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We present an atom interferometer using large momentum transfer without $k$-reversal. More specifically, we use a microwave $\pi$/2 pulse to manipulate the spin state of $^{87}$Rb atoms before applying a Raman light $\pi$ pulse to achieve 4$\hbar k$ momentum transfer per Raman light pulse. A microwave $\pi$ pulse in the middle of the interferometer sequence reverses the spin states, which allows closing of the interferometer arms by the same Raman light $\pi$ pulses without $k$-reversal. We discuss the scalability of this large momentum transfer technique. Our results extend the scope of using large momentum transfer atom optics into atom interferometers where $k$-reversal optics are not available., Comment: 6 pages, 3 figures + 3 pages supplemental

Measurements of the electron's electric dipole moment (eEDM) are demanding tests of physics beyond the Standard Model. We describe how ultracold YbF molecules could be used to improve the precision of eEDM measurements by two to three orders of magnitude. Using numerical simulations, we show how the combination of magnetic focussing, two-dimensional transverse laser cooling, and frequency-chirped laser slowing, can produce an intense, slow, highly-collimated molecular beam. We show how to make a magneto-optical trap of YbF molecules and how the molecules could be loaded into an optical lattice. eEDM measurements could be made using the slow molecular beam or using molecules trapped in the lattice. We estimate the statistical sensitivity that could be reached in each case and consider how sources of noise can be reduced so that the shot-noise limit of sensitivity can be reached. We also consider systematic effects due to magnetic fields and vector light shifts and how they could be controlled.

Extinction spectroscopy is a powerful tool for demonstrating the coupling of a single quantum emitter to a photonic structure. However, it can be challenging in all but the simplest of geometries to deduce an accurate value of the coupling efficiency from the measured spectrum. Here we develop a theoretical framework to deduce the coupling efficiency from the measured transmission and reflection spectra without precise knowledge of the photonic environment. We then consider the case of a waveguide interrupted by a transverse cut in which an emitter is placed. We apply that theory to a silicon nitride waveguide interrupted by a gap filled with anthracene that is doped with dibenzoterrylene molecules. We describe the fabrication of these devices, and experimentally characterise the waveguide coupling of a single molecule in the gap., Comment: 10 page article with 3 figures and 6 page supplementary information with 3 figures. Comments welcome

The electric dipole moment of the electron (eEDM) can be measured with high precision using heavy polar molecules. In this paper, we report on a series of new techniques that have improved the statistical sensitivity of the YbF eEDM experiment. We increase the number of molecules participating in the experiment by an order of magnitude using a carefully designed optical pumping scheme. We also increase the detection efficiency of these molecules by another order of magnitude using an optical cycling scheme. In addition, we show how to destabilise dark states and reduce backgrounds that otherwise limit the efficiency of these techniques. Together, these improvements allow us to demonstrate a statistical sensitivity of $1.8 \times 10^{-28}$ e cm after one day of measurement, which is 1.2 times the shot-noise limit. The techniques presented here are applicable to other high-precision measurements using molecules., Comment: 22 pages, 11 figures

We demonstrate the emission of photons from a single molecule into a hybrid gap plasmon waveguide (HGPW). Crystals of anthracene, doped with dibenzoterrylene (DBT), are grown on top of the waveguides. We investigate a single DBT molecule coupled to the plasmonic region of one of the guides, and determine its in-plane orientation, excited state lifetime and saturation intensity. The molecule emits light into the guide, which is remotely out-coupled by a grating. The second-order auto-correlation and cross-correlation functions show that the emitter is a single molecule and that the light emerging from the grating comes from that molecule. The coupling efficiency is found to be $\beta_{WG}=11.6(1.5)\%$. This type of structure is promising for building new functionality into quantum-photonic circuits, where localised regions of strong emitter-guide coupling can be interconnected by low-loss dielectric guides., Comment: 13 page article. Comments welcome

