with matter qubits. A key prerequisite for their use in optical quantum computing and solid-state networks is a high level of efficiency and indistinguishability. Pulsed resonance fluorescence (RF) has been anticipated as the optimum condition for the deterministic generation of high-quality photons with vanishing effects of dephasing. Here, we generate pulsed RF single photons on demand from a single, microcavity-embedded quantum dot under s-shell excitation with 3-ps laser pulses. The pi-pulse excited RF photons have less than 0.3% background contributions and a vanishing two-photon emission probability. Non-postselective Hong-Ou-Mandel interference between two successively emitted photons is observed with a visibility of 0.97(2), comparable to trapped atoms and ions. Two single photons are further used to implement a high-fidelity quantum controlled-NOT gate., Comment: 11 pages, 11 figures