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The invention of the laser unleashed the potential of optical metrology, leading to numerous advancements in modern science and technology. This reliance on lasers, however, also sets a bottleneck for precision optical metrology which is complicated by sophisticated photonic infrastructure required for delicate laser-wave control, leading to limited metrology performance and significant system complexity. Here we make a key step towards resolving this challenge, by demonstrating a Pockels laser with multi-functional capability that advances the optical metrology to a new level. The chip-scale laser exhibits a narrow intrinsic linewidth down to 167 Hz and a broad mode-hop-free tuning range up to 24 GHz. In particular, it offers an unprecedented frequency chirping rate up to 20 EHz/s, and an enormous modulation bandwidth >10 GHz, both orders of magnitude larger than any existing lasers. With this laser, we are able to successfully achieve velocimetry of 40 m/s at a short distance of 0.4 m, with a measurable velocity up to the first cosmic velocity at 1 m away, that is inaccessible by conventional ranging approaches, and distance metrology with a ranging resolution of <2 cm. Moreover, for the first time to the best of our knowledge, we are able to realize a dramatically simplified architecture for laser frequency stabilization, by direct locking the laser to an external reference gas cell without any extra external light control. We successfully achieve a long-term laser stability with a frequency fluctuation of only $\pm$ 6.5 MHz over 60 minutes. The demonstrated Pockels laser combines elegantly high laser coherence with ultrafast frequency reconfigurability and superior multifunctional capability that we envision to have profound impacts on many areas including communication, sensing, autonomous driving, quantum information processing, and beyond., Comment: 10 pages, 4 figures

Optical frequency comb underpins a wide range of applications from communication, metrology, to sensing. Its development on a chip-scale platform -- so called soliton microcomb -- provides a promising path towards system miniaturization and functionality integration via photonic integrated circuit (PIC) technology. Although extensively explored in recent years, challenges remain in key aspects of microcomb such as complex soliton initialization, high threshold, low power efficiency, and limited comb reconfigurability. Here we present an on-chip laser that directly outputs microcomb and resolves all these challenges, with a distinctive mechanism created from synergetic interaction among resonant electro-optic effect, optical Kerr effect, and optical gain inside the laser cavity. Realized with integration between a III-V gain chip and a thin-film lithium niobate (TFLN) PIC, the laser is able to directly emit mode-locked microcomb on demand with robust turnkey operation inherently built in, with individual comb linewidth down to 600 Hz, whole-comb frequency tuning rate exceeding $\rm 2.4\times10^{17}$ Hz/s, and 100% utilization of optical power fully contributing to comb generation. The demonstrated approach unifies architecture and operation simplicity, high-speed reconfigurability, and multifunctional capability enabled by TFLN PIC, opening up a great avenue towards on-demand generation of mode-locked microcomb that is expected to have profound impact on broad applications.

Epsilon-near-zero (ENZ) materials have shown significant potential for nonlinear optical applications due to their ultrafast hot carriers and consequent optical nonlinearity enhancement. Modified poly(3,4-ethylenedioxythiophene) (PEDOT) films show metallic characteristics and a resultant ENZ wavelength near 1550nm through polar solvent treatment and annealing. The metallic PEDOT film exhibits an intrinsic optical nonlinear response that is comparable to gold and 100-fold higher than typical inorganic semiconductor ENZ materials due to {\pi}-conjugated delocalized electrons. Hot carriers generate a 22-fold increase in the optical nonlinearity coefficient of metallic PEDOT films at 1550 nm. Hot holes in metallic PEDOT films have a smaller enhancement multiple of carrier temperature and a longer relaxation time than hot electrons in inorganic ENZ materials due to the larger imaginary permittivity and hot-phonon bottleneck for carrier cooling. Our findings suggest that {\pi}-conjugated ENZ polymer may have unique ultrafast and nonlinear optical properties compared to inorganic ENZ materials, enabling new possibilities in on-chip nanophotonic devices, nonlinear optics, and plasmonics., Comment: There is a mistake in our simulation part of two-temperature model. Thus we revise the parameter and reconstruct our idea. The new content is very different to this old one. Thus, we want to withdraw this paper and submit another new one