We introduce a scheme for deep laser cooling of molecules based on robust dark states at zero velocity. By simulating this scheme, we show it to be a widely applicable method that can reach the recoil limit or below. We demonstrate and characterise the method experimentally, reaching a temperature of 5.4(7) $\mu$K. We solve a general problem of measuring low temperatures for large clouds by rotating the phase-space distribution and then directly imaging the complete velocity distribution. Using the same phase-space rotation method, we rapidly compress the cloud. Applying the cooling method a second time, we compress both the position and velocity distributions., Comment: 9 pages, 7 figures

The accelerated expansion of the universe motivates a wide class of scalar field theories that modify gravity on large scales. In regions where the weak field limit of General Relativity has been confirmed by experiment, such theories need a screening mechanism to suppress the new force. We have measured the acceleration of an atom toward a macroscopic test mass inside a high vacuum chamber, where the new force is unscreened in some theories. Our measurement, made using atom interferometry, shows that the attraction between atoms and the test mass does not differ appreciably from Newtonian gravity. This result places stringent limits on the free parameters in chameleon and symmetron theories of modified gravity., Comment: 6 pages, 4 figures

A reliable photon source is required for many aspects of quantum technology. Organic molecules are attractive for this application because they can have high quantum yield and can be photostable, even at room temperature. To generate a photon with high probability, a laser must excite the molecule efficiently. We develop a simple model for that efficiency and discuss how to optimise it. We demonstrate the validity of our model through experiments on a single dibenzoterrylene (DBT) molecule in an anthracene crystal. We show that the excitation probability cannot exceed 75\% at room temperature, but can increase to over 99\% if the sample is cooled to liquid nitrogen temperature. The possibility of high photon generation efficiency with only modest cooling is a significant step towards a reliable photon source that is simple and practical., Comment: Main article (8 pages), Supplementary material (4 pages). Comments welcome

We demonstrate one-dimensional sub-Doppler laser cooling of a beam of YbF molecules to 100 $\mu$K. This is a key step towards a measurement of the electron's electric dipole moment using ultracold molecules. We compare the effectiveness of magnetically-assisted and polarization-gradient sub-Doppler cooling mechanisms. We model the experiment and find good agreement with our data.

We demonstrate coherent microwave control of the rotational, hyperfine and Zeeman states of ultracold CaF molecules, and the magnetic trapping of these molecules in a single, selectable quantum state. We trap about $5\times 10^{3}$ molecules for 2 s at a temperature of 65(11) $\mu$K and a density of $1.2 \times 10^{5}$ cm$^{-3}$. We measure the state-specific loss rate due to collisions with background helium., Comment: 6 pages, 4 figures

Experiments with cold molecules usually begin with a molecular source. We describe the construction and characteristics of a cryogenic buffer gas source of CaF molecules. The source emits pulses with a typical duration of 240 $\mu$s, a mean speed of about 150 m/s, and a flux of $5\times 10^{10}$ molecules per steradian per pulse in a single rotational state., Comment: 13 pages, 5 figures

We present the properties of a magneto-optical trap (MOT) of CaF molecules. We study the process of loading the MOT from a decelerated buffer-gas-cooled beam, and how best to slow this molecular beam in order to capture the most molecules. We determine how the number of molecules, the photon scattering rate, the oscillation frequency, damping constant, temperature, cloud size and lifetime depend on the key parameters of the MOT, especially the intensity and detuning of the main cooling laser. We compare our results to analytical and numerical models, to the properties of standard atomic MOTs, and to MOTs of SrF molecules. We load up to $2 \times 10^4$ molecules, and measure a maximum scattering rate of $2.5 \times 10^6$ s$^{-1}$ per molecule, a maximum oscillation frequency of 100 Hz, a maximum damping constant of 500 s$^{-1}$, and a minimum MOT rms radius of 1.5 mm. A minimum temperature of 730 $\mu$K is obtained by ramping down the laser intensity to low values. The lifetime, typically about 100 ms, is consistent with a leak out of the cooling cycle with a branching ratio of about $6 \times 10^{-6}$. The MOT has a capture velocity of about 11 m/s., Comment: 27 pages, 16 figures

The ability to cool atoms below the Doppler limit -- the minimum temperature reachable by Doppler cooling -- has been essential to most experiments with quantum degenerate gases, optical lattices and atomic fountains, among many other applications. A broad set of new applications await ultracold molecules, and the extension of laser cooling to molecules has begun. A molecular magneto-optical trap has been demonstrated, where molecules approached the Doppler limit. However, the sub-Doppler temperatures required for most applications have not yet been reached. Here we cool molecules to 50 uK, well below the Doppler limit, using a three-dimensional optical molasses. These ultracold molecules could be loaded into optical tweezers to trap arbitrary arrays for quantum simulation, launched into a molecular fountain for testing fundamental physics, and used to study ultracold collisions and ultracold chemistry., Comment: 8 pages, 6 figures

We describe a parallel pair of high voltage electric field plates designed and constructed to minimise magnetic Johnson noise. They are formed by laminating glass substrates with commercially available polyimide (Kapton) tape, covered with a thin gold film. Tested in vacuum, the outgassing rate is less than $5\times10^{-5}$ mbar.l/s. The plates have been operated at electric fields up to 8.3 kV/cm, when the leakage current is at most a few hundred pA. The design is discussed in the context of a molecular spin precession experiment to measure the permanent electric dipole moment of the electron., Comment: 9 pages, 3 figures

It is usually considered that the spectrum of an optical cavity coupled to an atomic medium does not exhibit a normal-mode splitting unless the system satisfies the strong coupling condition, meaning the Rabi frequency of the coherent coupling exceeds the decay rates of atom and cavity excitations. Here we show that this need not be the case, but depends on the way in which the coupled system is probed. Measurements of the reflection of a probe laser from the input mirror of an overdamped cavity reveal an avoided crossing in the spectrum which is not observed when driving the atoms directly and measuring the Purcell-enhanced cavity emission. We understand these observations by noting a formal correspondence with electromagnetically-induced transparency of a three-level atom in free space, where our cavity acts as the absorbing medium and the coupled atoms play the role of the control field.

The longitudinal ($\Gamma_1$) and transverse ($\Gamma_2$) decay rates of a two-level quantum system have profound influence on its evolution. Atomic systems with $\Gamma_2=\tfrac{1}{2}\Gamma_1$ have been studied extensively, but with the rise of solid-state quantum devices it is also important to consider the effect of stronger transverse relaxation due to interactions with the solid environment. Here we study the quantum dynamics of a single organic dye molecule driven by a laser. We measure the variation of $\Gamma_2$ with temperature and determine the activation energy for thermal dephasing of the optical dipole. Then we measure the second-order correlation function $g^{(2)}(\tau)$ of the light emitted by the molecule for various ratios $\Gamma_2/\Gamma_1$ and saturation parameters $S$. We show that the general solution to the optical Bloch equations accurately describes the observed quantum dynamics over a wide range of these parameters, and we discuss the limitations of the various approximate expressions for $g^{(2)}(\tau)$ that appear in the literature., Comment: 5 pages main text, 2 pages supplementary, 4 figures. Comments welcome

Using frequency-chirped radiation pressure slowing, we precisely control the velocity of a pulsed CaF molecular beam down to a few m/s, compressing its velocity spread by a factor of 10 while retaining high intensity: at a velocity of 15~m/s the flux, measured 1.3~m from the source, is 7$\times$10$^{5}$ molecules per cm$^{2}$ per shot in a single rovibrational state. The beam is suitable for loading a magneto-optical trap or, when combined with transverse laser cooling, improving the precision of spectroscopic measurements that test fundamental physics. We compare the frequency-chirped slowing method with the more commonly used frequency-broadened slowing method., Comment: 19 pages, 8 figures. Extension of earlier version to include detailed comparison of slowing methods

Single organic molecules offer great promise as bright, reliable sources of identical single photons on demand, capable of integration into solid-state devices. It has been proposed that such molecules in a crystalline organic matrix might be placed close to an optical waveguide for this purpose, but so far there have been no demonstrations of sufficiently thin crystals, with a controlled concentration of suitable dopant molecules. Here we present a method for growing very thin anthracene crystals from super-saturated vapour, which produces crystals of extreme flatness and controlled thickness. We show how this crystal can be doped with a widely adjustable concentration of dibenzoterrylene (DBT) molecules and we examine the optical properties of these molecules to demonstrate their suitability as quantum emitters in nanophotonic devices. Our measurements show that the molecules are available in the crystal as single quantum emitters, with a well-defined polarisation relative to the crystal axes, making them amenable to alignment with optical nanostructures. We find that the radiative lifetime and saturation intensity vary little within the crystal and are not in any way compromised by the unusual matrix environment. We show that a large fraction of these emitters are able to deliver more than $10^{12}$ photons without photo-bleaching, making them suitable for real applications., Comment: 12 pages, 10 figures, comments welcome

It has recently been shown that optical reflection gratings fabricated directly into an atom chip provide a simple and effective way to trap and cool substantial clouds of atoms [1,2]. In this article we describe how the gratings are designed and micro-fabricated and we characterise their optical properties, which determine their effectiveness as a cold atom source. We use simple scalar diffraction theory to understand how the morphology of the gratings determines the power in the diffracted beams.

We describe the design, construction and operation of a versatile dual-species Zeeman slower for both Cs and Yb, which is easily adaptable for use with other alkali metals and alkaline earths. With the aid of analytic models and numerical simulation of decelerator action, we highlight several real-world problems affecting the performance of a slower and discuss effective solutions. To capture Yb into a magneto-optical trap (MOT), we use the broad $^1S_0$ to $^1P_1$ transition at 399 nm for the slower and the narrow $^1S_0$ to $^3P_1$ intercombination line at 556 nm for the MOT. The Cs MOT and slower both use the D2 line ($6^2S_{1/2}$ to $6^2P_{3/2}$) at 852 nm. We demonstrate that within a few seconds the Zeeman slower loads more than $10^9$ Yb atoms and $10^8$ Cs atoms into their respective MOTs. These are ideal starting numbers for further experiments on ultracold mixtures and molecules., Comment: 15 pages, 15 figures, 4 tables, revtex4-1

We report a robust technique for laser frequency stabilisation that enables the reproducible loading of in excess of 10$^{9}$ Yb atoms from a Zeeman slower directly into a magneto-optical trap (MOT) operating on the $^{1}S_{0} \rightarrow \, ^{3}P_{1}$ transition, without the need for a first stage MOT on the $^{1}S_{0} \rightarrow \, ^{1}P_{1}$ transition. We use a simple atomic beam apparatus to generate narrow fluorescence signals on both the 399 nm $^{1}S_{0} \rightarrow \, ^{1}P_{1}$ transition used for the Zeeman slower and the 556 nm $^{1}S_{0} \rightarrow \, ^{3}P_{1}$ transition. We present in detail the methods for obtaining spectra with a high signal-to-noise ratio and demonstrate error signals suitable for robust frequency stabilisation. Finally we demonstrate the stability and precision of our technique through sensitive measurements of the gravitational sag of the Yb MOT as a function of the intensity of the laser cooling beams, which are in good agreement with theory. These results will be important for efficient loading of the atoms into an optical dipole trap., Comment: 15 pages, 9 figures

We describe an apparatus designed to trap and cool a Yb and Cs mixture. The apparatus consists of a dual species effusive oven source, dual species Zeeman slower, magneto-optical traps in a single ultra-high vacuum science chamber, and the associated laser systems. The dual species Zeeman slower is used to load sequentially the two species into their respective traps. Its design is flexible and may be adapted for other experiments with different mixtures of atomic species. The apparatus provides excellent optical access and can apply large magnetic bias fields to the trapped atoms. The apparatus regularly produces 10${}^{8}$ Cs atoms at 13.3 $\mu$K in an optical molasses, and 10${}^{9}$ Yb atoms cooled to 22 $\mu$K in a narrowband magneto-optical trap., Comment: 13 pages, 12 figures

We have measured the damped motion of a trapped Bose-Einstein condensate, oscillating with respect to a thermal cloud. The cigar-shaped trapping potential provides enough transverse confinement that the dynamics of the system are intermediate between three-dimensional and one-dimensional. We find that oscillations persist for longer than expected for a three-dimensional gas. We attribute this to the suppressed occupation of transverse momentum states, which are essential for damping.

We characterize a Fabry-Perot microwave cavity designed for trapping atoms and molecules at the antinode of a microwave field. The cavity is fed from a waveguide through a small coupling hole. Focussing on the compact resonant modes of the cavity, we measure how the electric field profile, the cavity quality factor, and the coupling efficiency, depend on the radius of the coupling hole. We measure how the quality factor depends on the temperature of the mirrors in the range from 77 to 293K. The presence of the coupling hole slightly changes the profile of the mode, leading to increased diffraction losses around the edges of the mirrors and a small reduction in quality factor. We find the hole size that maximizes the intra-cavity electric field. We develop an analytical theory of the aperture-coupled cavity that agrees well with our measurements, with small deviations due to enhanced diffraction losses. We find excellent agreement between our measurements and finite-difference time-domain simulations of the cavity., Comment: 16 pages, 8 figures

Theories of dark energy require a screening mechanism to explain why the associated scalar fields do not mediate observable long range fifth forces. The archetype of this is the chameleon field. Here we show that individual atoms are too small to screen the chameleon field inside a large high-vacuum chamber, and therefore can detect the field with high sensitivity. We derive new limits on the chameleon parameters from existing experiments, and show that most of the remaining chameleon parameter space is readily accessible using atom interferometry., Comment: 5 pages plus appendices, 4 figures v2. Error in Appendix C corrected, conclusions of the main text unchanged. This is an author-created, un-copyedited version of an article published in JCAP. IOP Publishing Ltd is not responsible for any errors or omissions in this version of the manuscript or any version derived from it. The Version of Record is available at doi:10.1088/1475-7516/2015/03/042

The Lambda-doublet transitions in CH at 3.3 and 0.7 GHz are unusually sensitive to variations in the fine-structure constant and the electron-to-proton mass ratio. We describe methods used to measure the frequencies of these transitions with Hz-level accuracy. We produce a pulsed supersonic beam of cold CH by photodissociation of CHBr3, and we measure the microwave transition frequencies as the molecules propagate through a parallel-plate transmission line resonator. We use the molecules to map out the amplitude and phase of the standing wave field inside the transmission line. We investigate velocity-dependent frequency shifts, showing that they can be strongly suppressed through careful timing of the microwave pulses. We measure the Zeeman and Stark effects of the microwave transitions, and reduce systematic shifts due to magnetic and electric fields to below 1 Hz. We also investigate other sources of systematic uncertainty in the experiment., Comment: 27 pages, 12 figures

We excite YbF molecules to low-lying vibrational levels of the $A^2\Pi_{1/2}$ state, and of the nearby perturber state sometimes called [18.6]0.5. By dispersing the fluorescence, we measure branching ratios for the radiative decay to vibrational levels of the $X^2\Sigma^+$ state. These ratios help to determine the optimum laser cooling scheme for the molecule. Our results establish the practicality of a scheme that was previously suggested [Tarbutt et al., New J. Phys. 15 (2013) 053034] and show how the scheme can be modified to provide a stronger radiative cooling force., Comment: 5 pages

Laser cooled atoms are central to modern precision measurements. They are also increasingly important as an enabling technology for experimental cavity quantum electrodynamics, quantum information processing and matter wave interferometry. Although significant progress has been made in miniaturising atomic metrological devices, these are limited in accuracy by their use of hot atomic ensembles and buffer gases. Advances have also been made in producing portable apparatus that benefit from the advantages of atoms in the microKelvin regime. However, simplifying atomic cooling and loading using microfabrication technology has proved difficult. In this letter we address this problem, realising an atom chip that enables the integration of laser cooling and trapping into a compact apparatus. Our source delivers ten thousand times more atoms than previous magneto-optical traps with microfabricated optics and, for the first time, can reach sub-Doppler temperatures. Moreover, the same chip design offers a simple way to form stable optical lattices. These features, combined with the simplicity of fabrication and the ease of operation, make these new traps a key advance in the development of cold-atom technology for high-accuracy, portable measurement devices., Comment: 5 pages, 5 figures

The CH radical offers a sensitive way to test the hypothesis that fundamental constants measured on earth may differ from those observed in other parts of the universe. The starting point for such a comparison is to have accurate laboratory frequencies. Here we measure the frequency of the lowest millimetre-wave transition of CH, near 535 GHz, with an accuracy of 0.6 kHz. This improves the uncertainty by roughly two orders of magnitude over previous determinations and opens the way for sensitive new tests of varying constants., Comment: 5 pages, 5 figures

We describe an experiment in which cold rubidium atoms, confined in an elongated magnetic trap, are excited by transverse oscillation of the trap centre. The temperature after excitation exhibits resonance as a function of the driving frequency. We measure these resonances at several different trap frequencies. In order to interpret the experiments, we develop a simple model that incorporates both collisions between atoms and the anharmonicity of the real three-dimensional trapping potential. As well as providing a precise connection between the transverse harmonic oscillation frequency and the temperature resonance frequency, this model gives insight into the heating and loss mechanisms, and into the dynamics of driven clouds of cold trapped atoms., Comment: 7 pages, 8 figures

Many modern theories predict that the fundamental constants depend on time, position, or the local density of matter. We develop a spectroscopic method for pulsed beams of cold molecules, and use it to measure the frequencies of microwave transitions in CH with accuracy down to 3 Hz. By comparing these frequencies with those measured from sources of CH in the Milky Way, we test the hypothesis that fundamental constants may differ between the high and low density environments of the Earth and the interstellar medium. For the fine structure constant we find \Delta\alpha/\alpha = (0.3 +/- 1.1)*10^{-7}, the strongest limit to date on such a variation of \alpha. For the electron-to-proton mass ratio we find \Delta\mu/\mu = (-0.7 +/- 2.2) * 10^{-7}. We suggest how dedicated astrophysical measurements can improve these constraints further and can also constrain temporal variation of the constants., Comment: 8 pages, 3 figures

We demonstrate slowing and longitudinal cooling of a supersonic beam of CaF molecules using counter-propagating laser light resonant with a closed rotational and almost closed vibrational transition. A group of molecules are decelerated by about 20 m/s by applying light of a fixed frequency for 1.8 ms. Their velocity spread is reduced, corresponding to a final temperature of about 300 mK. The velocity is further reduced by chirping the frequency of the light to keep it in resonance as the molecules slow down., Comment: 6 pages, 6 figures

High-precision measurements benefit from lock-in detection of small signals. Here we discuss the extension of lock-in detection to many channels, using mutually orthogonal modulation waveforms, and show how the the choice of waveforms affects the information content of the signal. We also consider how well the detection scheme rejects noise, both random and correlated. We address the particular difficulty of rejecting a background drift that makes a reproducible offset in the output signal and we show how a systematic error can be avoided by changing the waveforms between runs and averaging over many runs. These advances made possible a recent measurement of the electron's electric dipole moment., Comment: 11 pages, 3 figures

We have studied the surface quality of millimeter-scale optical mirrors produced by etching CZ and FZ silicon wafers in potassium hydroxide to expose the $\{111\}$ planes. We find that the FZ surfaces have four times lower noise power at spatial frequencies up to $500\, {mm}^{-1}$. We conclude that mirrors made using FZ wafers have higher optical quality.

We present a combined experimental and theoretical study of beam formation from a cryogenic buffer gas cell. Atoms and molecules are loaded into the cell by laser ablation of a target, and are cooled and swept out of the cell by a flow of cold helium. We study the thermalization and flow dynamics inside the cell and measure how the speed, temperature, divergence and extraction efficiency of the beam are influenced by the helium flow. We use a finite element model to simulate the flow dynamics and use the predictions of this model to interpret our experimental results., Comment: 10 pages, 14 figures

We demonstrate the elements of a coupled-resonator optical waveguide in a side-coupled Fabry-P\'erot configuration, and show that the coupling rate between adjacent waveguides can be widely tuned through the thermo-optic effect. The device is linearly scalable and can be combined with other integrated devices, with applications as an optical delay line or as a key element in a cavity-QED based quantum simulator., Comment: 3 pages, 4 figures

We propose an experiment to measure the electric dipole moment of the electron using ultracold YbF molecules. The molecules are produced as a thermal beam by a cryogenic buffer gas source, and brought to rest in an optical molasses that cools them to the Doppler limit or below. The molecular cloud is then thrown upward to form a fountain in which the electric dipole moment of the electron is measured., Comment: 18 pages, 8 figures, 53 references

Miniature concave hollows, made by wet etching silicon through a circular mask, can be used as mirror substrates for building optical micro-cavities on a chip. In this paper we investigate how ICP polishing improves both shape and roughness of the mirror substrates. We characterise the evolution of the surfaces during the ICP polishing using white-light optical profilometry and atomic force microscopy. A surface roughness of 1 nm is reached, which reduces to 0.5 nm after coating with a high reflectivity dielectric. With such smooth mirrors, the optical cavity finesse is now limited by the shape of the underlying mirror.

We recently reported a new measurement of the electron's electric dipole moment using YbF molecules [Nature 473, 493 (2011)]. Here, we give a more detailed description of the methods used to make this measurement, along with a fuller analysis of the data. We show how our methods isolate the electric dipole moment from imperfections in the experiment that might mimic it. We describe the systematic errors that we discovered, and the small corrections that we made to account for these. By making a set of additional measurements with greatly exaggerated experimental imperfections, we find upper bounds on possible uncorrected systematic errors which we use to determine the systematic uncertainty in the measurement. We also calculate the size of some systematic effects that have been important in previous electric dipole moment measurements, such as the motional magnetic field effect and the geometric phase, and show them to be negligibly small in the present experiment. Our result is consistent with an electric dipole moment of zero, so we provide upper bounds to its size at various confidence levels. Finally, we review the prospects for future improvements in the precision of the experiment., Comment: 35 pages, 15 figures

The Proceedings of the 2011 workshop on Fundamental Physics at the Intensity Frontier. Science opportunities at the intensity frontier are identified and described in the areas of heavy quarks, charged leptons, neutrinos, proton decay, new light weakly-coupled particles, and nucleons, nuclei, and atoms., Comment: 229 pages

We demonstrate the deceleration of heavy polar molecules in low-field seeking states by combining a cryogenic source and a travelling-wave Stark decelerator. The cryogenic source provides a high intensity beam with low speed and temperature, and the travelling-wave decelerator provides large deceleration forces and high phase-space acceptance. We prove these techniques using YbF molecules and find the experimental data to be in excellent agreement with numerical simulations. These methods extend the scope of Stark deceleration to a very wide range of molecules., Comment: 5 pages, 4 figures

The fluorescence spectrum resulting from laser excitation of the A^{2}\Pi_{1/2} - X^{2}\Sigma^{+} (0,0) band of ytterbium monofluoride, YbF, has been recorded and analyzed to determine the Franck-Condon factors. The measured values are compared with those predicted from Rydberg-Klein-Rees (RKR) potential energy curves. From the fluorescence decay curve the radiative lifetime of the A^{2}\Pi_{1/2} state is measured to be 28\pm2 ns, and the corresponding transition dipole moment is 4.39\pm0.16 D. The implications for laser cooling YbF are discussed., Comment: 5 pages, 5 figures

We describe a realistic scheme for coupling atoms or other quantum emitters with an array of coupled optical cavities. We consider open Fabry-Perot microcavities coupled to the emitters. Our central innovation is to connect the microcavities to waveguide resonators, which are in turn evanescently coupled to each other on a photonic chip to form a coupled cavity chain. In this paper, we describe the components, their technical limitations and the factors that need to be determined experimentally. This provides the basis for a detailed theoretical analysis of two possible experiments to realize quantum squeezing and controlled quantum dynamics. We close with an outline of more advanced applications., Comment: 30 pages, 8 figures. Submitted to New Journal of Physics

We analyze the evolution of an electromagnetic field inside a double cavity when the difference in length between the two cavities is changed, e.g. by translating the common mirror. We find that this allows photons to be moved deterministically from one cavity to the other. We are able to obtain the conditions for adiabatic transfer by first mapping the Maxwell wave equation for the electric field onto a Schroedinger-like wave equation, and then using the Landau-Zener result for the transition probability at an avoided crossing. Our analysis reveals that this mapping only rigorously holds when the two cavities are weakly coupled (i.e. in the regime of a highly reflective common mirror), and that, generally speaking, care is required when attempting a hamiltonian description of cavity electrodynamics with time-dependent boundary conditions., Comment: 24 pages, 18 figures. Version 2 includes a new section (Sec. VIII) on the regimes of validity of the Schroedinger-like equations and also of the adiabatic approximation, together with a new figure (Fig. 10). The discussion section (Sec. XI) has also been enhanced

We investigate the use of integrated, microfabricated photonic-atomic junctions for quantum information processing applications. The coupling between atoms and light is enhanced by using microscopic optics without the need for cavity enhancement. Qubits that are collectively encoded in hyperfine states of small ensembles of optically trapped atoms, coupled via the Rydberg blockade mechanism, seem a particularly promising implementation. Fast and high-fidelity gate operations, efficient readout, long coherence times and large numbers of qubits are all possible., Comment: submitted to special issue "Quantum Information with Neutral Particles" of "Quantum Information Processing"

We report the Stark deceleration of CaF molecules in the strong-field seeking ground state and in a weak-field seeking component of a rotationally-excited state. We use two types of decelerator, a conventional Stark decelerator for the weak-field seekers, and an alternating gradient decelerator for the strong-field seekers, and we compare their relative merits. We also consider the application of laser cooling to increase the phase-space density of decelerated molecules., Comment: 10 pages, 8 figures

We point out that individual organic dye molecules, deposited close to optical waveguides on a photonic chip, can act as single photon sources and can also provide localised, giant optical nonlinearities. This new atom-photon interface may be used as a resource for processing quantum information.

We present a technique for atomic density measurements by the off-resonant phase-shift induced on a two-frequency, coherently-synthesised light beam. We have used this scheme to measure the column density of a magnetically trapped atom cloud and to monitor oscillations of the cloud in real time by making over a hundred non-destructive local density measurments. For measurements using pulses of 10,000-100,000 photons lasting ~10 microsecond, the precision is limited by statistics of the photons and the photodiode avalanche. We explore the relationship between measurement precision and the unwanted loss of atoms from the trap and introduce a figure of merit that characterises it. This method can be used to probe the density of a BEC with minimal disturbance of its phase., Comment: Submitted to New Journal of Physics

We discuss an experiment underway at Imperial College London to measure the permanent electric dipole moment (EDM) of the electron using a molecular beam of YbF. We describe the measurement method, which uses a combination of laser and radiofrequency resonance techniques to detect the spin precession of the YbF molecule in a strong electric field. We pay particular attention to the analysis scheme and explore some of the possible systematic effects which might mimic the EDM signal. Finally, we describe technical improvements which should increase the sensitivity by more than an order of magnitude over the current experimental limit., Comment: 6 pages, 2 figures

We investigate the operation of pyramidal magneto-optical traps (MOTs) microfabricated in silicon. Measurements of the loading and loss rates give insight into the role of the nearby surface in the MOT dynamics. Studies of the fluorescence versus laser frequency and intensity allow us to develop a simple theory of operation. The number of $^{85}$Rb atoms trapped in the pyramid is approximately $L^6$, where $L \lesssim 6$ is the size in mm. This follows quite naturally from the relation between capture velocity and size and differs from the $L^{3.6}$ often used to describe larger MOTs. Our results constitute substantial progress towards fully integrated atomic physics experiments and devices.